arXiv subjects

Federico Belli

Publications and source records attributed to Federico Belli.

18 recordsLinked to original sources

arXiv2024

Supercontinuum generation in methane-filled hollow-core antiresonant fiber

We report the generation of a multi-octave supercontinuum spanning from 350 nm to 1700 nm with exceptional spectral flatness and high conversion efficiency to both the visible and near infrared region, by pumping a methane-filled hollow-core antiresonant fiber with 1030 nm laser pulses. The dynamics exhibited signs of both modulational instability and stimulated Raman scattering. Fiber lengths ranging from 15 to 200~cm were investigated along with gas pressures up to 50 bar and pump pulse durations from 220~fs up to 10~ps. The best supercontinuum, in terms of spectral width and flatness, was achieved with 220~fs pulses, 25~bar filling pressure, and 60~cm propagation length. Comparison with argon-filled fiber with matched nonlinearity and dispersion showed that the Raman contribution enhances the supercontinuum generation process compared to a pure modulational instability-based process. The average power was scaled up by increasing the pulse repetition rate to 50~kHz, but further scaling was hindered by linear and nonlinear absorption leading to fiber damage.

physics.optics↗

arXiv2024

Optimizing Spectral Phase Transfer in Four-Wave Mixing with Gas-filled Capillaries: A Trade-off Study

Four-wave mixing (FWM) in gas-filled hollow-core capillaries, a nonlinear optical process that mixes signal and pump photon frequencies to generate idler frequency photons, offers a method for precise spectral phase transfer from signal to idler at ultrashort timescales and extreme powers. However, this regime is challenged by competing linear and nonlinear dynamics, leading to significant trade-offs between spectral phase transfer and conversion efficiency. Our computational investigation focuses on upconversion of femtosecond pulses from the infrared (IR) to the ultraviolet (UV), a range notoriously difficult to manipulate. We explore an intermediate energy regime that strikes an optimal balance between FWM-mediated phase-transfer fidelity and nonlinear conversion efficiency. By adjusting the energy ratios and spectral phase profiles of the input signal, we achieve conversion efficiencies of approximately 5%-15% while maintaining an effectively quasi-linear spectral phase transfer. These findings contribute to establishing first-principles and scaling laws essential for applications such as high-precision imaging, spectroscopy, quantum transduction, and distributed entangled interconnects, facilitating advanced control of ultrafast photonic and electronic wavepackets in quantum materials with unprecedented spatial and temporal precision.

physics.optics↗

arXiv2023

On-target delivery of intense ultrafast laser pulses through hollow-core anti-resonant fibers

We report the flexible on-target delivery of 800 nm wavelength, 5 GW peak power, 40 fs duration laser pulses through an evacuated and tightly coiled 10 m long hollow-core nested anti-resonant fiber by positively chirping the input pulses to compensate for the anomalous dispersion of the fiber. Near-transform-limited output pulses with high beam quality and a guided peak intensity of 3 PW/cm2 were achieved by suppressing plasma effects in the residual gas by pre-pumping the fiber after evacuation. This appears to cause a long-term removal of molecules from the fiber core. Identifying the fluence at the fiber core-wall interface as the damage origin, we scaled the coupled energy to 2.1 mJ using a short piece of larger-core fiber to obtain 20 GW at the fiber output. This scheme can pave the way towards the integration of anti-resonant fibers in mJ-level nonlinear optical experiments and laser-source development.

physics.optics↗

arXiv2023

The effect of rotational Raman response on ultra-flat supercontinuum generation in gas-filled hollow-core photonic crystal fibers

We experimentally and numerically investigate flat supercontinuum generation in gas-filled anti-resonant guiding hollow-core photonic crystal fiber. By comparing results obtained with either argon or nitrogen we determine the role of the rotational Raman response on the supercontinuum formation. When using argon, a supercontinuum extending from 350 nm to 2 {\mu}m is generated through modulational instability. Although argon and nitrogen exhibit similar Kerr nonlinearity and dispersion, we find that the energy density of the continuum in the normal dispersion region is significantly lower when using nitrogen. Using numerical simulations, we find that due to the closely spaced rotational lines in nitrogen, gain suppression in the fundamental mode causes part of the pump pulse to be coupled into higher-order modes which reduces the energy transfer to wavelengths shorter than the pump.

physics.optics↗

arXiv2023

Dispersion-tuning of nonlinear optical pulse dynamics in gas-filled hollow capillary fibers

We experimentally investigate the nonlinear optical pulse dynamics of ultrashort laser pulses propagating in gas-filled hollow capillary fibers in different dispersion regimes, which are achieved by tuning the gas pressure. When the pulse propagates in the anomalous dispersion regime we observe soliton dynamics accompanied with soliton-plasma effects, such as self-compression, resonant dispersive-wave emission in the fundamental as well as in higher-order modes, soliton blue-shifting and ionization-induced pulse splitting. Propagation of the pulse in the vicinity of the zero-dispersion wavelength results in pulse splitting and subsequent cross-phase modulation leading to the generation of an additional frequency-shifted band and a 3-octave broad supercontinuum. In the case of pulses propagating in normal dispersion we observe the generation of a broad and flat supercontinuum. In this regime, the experimental results are less well described by simulations that consider only the propagation dynamics inside the fiber. Free-space simulations of the beam propagation in the bulk gas, before the capillary entrance, suggest that this discrepancy is caused by self-focusing and ionization altering the pulse spatial and temporal shape, affecting both the coupling efficiency and the subsequent propagation inside the capillary.

physics.optics↗

arXiv2022

Generation and characterization of frequency tuneable sub-15 fs pulses in a gas-filled hollow-core fiber pumped by a Yb:KGW laser

We investigate soliton self-compression and photoionization effects in an argon-filled antiresonant hollow-core photonic crystal fiber pumped with a commercial Yb:KGW laser. Before the onset of photoionization, we demonstrate self-compression of our 220~fs pump laser to 13~fs in a single and compact stage. By using the plasma driven soliton self-frequency blueshift, we also demonstrate a tuneable source from 1030 to ~700 nm. We fully characterize the compressed pulses using sum-frequency generation time-domain ptychography, experimentally revealing the full time-frequency plasma-soliton dynamics in hollow-core fibre for the first time.

physics.optics↗

arXiv2022

From Raman frequency combs to supercontinuum generation in nitrogen-filled hollow-core anti-resonant fiber

We demonstrate a route to supercontinuum generation in gas-filled hollow-core anti-resonant fibers through the creation of a broad vibrational Raman frequency comb followed by continuous broadening and merging of the comb lines through either rotational Raman scattering or the optical Kerr effect. Our demonstration experiments, utilizing a single pump pulse with 20 ps duration at 532 nm in a nitrogen-filled fiber, produce a supercontinuum spanning from 440 nm to 1200 nm, with an additional deep ultraviolet continuum from 250 nm to 360 nm. Numerical results suggest that this approach can produce even broader supercontinuum spectra extending from the ultraviolet to mid-infrared.

physics.optics↗

arXiv2021

Ultrafast circularly polarized pulses tunable from the vacuum to deep ultraviolet

We experimentally demonstrate the efficient generation of circularly polarized pulses tunable from the vacuum to deep ultraviolet (160-380 nm) through resonant dispersive wave emission from optical solitons in a gas-filled hollow capillary fiber. In the deep ultraviolet we measure up to 13 microjoule of pulse energy, and from numerical simulations, we estimate the shortest output pulse duration to be 8.5 fs. We also experimentally verify that simply scaling the pulse energy by 3/2 between linearly and circularly polarized pumping closely reproduces the soliton and dispersive wave dynamics. Based on previous results with linearly polarized self-compression and resonant dispersive wave emission, we expect our technique to be extended to produce circularly polarized few-fs pulses further into the vacuum ultraviolet, and few to sub-fs circularly polarized pulses in the near-infrared.

physics.optics↗

arXiv2020

Generation of broadband circularly polarized deep-ultraviolet pulses in hollow capillary fibers

We demonstrate an efficient scheme for the generation of broadband, high-energy, circularly polarized femtosecond laser pulses in the deep ultraviolet through seeded degenerate four-wave mixing in stretched gas-filled hollow capillary fibers. Pumping and seeding with circularly polarized 35 fs pulses centered at 400 nm and 800 nm, respectively, we generate idler pulses centered at 266 nm with more than 25 microjoule of energy and over 95% spectrally averaged ellipticity. Even higher idler energies and broad spectra (27 nm bandwidth) can be obtained at the cost of reduced ellipticity. Our system can be scaled in average power and used in different spectral regions, including the vacuum ultraviolet.

physics.optics↗

arXiv2020

Resonant dispersive wave emission in hollow capillary fibres filled with pressure gradients

Resonant dispersive wave (RDW) emission in gas-filled hollow waveguides is a powerful technique for the generation of bright few-femtosecond laser pulses from the vacuum ultraviolet to the near infrared. Here we investigate deep-ultraviolet RDW emission in a hollow capillary fibre filled with a longitudinal gas pressure gradient. We obtain broadly similar emission to the constant-pressure case by applying a surprisingly simple scaling rule for the gas pressure and study the energy-dependent dispersive-wave spectrum in detail using simulations. We further find that in addition to enabling dispersion-free delivery to experimental targets, a decreasing gradient also reduces the pulse stretching within the waveguide itself, and that transform-limited pulses with 3 fs duration can be generated by using short waveguides. Our results illuminate the fundamental dynamics underlying this frequency conversion technique and will aid in fully exploiting it for applications in ultrafast science and beyond.

physics.optics↗

arXiv2020

High-energy pulse self-compression and ultraviolet generation through soliton dynamics in hollow capillary fibres

Optical soliton dynamics can cause the extreme alteration of the temporal and spectral shape of a propagating light pulse. They occur at up to kilowatt peak powers in glass-core optical fibres and the gigawatt level in gas-filled microstructured hollow-core fibres. Here we demonstrate optical soliton dynamics in large-core hollow capillary fibres. This enables scaling of soliton effects by several orders of magnitude to the multi-mJ energy and terawatt peak power level. We experimentally demonstrate two key soliton effects. First, we observe self-compression to sub-cycle pulses and infer the creation of sub-femtosecond field waveforms - a route to high-power optical attosecond pulse generation. Second, we efficiently generate continuously tunable high-energy (1 to 16 $μ$J) pulses in the vacuum and deep ultraviolet (110 nm to 400 nm) through resonant dispersive-wave emission.These results promise to be the foundation of a new generation of table-top light sources for ultrafast strong-field physics and advanced spectroscopy.

physics.optics↗

arXiv2020

Infrared attosecond field transients and UV to IR few-femtosecond pulses generated by high-energy soliton self-compression

Infrared femtosecond laser pulses are important tools both in strong-field physics, driving X-ray high-harmonic generation, and as the basis for widely tuneable, if inefficient, ultrafast sources in the visible and ultraviolet. Although anomalous material dispersion simplifies compression to few-cycle pulses, attosecond pulses in the infrared have remained out of reach. We demonstrate soliton self-compression of 1800 nm laser pulses in hollow capillary fibers to sub-cycle envelope duration (2 fs) with 27 GW peak power, corresponding to attosecond field transients. In the same system, we generate wavelength-tuneable few-femtosecond pulses from the ultraviolet (300 nm) to the infrared (740 nm) with energy up to 25 $μ$J and efficiency up to 12 %, and experimentally characterize the generation dynamics in the time-frequency domain. A compact second stage generates multi-$μ$J pulses from 210 nm to 700 nm using less than 200 $μ$J of input energy. Our results significantly expand the toolkit available to ultrafast science.

physics.optics↗

arXiv2019

Highly Efficient Deep UV Generation by Four-Wave Mixing in Gas-Filled Hollow Core Photonic Crystal Fiber

We report on a highly-efficient experimental scheme for the generation of deep-ultraviolet ultrashort light pulses using four-wave mixing in gas-filled kagomé-style photonic crystal fiber. By pumping with ultrashort, few $μ$J, pulses centered at 400 nm, we generate an idler pulse at 266 nm, and amplify a seeded signal at 800 nm. We achieve remarkably high pump-to-idler energy conversion efficiencies of up to 38%. Although the pump and seed pulse durations are ~100 fs, the generated ultraviolet spectral bandwidths support sub-15 fs pulses. These can be further extended to support few-cycle pulses. Four-wave mixing in gas-filled hollow-core fibres can be scaled to high average powers and different spectral regions such as the vacuum ultraviolet (100-200 nm).

physics.optics↗

arXiv2019

High-energy ultraviolet dispersive-wave emission in compact hollow capillary systems

We demonstrate high-energy resonant dispersive-wave emission in the deep ultraviolet (218 to 375 nm) from optical solitons in short (15 to 34cm) hollow capillary fibres. This down-scaling in length compared to previous results in capillaries is achieved by using small core diameters (100 and 150 $μ$m) and pumping with 6.3 fs pulses at 800 nm. We generate pulses with energies of 4 to 6 $μ$J across the deep ultraviolet in a 100 $μ$m capillary and up to 11 $μ$J in a 150 $μ$m capillary. From comparisons to simulations we estimate the ultraviolet pulse to be 2 to 2.5 fs in duration. We also numerically study the influence of pump duration on the bandwidth of the dispersive wave.

physics.optics↗

arXiv2018

Ultrafast Molecular Spectroscopy Using a Hollow-Core Photonic Crystal Fibre Light Source

We demonstrate, for the first time, the application of rare-gas filled hollow-core photonic crystal fibres (HC-PCFs) as tuneable ultraviolet light sources in femtosecond pump-probe spectroscopy. The time-resolved photoelectron imaging technique reveals non-adiabatic dynamical processes operating on three distinct timescales in the styrene molecule following excitation over the 242-258 nm region. These include ultrafast (<100 fs) internal conversion between the S2(pipi*) and S1(pipi*) electronic states and subsequent intramolecular vibrational energy redistribution within S1(pipi*). Compact, cost-effective and highly efficient bench-top HC-PCF sources have huge potential to open up many exciting new avenues for ultrafast spectroscopy in the ultraviolet and vacuum ultraviolet spectral regions. We anticipate that our initial validation of this approach will generate important impetus in this area

physics.chem-ph↗

arXiv2017

Control of ultrafast pulses in hydrogen-filled hollow-core photonic crystal fiber by Raman coherence

We present the results of an experimental and numerical investigation into temporally non-local coherent interactions between ultrashort pulses, mediated by Raman coherence, in gas-filled kagomé-style hollow-core photonic crystal fiber. A pump pulse first set up the Raman coherence, creating a refractive index grating in the gas that travels at the group velocity of the pump pulse. Varying the arrival time of a second probe pulse allows high degree of control over its evolution as it propagates along the fiber, in particular soliton self-compression and dispersive wave (DW) emission. In the experiments reported, a DW is emitted at ~300 nm, with a central frequency that oscillates with the pump-probe delay. The results demonstrate that strong Raman coherence created in broadband guiding gas-filled kagomé-PCF can be used to control the dynamics of ultrashort probe pulses, even in difficult-to-access spectral regions such as the deep and vacuum ultraviolet.

physics.optics↗

arXiv2015

Vacuum-UV to IR supercontinuum in hydrogen-filled photonic crystal fiber

Although supercontinuum sources are readily available for the visible and near infrared, and recently also for the mid-IR, many areas of biology, chemistry and physics would benefit greatly from the availability of compact, stable and spectrally bright deep ultraviolet (DUV) and vacuum ultraviolet (VUV) supercontinuum sources. Such sources have however not yet been developed. Here we report the generation of a bright supercontinuum, spanning more than three octaves from 124 nm to beyond 1200 nm, in hydrogen-filled kagomé-style hollow-core photonic crystal fiber (kagomé-PCF). Few-μJ, 30 fs pump pulses at wavelength 805 nm are launched into the fiber, where they undergo self-compression via the Raman-enhanced Kerr effect. Modeling indicates that before reaching a minimum sub-cycle pulse duration of ~1 fs, much less than one period of molecular vibration (8 fs), nonlinear reshaping of the pulse envelope, accentuated by self-steepening and shock formation, creates an ultrashort feature that causes impulsive excitation of long-lived coherent molecular vibrations. These phase-modulate a strong VUV dispersive wave (at 182 nm or 6.8 eV) on the trailing edge of the pulse, further broadening the spectrum into the VUV. The results also show for the first time that kagomé-PCF guides well in the VUV.

physics.optics↗

arXiv2014

Temporal condensed matter physics in gas-filled photonic crystal fibers

Raman effect in gases can generate an extremely long-living wave of coherence that can lead to the establishment of an almost perfect periodic variation of the medium refractive index. We show theoretically and numerically that the equations, regulate the pulse propagation in hollow-core photonic crystal fibers filled by Raman-active gas, are exactly identical to a classical problem in quantum condensed matter physics -- but with the role of space and time reversed -- namely an electron in a periodic potential subject to a constant electric field. We are therefore able to infer the existence of Wannier-Stark ladders, Bloch oscillations, and Zener tunneling, phenomena that are normally associated with condensed matter physics only, now realized with purely optical means in the temporal domain.

physics.optics↗