arXiv subjects

Feiyu Li

Publications and source records attributed to Feiyu Li.

At least 19 recordsLinked to original sources

arXiv2026

Particle-in-Cell Simulation of the Parametric Decay Instability of Alfv\'en Waves with Absorbing Boundary Conditions

The Alfv\'en wave parametric decay instability (PDI) facilitates energy transfer, plasma heating, and turbulence generation in space, astrophysical, and fusion plasmas. Most simulation studies of Alfv\'en wave PDI have focused on kinetic ions under periodic boundary conditions. Here, we present fully kinetic one-dimensional simulations (perpendicular wave-vector $k_\perp=0$) of the Alfv\'en wave PDI at low plasma beta using absorbing boundary conditions for the waves to understand the energy partition in an open system. For $\beta=5\times 10^{-4}$ and a normalized wave amplitude $\frac{\delta B}{B_0}=0.01$, nearly 92\% of the pump wave energy is transferred to the backward-propagating child Alfv\'en wave, and the remaining energy is partitioned between electrons ($\sim 1$-$2\%$) and ions ($\sim 6$-$7\%$). In the parameter regime considered, the ion and electron heating appears only when the PDI has sufficiently developed, and their rates are approximately twice the linear PDI growth rate, which roughly corresponds to the quadratic dependence of energy on the fluctuation amplitude. Furthermore, we find a qualitative agreement between theoretical and numerical growth rates over a range of plasma and wave parameters. This work establishes critical steps for future extension to finite $k_\perp$ waves in high dimensions, where stronger electron heating may be induced.

physics.plasm-ph↗

arXiv2026

Non-Local and Non-Markovian Effects of a Microscopic Two-Level Defect in Superconducting Quantum Circuits

Microscopic two-level systems (TLS) -- ubiquitous atomic-scale defects in solid-state quantum devices -- are a dominant source of qubit decoherence, yet their role is often considered local and short-memoried. Here, we report the observation of a coherent TLS that couples simultaneously to two spatially distant superconducting qubits. The TLS is identified to reside within the tunable coupler linking the qubits, enabling controllability of the TLS-qubit coupling strength via coupler frequency -- a capability absent in earlier studies. This tunability allows us to systematically probe how TLS distorts qubit dynamics, revisiting the decoherence model in the presence of non-Markovian TLS dephasing noise. This is corroborated by the reconstructed $1/f$ noise spectrum of TLS frequency fluctuation spanning more than ten orders of magnitude (0.1\,mHz -- 1\,MHz) that reveals discrete fluctuator signatures. Quantum process tomography further unveils TLS-induced correlated qubit dynamics, highlighting the long-lived TLS as an effective source of non-Markovianity. Our findings expose a previously overlooked interaction mechanism in scalable quantum architectures: defects embedded in coupling elements can simultaneously affect multiple qubits with variable impact. Beyond immediate implications for system characterization and calibration, this situation provides a powerful testbed for studying defect-driven quantum dynamics, refining error suppression strategies, and advancing architecture design for scalable quantum technologies.

quant-ph↗

arXiv2026

On estimating superconducting shielding volume fraction from susceptibility in pressurized Ruddlesden-Popper nickelates: Response to arXiv:2602.19282

In a recent preprint (arXiv:2602.19282) [1], the authors questioned the procedure we used to evaluate the demagnetization-corrected superconducting shielding volume fraction in pressurized Ruddlesden-Popper nickelates [2-5]. They further claimed that this methodology has neither been derived nor used previously, and they proposed an alternative normalization scheme. Here we clarify that our evaluation follows directly from the standard magnetostatic self-consistency relation for finite samples and has been widely adopted in the superconductivity literature for decades. We also demonstrate that the discrepancies claimed in Ref. [1] stem from a fundamental flaw in their approach, namely, the assumption that the measured diamagnetic moment is linearly proportional to the superconducting shielding volume fraction in the presence of a finite demagnetization factor N. This assumption is not valid for strongly demagnetized, thin disk-like specimens, where the internal field and the measured moment are coupled self-consistently through the demagnetizing field.

cond-mat.supr-con↗

arXiv2026

Reply to "Threefold error in the reported zero-field cooled magnetic moment of single crystal $La_2SmNi_2O_7$ (arXiv: 2602.23240)"

We respond to the critique by Aleksandr V. Korolev and Evgeny F. Talantsev on the superconducting phase fraction ($f$) calculations in Li et al. Nature 649, 871-878 (2026). First, the weak upturn in the low-temperature tail of our data has been confirmed to originate from the background, and the paramagnetic Meissner effect is absent in our case; thus, field-cooled (FC) data can be used for superconducting phase fraction calculations. Second, demagnetization effect must be calculated based on the actual measured moment as a function of $f$, which has been well-established and routinely employed in the superconductivity community. In contrast, Korolev and Talantsev treated the demagnetization field as a constant; thus, their calculation underestimates $f$ by a factor of $(1-N\chi_{meas})(1-N)$. This factor is close to 1/3, given $N$ = 0.849, $\chi_{meas}$ = -1.313 in our study, which explains the origin of their deviated result (nearly three times smaller than our results). Third, our sample is a homogeneous high-quality bulk single crystal, evidenced by various techniques, making the existence of multiple discrete superconducting regions highly unlikely. We conclude that the superconducting phase fraction calculations reported in Li et al. Nature 649, 871-878 (2026) are not invalidated by the analyses presented in Korolev et al. arXiv: 2602.23240 (2026).

cond-mat.supr-con↗

arXiv2026

Intertwined Charge and Spin Density Waves in Trilayer Nickelate La$_4$Ni$_3$O$_{10}$ Revealed by $^{139}$La NQR

The discovery of superconducting transitions in pressurized La$_3$Ni$_2$O$_{7}$ and La$_4$Ni$_3$O$_{10}$ has highlighted the pivotal role of density wave (DW) orders in nickelate superconductors. To gain a comprehensive understanding of the superconducting state, it is essential to elucidate the nature of the DW order. In this study, we utilized $^{139}$La nuclear quadrupole resonance (NQR) to investigate the charge density wave (CDW) and spin density wave (SDW) orders in both single-crystal and polycrystalline La$_4$Ni$_3$O$_{10}$. Near $T_{\rm{DW}} \approx 133$ K, an abrupt change in both the linewidth and frequency of the La(2) site in the single-crystal sample provides compelling evidence for a first-order-like phase transition. The pronounced broadening of the NQR lines indicates the incommensurate nature of the DW order. Furthermore, the spin-lattice relaxation rate divided by temperature 1/$T_1$$T$ exhibits a strong enhancement at $T_{\rm{DW}}$, indicating the strong spin fluctuations above the first-order DW transition. These observations suggest an intricate interplay between incommensurate CDW and SDW orders. Our findings offer critical insights into the microscopic mechanisms of the DW state in La$_4$Ni$_3$O$_{10}$ and establish an essential framework for exploring the interplay between DW and superconducting phases in nickelate superconductors.

cond-mat.supr-con↗

arXiv2025

Mitigating Measurement Crosstalk via Pulse Shaping

Quantum error correction protocols require rapid and repeated qubit measurements. While multiplexed readout in superconducting quantum systems improves efficiency, fast probe pulses introduce spectral broadening, leading to signal leakage into neighboring readout resonators. This crosstalk results in qubit dephasing and degraded readout fidelity. Here, we introduce a pulse shaping technique inspired by the derivative removal by adiabatic gate (DRAG) protocol to suppress measurement crosstalk during fast readout. By engineering a spectral notch at neighboring resonator frequencies, the method effectively mitigates spurious signal interference. Our approach integrates seamlessly with existing readout architectures, enabling fast, low-crosstalk multiplexed measurements without additional hardware overhead - a critical advancement for scalable quantum computing.

quant-ph↗

arXiv2025

A novel scheme for measuring the growth of Alfven wave parametric decay instability using counter-propagating waves

The parametric decay instability (PDI) of Alfven waves -- where a pump Alfven wave decays into a backward-propagating child Alfven wave and a forward ion acoustic wave -- is a fundamental nonlinear wave-wave interaction and holds significant implications for space and laboratory plasmas. However, to date there has been no direct experimental measurement of PDI. Here, we propose a novel and experimentally viable scheme to quantify the growth of Alfven wave PDI on a linear device using a large pump Alfven wave and a small counter-propagating seed Alfven wave, with the seed wave frequency tuned to match the backward Alfven wave generated by standard PDI. Using hybrid simulations, we show that energy transfer from the pump to the seed reduces the latter's spatial damping. By comparing seed wave amplitudes with and without the pump wave, this damping reduction can be used as a direct and reliable proxy for PDI growth. The method is validated in our simulations across a range of plasma and wave parameters and agrees well with theoretical predictions. Notably, the scheme exhibits no threshold for PDI excitation and is, in principle, readily implementable under current laboratory conditions. This scheme is a critical step toward solving the challenge of experimentally accessing Alfven wave PDI and provides an elegant method that may be used to validate fundamental theories of parametric instabilities in controlled laboratory settings.

physics.plasm-ph↗

arXiv2025

$La_3Pd_2NaO_9$: A High-Valent Insulating Palladate

A high-valent palladate, $La_3Pd_2NaO_9$, has been synthesized for the first time. Single crystals with dimensions of 20 ${\mu}$m on edge were successfully grown using the flux method at 420 $^o$C and 70 bar oxygen pressure. Energy dispersive spectroscopy (EDS) and inductively coupled plasma mass spectroscopy (ICP) measurements show that the atomic ratio of La: (Pd+Na) is 3: 3 and Pd: Na is 2: 1. X-ray photoelectron spectroscopy (XPS) measurements show that the oxidation state of Pd is dominated by +4. Synchrotron X-ray single-crystal diffraction measurements revealed that this material crystallizes in the monoclinic $P2_1/c$ space group with charge ordering of Na and Pd. Real-space imaging via scanning transmission electron microscopy (STEM) confirmed the crystal structure and revealed excellent sample homogeneity. Electrical resistivity measurements show an insulating behavior. Magnetic measurements show an unexpected paramagnetic behavior, which probably originate from a small fraction of high-spin Pd$^{2+}$ evidenced by XPS. The successful growth of $La_3Pd_2NaO_9$ single crystals with a high-valent oxidation state of Pd offers an approach for exploring interesting palladates, including potential bilayer Ruddlesden-Popper palladates analogous to the high temperature superconducting $La_3Ni_2O_7$.

cond-mat.str-el↗

arXiv2025

PassiveBLE: Towards Fully Commodity-Compatible BLE Backscatter

Bluetooth Low Energy (BLE) backscatter is a promising candidate for battery-free Internet of Things (IoT) applications. Unlike existing commodity-level BLE backscatter systems that only enable one-shot communication through BLE advertising packets, we propose PassiveBLE, a backscatter system that can establish authentic and fully compatible BLE connections on data channels. The key enabling techniques include (i) a synchronization circuit that can wake up tags and activate backscatter communications with symbol-level accuracy to facilitate BLE data packet generation; (ii) a distributed coding scheme that offloads the major encoding and processing burdens from tags to the excitation source while achieving high throughput; (iii) a BLE connection scheduler to enable fully compatible BLE connection interactions, including connection establishment, maintenance and termination for multiple backscatter tags. We prototype PassiveBLE tags with off-the-shelf components and also convert the circuits and control logic into ASIC design sketch, whose power consumptions are 491 uW and 9.9 uW, respectively. Experimental results demonstrate that PassiveBLE achieves a success rate of over 99.9% in establishing commodity BLE connections. PassiveBLE also achieves commodity-compatible BLE communication with a high goodput of up to 974 kbps in LE 2M PHY mode and 532 kbps in LE 1M PHY mode, which is about 63.3 times higher than the previous commodity-level BLE backscatter system in the same mode.

cs.NI↗

arXiv2025

Efficient Implementation of Arbitrary Two-Qubit Gates via Unified Control

The native gate set is fundamental to the performance of quantum devices, as it governs the accuracy of basic quantum operations and dictates the complexity of implementing quantum algorithms. Traditional approaches to extending gate sets often require accessing multiple transitions within an extended Hilbert space, leading to increased control complexity while offering only a limited set of gates. Here, we experimentally demonstrate a unified and highly versatile gate scheme capable of natively generating arbitrary two-qubit gates using only exchange interaction and qubit driving on a superconducting quantum processor, achieving maximum expressivity. Using a state-of-the-art transmon-coupler-transmon architecture, we achieve high fidelities averaging $99.37 \pm 0.07\%$ across a wide range of commonly used two-qubit unitaries. This outstanding performance, combined with reduced complexity, enables precise multipartite entangled state preparation, as demonstrated. To further enhance its applicability, we also show the high-fidelity realization of the unique B gate, which efficiently synthesizes the entire family of two-qubit gates. Our results highlight that fully exploiting the capabilities of a single interaction can yield a comprehensive and highly accurate gate set. With maximum expressivity, gate-time optimality, demonstrated high fidelity, and easy adaptability to other quantum platforms, our unified control scheme paves the way for optimal performance in quantum devices, offering exciting prospects for advancing quantum hardware and algorithm development.

quant-ph↗

arXiv2025

Damage of bilayer structure in La3Ni2O7-d induced by high pO2 annealing

The discovery of superconductivity with onset temperature of ~80 K in pressurized bilayer Ruddlesden-Popper La3Ni2O7-d has attracted much attention. Despite intense research, determination of the exact oxygen content and understanding of the relationship between superconductivity and oxygen content remain a big challenge. Here, we report a systematical study on the structure and physical properties of La3Ni2O7-d polycrystalline powders which were prepared using sol-gel method at ambient pressure and then annealed under various oxygen pressure. We found that high pO2 annealing with slow cooling results in a new phase, which can be modeled using the hybrid single-layer-trilayer La3Ni2O7 or the tetragonal bilayer La3Ni2O7. Scanning transmission electron microscopy (STEM) measurements revealed significant single layers and trilayers after high oxygen pressure annealing, evidencing damage of the bilayer structure. The superconducting transition under high pressure became weak for high pO2 annealed samples, which is consistent with the damage of the bilayer structure. Our results reveal that the bilayer structure is fragile and post-annealing under near atmosphere pressure of oxygen is suitable to maintain bilayer structure and increase oxygen content at the same time.

cond-mat.supr-con↗

arXiv2025

Pyrochlore NaYbO2: A potential Quantum Spin Liquid Candidate

The search for quantum spin liquids (QSL) and chemical doping in such materials to explore superconductivity have continuously attracted intense interest. Here, we report the discovery of a potential QSL candidate, pyrochlore-lattice beta-NaYbO2. Colorless and transparent NaYbO2 single crystals, layered alpha-NaYbO2 (~250 um on edge) and octahedral beta-NaYbO2 (~50 um on edge), were grown for the first time. Synchrotron X-ray single crystal diffraction unambiguously determined that the newfound beta-NaYbO2 belongs to the three-dimensional pyrochlore structure characterized by the R-3m space group, corroborated by synchrotron X-ray and neutron powder diffraction and pair distribution function. Magnetic measurements revealed no long-range magnetic order or spin glass behavior down to 0.4 K with a low boundary spin frustration factor of 17.5, suggesting a potential QSL ground state. Under high magnetic fields, the potential QSL state was broken and spins order. Our findings reveal that NaYbO2 is a fertile playground for studying novel quantum states.

cond-mat.str-el↗

arXiv2025

Bulk superconductivity up to 96 K in pressurized nickelate single crystals

Recently, the Ruddlesden-Popper bilayer nickelate $La_3Ni_2O_7$ has emerged as a superconductor with a transition temperature ($T_c$) of approximately 80 K above 14 GPa (Refs. 1-3). Achieving higher $T_c$ in nickelate superconductors, along with the synthesis of reproducible high-quality single crystals without relying on high-oxygen-pressure growth conditions, remains a significant challenge$^{[4-7]}$. Here we report superconductivity up to 96 K under high pressure in bilayer nickelate single crystals synthesized at ambient pressure. Energy-dispersive spectroscopy, single-crystal X-ray diffraction, nuclear quadrupole resonance and scanning transmission electron microscopy evidenced high crystal quality of the flux-grown $La_2SmNi_2O_{7-{\delta}}$ single crystals. $La_2SmNi_2O_7$ exhibits clear bulk superconductivity, including zero resistivity ($T_{c,max}^{onset}$ = 92 K and $T_{c,max}^{zero}$ = 73 K at 21.6 GPa) and the Meissner effect ($T_c$= 60 K at 20.6 GPa). A low-temperature high-pressure structural study indicates that both monoclinic and tetragonal structures can support superconductivity in this bilayer nickelate. Furthermore, we established a correlation between higher $T_c$ under high pressures and larger in-plane lattice distortion under ambient conditions, corroborated by observing even higher $T_c^{onset}$ of 96 K in $La_{1.57}Sm_{1.43}Ni_2O_{7-{\delta}}$. This study overcomes key limitations in growing nickelate superconductor crystals, resolves the crystal structure in the superconducting state and demonstrates an effective pathway towards achieving higher $T_c$.

cond-mat.supr-con↗

arXiv2025

Signature of superconductivity in pressurized La4Ni3O10-x single crystals grown at ambient pressure

Nickelates have attracted enormous attention since the discovery of high-temperature superconductivity in La3Ni2O7 under high pressure. However, whether superconducting nickelate single crystals can be prepared at ambient pressure remains elusive. Here we report signature of superconductivity in pressurized La4Ni3O10-x single crystals grown from potassium carbonate flux at ambient pressure. Single crystal X-ray diffraction and scanning transmission electron microscopy investigations re-vealed high-quality single crystals with perfect stacking of trilayers. Resistivity measurements indicate that the metal-to-metal transition observed at ambient pressure was suppressed under high pressure, and a sharp drop occurred at ~30 K at 77.9 GPa, consistent with superconductivity in pressurized La4Ni3O10 single crystals grown by the floating zone method at an oxygen pressure of >18 bar. Our results not only provide an important path to prepare high-quality nickelate single crystals but also support superconductivity in nickelates under high pressure, promoting more systematic and in-depth research in this compelling field.

cond-mat.supr-con↗

arXiv2024

Bulk Crystal Growth and Single-Crystal-to-Single-Crystal Phase Transitions in the Averievite CsClCu5V2O10

Quasi-two-dimensional averievites with triangle-kagome-triangle trilayers are of interest due to their rich structural and magnetic transitions and strong spin frustration that are expected to host quantum spin liquid ground state with suitable substitution or doping. Herein, we report growth of bulk single crystals of averievite CsClCu5V2O10 with dimensions of several millimeters on edge in order to (1) address the open question whether the room temperature crystal structure is P-3m1, P-3, P21/c or else, (2) to elucidate the nature of phase transitions, and (3) to study direction-dependent physical properties. Single-crystal-to-single-crystal structural transitions at ~305 K and ~127 K were observed in the averievite CsClCu5V2O10 single crystals. The nature of the transition at ~305 K, which was reported as P-3m1-P21/c transition, was found to be a structural transition from high temperature P-3m1 to low temperature P-3 by combining variable temperature synchrotron X-ray single crystal and high-resolution powder diffraction. In-plane and out-of-plane magnetic susceptibility and heat capacity measurements confirm a first-order transition at 305 K, a structural transition at 127 K and an antiferromagnetic transition at 24 K. These averievites are thus ideal model systems for a deeper understanding of structural transitions and magnetism.

cond-mat.str-el↗

arXiv2024

Cascade of phase transitions and large magnetic anisotropy in a triangle-kagome-triangle trilayer antiferromagnet

Spins in strongly frustrated systems are of intense interest due to the emergence of intriguing quantum states including superconductivity and quantum spin liquid. Herein we report the discovery of cascade of phase transitions and large magnetic anisotropy in the averievite CsClCu5P2O10 single crystals. Under zero field, CsClCu5P2O10 undergoes a first-order structural transition at around 225 K from high temperature centrosymmetric P-3m1 to low temperature noncentrosymmetric P321, followed by an AFM transition at 13.6 K, another structural transition centering at ~3 K, and another AFM transition at ~2.18 K. Based upon magnetic susceptibility and magnetization data with magnetic fields perpendicular to the ab plane, a phase diagram, consisting of a paramagnetic state, two AFM states and four field-induced states including two magnetization plateaus, has been constructed. Our findings demonstrate that the quasi-2D CsClCu5P2O10 exhibits rich structural and metamagnetic transitions and the averievite family is a fertile platform for exploring novel quantum states.

cond-mat.str-el↗

arXiv2024

Multi-Purpose Architecture for Fast Reset and Protective Readout of Superconducting Qubits

The ability to fast reset a qubit state is crucial for quantum information processing. However, to actively reset a qubit requires engineering a pathway to interact with a dissipative bath, which often comes with the cost of reduced qubit protection from the environment. Here, we present a novel multi-purpose architecture that enables fast reset and protection of superconducting qubits during control and readout. In our design, two on-chip diplexers are connected by two transmission lines. The high-pass branch provides a flat passband for convenient allocation of readout resonators above the qubit frequencies, which is preferred for reducing measurement-induced state transitions. In the low-pass branch, we leverage a standing-wave mode below the maximum qubit frequency for a rapid reset. The qubits are located in the common stopband to inhibit dissipation during coherent operations. We demonstrate resetting a transmon qubit from its first excited state to the ground state in 100 ns, achieving a residual population of 2.7%. The reset time may be further shortened to 27 ns by exploiting the coherent population inversion effect. We further extend the technique to resetting the qubit from its second excited state. Our approach promises scalable implementation of fast reset and qubit protection during control and readout, adding to the toolbox of dissipation engineering.

quant-ph↗

arXiv2024

Effects of wave damping and finite perpendicular scale on three-dimensional Alfven wave parametric decay in low-beta plasmas

Shear Alfven wave parametric decay instability (PDI) provides a potential path toward significant wave dissipation and plasma heating. However, fundamental questions regarding how PDI is excited in a realistic three-dimensional (3D) open system and how critically the finite perpendicular wave scale--as found in both laboratory and space plasmas--affects the excitation remain poorly understood. Here, we present the first 3D, open-boundary, hybrid kinetic-fluid simulations of kinetic Alfven wave PDI in low-beta plasmas. Key findings are that the PDI excitation is strongly limited by the wave damping present, including electron-ion collisional damping (represented by a constant resistivity) and geometrical attenuation associated with the finite-scale Alfven wave, and ion Landau damping of the child acoustic wave. The perpendicular wave scale alone, however, plays no discernible role: waves of different perpendicular scales exhibit similar instability growth as long as the magnitude of the parallel ponderomotive force remains unchanged. These findings are corroborated by theoretical analysis and estimates. The new understanding of 3D kinetic Alfvén wave PDI physics is essential for laboratory study of the basic plasma process and may also help evaluate the relevance/role of PDI in low-beta space plasmas.

physics.plasm-ph↗