arXiv subjects

Felix Flicker

Publications and source records attributed to Felix Flicker.

At least 37 records · Page 2Linked to original sources

arXiv2020

Charge order from structured coupling in VSe$_2$

Charge order--ubiquitous among correlated materials--is customarily described purely as an instability of the electronic structure. However, the resulting theoretical predictions often do not match high-resolution experimental data. A pertinent case is $1T$-VSe$_2$, whose single-band Fermi surface and weak-coupling nature make it qualitatively similar to the Peierls model underlying the traditional approach. Despite this, its Fermi surface is poorly nested, the thermal evolution of its charge density wave (CDW) ordering vectors displays an unexpected jump, and the CDW gap itself evades detection in direct probes of the electronic structure. We demonstrate that the thermal variation of the CDW vectors is naturally reproduced by the electronic susceptibility when incorporating a structured, momentum-dependent electron-phonon coupling, while the evasive CDW gap presents itself as a localized suppression of spectral weight centered above the Fermi level. Our results showcase the general utility of incorporating a structured coupling in the description of charge ordered materials, including those that appear unconventional.

cond-mat.str-el↗

arXiv2019

Conformal Quasicrystals and Holography

Recent studies of holographic tensor network models defined on regular tessellations of hyperbolic space have not yet addressed the underlying discrete geometry of the boundary. We show that the boundary degrees of freedom naturally live on a novel structure, a conformal quasicrystal, that provides a discrete model of conformal geometry. We introduce and construct a class of one-dimensional conformal quasicrystals, and discuss a higher-dimensional example (related to the Penrose tiling). Our construction permits discretizations of conformal field theories that preserve an infinite discrete subgroup of the global conformal group at the cost of lattice periodicity.

hep-th↗

arXiv2019

Superconducting order of $\mathrm{Sr}_2\mathrm{RuO}_4$ from a three-dimensional microscopic model

We compute and compare even- and odd-parity superconducting order parameters of strontium ruthenate ($\mathrm{Sr}_2\mathrm{RuO}_4$) in the limit of weak interactions, resulting from a fully microscopic three-dimensional model including spin-orbit coupling. We find that odd-parity helical and even-parity $d$-wave order are favored for smaller and larger values of the Hund's coupling parameter $J$, respectively. Both orders are found compatible with specific heat data and the recently-reported nuclear magnetic resonance (NMR) Knight shift drop [A. Pustogow et al. Nature 574, 72 (2019)]. The chiral $p$-wave order, numerically very competitive with helical order, sharply conflicts with the NMR experiment.

cond-mat.supr-con↗

arXiv2019

Classical Dimers on Penrose Tilings

We study the classical dimer model on rhombic Penrose tilings, whose edges and vertices may be identified with those of a bipartite graph. We find that Penrose tilings do not admit perfect matchings (defect-free dimer coverings). Instead, their maximum matchings have a monomer density of $81-50φ\approx 0.098$ in the thermodynamic limit, with $φ=\left(1+\sqrt{5}\right)/2$ the golden ratio. Maximum matchings divide the tiling into a fractal of nested closed regions bounded by loops that cannot be crossed by monomers. These loops connect second-nearest neighbour even-valence vertices, each of which lies on such a loop. Assigning a charge to each monomer with a sign fixed by its bipartite sublattice, we find that each bounded region has an excess of one charge, and a corresponding set of monomers, with adjacent regions having opposite net charge. The infinite tiling is charge neutral. We devise a simple algorithm for generating maximum matchings, and demonstrate that maximum matchings form a connected manifold under local monomer-dimer rearrangements. We show that dart-kite Penrose tilings feature an imbalance of charge between bipartite sub-lattices, leading to a minimum monomer density of $\left(7-4φ\right)/5\approx 0.106$ all of one charge.

cond-mat.str-el↗

arXiv2019

Magnetic Monopole Noise

Magnetic monopoles are hypothetical elementary particles exhibiting quantized magnetic charge $m_0=\pm(h/μ_0e)$ and quantized magnetic flux $Φ_0=\pm h/e$. A classic proposal for detecting such magnetic charges is to measure the quantized jump in magnetic flux $Φ$ threading the loop of a superconducting quantum interference device (SQUID) when a monopole passes through it. Naturally, with the theoretical discovery that a plasma of emergent magnetic charges should exist in several lanthanide-pyrochlore magnetic insulators, including Dy$_2$Ti$_2$O$_7$, this SQUID technique was proposed for their direct detection. Experimentally, this has proven extremely challenging because of the high number density, and the generation-recombination (GR) fluctuations, of the monopole plasma. Recently, however, theoretical advances have allowed the spectral density of magnetic-flux noise $S_Φ(ω,T)$ due to GR fluctuations of $\pm m_*$ magnetic charge pairs to be determined. These theories present a sequence of strikingly clear predictions for the magnetic-flux noise signature of emergent magnetic monopoles. Here we report development of a high-sensitivity, SQUID based flux-noise spectrometer, and consequent measurements of the frequency and temperature dependence of $S_Φ(ω,T)$ for Dy$_2$Ti$_2$O$_7$ samples. Virtually all the elements of $S_Φ(ω,T)$ predicted for a magnetic monopole plasma, including the existence of intense magnetization noise and its characteristic frequency and temperature dependence, are detected directly. Moreover, comparisons of simulated and measured correlation functions $C_Φ(t)$ of the magnetic-flux noise $Φ(t)$ imply that the motion of magnetic charges is strongly correlated because traversal of the same trajectory by two magnetic charges of same sign is forbidden.

cond-mat.quant-gas↗

arXiv2019

Finite temperature effects on Majorana bound states in chiral $p$-wave superconductors

We study Majorana fermions bound to vortex cores in a chiral $p$-wave superconductor at temperatures non-negligible compared to the superconducting gap. Thermal occupation of Caroli de Gennes-Matricon states, below the full gap, causes the free energy difference between the two fermionic parity sectors to decay algebraically with increasing temperature. The power law acquires an additional factor of $T^{-1}$ for each bound state thermally excited. The zero-temperature result is exponentially recovered well below the minigap (lowest-lying CdGM level). Our results suggest that temperatures larger than the minigap may not be disastrous for topological quantum computation. We discuss the prospect of precision measurements of pinning forces on vortices as a readout scheme for Majorana qubits.

cond-mat.str-el↗

arXiv2019

Uniaxial Strain Tuning of Superconductivity in 2$H$-NbSe$_{2}$

We explore the effect of lattice anisotropy on the charge-ordered superconductor 2H-NbSe$_{2}$. Using a novel strain apparatus, we measure the superconducting transition temperature $T_{sc}$ as a function of uniaxial strain. It is found that $T_{sc}$ is independent of tensile(compressive) strain below a threshold of 0.2\% (0.1\%), but decreases strongly with larger strains with an average rate of $1.3\,$K/\% ($2.5\,$K/\%). Transport signatures of charge order are largely unaffected as a function of strain. Theoretical considerations show that the change in the behavior of $T_{sc}$ with strain coincides with a phase transition from 3Q to 1Q charge order in the material. The spectral weight on one of the Fermi surface bands is found to change strongly as a consequence of this phase transition, providing a pathway to tune superconducting order.

cond-mat.supr-con↗

arXiv2018

Weak-coupling superconductivity in an anisotropic three-dimensional repulsive Hubbard model

We study a three-dimensional single-band repulsive Hubbard model at weak coupling. We establish the superconducting phase diagram in the parameter space of the chemical potential and the out-of-plane hopping strength. The model continuously connects the Hubbard model in two and three dimensions. We confirm previously-established results in these limits, and identify a rich structure of competing order parameters in between. Specifically, we find five types of $p$- and $d$-wave orders. In several regions of the phase diagram, even when the Fermi surface is a corrugated cylinder, the ground state is a time-reversal-symmetry-breaking superconductor with nodes, i.e. a Weyl superconductor.

cond-mat.supr-con↗

arXiv2018

Superconvergence of Topological Entropy in the Symbolic Dynamics of Substitution Sequences

We consider infinite sequences of superstable orbits (cascades) generated by systematic substitutions of letters in the symbolic dynamics of one-dimensional nonlinear systems in the logistic map universality class. We identify the conditions under which the topological entropy of successive words converges as a double exponential onto the accumulation point, and find the convergence rates analytically for selected cascades. Numerical tests of the convergence of the control parameter reveal a tendency to quantitatively universal double-exponential convergence. Taking a specific physical example, we consider cascades of stable orbits described by symbolic sequences with the symmetries of quasilattices. We show that all quasilattices can be realised as stable trajectories in nonlinear dynamical systems, extending previous results in which two were identified.

nlin.CD↗

arXiv2018

Chiral Optical Response of Multifold Fermions

Multifold fermions are generalizations of two-fold degenerate Weyl fermions with three-, four-, six- or eight-fold degeneracies protected by crystal symmetries, of which only the last type is necessarily non-chiral. Their low energy degrees of freedom can be described as emergent particles not present in the Standard Model of particle physics. We propose a range of experimental probes for multifold fermions in chiral symmetry groups based on the gyrotropic magnetic effect (GME) and the circular photo-galvanic effect (CPGE). We find that, in contrast to Weyl fermions, multifold fermions can have zero Berry curvature yet a finite GME, leading to an enhanced response. The CPGE is quantized and independent of frequency provided that the frequency region at which it is probed defines closed optically-activated momentum surfaces. We confirm the above properties by calculations in symmetry-restricted tight binding models with realistic density functional theory parameters. We identify a range of previously-unidentified ternary compounds able to exhibit chiral multifold fermions of all types (including a range of materials in the families AsBaPt and Gd$_3$Cl$_3$C), and provide specific predictions for the known multifold material RhSi.

cond-mat.mes-hall↗

arXiv2018

Atomic-Scale Strain Manipulation of a Charge Density Wave

A charge density wave (CDW) is one of the fundamental instabilities of the Fermi surface occurring in a wide range of quantum materials. In dimensions higher than one, where Fermi surface nesting can play only a limited role, the selection of the particular wave vector and geometry of an emerging CDW should in principle be susceptible to controllable manipulation. In this work, we implement a simple method for straining materials compatible with low-temperature scanning tunneling microscopy/spectroscopy (STM/S), and use it to strain-engineer new CDWs in 2H-NbSe2. Our STM/S measurements combined with theory reveal how small strain-induced changes in the electronic band structure and phonon dispersion lead to dramatic changes in the CDW ordering wave vector and geometry. Our work unveils the microscopic mechanism of a CDW formation in this system, and can serve as a general tool compatible with a range of spectroscopic techniques to engineer novel electronic states in any material where local strain or lattice symmetry breaking plays a role.

cond-mat.str-el↗

arXiv2018

Time Quasilattices in Dissipative Dynamical Systems

We establish the existence of `time quasilattices' as stable trajectories in dissipative dynamical systems. These tilings of the time axis, with two unit cells of different durations, can be generated as cuts through a periodic lattice spanned by two orthogonal directions of time. We show that there are precisely two admissible time quasilattices, which we term the infinite Pell and Clapeyron words, reached by a generalization of the period-doubling cascade. Finite Pell and Clapeyron words of increasing length provide systematic periodic approximations to time quasilattices which can be verified experimentally. The results apply to all systems featuring the universal sequence of periodic windows. We provide examples of discrete-time maps, and periodically-driven continuous-time dynamical systems. We identify quantum many-body systems in which time quasilattices develop rigidity via the interaction of many degrees of freedom, thus constituting dissipative discrete `time quasicrystals'.

nlin.CD↗

arXiv2018

Signatures of exciton condensation in a transition metal dichalcogenide

Bose condensation has shaped our understanding of macroscopic quantum phenomena, having been realized in superconductors, atomic gases, and liquid helium. Excitons are bosons that have been predicted to condense into either a superfluid or an insulating electronic crystal. Using the recently developed momentum-resolved electron energy-loss spectroscopy (M-EELS), we study electronic collective modes in the transition metal dichalcogenide semimetal, 1T-TiSe$_2$. Near the phase transition temperature, T$_c$ = 190 K, the energy of the electronic mode falls to zero at nonzero momentum, indicating dynamical slowing down of plasma fluctuations and crystallization of the valence electrons into an exciton condensate. Our study provides compelling evidence for exciton condensation in a three-dimensional solid and establishes M-EELS as a versatile technique sensitive to valence band excitations in quantum materials.

cond-mat.str-el↗

arXiv2017

Pell and Clapeyron Words as Stable Trajectories in Dynamical Systems

We establish the existence of `time quasicrystals', tilings of the time axis with two unit cells of different duration. These aperiodic tilings can be constructed as slices through regular tilings of a space spanned by two orthogonal time directions. We establish the result rigorously using the tools of symbolic dynamics. We show that, of the ten physically-relevant classes of one-dimensional quasicrystal, precisely two can appear as stable, attracting trajectories in dynamical systems, which we term the infinite Pell and Clapeyron words. These grow, via a generalization of the period-doubling cascade, as a sequence of stable orbits with periods increasing as the Pell and Clapeyron numbers, providing systematic approximations which can be experimentally implemented. The results apply to a wide universality class of dissipative nonlinear systems: we consider discrete-time maps, and continuous-time dynamical systems, both autonomous and periodically driven. This Paper proves and extends the results of a companion Letter, as well as providing a pedagogical background.

nlin.CD↗

arXiv2017

Proposal for the Detection of Magnetic Monopoles in Spin Ice via Nanoscale Magnetometry

We present a proposal for applying nanoscale magnetometry to the search for magnetic monopoles in the spin ice materials holmium and dysprosium titanate. Employing Monte Carlo simulations of the dipolar spin ice model, we find that when cooled to below $1.5\,$K these materials exhibit a sufficiently low monopole density to enable the direct observation of magnetic fields from individual monopoles. At these temperatures we demonstrate that noise spectroscopy can capture the intrinsic fluctuations associated with monopole dynamics, allowing one to isolate the qualitative effects associated with both the Coulomb interaction between monopoles and the topological constraints implied by Dirac strings. We describe in detail three different nanoscale magnetometry platforms (muon spin rotation, nitrogen vacancy defects, and nanoSQUID arrays) that can be used to detect monopoles in these experiments, and analyze the advantages of each.

cond-mat.str-el↗

arXiv2017

Inducing superconductivity in Weyl semi-metal microstructures by selective ion sputtering

By introducing a superconducting gap in Weyl- or Dirac semi-metals, the superconducting state inherits the non-trivial topology of their electronic structure. As a result, Weyl superconductors are expected to host exotic phenomena such as non-zero-momentum pairing due to their chiral node structure, or zero- energy Majorana modes at the surface. These are of fundamental interest to improve our understanding of correlated topological systems, and moreover practical applications in phase coherent devices and quantum applications have been proposed. Proximity-induced superconductivity promises to allow such experiments on non-superconducting Weyl semi-metals. Here we show a new route to reliably fabricating superconducting microstructures from the non-superconducting Weyl semi-metal NbAs under ion irradiation. The significant difference in the surface binding energy of Nb and As leads to a natural enrichment of Nb at the surface during ion milling, forming a superconducting surface layer (Tc~3.5K). Being formed from the target crystal itself, the ideal contact between the superconductor and the bulk may enable an effective gapping of the Weyl nodes in the bulk due to the proximity effect. Simple ion irradiation may thus serve as a powerful tool to fabricating topological quantum devices from mono-arsenides, even on an industrial scale.

cond-mat.mtrl-sci↗

arXiv2016

Charge Order in NbSe$_2$

We develop in detail a model of the charge order in NbSe$_2$ deriving from a strong electron-phonon coupling dependent on the ingoing and outgoing electron momenta as well as the electronic orbitals scattered between. Including both dependencies allows us to reproduce the full range of available experimental observations on this material. The stability of both experimentally-observed charge-ordered geometries (1Q and 3Q) is studied within this model as a function of temperature and uniaxial strain. It is found that a small amount of bulk strain suffices to stabilize the unidirectional order, and that in both ordering geometries, lattice fluctuations arising from the strong electron-phonon coupling act to suppress the onset temperature of charge order, giving a pseudogap regime characterized by local order and strong phase fluctuations.

cond-mat.str-el↗

arXiv2015

One-Dimensional Quasicrystals from Incommensurate Charge Order

Artificial quasicrystals are nowadays routinely manufactured, yet only two naturally occurring examples are known. We present a class of systems with the potential to be realized both artificially and in nature, in which the lowest energy state is a one-dimensional quasicrystal. These systems are based on incommensurately charge-ordered materials, in which the quasicrystalline phase competes with the formation of a regular array of discommensurations as a way of interpolating between incommensurate charge order at high temperatures and commensurate order at low temperatures. The nonlocal correlations characteristic of the quasicrystalline state emerge from a free-energy contribution localized in reciprocal space. We present a theoretical phase diagram showing that the required material properties for the appearance of such a ground state allow for one-dimensional quasicrystals to form in real materials. The result is a potentially wide class of one-dimensional quasicrystals.

cond-mat.str-el↗