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Fanqiang Chen

Publications and source records attributed to Fanqiang Chen.

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Tunable Extended Magnetic Non-Fermi Liquid in Graphene Moir\'e Heterostructures

Exploring exotic quantum metallic states beyond Landau's Fermi liquid theory remains a central focus in condensed matter physics. Such non-Fermi liquid behavior is mostly observed near quantum criticality, yet growing attention is directed toward extended NFL phases with intrinsic quantum fluctuations rooted in the extended ground state. While these extended NFL states have been previously reported only in a limited set of d- and f-electron systems, realizing a single, highly tunable platform capable of exhibiting multiple resistance exponent values is essential for uncovering the connection between the resistance exponent and the dominant quantum fluctuations coupled to quasiparticles. However, corresponding experimental progress remains elusive. Here, we report the observation of tunable extended non-Fermi liquid behavior in twisted double bilayer graphene encapsulated by aligned hBN layers. This NFL phase spans a broad range of carrier densities and exhibiting a carrier density dependent resistance exponent. Combined with temperature dependent resistance, magnetotransport and differential resistance measurements, these findings support a scenario where strong quantum fluctuations emerge from the interplay between localized and itinerant carriers. Our work establishes a highly tunable platform beyond conventional frameworks to investigate the organizing principles of non-Fermi liquid physics manifested in diverse behaviors.

cond-mat.mes-hall

Orientation-tunable correlated Chern insulating states in chiral twisted double bilayer graphene proximitized by WSe2

Moire flat bands in graphene systems proximitized by transition-metal dichalcogenides (TMDCs) provide a setting where spin-orbit coupling (SOC) can reshape band topology. The crystallographic alignment angle twist angle between TMDC and graphene layers is predicted to tune the balance of Ising and Rashba SOC, but a combined theoretical and experimental understanding of how twist angle governs the topological character of correlated states has not been systematically established. Here we show that in chiral-stacked twisted double bilayer graphene in proximity to WSe2, twist angle between graphene and WSe2 determines the topological character of correlated Chern insulators. Continuum model calculations reveal that Ising spin-orbit coupling dominates at zero twist angle, giving rise to flat bands with finite valley Chern numbers, whereas Rashba coupling dominates at larger twist angle, resulting in topologically trivial bands. Transport measurements at quarter filling confirm this picture: twist angle = 0 deg devices exhibit C = +1 Chern insulators, consistent with spontaneous isospin polarization, whereas twist angle = 15 degree devices show C = 0 despite exhibiting similar correlated insulating behavior. The sharp contrast establishes crystallographic alignment as a new tuning knob, complementary to twist angle, displacement field, and carrier density, for engineering correlated topological states in van der Waals heterostructures.

cond-mat.mes-hall

Skin-inspired in-sensor encoding of strain vector using tunable quantum geometry

Human skin provides crucial tactile feedback, allowing us to skillfully perceive various objects by sensing and encoding complex deformations through multiple parameters in each tactile receptor. However, replicating this high-dimensional tactile perception with conventional materials' electronic properties remains a daunting challenge. Here, we present a skin-inspired method to encode strain vectors directly within a sensor. This is achieved by leveraging the strain-tunable quantum properties of electronic bands in the van der Waals topological semimetal Td -WTe2. We observe robust and independent responses from the second-order and third-order nonlinear Hall signals in Td -WTe2 when subjected to variations in both the magnitude and direction of strain. Through rigorous temperature-dependent measurements and scaling law analysis, we establish that these strain responses primarily stem from quantum geometry-related phenomena, including the Berry curvature and Berry-connection polarizability tensor. Furthermore, our study demonstrates that the strain-dependent nonlinear Hall signals can efficiently encode high-dimensional strain information using a single device. This capability enables accurate and comprehensive sensing of complex strain patterns in the embossed character "NJU". Our findings highlight the promising application of topological quantum materials in advancing next-generation, bio-inspired flexible electronics.

cond-mat.mes-hall

Selective and Quasi-continuous Switching of Ferroelectric Chern Insulator Device for Neuromorphic Computing

Topologically protected edge state transport in quantum materials is dissipationless and features quantized Hall conductance, and shows great potential in highly fault-tolerant computing technologies. However, it remains elusive about how to develop topological edge state-based computing devices. Recently, exploration and understanding of interfacial ferroelectricity in various van der Waals heterostructure material systems have received widespread attention among the community of materials science and condensed matter physics3-11. Such ferroelectric polarization emergent at the vdW interface can coexist with other quantum states and thus provides an unprecedented opportunity to electrically switch the topological edge states of interest, which is of crucial significance to the fault-tolerant electronic device applications based on the topological edge states. Here, we report the selective and quasi-continuous ferroelectric switching of topological Chern insulator devices and demonstrate its promising application in noise-immune neuromorphic computing. We fabricate this ferroelectric Chern insulator device by encapsulating magic-angle twisted bilayer graphene with doubly-aligned h-BN layers, and observe the coexistence of the interfacial ferroelectricity and the topological Chern insulating states. This ferroelectricity exhibits an anisotropic dependence on the in-plane magnetic field. By using a VBG pulse with delicately controlled amplitude, we realize the nonvolatile switching between any pair of Chern insulating states and achieve 1280 distinguishable nonvolatile resistance levels on a single device. Furthermore, we demonstrate deterministic switching between two arbitrary levels among the record-high number of nonvolatile resistance levels.

cond-mat.mes-hall

Tunable moiré bandgap in hBN-aligned bilayer graphene device with in-situ electrostatic gating

Over the years, great efforts have been devoted in introducing a sizable and tunable band gap in graphene for its potential application in next-generation electronic devices. The primary challenge in modulating this gap has been the absence of a direct method for observing changes of the band gap in momentum space. In this study, we employ advanced spatial- and angle-resolved photoemission spectroscopy technique to directly visualize the gap formation in bilayer graphene, modulated by both displacement fields and moiré potentials. The application of displacement field via in-situ electrostatic gating introduces a sizable and tunable electronic bandgap, proportional to the field strength up to 100 meV. Meanwhile, the moiré potential, induced by aligning the underlying hexagonal boron nitride substrate, extends the bandgap by ~ 20 meV. Theoretical calculations, effectively capture the experimental observations. Our investigation provides a quantitative understanding of how these two mechanisms collaboratively modulate the band gap in bilayer graphene, offering valuable guidance for the design of graphene-based electronic devices.

cond-mat.mes-hall

Tunable quantum criticalities in an isospin extended Hubbard model simulator

Studying strong electron correlations has been an essential driving force for pushing the frontiers of condensed matter physics. In particular, in the vicinity of correlation-driven quantum phase transitions (QPTs), quantum critical fluctuations of multiple degrees of freedom facilitate exotic many-body states and quantum critical behaviors beyond Landau's framework. Recently, moiré heterostructures of van der Waals materials have been demonstrated as a highly tunable quantum platform for exploring fascinating strongly correlated quantum physics. Here, we report the observation of tunable quantum criticalities in an experimental simulator of extended Hubbard model with spin-valley isospins arising in chiral-stacked twisted double bilayer graphene. Scaling analysis shows a quantum two-stage criticality manifesting two distinct quantum critical points as the generalized Wigner crystal transits to a Fermi liquid by varying the displacement field, suggesting the emergence of a critical intermediate phase. The quantum two-stage criticality evolves into a quantum pseudo criticality as a high parallel magnetic field is applied. In such pseudo criticality, we find that the quantum critical scaling is only valid above a critical temperature, indicating a weak first-order QPT therein. Our results demonstrate a highly tunable solid-state simulator with intricate interplay of multiple degrees of freedom for exploring exotic quantum critical states and behaviors.

cond-mat.mes-hall

Observation of Coexisting Dirac Bands and Moiré Flat Bands in Magic-Angle Twisted Trilayer Graphene

Moiré superlattices that consist of two or more layers of two-dimensional materials stacked together with a small twist angle have emerged as a tunable platform to realize various correlated and topological phases, such as Mott insulators, unconventional uperconductivity and quantum anomalous Hall effect. Recently, the magic-angle twisted trilayer graphene (MATTG) has shown both robust superconductivity similar to magic-angle twisted bilayer graphene (MATBG) and other unique properties, including the Pauli-limit violating and re-entrant superconductivity. These rich properties are deeply rooted in its electronic structure under the influence of distinct moiré potential and mirror symmetry. Here, combining nanometer-scale spatially resolved angle-resolved photoemission spectroscopy (nano-ARPES) and scanning tunneling microscopy/spectroscopy (STM/STS), we systematically measure the yet unexplored band structure of MATTG near charge neutrality. Our measurements reveal the coexistence of the distinct dispersive Dirac band with the emergent moiré flat band, showing nice agreement with the theoretical calculations. These results serve as a stepstone for further understanding of the unconventional superconductivity in MATTG.

cond-mat.mtrl-sci