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Falko Pientka

Publications and source records attributed to Falko Pientka.

At least 19 recordsLinked to original sources

Non-linear Faraday Precession of Light Polarization in Time-Reversal Invariant Materials

We investigate the propagation of electromagnetic waves through materials displaying a non-linear Hall effect. The coupled Maxwell-Boltzmann equations for traveling waves can be mapped onto ordinary differential equations that resemble those for the motion of a pendulum. In the weakly non-linear regime relevant for most experiments, we find that the polarization of light displays a Faraday-like precession of its polarization direction that swings back and forth around the direction of Berry dipole vector as the light beam traverses the material. This occurs concomitantly with an oscillation of its degree of polarization, with a characteristic frequency that increases linearly with the intensity of the traveling wave. These effects could be observed by measuring thickness dependent Faraday rotations as well as the emission of lower frequency radiation associated with the polarization oscillations in materials displaying the non-linear Hall effect.

cond-mat.mes-hall

Signatures of Mode-Resolved, Nonlocal Electron-Phonon Coupling in Two-Dimensional Spectroscopy

Electron-phonon coupling (EPC) is foundational in condensed matter physics, determining intriguing phenomena and properties in both conventional and quantum materials. In this manuscript, we propose and demonstrate a novel two dimensional (2D) EPC spectroscopy which allows for direct extraction of EPC matrix elements for specific phonon modes and different electron energies, simultaneously. Using this technique, we are able to measure the electron-energy dependence of the EPC strength for individual phonon modes. This capability allows us to identify unique signatures distinguishing nonlocal Su-SchriefferHeeger (SSH)-type couplings from local Holstein-type couplings. In application to a methylammonium lead iodide (MAPI) perovskite, we find that two pronounced phonon modes at room temperature exhibit highly distinctive EPC behaviors, concerning strength, anisotropy, and temperature-dependence across the structural phase transition. Our approach paves the way for unraveling the microscopic origin of EPC, the change of the phonon-mode-specific EPC with external conditions, and phonon-mediated ultrafast control of condensed materials.

cond-mat.mtrl-sci

Collective modes in the charge-density wave state of K$_{0.3}$MoO$_3$: The role of long-range Coulomb interactions revisited

We re-examine the effect of long-range Coulomb interactions on the collective amplitude and phase modes in the incommensurate charge-density-wave ground state of quasi-one-dimensional conductors. Using an effective action approach we show that the longitudinal acoustic phonon protects the gapless linear dispersion of the lowest phase mode in the presence of long-range Coulomb interactions. Moreover, in Gaussian approximation, amplitude fluctuations are not affected by long-range Coulomb interactions. We also calculate the collective mode dispersions at finite temperatures and compare our results with the measured energies of amplitude and phase modes in K$_{0.3}$MoO$_3$. With the exception of the lowest phase mode, the temperature dependence of the measured mode energies can be quantitatively described within a multi-phonon Fr\"{o}hlich model for generic electron-phonon interactions neglecting long-range Coulomb interactions.

cond-mat.str-el

Probing the Quantum Noise of the Spinon Fermi Surface with NV Centers

We study the transverse electrical conductivity and the corresponding magnetic noise of a two-dimensional U(1) spin liquid state with a spinon Fermi surface. We show that in the quasi-static regime these responses have the same wave-vector dependence as that of a metal but are reduced by a dimensionless pre-factor controlled by the ratio of orbital diamagnetic susceptibilities of the spinons and chargons, correcting previous work. We estimate that this quasi-static regime is comfortably accessed by the typical NV center splittings of a few GHz and estimate that the expected T1 times for an NV center placed above candidate materials, such as the organic dmit and ET salts, monolayer 1T-TaS2/Se2, would range from several tens to a few hundred milliseconds.

cond-mat.str-el

The universal shear conductivity of Fermi liquids and spinon Fermi surface states and its detection via spin qubit noise magnetometry

We demonstrate a remarkable property of metallic Fermi liquids: the transverse conductivity assumes a universal value in the quasi-static ($ω\rightarrow 0$) limit for wavevectors $q$ in the regime $l_{\rm mfp}^{-1} \ll q \ll p_{\rm F}$, where $l_{\rm mfp}$ is the mean free path and $p_{\rm F}$ is the Fermi momentum. This value is $(e^2/h) \mathcal{R}_{\rm FS}/q$ in two dimensions (2D), where $\mathcal{R}_{\rm FS}$ measures the local radius of curvature of the Fermi surface in momentum space. Even more surprisingly, we find that U(1) spin liquids with a spinon Fermi surface have the same universal transverse conductivity. This means such spin liquids behave effectively as metals in this regime, even though they appear insulating in standard transport experiments. Moreover, we show that transverse current fluctuations result in a universal low-frequency magnetic noise that can be directly probed by a spin qubit, such as a nitrogen-vacancy center in diamond, placed at a distance $z$ above of the 2D metal or spin liquid. Specifically the magnetic noise is given by $Cω\mathcal{P}_{\rm FS}/z$, where $\mathcal{P}_{\rm FS}$ is the perimeter of the Fermi surface in momentum space and $C$ is a combination of fundamental constants of nature. Therefore these observables are controlled purely by the geometry of the Fermi surface and are independent of kinematic details of the quasi-particles, such as their effective mass and interactions. This behavior can be used as a new technique to measure the size of the Fermi surface of metals and as a smoking gun probe to pinpoint the presence of the elusive spinon Fermi surface in two-dimensional systems. We estimate that this universal regime is within reach of current nitrogen-vacancy center spectroscopic techniques for several spinon Fermi surface candidate materials.

cond-mat.mes-hall

Fermi polaron laser in two-dimensional semiconductors

We study the relaxation dynamics of driven, two-dimensional semiconductors, where itinerant electrons dress optically pumped excitons to form two Fermi-polaron branches. Repulsive polarons excited around zero momentum quickly decay to the attractive branch at high momentum. Collisions with electrons subsequently lead to a slower relaxation of attractive polarons, which accumulate at the edge of the light-cone around zero momentum where the radiative loss dominates. The bosonic nature of exciton polarons enables stimulated scattering, which results in a lasing transition at higher pump power. The latter is characterized by a superlinear increase of light emission as well as extended spatiotemporal coherence. As the coherent peak is at the edge of the light-cone and not at the center, the many-body dressing of excitons can reduce the linewidth below the limit set by the exciton nonradiative lifetime.

cond-mat.mes-hall

Topological superconductivity in proximity to type-II superconductors

One-dimensional systems proximity-coupled to a superconductor can be driven into a topological superconducting phase by an external magnetic field. Here, we investigate the effect of vortices created by the magnetic field in a type-II superconductor providing the proximity effect. We identify different ways in which the topological protection of Majorana modes can be compromised and discuss strategies to circumvent these detrimental effects. Our findings are also relevant to topological phases of proximitized quantum Hall edge states.

cond-mat.mes-hall

Quantum Paracrystalline Shear Modes of the Electron Liquid

Unlike classical fluids, a quantum Fermi liquid can support a long-lived and propagating shear sound wave at arbitrarily small wave vectors and frequencies, reminiscent of the transverse sound in crystals, despite lacking any form of long-range crystalline order. This mode is expected to be present in moderately interacting metals where the quasiparticle mass is renormalized to be more than twice the bare mass in two dimensions (2D), but it has remained undetected because it is hard to excite since it does not involve charge density fluctuations, in contrast to the conventional plasma mode. In this work we propose a strategy to excite and detect this unconventional mode in clean metallic channels. We show that the shear sound is responsible for the appearance of sharp dips in the ac conductance of narrow channels at resonant frequencies matching its dispersion. The liquid resonates while minimizing its dissipation in an analogous fashion to a sliding crystal. Ultra-clean 2D materials that can be tuned towards the Wigner crystallization transition such as silicon metal-oxide-semiconductor field-effect transistors, MgZnO/ZnO, p-GaAs, and AlAs quantum wells are promising platforms to experimentally discover the shear sound.

cond-mat.mes-hall

Tuning Topological Superconductivity in Phase-Controlled Josephson Junctions with Rashba and Dresselhaus Spin-Orbit Coupling

Recently, topological superconductors based on Josephson junctions in two-dimensional electron gases with strong Rashba spin-orbit coupling have been proposed as attractive alternatives to wire-based setups. Here, we elucidate how phase-controlled Josephson junctions based on quantum wells with [001] growth direction and an arbitrary combination of Rashba and Dresselhaus spin-orbit coupling can also host Majorana bound states for a wide range of parameters as long as the magnetic field is oriented appropriately. Hence, Majorana bound states based on Josephson junctions can appear in a wide class of two-dimensional electron gases. We study the effect of spin-orbit coupling, the Zeeman energies, and the superconducting phase difference to create a full topological phase diagram and find the optimal stability region to observe Majorana bound states in narrow junctions. Surprisingly, for equal Rashba and Dresselhaus spin-orbit coupling, well localized Majorana bound states can appear only for phase differences $ϕ\neqπ$ as the topological gap protecting the Majorana bound states vanishes at $ϕ=π$. Our results show that the ratio between Rashba and Dresselhaus spin-orbit coupling or the choice of the in-plane crystallographic axis along which the superconducting phase bias is applied offer additional tunable knobs to test Majorana bound states in these systems. Finally, we discuss signatures of Majorana bound states that could be probed experimentally by tunneling conductance measurements at the edge of the junction.

cond-mat.supr-con

Topological Superconductivity in a Phase-Controlled Josephson Junction

Topological superconductors can support localized Majorana states at their boundaries. These quasi-particle excitations have non-Abelian statistics that can be used to encode and manipulate quantum information in a topologically protected manner. While signatures of Majorana bound states have been observed in one-dimensional systems, there is an ongoing effort to find alternative platforms that do not require fine-tuning of parameters and can be easily scalable to large numbers of states. Here we present a novel experimental approach towards a two-dimensional architecture. Using a Josephson junction made of HgTe quantum well coupled to thin-film aluminum, we are able to tune between a trivial and a topological superconducting state by controlling the phase difference $\phi$ across the junction and applying an in-plane magnetic field. We determine the topological state of the induced superconductor by measuring the tunneling conductance at the edge of the junction. At low magnetic fields, we observe a minimum in the tunneling spectra near zero bias, consistent with a trivial superconductor. However, as the magnetic field increases, the tunneling conductance develops a zero-bias peak which persists over a range of $\phi$ that expands systematically with increasing magnetic fields. Our observations are consistent with theoretical predictions for this system and with full quantum mechanical numerical simulations performed on model systems with similar dimensions and parameters. Our work establishes this system as a promising platform for realizing topological superconductivity and for creating and manipulating Majorana modes and will therefore open new avenues for probing topological superconducting phases in two-dimensional systems.

cond-mat.mes-hall

Simulating spin systems with Majorana networks

With the discovery of Majorana quasiparticles in semiconductor-superconductor hybrid structures, topologically protected qubits have emerged as a promising contender for quantum information processing. While the construction of a universal quantum computer with topological protection likely requires significant advances in materials science, intermediate-scale devices are nearly within the reach of current technology. As a near-term milestone for topological qubits, we propose a network of topological superconductors as a simulator of a large variety of quantum spin systems, including those with frustration. Our proposal is founded on existing technology, combining advantages of semiconducting and superconducting qubits. We identify local measurement protocols that give access to information about ground and excited states as well as dynamic correlations. The topological protection of the qubits results in longer coherence times, and relaxation to the groundstate can be controlled by coupling the network an external bath. We conclude by pointing out specific applications of the quantum simulator, e.g., spin liquids, quantum criticality, and thermalization.

cond-mat.mes-hall

Transport of neutral optical excitations using electric fields

Mobile quantum impurities interacting with a fermionic bath form quasiparticles known as Fermi polarons. We demonstrate that a force applied to the bath particles can generate a drag force of similar magnitude acting on the impurities, realizing a novel, nonperturbative Coulomb drag effect. To prove this, we calculate the fully self-consistent, frequency-dependent transconductivity at zero temperature in the Baym-Kadanoff conserving approximation. We apply our theory to excitons and exciton polaritons interacting with a bath of charge carriers in a doped semiconductor embedded in a microcavity. In external electric and magnetic fields, the drag effect enables electrical control of excitons and may pave the way for the implementation of gauge fields for excitons and polaritons. Moreover, a reciprocal effect may facilitate optical manipulation of electron transport. Our findings establish transport measurements as a novel, powerful tool for probing the many-body physics of mobile quantum impurities.

cond-mat.mes-hall

Thermal Transport Signatures of Broken-Symmetry Phases in Graphene

In the half-filled zero-energy Landau level of bilayer graphene, competing phases with spontaneously broken symmetries and an intriguing quantum critical behavior have been predicted. Here we investigate signatures of these broken-symmetry phases in thermal transport measurements. To this end we calculate the spectrum of spin and valley waves in the $ν=0$ quantum Hall state of bilayer graphene. The presence of Goldstone modes enables heat transport even at low temperatures, which can serve as compelling evidence for spontaneous symmetry breaking. By varying external electric and magnetic fields it is possible to determine the nature of the symmetry breaking and temperature-dependent measurements may yield additional information about gapped modes.

cond-mat.mes-hall

Topological Superconductivity in a Planar Josephson Junction

We consider a two-dimensional electron gas with strong spin-orbit coupling contacted by two superconducting leads, forming a Josephson junction. We show that in the presence of an in-plane Zeeman field the quasi-one-dimensional region between the two superconductors can support a topological superconducting phase hosting Majorana bound states at its ends. We study the phase diagram of the system as a function of the Zeeman field and the phase difference between the two superconductors (treated as an externally controlled parameter). Remarkably, at a phase difference of $π$, the topological phase is obtained for almost any value of the Zeeman field and chemical potential. In a setup where the phase is not controlled externally, we find that the system undergoes a first-order topological phase transition when the Zeeman field is varied. At the transition, the phase difference in the ground state changes abruptly from a value close to zero, at which the system is trivial, to a value close to $π$, at which the system is topological. The critical current through the junction exhibits a sharp minimum at the critical Zeeman field, and is therefore a natural diagnostic of the transition. We point out that in presence of a symmetry under a modified mirror reflection followed by time reversal, the system belongs to a higher symmetry class and the phase diagram as a function of the phase difference and the Zeeman field becomes richer.

cond-mat.mes-hall

Signatures of topological Josephson junctions

Quasiparticle poisoning and diabatic transitions may significantly narrow the window for the experimental observation of the $4π$-periodic $dc$ Josephson effect predicted for topological Josephson junctions. Here, we show that switching current measurements provide accessible and robust signatures for topological superconductivity which persist in the presence of quasiparticle poisoning processes. Such measurements provide access to the phase-dependent subgap spectrum and Josephson currents of the topological junction when incorporating it into an asymmetric SQUID together with a conventional Josephson junction with large critical current. We also argue that pump-probe experiments with multiple current pulses can be used to measure the quasiparticle poisoning rates of the topological junction. The proposed signatures are particularly robust, even in the presence of Zeeman fields and spin-orbit coupling, when focusing on short Josephson junctions. Finally, we also consider microwave excitations of short topological Josephson junctions which may complement switching current measurements.

cond-mat.mes-hall

Robust Majorana conductance peaks for a superconducting lead

Experimental evidence for Majorana bound states largely relies on measurements of the tunneling conductance. While the conductance into a Majorana state is in principle quantized to $2e^2/h$, observation of this quantization has been elusive, presumably due to temperature broadening in the normal-metal lead. Here, we propose to use a superconducting lead instead, whose gap strongly suppresses thermal excitations. For a wide range of tunneling strengths and temperatures, a Majorana state is then signaled by symmetric conductance peaks at $eV=\pmΔ$ with quantized height $G=(4-π)2e^2/h$. For a superconducting scanning tunneling microscope tip, Majorana states appear as spatial conductance plateaus while the conductance varies with the local wavefunction for trivial Andreev bound states. We discuss effects of nonresonant (bulk) Andreev reflections and quasiparticle poisoning.

cond-mat.mes-hall

End states and subgap structure in proximity-coupled chains of magnetic adatoms

A recent experiment [Nadj-Perge et al., Science 346, 602 (2014)] provides evidence for Majorana zero modes in iron (Fe) chains on the superconducting Pb(110) surface. Here, we study this system by scanning tunneling microscopy using superconducting tips. This high-resolution technique resolves a rich subgap structure, including zero-energy excitations in some chains. We compare the symmetry properties of the data under voltage reversal against theoretical expectations and provide evidence that the putative Majorana signature overlaps with a previously unresolved low-energy resonance. Interpreting the data within a Majorana framework suggests that the topological gap is significantly smaller than previously believed. Aided by model calculations, we also analyze higher-energy features of the subgap spectrum and their relation to high-bias peaks which we associate with the Fe d-bands.

cond-mat.mes-hall

Strong localization of Majorana end states in chains of magnetic adatoms

A recent experiment [Nadj-Perge et al., Science 346, 602 (2014)] gives possible evidence for Majorana bound states in chains of magnetic adatoms placed on a superconductor. While many features of the observed end states are naturally interpreted in terms of Majoranas, their strong localization remained puzzling. We consider a linear chain of Anderson impurities on a superconductor as a minimal model and treat it largely analytically within mean-field theory. We explore the phase diagram, the subgap excitation spectrum, and the Majorana wavefunctions. Owing to a strong velocity renormalization, the latter are localized on a scale which is parametrically small compared to the coherence length of the host superconductor.

cond-mat.mes-hall