arXiv subjects

Federico Paolucci

Publications and source records attributed to Federico Paolucci.

At least 19 recordsLinked to original sources

arXiv2026

Strong nonlinear thermoelectricity generation and close-to-Carnot efficient heat engines in Superconductor-Insulator-2D electron gas junctions

We propose and theoretically analyse a novel Superconductor-Insulator-2D electron gas tunnel junction (SI2DEG) that strongly and efficiently generates thermoelectricity via a nonlinear mechanism. By varying the position of the electrochemical potential of the 2DEG, the SI2DEG junction shows different thermoelectric generation regimes with performance exceeding state-of-the-art tunnel systems. Indeed, the generated Seebeck potential can reach $6.75Δ_0/e$ with a nonlinear Seebeck coefficient as high as $\mathcal{S}=5\,Δ_0/e{\rm K}$. When operated as a quantum heat engine, the system efficiency gets very close to the Carnot limit with a maximum value $η=0.92η_C$ with a non-negligible power output. The SI2DEG junction also shows peculiar features such as bidirectional cooling controlled by the potential bias and bistability of the thermoelectric generation. These features, together with its strong temperature response, make the SI2DEG system an interesting general platform for quantum science and technology applications, such as quantum thermodynamics, ultrasensitive cosmology and dark-matter detection, and qubit refrigeration.

cond-mat.mes-hall↗

arXiv2026

Graphene-Insulator-Superconductor junctions as thermoelectric bolometers

We design a superconducting thermoelectric bolometer made of a Graphene-Insulator-Superconductor tunnel junction. Our detector has the advantage of being passive, as it directly transduces input power to a voltage without the need to modulate an external bias. We characterize the device via numerical simulation of the full nonlinear thermal dynamical model of the junction, considering heating of both sides of the junction. While estimating noise contributions, we found novel expressions due to the temperatures of both sides being different than the bath temperature. Numerical simulations show a Noise Equivalent Power ${\rm NEP}\sim 4\times 10^{-17}\,{\rm W}/\sqrt{\rm Hz}$ for an input power of $\sim10^{-16}\,{\rm W}$, a response time of $τ_{th}\sim 200\, {\rm ns}$ and an integration time to obtain a Signal-to-Noise Ratio ${\rm SNR}=1$ of $τ_{\rm SNR=1}\sim 100\,μ{\rm s}$ for an input power $\sim 10^{-13}\,{\rm W}$. Therefore, the device shows promise for large-array cosmological experiment applications, also considering its advantages for fabrication and heat budget.

cond-mat.mes-hall↗

arXiv2025

Active electron cooling of graphene

In the emergent field of quantum technology, the ability to manage heat at the nanoscale and in cryogenic conditions is crucial for enhancing device performance in terms of noise, coherence, and sensitivity. Here, we demonstrate the active cooling and refrigeration of the electron gas in a graphene thermal transistor, by taking advantage of nanoscale superconductive tunnel contacts able to pump or extract heat directly from the electrons in the device. Our prototypes achieved a top cooling of electrons in graphene of about 15 mK at a bath temperature of about 450 mK, demonstrating the viability of the proposed device architecture. Our experimental findings are backed by a detailed thermal model that accurately replicated the observed device behavior. Alternative cooling schemes and perspectives are discussed in light of the reported results. Finally, our graphene thermal transistor could find application in superconducting hybrid quantum technologies.

cond-mat.mes-hall↗

arXiv2025

Out-of-equilibrium nonlinear model of thermoelectricity in superconducting tunnel junctions

Thermoelectricity in superconducting tunnel junctions has always been studied under the hypothesis of equilibrium between the cold side and the thermal bath, usually in the linear regime. We define a more complete out-of-equilibrium nonlinear numerical model that reduces to the equilibrium linear model in the low-power limit. We find that the linear model does not correctly describe the behavior of superconducting tunnel junctions for parameters that are reasonable in practical experimental setups. Subsequently, we present the qualitative and quantitative differences between the models, discovering that for high power, the junction saturates and then inverts its behavior. Finally, we also clarify the difference between linear and nonlinear thermoelectricity and devise a new criterion to find nonlinear thermoelectricity in the parameter space.

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arXiv2025

Electrostatic field-driven supercurrent suppression in ionic-gated metallic Josephson nanotransistors

Recent experiments have shown the possibility of tuning the transport properties of metallic nanosized superconductors through a gate voltage. These results renewed the longstanding debate on the interaction between electrostatic fields and superconductivity. Indeed, different works suggested competing mechanisms as the cause of the effect: an unconventional electric field-effect or quasiparticle injection. Here, we provide conclusive evidence for the electrostatic-field-driven control of the supercurrent in metallic nanosized superconductors, by realizing ionic-gated superconducting field-effect nanotransistors (ISFETs) where electron injection is impossible. Our Nb ISFETs show giant suppression of the superconducting critical current of up to 45%. Moreover, the bipolar supercurrent suppression observed in different ISFETs, together with invariant critical temperature and normal-state resistance, also excludes conventional charge accumulation/depletion. Therefore, the microscopic explanation of this effect calls upon a novel theory able to describe the nontrivial interaction of static electric fields with conventional superconductivity.

cond-mat.supr-con↗

arXiv2025

Bipolar Thermoelectric Josephson Engine

Thermoelectric effects in metals are typically small due to the nearly-perfect particle-hole (PH) symmetry around their Fermi surface [1, 2]. Despite being initially considered paradoxical [3], thermophase effects [4-8] and linear thermoelectricity [9] in superconducting systems were identified only when PH symmetry is explicitly broken [10-14]. Here, we experimentally demonstrate that a superconducting tunnel junction can develop a very large bipolar thermoelectric effect in the presence of a nonlinear thermal gradient thanks to spontaneous PH symmetry breaking [15]. Our junctions show a maximum thermovoltage of $\pm150\; μ$ V at $\pm650$ mK, directly proportional to the superconducting gap. Notably, the corresponding Seebeck coefficient of $\pm300\; μ$V/K is roughly $10^5$ times larger than the one expected for a normal metal at the same temperature [16, 17]. Moreover, by integrating our junctions into a Josephson interferometer, we realize a bipolar thermoelectric Josephson engine (BTJE) [18] with phase-coherent thermopower control [19]. When connected to a generic load, the BTJE generates a phase-tunable electric power up to about 140 mW/m$^2$ at subKelvin temperatures. In addition, our device implements the prototype for a persistent thermoelectric memory cell, written or erased by current injection [20]. We expect that our findings will trigger thermoelectricity in PH symmetric systems, and will lead to a number of groundbreaking applications in superconducting electronics [21], cutting-edge quantum technologies [22-24] and sensing [25].

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arXiv2024

Tailoring coherent charge transport in graphene by deterministic defect generation

Harnessing the wave-nature of charge carriers in solid state devices, electron optics investigates and exploits coherent phenomena, in analogy with optics and photonics. Typically, this requires complex electronic devices leveraging macroscopically coherent charge transport in two-dimensional electron gases and superconductors. Here, collective coherent effects are induced in a simple counterintuitive architecture by defect engineering. Deterministically introduced lattice defects in graphene enable the phase coherent charge transport by playing the role of potential barriers, instead of scattering centres as conventionally considered. Thus, graphene preserves its quasi-ballistic quantum transport and can support phase-matched charge carrier waves. Based on this approach, multiple electronic Fabry-Pèrot cavities are formed by creating periodically alternating defective and pristine nano-stripes through low energy electron-beam irradiation. Indeed, defective stripes behave as partially reflecting mirrors and resonantly confine the charge carrier waves within the pristine areas, giving rise to Fabry-Pèrot resonant modes. These modes experimentally manifest as sheet resistance oscillations, as also confirmed by Landauer-Büttiker simulations. Moreover, these coherent phenomena survive up to 30 K for both polarities of charge carriers, contrarily to traditional monopolar electrostatically created Fabry-Pèrot interferometers. Our study positions defective graphene as an innovative platform for coherent electronic devices, with potential applications in nano and quantum technologies.

cond-mat.mes-hall↗

arXiv2024

Transition Edge Sensors: Physics and Applications

Transition Edge Sensors (TESs) are amongst the most sensitive cryogenic detectors and can be easily optimized for the detection of massive particles or photons ranging from X-rays all the way down to millimetre radiation. Furthermore, TESs exhibit unmatched energy resolution while being easily frequency domain multiplexed in arrays of several hundred pixels. Such great performance, along with rather simple and sturdy readout and amplification chains make TESs extremely compelling for applications in many fields of scientific endeavour. While the first part of this article is an in-depth discussion on the working principles of Transition Edge Sensors, the remainder of this review article focuses on the applications of Transition Edge Sensors in advanced scientific instrumentation serving as an accessible and thorough list of possible starting points for more comprehensive literature research.

physics.ins-det↗

arXiv2024

Side-gate modulation of supercurrent in InSb nanoflag-based Josephson junctions

InSb nanoflags, due to their intrinsic spin-orbit interactions, are an interesting platform in the study of planar Josephson junctions. Ballistic transport, combined with high transparency of the superconductor/semiconductor interfaces, was reported to lead to interesting phenomena such as the Josephson diode effect. The versatility offered by the planar geometry can be exploited to manipulate both carrier concentration and spin-orbit strength by electrical means. Here we present experimental results on InSb nanoflag-based Josephson junctions fabricated with side-gates placed in close proximity to the junction. We show that side-gates can efficiently modulate the current through the junction, both in the dissipative and in the dissipation-less regimes, similarly to what obtained with a conventional back-gate. Furthermore, the side-gates can be used to influence the Fraunhofer interference pattern induced by the presence of an external out-of-plane magnetic field.

cond-mat.supr-con↗

arXiv2024

Design and simulation of a transmon qubit chip for Axion detection

Quantum Sensing is a rapidly expanding research field that finds one of its applications in Fundamental Physics, as the search for Dark Matter. Devices based on superconducting qubits have already been successfully applied in detecting few-GHz single photons via Quantum Non-Demolition measurement (QND). This technique allows us to perform repeatable measurements, bringing remarkable sensitivity improvements and dark count rate suppression in experiments based on high-precision microwave photon detection, such as for Axions and Dark Photons search. In this context, the INFN Qub-IT project goal is to realize an itinerant single-photon counter based on superconducting qubits that will exploit QND for enhancing Axion search experiments. In this study, we present Qub-IT's status towards the realization of its first superconducting qubit device, illustrating design and simulation procedures and the characterization of fabricated Coplanar Waveguide Resonators (CPWs) for readout. We match target qubit parameters and assess a few-percent level agreement between lumped and distributed element simulation models. We reach a maximum internal quality factor of 9.2x10^5 for -92 dBm on-chip readout power.

quant-ph↗

arXiv2023

Thermoelectric single-photon detection through superconducting tunnel junctions

Bipolar thermoelectricity in tunnel junctions between superconductors of different energy gap has been recently predicted and experimentally demonstrated. This effect showed thermovoltages up to $\pm150\;μ$V at milliKelvin temperatures. Thus, superconducting tunnel junctions can be exploited to realize a passive single-photon thermoelectric detector $TED$ operating in the broadband range 15 GHz - 50 PHz. In particular, this detector is expected to show a signal-to-noise ratio of about 15 down to $ν=50$ GHz and a operating window of more than 4 decades. Therefore, the $TED$ might find applications in quantum computing, telecommunications, optoelectronics, spectroscopy and astro-particle physics.

cond-mat.mes-hall↗

arXiv2023

Optical grade bromide-based thin film electrolytes

Controlling the charge density in low-dimensional materials with an electrostatic potential is a powerful tool to explore and influence their electronic and optical properties. Conventional solid gates impose strict geometrical constraints to the devices and often absorb electromagnetic radiation in the infrared (IR) region. A powerful alternative is ionic liquid (IL) gating. This technique only needs a metallic electrode in contact with the IL and the highest achievable electric field is limited by the electrochemical interactions of the IL with the environment. Despite the excellent gating properties, a large number of ILs is hardly exploitable for optical experiments in the mid-IR region, because they typically suffer from low optical transparency and degradation in ambient conditions. Here, we report the realization of two electrolytes based on bromide ILs dissolved in polymethyl methacrylate (PMMA). We demonstrate that such electrolytes can induce state-of-the-art charge densities as high as $20\times10^{15}\ \mathrm{cm^{-2}}$. Thanks to the low water absorption of PMMA, they work both in vacuum and in ambient atmosphere after a simple vacuum curing. Furthermore, our electrolytes can be spin coated into flat thin films with optical transparency in the range from 600 cm$^{-1}$ to 4000 cm$^{-1}$. Thanks to these properties, the electrolytes are excellent candidates to fill the gap as versatile gating layers for electronic and mid-IR optoelectronic devices.

cond-mat.mes-hall↗

arXiv2023

Non-local superconducting single-photon detector

We present and theoretically analyse the performance of an innovative non-local superconducting single-photon detector. The device operates thanks to the energy-to-phase conversion mechanism, where the energy of the absorbed single-photon is transformed in a variation of the superconducting phase. To this scope, the detector is designed in the form of a double-loop superconductor/normal metal/superconductors (SNS) Josephson interferometer, where the detection occurs in a long SNS junction and the read-out is operated by a short SNS junction. The variation of the superconducting phase across the read-out junction is measured by recording the quasiparticle current flowing through a tunnel coupled superconducting probe. By exploiting realistic geometry and materials, the detector is able to reveal single-photons of frequency down to 10 GHz when operated at 10 mK. Furthermore, the device provides value of signal-to-noise ratio up 10^4 in the range 10 GHz-10 THz by selecting the magnetic flux and the bias voltage. This device can find direct applications as single-photon detector in both basic science and quantum technology, while the energy-to-phase conversion mechanism can be at the basis of non-local read-out and memory architectures for superconducting qubits.

cond-mat.mes-hall↗

arXiv2023

A highly-sensitive broadband superconducting thermoelectric single-photon detector

We propose a passive single-photon detector based on the bipolar thermoelectric effect occurring in tunnel junctions between two different superconductors thanks to spontaneous electron-hole symmetry breaking. Our thermoelectric detector (TED) converts a finite temperature difference caused by the absorption of a single photon into an open circuit thermovoltage. Designed with feasible parameters, our TED is able to reveal single-photons of frequency ranging from about 15 GHz to about 150 PHz depending on the chosen design and materials. In particular, this detector is expected to show values of signal-to-noise ratio SNR about 15 at ν = 50 GHz when operated at a temperature of 10 mK. Interestingly, this device can be viewed as a digital single-photon detector, since it generates an almost constant voltage VS for the full operation energies. Our TED can reveal single photons in a frequency range wider than 4 decades with the possibility to discern the energy of the incident photon by measuring the time persistence of the generated thermovoltage. Its broadband operation suggests that our TED could find practical applications in several fields of quantum science and technology, such as quantum computing, telecommunications, optoelectronics, THz spectroscopy and astro-particle physics.

cond-mat.mes-hall↗

arXiv2022

A gate- and flux-controlled supercurrent diode

Non-reciprocal charge transport in supercurrent diodes (SDs) polarized growing interest in the last few years for its potential applications in superconducting electronics (SCE). So far, SD effects have been reported in complex hybrid superconductor/semiconductor structures or metallic systems subject to moderate magnetic fields, thus showing a limited potentiality for practical applications in SCE. Here, we report the design and the realization of a monolithic SD by exploiting a Dayem bridge-based superconducting quantum interference device (SQUID). Our structure allows reaching rectification efficiencies ($η$) up to about 6%. Moreover, the absolute value and the polarity of $η$ can be selected on demand by the modulation of an external magnetic flux or by a gate voltage, thereby guaranteeing high versatility and improved switching speed. Furthermore, our SD operates in a wide range of temperatures up to about the 70% of the superconducting critical temperature of the titanium film composing the interferometer. Our SD can find extended applications in SCE by operating in synergy with widespread superconducting technologies, such as nanocryotrons, rapid single flux quanta (RSFQs) and memories.

cond-mat.mes-hall↗

arXiv2022

Phase-control of bipolar thermoelectricity in Josephson tunnel junctions

Not so long ago, thermoelectricity in superconductors was believed to be possible only by breaking explicitly the particle-hole symmetry. Recently, it has been theoretically predicted that a superconducting tunnel junction can develop bipolar thermoelectric phenomena in the presence of a large thermal gradient owing to non-equilibrium spontaneous PH symmetry breaking. The experimental realization of the first thermoelectric Josephson engine then followed. Here, we give a more extended discussion and focus on the impact of the Josephson contribution on thermoelectricity modulating the Cooper pairs transport in a double-loop SQUID. When the Cooper pairs current prevails on the quasiparticle one, the Josephson contribution short-circuits the junction thereby screening the thermoelectric effect. We demonstrate that the thermoelectric generation due to the pure quasiparticle transport is phase-independent, once Josephson contribution is appropriately removed from the net current measured. At the same time, we investigate an additional metastable state at V\simeq0 determined by the presence of the Josephson coupling, which peculiarly modifies the hysteretic behavior of our thermoelectric engine realized. At the end, we also discuss how the current-voltage characteristics are affected by the presence of multiple thermoelectric elements, which improve the generated output power.

cond-mat.supr-con↗

arXiv2022

Thermal superconducting quantum interference proximity transistor

Superconductors are known to be excellent thermal insulators at low temperature owing to the presence of the energy gap in their density of states (DOS). In this context, the superconducting \textit{proximity effect} allows to tune the local DOS of a metallic wire by controlling the phase bias ($φ$) imposed across it. As a result, the wire thermal conductance can be tuned over several orders of magnitude by phase manipulation. Despite strong implications in nanoscale heat management, experimental proofs of phase-driven control of thermal transport in superconducting proximitized nanostructures are still very limited. Here, we report the experimental demonstration of efficient heat current control by phase tuning the superconducting proximity effect. This is achieved by exploiting the magnetic flux-driven manipulation of the DOS of a quasi one-dimensional aluminum nanowire forming a weal-link embedded in a superconducting ring. Our thermal superconducting quantum interference transistor (T-SQUIPT) shows temperature modulations up to $\sim 16$ mK yielding a temperature-to-flux transfer function as large as $\sim 60$ mK/$Φ_0$. Yet, phase-slip transitions occurring in the nanowire Josephson junction induce a hysteretic dependence of its local DOS on the direction of the applied magnetic field. Thus, we also prove the operation of the T-SQUIPT as a phase-tunable \textit{thermal memory}, where the information is encoded in the temperature of the metallic mesoscopic island. Besides their relevance in quantum physics, our results are pivotal for the design of innovative coherent caloritronics devices such as heat valves and temperature amplifiers suitable for thermal logic architectures.

cond-mat.mes-hall↗

arXiv2021

Spontaneous symmetry breaking-induced thermospin effect in superconducting tunnel junctions

We discuss the charge and the spin tunneling currents between two Bardeen-Cooper-Schrieffer (BCS) superconductors, where one density of states is spin-split. In the presence of a large temperature bias across the junction, we predict the generation of a spin-polarized thermoelectric current. This thermo-spin effect is the result of a spontaneous particle-hole symmetry breaking in the absence of a polarizing tunnel barrier. The two spin components, which move in opposite directions, generate a spin current larger than the purely polarized case when the thermo-active component dominates over the dissipative one.

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