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Fabrizio Croccolo

Publications and source records attributed to Fabrizio Croccolo.

9 recordsLinked to original sources

Non-Equilibrium Stratification in Supercritical CO2

The supercritical state of matter is usually described as a continuous phase without sharp boundaries between liquid and gas regions. However, under non-equilibrium conditions, this view breaks down. Here we report an experimental investigation of non-equilibrium fluctuations in supercritical carbon dioxide (CO2) subjected to a stabilising temperature gradient. Using shadowgraphy, we reveal spontaneous stratification of the fluid into different layers, separated by transition regions, where thermodynamic properties vary dramatically. These signatures are particularly evident when the system crosses the Widom lines, loci of the extrema of the response function in the supercritical domain. The analysis of the intermediate scattering function of temperature fluctuations highlights the presence of Brunt-Vaisala oscillations within the fluid at multiple frequencies. These oscillations arise from the coupling of thermal and viscous modes under gravity and are a clear signature of the layered structure of the fluid. Our approach enables systematic exploration of a wide range of thermodynamic conditions in a single experiment. These findings suggest that the Widom region cannot be described as a homogeneous phase, but rather as a dynamic assembly of phase-like behaviours, challenging the applicability of classical thermodynamics in non-equilibrium supercritical regimes.

physics.chem-ph

Levitation, oscillations, and wave propagation in a stratified fluid

We present an engaging levitation experiment that students can perform at home or in a simple laboratory using everyday objects. A cork, modified to be slightly denser than water, is placed in a jug containing tap water and coarse kitchen salt delivered at the bottom without stirring. The salt gradually diffuses and determines a stable density stratification of water, the bottom layers being denser than the top ones. During the dissolution of salt, the cork slowly rises at an increasing height, where at any instant its density is balanced by that of the surrounding water. If the cork is gently pushed off its temporary equilibrium position, it experiences a restoring force and starts to oscillate. Students can perform many different measurements of the phenomena involved and tackle non-trivial physical issues related to the behaviour of a macroscopic body immersed in a stratified fluid. Despite its simplicity, this experiment allows to introduce various theoretical concepts of relevance for the physics of the atmosphere and stars and offers students the opportunity of getting acquainted with a simple system that can serve as a model to understand complex phenomena such as oscillations at the Brunt-Väisälä frequency and the propagation of internal gravity waves in a stratified medium.

physics.ed-ph

Spreading of infections on random graphs: A percolation-type model for COVID-19

We introduce an epidemic spreading model on a network using concepts from percolation theory. The model is motivated by discussing the standard SIR model, with extensions to describe effects of lockdowns within a population. The underlying ideas and behavior of the lattice model, implemented using the same lockdown scheme as for the SIR scheme, are discussed in detail and illustrated with extensive simulations. A comparison between both models is presented for the case of COVID-19 data from the USA. Both fits to the empirical data are very good, but some differences emerge between the two approaches which indicate the usefulness of having an alternative approach to the widespread SIR model.

physics.soc-ph

Modelling the spread of Covid19 in Italy using a revised version of the SIR model

In this paper, we present a model to predict the spread of the Covid-19 epidemic and apply it to the specific case of Italy. We started from a simple Susceptible, Infected, Recovered (SIR) model and we added the condition that, after a certain time, the basic reproduction number $R_0$ exponentially decays in time, as empirically suggested by world data. Using this model, we were able to reproduce the real behavior of the epidemic with an average error of 5\%. Moreover, we illustrate possible future scenarios, associated to different intervals of $R_0$. This model has been used since the beginning of March 2020, predicting the Italian peak of the epidemic in April 2020 with about 100.000 detected active cases. The real peak of the epidemic happened on the 20th of April 2020, with 108.000 active cases. This result shows that the model had predictive power for the italian case.

physics.soc-ph

Slowing-down of non-equilibrium concentration fluctuations in confinement

Fluctuations in a fluid are strongly affected by the presence of a macroscopic gradient making them long-ranged and enhancing their amplitude. While small-scale fluctuations exhibit diffusive lifetimes, larger-scale fluctuations live shorter because of gravity, as theoretically and experimentally well-known. We explore here fluctuations of even larger size, comparable to the extent of the system in the direction of the gradient, and find experimental evidence of a dramatic slowing-down in their dynamics. We recover diffusive behaviour for these strongly-confined fluctuations, but with a diffusion coefficient that depends on the solutal Rayleigh number. Results from dynamic shadowgraph experiments are complemented by theoretical calculations and numerical simulations based on fluctuating hydrodynamics, and excellent agreement is found. The study of the dynamics of non-equilibrium fluctuations allows to probe and measure the competition of physical processes such as diffusion, buoyancy and confinement.

cond-mat.soft

Effect of a marginal inclination on pattern formation in a binary liquid mixture under thermal stress

Convective motions in a fluid layer are affected by its orientation with respect to the gravitational field. We investigate the long-term stability of a thermally-stressed layer of a binary liquid mixture and show that pattern formation is strongly affected by marginal inclinations as small as a few milliradians. At small Rayleigh numbers the mass transfer is dominated by the induced large scale shear flow, while at larger Rayleigh numbers it is dominated by solutal convection. At the transition, the balance between the solutal and shear flows gives rise to drifting columnar flows moving in opposite directions along parallel lanes in a Super-Highway configuration.

physics.flu-dyn

Quasi-real-time analysis of dynamic near field scattering data using a graphics processing unit

We present an implementation of the analysis of dynamic near field scattering (NFS) data using a graphics processing unit (GPU). We introduce an optimized data management scheme thereby limiting the number of operations required. Overall, we reduce the processing time from hours to minutes, for typical experimental conditions. Previously the limiting step in such experiments, the processing time is now comparable to the data acquisition time. Our approach is applicable to various dynamic NFS methods, including shadowgraph, Schlieren and differential dynamic microscopy.

physics.data-an

Characterization of anisotropic nano-particles by using depolarized dynamic light scattering in the near field

Light scattering techniques are widely used in many fields of condensed and sof t matter physics. Usually these methods are based on the study of the scattered light in the far field. Recently, a new family of near field detection schemes has been developed, mainly for the study of small angle light scattering. These techniques are based on the detection of the light intensity near to the sample, where light scattered at different directions overlaps but can be distinguished by Fourier transform analysis. Here we report for the first time data obtained with a dynamic near field scattering instrument, measuring both polarized and depolarized scattered light. Advantages of this procedure over the traditional far field detection include the immunity to stray light problems and the possibility to obtain a large number of statistical samples for many different wave vectors in a single instantaneous measurement. By using the proposed technique we have measured the translational and rotational diffusion coefficients of rod-like colloidal particles. The obtained data are in very good agreement with the data acquired with a traditional light scattering apparatus.

physics.optics

Nano-particle characterization by using Exposure Time Dependent Spectrum and scattering in the near field methods: how to get fast dynamics with low-speed CCD camera

Light scattering detection in the near field, a rapidly expanding family of scattering techniques, has recently proved to be an appropriate procedure for performing dynamic measurements. Here we report an innovative algorithm, based on the evaluation of the Exposure Time Dependent Spectrum (ETDS), which makes it possible to measure the fast dynamics of a colloidal suspension with the aid of a simple near field scattering apparatus and a CCD camera. Our algorithm consists in acquiring static spectra in the near field at different exposure times, so that the measured decay times are limited only by the exposure time of the camera and not by its frame rate. The experimental set-up is based on a modified microscope, where the light scattered in the near field is collected by a commercial objective, but (unlike in standard microscopes) the light source is a He-Ne laser which increases the instrument sensitivity. The apparatus and the algorithm have been validated by considering model systems of standard spherical nano-particle.

physics.optics