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Federico Garcia-Gaitan

Publications and source records attributed to Federico Garcia-Gaitan.

8 recordsLinked to original sources

Long-range and steady-state entanglement of driven-dissipative nitrogen vacancy centers using microwaves as a drive and synthetic antiferromagnet as a dissipator

The search for optimal schemes and dissipative environments for mediating long-range entanglement between two distant nitrogen-vacancy centers (NVCs) in diamond is the subject of ongoing vigorous efforts due to potential applications of such microscopic solid-state qubits in quantum sensing and quantum computing. However, stabilizing entanglement of NVCs into steady-state poses a significant challenge, typically requiring tuning the environment into a {\em nonequilibrium} state. Here we microscopically derive a Lindblad quantum master equation for a system of two driven-dissipative NVCs, where the drive is microwave radiation and dissipation is provided by a single magnetic bath that is kept in {\em equilibrium}. This equation allows us to predict precise conditions for long-range and steady-state entanglement of NVCs, while it also suggests synthetic antiferromagnet as an optimal choice for a dissipative environment. By using realistic parameters from available experiments, we estimate steady-state concurrence reaching $\mathcal{C}\simeq 0.28$ for two NVCs separated by $\sim 100 \: \mathrm{nm}$.

cond-mat.mes-hall↗

Fate of entanglement in open quantum spin liquid: Time evolution of its genuine multipartite negativity upon sudden coupling to a dissipative bosonic environment

Many-body entanglement properties of quantum spin liquids (QSLs), persisting at arbitrarily long distances, have been intensely explored over the past two decades, but mostly for QSLs viewed as {\em closed} quantum systems. However, in experiments and potential quantum computing applications, candidate materials for this exotic phase of quantum matter will always interact with a dissipative environment, such as the one generated by bosonic quasiparticles in solids at finite temperature. Here we investigate both the {\em stability} and {\em spatial distribution} of entanglement for the Kitaev model of QSL, which is made {\em open} by its sudden coupling to an infinite bosonic bath of Caldeira-Leggett type and then time-evolved in both Markovian and non-Markovian regimes. From the time-dependent density matrix of QSL subregions, we extract genuine multipartite negativity (GMN), quantum Fisher information, spin-spin correlators, and the expectation value (EV) of the Wilson loop operator. In particular, time dependence of GMN offers the most penetrating insights: ({\em i}) in the Markovian regime, it remains nonzero only in hexagonal loopy subregions of QSL (as also discovered very recently for closed QSLs), eventually vanishing on the same timescale on which the EV of the Wilson loop operator vanishes; ({\em ii}) in the non-Markovian regime with pronounced memory effects, surprisingly, GMN remains nonzero up to much higher temperatures while also remaining zero in non-loopy subregions. In addition, the non-Markovian dynamics generates emergent interactions between spins, thereby opening avenues for tailoring properties of QSL via engineering of dissipation.

cond-mat.str-el↗

FermiLink: A Unified Agent Framework for Multidomain Autonomous Scientific Simulations

Artificial-intelligence (AI) agent frameworks have been developed for autonomous scientific simulations, but most current agent frameworks are tailored to a single or a small set of software packages. Herein, FermiLink, a unified and extensible open-source agent framework is introduced for multidomain scientific simulations. Its key design principle is the separation of package knowledge bases from simulation workflows, so that simulation workflows in FermiLink, from figure-level simulations to full-paper-level research on high-performance computing clusters, operate uniformly among supported packages via a four-layer progressive disclosure mechanism. Using OpenAI Codex as the agent provider, the capabilities of FermiLink are demonstrated across approximately 50 scientific software packages spanning nine research domains from physics to engineering. Systematic benchmarks on 132 real-world figure-level reproduction tasks with 44 packages show that FermiLink reproduces 74 (56.1%) of published figures with simulations, among which 30 achieve high-fidelity agreement and 35 reach qualitative agreement with the target figures. A smaller set of human expert-guided reproduction benchmarks with 10 packages further highlights the importance of expert insights for improving the simulation fidelity. Beyond reproduction, a single-blinded study demonstrates that FermiLink can produce research-grade results on unpublished polariton physics problems when provided with sufficiently detailed research objectives and source code, even in the absence of external documentation or tutorials. Overall, FermiLink provides a scalable research infrastructure that may accelerate the path from scientific questions to computational results across diverse domains.

physics.chem-ph↗

Schwinger-Keldysh non-perturbative field theory of open quantum systems beyond the Markovian regime: Application to spin-boson and spin-chain-boson models

We develop a unified framework for open quantum systems composed of many mutually interacting quantum spins, or any isomorphic systems like qubits and qudits, surrounded by one or more independent bosonic baths. Our framework, based on Schwinger-Keldysh field theory (SKFT), can handle arbitrary spin value S, dimensionality of space, and geometry, while being applicable to a large parameter space for system and bath or their coupling. It can probe regimes in which non-Markovian dynamics and nonperturbative effects pose formidable challenges for other state-of-the-art theoretical methods. This is achieved by working with the two-particle irreducible (2PI) effective action, which resums classes of Feynman diagrams of SKFT to an infinite order. Furthermore, such diagrams are generated via an expansion in 1/N, where N is the number of Schwinger bosons we employ to map spin operators onto canonically commuting ones, rather than via conventional expansion in system-bath coupling constant. We carefully benchmark our SKFT+2PI-computed results vs. numerically (quasi)exact ones from tensor network calculations applied to the archetypical spin-boson model where both methodologies are applicable. Additionally, we demonstrate the capability of SKFT+2PI to handle a much more complex spin-chain-boson model with multiple baths interacting with each spin where no benchmark from other methods is available at present. The favorable numerical cost of solving integro-differential equations produced by the SKFT+2PI framework with an increasing number of spins and time steps makes it a promising route for simulating driven-dissipative systems in quantum computing, quantum magnonics, and quantum spintronics.

quant-ph↗

Nonclassical dynamics of Néel vector and magnetization accompanied by THz and high-harmonic radiation from ultrafast-light-driven NiO antiferromagnet insulator

Ultrafast-light-driven strongly correlated antiferromagnetic insulators, such as prototypical NiO with large energy gap 4 eV, have recently attracted experimental attention using either above-gap [K. Gillmeister et al., Nat. Commun. 11, 4095 (2020)] or subgap [H. Qiu et al., Nat. Phys. 17, 388 (2021)] energy photons that are of fundamental interest in far-from-equilibrium quantum matter or spintronic applications, respectively. In the latter context, emission of THz radiation is also observed from NiO/Pt bilayers, where heavy metal (HM) Pt introduces strong spin-orbit coupling (SOC). However, microscopic mechanisms of such emission remain obscure because spintronic THz emitters have been amply studied using FM/HM (FM-ferromagnetic metal of conventional type) bilayers, where ultrafast demagnetization takes place and is directly related to THz emission. Conversely, in NiO total magnetization is zero prior to the fs laser pulse (fsLP) application. Here we employ the two-orbital Hubbard-Hund-Heisenberg model and study, via numerically exact nonequilibrium quantum many-body methods, the dynamics of its Neel vector and nonequilibrium magnetization. Additionally, we compute electromagnetic radiation by both time-dependent magnetization and local charge currents arising in either plain NiO or NiO with proximity SOC introduced by HM layer. Our analysis reveals nonclassical dynamics of Neel vector and nonequilibrium magnetization, changing only in length while not rotating, where the former is substantially reduced only in the case above-gap fsLP. In the plain NiO case, THz radiation of interest to applications is insignificant, but adding SOC enhances both current and magnetic dipole contributions to it. Above THz range, we find integer high-harmonic generation, as well as unusual noninteger harmonics for above-gap fsLP pump.

cond-mat.str-el↗

Magnon spectrum of altermagnets beyond linear spin wave theory: Magnon-magnon interactions via time-dependent matrix product states vs. atomistic spin dynamics

The energy-momentum dispersion of magnons, as collective low-energy excitations of magnetic material, is computed from an effective quantum spin Hamiltonian but simplified via linearized Holstein-Primakoff transformations to describe noninteracting magnons. The dispersion produced by such linear spin wave theory (LSWT) is then plotted as ``sharp bands'' of infinitely long-lived quasiparticles. However, magnons are prone to many-body interactions with other quasiparticles -- such as electrons, phonons or other magnons -- which can lead to shifting (i.e., band renormalization) and broadening of ``sharp bands'' as the signature of finite quasiparticle lifetime. The magnon-magnon interactions can be particularly important in antiferromagnets (AFs), and, therefore, possibly in newly classified altermagnets sharing many features of collinear AFs. Here, we employ nonperturbative quantum many-body calculations, via time-dependent matrix product states (TDMPS), to obtain magnon spectral function for RuO$_2$ altermagnet whose effective quantum spin Hamiltonian is put onto 4-leg cylinder. Its upper band is shifted away from upper ``sharp band'' of LSWT, as well as broadened, which is explained as the consequence of {\em hybridization} of the latter with three-magnon continuum. This implies that two-magnon Raman scattering spectra {\em cannot} be computed from LSWT bands, which offers a litmus test for the relevance of magnon-magnon interactions. Finally, we employ atomistic spin dynamics (ASD) simulations, based on classical Landau-Lifshitz-Gilbert (LLG) equation, to obtain magnon spectrum at finite temperature and/or at a fraction of the cost of TDMPS calculations. Despite including magnon-magnon interactions via nonlinearity of LLG equation, ASD simulations {\em cannot} match the TDMPS-computed magnon spectrum, thereby signaling {\em nonclassical} effects harbored by AFs and altermagnets.

cond-mat.str-el↗

Electric polarization induced by magnons and magnon Nernst effects

Magnons offer a promising path toward energy-efficient information transmission and the development of next-generation classical and quantum computing technologies. However, methods to efficiently excite, manipulate, and detect magnons remain a critical need. Here, we show that magnons, despite their charge-neutrality, can induce electric polarization as a result of both their spin and orbital moments. We demonstrate this by calculating the electric polarization induced by magnons in two-dimensional (2D) honeycomb antiferromagnets. The electric polarization becomes finite when the Dzyaloshinskii-Moriya Interaction (DMI) is present and its magnitude can be increased by symmetries of the system. We illustrate this by computing and comparing the electric polarizations induced by the magnon Nernst effects in 2D materials with Néel and Zigzag ordering. Our findings show that in the Zigzag order, where the effect is dominated by the magnon orbital moment, the induced electric polarization is approximately three orders of magnitude greater than in the Néel phase. These findings reveal that electric fields could enable both detection and manipulation of magnons under certain conditions by leveraging their spin and orbital angular moment. They also suggest that the discovery or engineering of materials with substantial magnon orbital moments could lead to more practical use of magnons for future computing and information transmission device applications.

cond-mat.mes-hall↗

Fate of entanglement in magnetism under Lindbladian or non-Markovian dynamics and conditions for their transition to Landau-Lifshitz-Gilbert classical dynamics

It is commonly assumed in spintronics and magnonics that localized spins within antiferromagnets are in the Néel ground state (GS), as well as that such state evolves, when pushed out of equilibrium by current or external fields, according to the Landau-Lifshitz-Gilbert (LLG) equation viewing localized spins as classical vectors of fixed length. On the other hand, the true GS of antiferromagnets is highly entangled, as confirmed by very recent neutron scattering experiments witnessing their entanglement. Although GS of ferromagnets is always unentangled, their magnonic low-energy excitation are superpositions of many-body spin states and, therefore, entangled. In this study, we initialize quantum Heisenberg ferro- or antiferromagnetic chains hosing localized spins $S=1/2$, $S=1$ or $S=5/2$ into unentangled pure state and then evolve them by quantum master equations (QMEs) of Lindblad or non-Markovian type, derived by coupling localized spins to a bosonic bath (such as due to phonons) or by using additional ``reaction coordinate'' in the latter case. The time evolution is initiated by applying an external magnetic field, and entanglement of time-evolving {\em mixed} quantum states is monitored by computing its logarithmic negativity. We find that non-Markovian dynamics maintains some degree of entanglement, which shrinks the length of the vector of spin expectation values, thereby making the LLG equation inapplicable. Conversely, Lindbladian (i.e., Markovian) dynamics ensures that entanglement goes to zero, thereby enabling quantum-to-classical (i.e., to LLG) transition in all cases -- $S=1/2$, $S=1$ and $S=5/2$ ferromagnet or $S=5/2$ antiferromagnet -- {\em except} for $S=1/2$ and $S=1$ antiferromagnet. We also investigate the stability of entangled antiferromagnetic GS upon suddenly coupling it to the bosonic bath.

cond-mat.str-el↗