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Fabrice P. Laussy

Publications and source records attributed to Fabrice P. Laussy.

At least 37 records · Page 2Linked to original sources

$N$-phonon bundle emission via the anti-Stokes process

We demonstrate theoretically the bundle emission of $n$ strongly correlated phonons in an acoustic cavity QED system. The mechanism relies on anti-Stokes resonances that generate super-Rabi oscillations between states with a large difference in their number of excitations, which, combined with dissipation, transfer coherently pure $n$-phonon states outside of the cavity. This process works with close to perfect purity over a wide range of parameters and is tunable optically with well-resolved operation conditions. This broadens the realm of quantum phononics, with potential applications for on-chip quantum information processing, quantum metrology, and engineering of new types of quantum devices, such as optically heralded $N$-phonon guns.

quant-ph↗

Formation of nonlinear X-waves in condensed matter systems

X-waves are an example of a localized wave packet solution of the homogeneous wave equation, and can potentially arise in any area of physics relating to wave phenomena, such as acoustics, electromagnetism, or quantum mechanics. They have been predicted in condensed matter systems such as atomic Bose-Einstein condensates in optical lattices, and were recently observed in exciton-polariton condensates. Here we show that polariton X-waves result from an interference between two separating wave packets that arise from the combination of a locally hyperbolic dispersion relation and nonlinear interactions. We show that similar X-wave structures could also be observed in expanding spin-orbit coupled Bose-Einstein condensates.

cond-mat.quant-gas↗

Negative-mass effects in spin-orbit coupled Bose-Einstein condensates

Negative effective masses can be realised by engineering the dispersion relation in a variety of quantum systems. A recent experiment with spin-orbit coupled Bose-Einstein condensates has shown that a negative effective mass can halt the free expansion of the condensate and produce fringes in the density [M. Khamehchi et al., Phys. Rev. Lett. 118, 155301 (2017)]. Here, we show that the observed fringes are due to the negativity of only one of the two effective mass parameters that characterise the dispersion, which leads to previously predicted self-interference of the wave packet. We show how confgurations are nevertheless accessible to spin-orbit coupled Bose-Einstein condensates where both mass parameters controlling the propagation and diffusion of the condensate are negative, resulting in the novel phenomenon of counter-propagating self-interfering packets.

cond-mat.quant-gas↗

Joint subnatural-linewidth and single-photon emission from resonance fluorescence

Resonance fluorescence---the light emitted when exciting resonantly a two-level system---is a popular quantum source as it seems to inherit its spectral properties from the driving laser and its statistical properties from the two-level system, thus providing a subnatural-linewidth single-photon source. However, these two qualities do not actually coexist in resonance fluorescence, since an optical target detecting these antibunched photons will either be spectrally broad itself and not benefit from the spectrally narrow source, or match spectrally with the source but in this case the antibunching will be spoiled. We first explain this failure through a decomposition of the field-emission and how this gets affected by frequency resolution. We then show how to restore the sought joint subnatural linewidth and antibunched properties, by interfering the resonance fluorescence output with a coherent beam. We finally discuss how the signal that is eventually generated in this way features a new type of quantum correlations, with a plateau of antibunching which suppresses much more strongly close photon pairs. This introduces a new concept of perfect single-photon source.

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Impact of detuning and dephasing on a laser-corrected subnatural-linewidth single-photon source

The elastic scattering peak of a resonantly driven two-level system has been argued to provide narrow-linewidth antibunched photons. Although independent measurements of spectral width on the one hand and antibunching on the other hand do seem to show that this is the case, a joint measurement reveals that only one or the other of these attributes can be realised in the direct emission. We discuss a scheme which interferes the emission with a laser to produce simultaneously single photons of subnatural linewidth. In particular, we consider the effect of dephasing and of the detuning between the driving laser and/or the detector with the emitter. We find that also in presence of dephasing, our scheme brings considerable improvement as compared to the standard scheme.

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Photon correlations in both time and frequency

We summarise the main results that follow from our theory of frequency- and time-resolved photon correlations, which provides exact computations in nontrivial systems. We illustrate the theory with original results as interesting cases can be picked up from the endless configurations that abound in any quantum optical system. In particular, we compare our exact results with previous approximations, upgrade correlations to the case of photon bundles as otherwise no clear physical picture emerge, highlight the interest of measuring away from the peaks in rich landscapes of correlations and emphasize the joint time and frequency aspect of our theory.

quant-ph↗

Photon correlations in both time and frequency

While quantum mechanics precludes the perfect knowledge of so-called "conjugate" variables, such as time and frequency, we discuss the importance of compromising to retain a fair knowledge of their combined values. In the case of light, we show how time and frequency photon correlations allow us to identify a new type of photon emission, which can be used to design a new type of quantum source where we can choose the distribution in time and energy of the emitted photons.

quant-ph↗

Frequency-resolved Monte Carlo

We adapt the Quantum Monte Carlo method to the cascaded formalism of quantum optics, allowing us to simulate the emission of photons of known energy. Statistical processing of the photon clicks thus collected agrees with the theory of frequency-resolved photon correlations, extending the range of applications based on correlations of photons of prescribed energy, in particular those of a photon-counting character. We apply the technique to autocorrelations of photon streams from a two-level system under coherent and incoherent pumping, including the Mollow triplet regime where we demonstrate the direct manifestation of leapfrog processes in producing an increased rate of two-photon emission events.

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Filtering Multiphoton Emission from State-of-the-Art Cavity QED

Engineering multiphoton states is an outstanding challenge with applications in multiple fields, such as quan- tum metrology, quantum lithography or even biological systems. State-of-the-art methods to obtain them rely on post-selection, multi-level systems or Rydberg atomic ensembles. Recently, it was shown that a strongly driven two-level system interacting with a detuned cavity mode can be engineered to continuously emit n-photon states. In the present work, we show that spectral filtering of its emission relaxes considerably the requirements on the system parameters even to the more accessible bad-cavity situation, opening up the possibility of implementing this protocol in a much wider landscape of different platforms. This improvement is based on a key observation: in the imperfect case where only a certain fraction of emission is composed of n-photon states, these have a well defined energy separated from the rest of the signal, which allows to reveal and purify multiphoton emission just by frequency filtering. We demonstrate these results by obtaining analytical expressions for relevant figures of merit of multiphoton emission, such as the n-photon coupling rate between cavity and emitter, the fraction of light emitted as n-photon states, and n-photon emission rates. This allows us to make a systematic study of such figures of merit as a function of the system parameters and demonstrate the viability of the protocol in several relevant types of cavity QED setups, where we take into account the impact of their respective experimental limitations.

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Entangling one polariton with a photon: effect of interactions on a single-polariton quantum state

Polaritons are quasi-particles originating from the coupling of light with matter that demonstrated quantum phenomena at the many-particle mesoscopic level, such as BEC and superfluidity. A highly sought and long-time missing feature of polaritons is a genuine quantum manifestation of their dynamics at the single-particle level. Although they are conceptually perceived as entangled states and theoretical proposals abound for an explicit manifestation of their single-particle properties, so far their behaviour has remained fully accountable for by classical and mean-field theories. In this Article, we report the first experimental demonstration of a genuinely-quantum manifestation of microcavity polaritons, by swapping, in a two-photon entangled state generated by parametric down-conversion, a photon for a polariton. Furthermore, we show how single polaritons are affected by polariton-polariton interactions in a propaedeutic demonstration of their qualities for quantum information applications.

cond-mat.mes-hall↗

Photon Correlations from the Mollow Triplet

Photon correlations between the photoluminescence peaks of the Mollow triplet have been known for a long time, and recently hailed as a resource for heralded single-photon sources. Here, we provide the full picture of photon-correlations at all orders (we deal explicitly with up to four photons) and with no restriction to the peculiar frequency windows enclosing the peaks. We show that a rich multi-photon physics lies between the peaks, due to transition involving virtual photons, and thereby much more strongly correlated than those transiting through the dressed states. Specifically, we show that such emissions occur in bundles of photons rather than as successive, albeit correlated, photons. We provide the recipe to frequency-filter the emission of the Mollow triplet to turn it into a versatile and tunable photon source, allowing in principle all scenarios of photon emission, with advantages already at the one-photon level, i.e., providing more strongly correlated heralded single-photon sources than those already known.

quant-ph↗

Criterion for Single Photon Sources

We propose a criterion to classify and compare sources of single photons: the $p$-norm of their $k$th-order photon correlations. While ideally one should use the uniform norm with $p\rightarrow\infty$, in practice, the 3-norm already allows a meaningful comparison and shows the serious limitations of the usual criterion based on the second order correlation $g^{(2)}$ only. We apply this new criterion to a large family of popular single photon sources and show that some of them do not, in fact, qualify for this function. The best sources from our selections consist of a cascade of two-level systems, improving on the otherwise standard low-power resonant excitation of a single two-level system.

quant-ph↗

Topological order and equilibrium in a condensate of exciton-polaritons

We report the observation of the Berezinskii-Kosterlitz-Thouless transition for a 2D gas of exciton-polaritons, and through the joint measurement of the first-order coherence both in space and time we bring compelling evidence of a thermodynamic equilibrium phase transition in an otherwise open driven/dissipative system. This is made possible thanks to long polariton lifetimes in high-quality samples with small disorder and in a reservoir-free region far away from the excitation spot, that allow topological ordering to prevail. The observed quasi-ordered phase, characteristic for an equilibrium 2D bosonic gas, with a decay of coherence in both spatial and temporal domains with the same algebraic exponent, is reproduced with numerical solutions of stochastic dynamics, proving that the mechanism of pairing of the topological defects (vortices) is responsible for the transition to the algebraic order. Finally, measurements in the weak-coupling regime confirm that polariton condensates are fundamentally different from photon lasers and constitute genuine quantum degenerate macroscopic states.

cond-mat.quant-gas↗

Enhanced two-photon emission from a dressed biexciton

Radiative two-photon cascades from biexcitons in semiconductor quantum dots under resonant two-photon excitation are promising candidates for the generation of photon pairs. In this work, we propose a scheme to obtain two-photon emission that allows to operate under very intense driving fields. This approach relies on the Purcell enhancement of two-photon virtual transitions between states of the biexciton dressed by the laser. The richness provided by the biexcitonic level structure allows to reach a variety of regimes, from antibunched and bunched photon pairs with polarization orthogonal to the driving field, to polarization entangled two-photon emission. This evidences that the general paradigm of two-photon emission from a ladder of dressed states can find interesting, particular implementations in a variety of systems.

quant-ph↗

Coherent generation of nonclassical light on chip via detuned photon blockade

The on-chip generation of non-classical states of light is a key-requirement for future optical quantum hardware. In solid-state cavity quantum electrodynamics, such non-classical light can be generated from self-assembled quantum dots strongly coupled to photonic crystal cavities. Their anharmonic strong light-matter interaction results in large optical nonlinearities at the single photon level, where the admission of a single photon into the cavity may enhance (photon-tunnelling) or diminish (photon-blockade) the probability for a second photon to enter the cavity. Here, we demonstrate that detuning the cavity and QD resonances enables the generation of high-purity non-classical light from strongly coupled systems. For specific detunings we show that not only the purity but also the efficiency of single-photon generation increases significantly, making high-quality single-photon generation by photon-blockade possible with current state-of-the-art samples.

cond-mat.mes-hall↗

Violation of classical inequalities by photon frequency-filtering

The violation of the Cauchy-Schwarz and Bell inequalities ranks among the major evidences of the genuinely quantum nature of an emitter. We show that by dispensing from the usual approximation of mode correlations and studying directly correlations between the physical reality -the photons- these violations can be optimized. This is achieved by extending the concept of photon correlations to all frequencies in all the possible windows of detections, with no prejudice to the supposed origin of the photons. We identify the regions of quantum emission as rooted in collective de-excitation involving virtual states instead of, as previously assumed, cascaded transitions between real states.

quant-ph↗

Relaxation Oscillations in the Formation of a Polariton Condensate

We report observation of oscillations in the dynamics of a microcavity polariton condensate formed under pulsed non resonant excitation. While oscillations in a condensate have always been attributed to Josephson mechanisms due to a chemical potential unbalance, here we show that under some localisation conditions of the condensate, they may arise from relaxation oscillations, a pervasive classical dynamics that repeatedly provokes the sudden decay of a reservoir, shutting off relaxation as the reservoir is replenished. Using non-resonant excitation, it is thus possible to obtain condensate injection pulses with a record frequency of 0:1 THz.

cond-mat.mes-hall↗

Theory of frequency-filtered and time-resolved N-photon correlations

A theory of correlations between N photons of given frequencies and detected at given time delays is presented. These correlation functions are usually too cumbersome to be computed explicitly. We show that they are obtained exactly through intensity correlations between two-level sensors in the limit of their vanishing coupling to the system. This allows the computation of correlation functions hitherto unreachable. The uncertainties in time and frequency of the detection, which are necessary variables to describe the system, are intrinsic to the theory. We illustrate the formalism with the Jaynes--Cummings model, showing how correlations of various peaks at zero or finite time delays bring new insights into the dynamics of open quantum systems.

quant-ph↗