arXiv subjects

Felix von Oppen

Publications and source records attributed to Felix von Oppen.

At least 55 records · Page 3Linked to original sources

arXiv2022

Diode effect in Josephson junctions with a single magnetic atom

Current flow in electronic devices can be asymmetric with bias direction, a phenomenon underlying the utility of diodes and known as non-reciprocal charge transport. The promise of dissipationless electronics has recently stimulated the quest for superconducting diodes, and non-reciprocal superconducting devices have been realized in various non-centrosymmetric systems. Probing the ultimate limits of miniaturization, we have created atomic-scale Pb--Pb Josephson junctions in a scanning tunneling microscope. Pristine junctions stabilized by a single Pb atom exhibit hysteretic behavior, confirming the high quality of the junctions, but no asymmetry between the bias directions. Non-reciprocal supercurrents emerge when inserting a single magnetic atom into the junction, with the preferred direction depending on the atomic species. Aided by theoretical modelling, we trace the non-reciprocity to quasiparticle currents flowing via Yu-Shiba-Rusinov (YSR) states inside the superconducting energy gap. Our results open new avenues for creating atomic-scale Josephson diodes and tuning their properties through single-atom manipulation.

cond-mat.supr-con↗

arXiv2022

Anderson's theorem for correlated insulating states in twisted bilayer graphene

The emergence of correlated insulating phases in magic-angle twisted bilayer graphene exhibits strong sample dependence. Here, we derive an Anderson theorem governing the robustness against disorder of the Kramers intervalley coherent (K-IVC) state, a prime candidate for describing the correlated insulators at even fillings of the moiré flat bands. We find that the K-IVC gap is robust against local perturbations, which are odd under $\mathcal{PT}$, where $\mathcal{P}$ and $\mathcal{T}$ denote particle-hole conjugation and time reversal, respectively. In contrast, $\mathcal{PT}$-even perturbations will in general induce subgap states and reduce or even eliminate the gap. We use this result to classify the stability of the K-IVC state against various experimentally relevant perturbations. The existence of an Anderson theorem singles out the K-IVC state from other possible insulating ground states.

cond-mat.mes-hall↗

arXiv2022

Hierarchy of Symmetry Breaking Correlated Phases in Twisted Bilayer Graphene

Twisted bilayer graphene (TBG) near the magic twist angle of $\sim1.1^{o}$ exhibits a rich phase diagram. However, the interplay between different phases and their dependence on twist angle is still elusive. Here, we explore the stability of various TBG phases and demonstrate that superconductivity near filling of two electrons per moiré unit cell alongside Fermi surface reconstructions, as well as entropy-driven high-temperature phase transitions and linear-in-T resistance occur over a range of twist angles which extends far beyond those exhibiting correlated insulating phases. In the vicinity of the magic angle, we also find a metallic phase that displays a hysteretic anomalous Hall effect and incipient Chern insulating behaviour. Such a metallic phase can be rationalized in terms of the interplay between interaction-driven deformations of TBG bands leading to Berry curvature redistribution and Fermi surface reconstruction. Our results provide an extensive perspective on the hierarchy of correlated phases in TBG as classified by their robustness against deviations from the magic angle or, equivalently, their electronic interaction requirements.

cond-mat.str-el↗

arXiv2022

Quantum spins and hybridization in artificially-constructed chains of magnetic adatoms on a superconductor

Magnetic adatom chains on surfaces constitute fascinating quantum spin systems. Superconducting substrates suppress interactions with bulk electronic excitations but couple the adatom spins to a chain of subgap Yu-Shiba-Rusinov (YSR) quasiparticles. Using a scanning tunneling microscope, we investigate such correlated spin-fermion systems by constructing Fe chains adatom by adatom on superconducting NbSe$_2$. The adatoms couple entirely via the substrate, retaining their quantum spin nature. In dimers, we observe that the deepest YSR state undergoes a quantum phase transition due to Ruderman-Kittel-Kasuya-Yosida interactions, a distinct signature of quantum spins. Chains exhibit coherent hybridization and band formation of the YSR excitations, indicating ferromagnetic coupling. Longer chains develop separate domains due to coexisting charge-density-wave order of NbSe$_2$. Despite the spin-orbit-coupled substrate, we find no signatures of Majoranas, possibly because quantum spins reduce the parameter range for topological superconductivity. We suggest that adatom chains are versatile systems for investigating correlated-electron physics and its interplay with topological superconductivity.

cond-mat.mes-hall↗

arXiv2022

Quantum Yu-Shiba-Rusinov dimers

Magnetic adatoms on a superconducting substrate undergo a quantum phase transition as their exchange coupling to the conduction electrons increases. For quantum spins, this transition is accompanied by screening of the adatom spin. Here, we explore the consequences of this screening for the phase diagrams and subgap excitation spectra of dimers of magnetic adatoms coupled by hybridization of their Yu-Shiba-Rusinov states and spin-spin interactions. We specifically account for higher spins, single-ion anisotropy, Ruderman-Kittel-Kasuya-Yosida coupling, and Dzyaloshinsky-Moriya interactions relevant in transition-metal and rare-earth systems. Our flexible approach based on a zero-bandwidth approximation provides detailed physical insight and is in excellent qualitative agreement with available numerical-renormalization group calculations on monomers and dimers. Remarkably, we find that even in the limit of large impurity spins or strong single-ion anisotropy, the phase diagrams for dimers of quantum spins remain qualitatively distinct from phase diagrams based on classical spins, highlighting the need for a theory of quantum Yu-Shiba-Rusinov dimers.

cond-mat.mes-hall↗

arXiv2021

Ascendance of Superconductivity in Magic-Angle Graphene Multilayers

Graphene moire superlattices have emerged as a platform hosting and abundance of correlated insulating, topological, and superconducting phases. While the origins of strong correlations and non-trivial topology are shown to be directly linked to flat moire bands, the nature and mechanism of superconductivity remain enigmatic. In particular, only alternating twisted stacking geometries of bilayer and trilayer graphene are found to exhibit robust superconductivity manifesting as zero resistance and Fraunhofer interference patterns. Here we demonstrate that magic-angle twisted tri-, quadri-, and pentalayers placed on monolayer tungsten diselenide exhibit flavour polarization and superconductivity. We also observe insulating states in the trilayer and quadrilayer arising at finite electric displacement fields, despite the presence of dispersive bands introduced by additional graphene layers. Moreover, the three multilayer geometries allow us to identify universal features in the family of graphene moire structures arising from the intricate relations between superconducting states, symmetry-breaking transitions, and van Hove singularities. Remarkably, as the number of layers increases, superconductivity emerges over a dramatically enhanced filling-factor range. In particular, in twisted pentalayers, superconductivity extends well beyond the filling of four electrons per moire unit cell, demonstrating the non-trivial role of the additional bands. Our results highlight the importance of the interplay between flat and dispersive bands in extending superconducting regions in graphene moire superlattices and open new frontiers for developing graphene-based superconductors.

cond-mat.supr-con↗

arXiv2021

Direct observation of intrinsic surface magnetic disorder in amorphous superconducting films

The interplay between disorder and interactions can dramatically influence the physical properties of thin-film superconductors. In the most extreme case, strong disorder is able to suppress superconductivity as an insulating phase emerges. Due to the known pair-breaking potential of magnetic disorder on superconductors, the research focus is on the influence of non-magnetic disorder. Here we provide direct evidence that magnetic disorder is also present at the surface of amorphous superconducting films. This magnetic disorder is present even in the absence of magnetic impurity atoms and is intimately related to the surface termination itself. While bulk superconductivity survives in sufficiently thick films, we suggest that magnetic disorder may crucially affect the superconductor-to-insulator transition in the thin-film limit.

cond-mat.supr-con↗

arXiv2021

Topological States in Dimerized Quantum-Dot Chains Created by Atom Manipulation

Topological electronic phases exist in a variety of naturally occurring materials but can also be created artificially. We used a cryogenic scanning tunneling microscope to create dimerized chains of identical quantum dots on a semiconductor surface and to demonstrate that these chains give rise to one-dimensional topological phases. The dots were assembled from charged adatoms, creating a confining potential with single-atom precision acting on electrons in surface states of the semiconductor. Quantum coupling between the dots leads to electronic states localized at the ends of the chains, as well as at deliberately created internal domain walls, in agreement with the predictions of the Su-Schrieffer-Heeger model. Scanning tunneling spectroscopy also reveals deviations from this well-established model manifested in an asymmetric level spectrum and energy shifts of the boundary states. The deviations arise because the dots are charged and hence lead to an onsite potential that varies along the chain. We show that this variation can be mitigated by electrostatic gating using auxiliary charged adatoms, enabling fine-tuning of the boundary states and control of their quantum superposition. The experimental data, which are complemented by theoretical modeling of the potential and the resulting eigenstates, reveal the important role of electrostatics in these engineered quantum structures.

cond-mat.mes-hall↗

arXiv2021

Quantum magnetism and topological superconductivity in Yu-Shiba-Rusinov chains

Chains of magnetic adatoms on superconductors have been discussed as promising systems for realizing Majorana end states. Here, we show that dilute Yu-Shiba-Rusinov (YSR) chains are also a versatile platform for quantum magnetism and correlated electron dynamics, with widely adjustable spin values and couplings. Focusing on subgap excitations, we derive an extended $t-J$ model for dilute quantum YSR chains and use it to study the phase diagram as well as tunneling spectra. We explore the implications of quantum magnetism for the formation of a topological superconducting phase, contrasting it to existing models assuming classical spin textures.

cond-mat.mes-hall↗

arXiv2021

Yu-Shiba-Rusinov states in real metals

Theoretical descriptions of Yu-Shiba-Rusinov (YSR) states induced by magnetic impurities inside the gap of a superconductor typically rely on a classical spin model or are restricted to spin-1/2 quantum spins. These models fail to account for important aspects of YSR states induced by transition-metal impurities, including the effects of higher quantum spins coupled to several conduction-electron channels, crystal or ligand-field effects, and magnetic anisotropy. We introduce and explore a zero-bandwidth model, which incorporates these aspects, is readily solved numerically, and analytically tractable in several limiting cases. The principal simplification of the model is to neglect Kondo renormalizations of the exchange couplings between impurity spin and conduction electrons. Nevertheless, we find excellent correspondence in those cases, in which we can compare our results to existing numerical-renormalization-group calculations. We apply the model to obtain and understand phase diagrams as a function of pairing strength and magnetic anisotropy as well as subgap excitation spectra. The single-channel case is most relevant for transition-metal impurities embedded into metallic coordination complexes on superconducting substrates, while the multi-channel case models transition-metal adatoms.

cond-mat.mes-hall↗

arXiv2021

Moiré tuning of spin excitations: Individual Fe atoms on MoS$_2$/Au(111)

Magnetic adatoms on surfaces are exchange coupled to their environment, inducing fast relaxation of excited spin states and decoherence. These interactions can be suppressed by inserting decoupling layers between the magnetic adsorbate and the metallic substrate. Using low-temperature scanning tunneling microscopy and spectroscopy, we investigate the magnetic properties of single Fe atoms on Au(111) covered by a monolayer of MoS$_2$ and explore the influence of the moiré structure on the spin excitation spectra. Fe adatoms absorbed at minima of the moiré structure exhibit almost pure inelastic spin excitations. Kondo correlations develop for adsorption sites off the moiré minimum, culminating in fully developed Kondo resonances on moiré maxima. The increase in Kondo correlations is accompanied by a decrease in the single-ion anisotropy, which we rationalize by poor-person's scaling. Local variations in the tunneling spectra indicate pronounced interference between tunneling paths involving the spin-carrying orbitals and a hybrid Fe-S orbital, which forms despite the nominally inert nature of the terminating S layer.

cond-mat.mes-hall↗

arXiv2021

Three-phase Majorana zero modes at tiny magnetic fields

Proposals for realizing Majorana fermions in condensed matter systems typically rely on magnetic fields, which degrade the proximitizing superconductor and plague the Majoranas' detection. We propose an alternative scheme to realize Majoranas based only on phase-biased superconductors. The phases (at least three of them) can be biased by a tiny magnetic field threading macroscopic superconducting loops, focusing and enhancing the effect of the magnetic field onto the junction, or by supercurrents. We show how a combination of the superconducting phase winding and the spin-orbit phase induced in closed loops (Aharonov-Casher effect) facilitates a topological superconducting state with Majorana end states. We demontrate this scheme by an analytically tractable model as well as simulations of realistic setups comprising only conventional materials.

cond-mat.mes-hall↗

arXiv2021

Engineered platforms for topological superconductivity and Majorana zero modes

Among the major approaches that are being pursued for realizing quantum bits, the Majorana-based platform has been the most recent to be launched. It attempts to realize qubits which store quantum information in a topologically-protected manner. The quantum information is protected by its nonlocal storage in localized and well-separated Majorana zero modes, and manipulated by exploiting their nonabelian quantum exchange properties. Realizing these topological qubits is experimentally challenging, requiring superconductivity, helical electrons (created by spin-orbit coupling) and breaking of time reversal symmetry to all cooperate in an uncomfortable alliance. Over the past decade, several candidate material systems for realizing Majorana-based topological qubits have been explored, and there is accumulating, though still debated, evidence that zero modes are indeed being realized. This paper reviews the basic physical principles on which these approaches are based, the material systems that are being developed, and the current state of the field. We highlight both the progress made and the challenges that still need to be overcome.

cond-mat.mes-hall↗

arXiv2021

Photon-assisted resonant Andreev reflections: Yu-Shiba-Rusinov and Majorana states

Photon-assisted tunneling frequently provides detailed information on the underlying charge-transfer process. In particular, the Tien-Gordon approach and its extensions predict that the sideband spacing in bias voltage is a direct fingerprint of the number of electrons transferred in a single tunneling event. Here, we analyze photon-assisted tunneling into subgap states in superconductors in the limit of small temperatures and bias voltages where tunneling is dominated by resonant Andreev processes and does not conform to the predictions of simple Tien-Gordon theory. Our analysis is based on a systematic Keldysh calculation of the subgap conductance and provides a detailed analytical understanding of photon-assisted tunneling into subgap states, in excellent agreement with a recent experiment. We focus on tunneling from superconducting electrodes and into Yu-Shiba-Rusinov states associated with magnetic impurities or adatoms, but we also explicitly extend our results to include normal-metal electrodes or other types of subgap states in superconductors. In particular, we argue that photon-assisted Andreev reflections provide a high-accuracy method to measure small, but nonzero energies of subgap states which can be important for distinguishing conventional subgap states from Majorana bound states.

cond-mat.mes-hall↗

arXiv2020

Topological superconductivity in tripartite superconductor-ferromagnet-semiconductor nanowires

Motivated by recent experiments searching for Majorana zero modes in tripartite semiconductor nanowires with epitaxial superconductor and ferromagnetic-insulator layers, we explore the emergence of topological superconductivity in such devices for paradigmatic arrangements of the three constituents. Accounting for the competition between magnetism and superconductivity, we treat superconductivity self consistently and describe the electronic properties, including the superconducting and ferromagnetic proximity effects, within a direct wave-function approach. We conclude that the most viable mechanism for topological superconductivity relies on a superconductor-semiconductor-ferromagnet arrangement of the constituents, in which spin splitting and superconductivity are independently induced in the semiconductor by proximity and superconductivity is only weakly affected by the ferromagnetic insulator.

cond-mat.mes-hall↗

arXiv2020

Hilbert-space geometry of random-matrix eigenstates

The geometry of multi-parameter families of quantum states is important in numerous contexts, including adiabatic or nonadiabatic quantum dynamics, quantum quenches, and the characterization of quantum critical points. Here, we discuss the Hilbert-space geometry of eigenstates of parameter-dependent random-matrix ensembles, deriving the full probability distribution of the quantum geometric tensor for the Gaussian Unitary Ensemble. Our analytical results give the exact joint distribution function of the Fubini-Study metric and the Berry curvature. We discuss relations to Levy stable distributions and compare our results to numerical simulations of random-matrix ensembles as well as electrons in a random magnetic field.

cond-mat.dis-nn↗

arXiv2020

Interfering tunneling paths through magnetic molecules on superconductors: Asymmetries of Kondo and Yu-Shiba-Rusinov resonances

Magnetic adsorbates on superconductors induce a Kondo resonance outside and Yu-Shiba-Rusinov (YSR) bound states inside the superconducting energy gap. When probed by scanning tunneling spectroscopy, the associated differential-conductance spectra frequently exhibit characteristic bias-voltage asymmetries. Here, we observe correlated variations of Kondo and YSR asymmetries across an Fe-porphyrin molecule adsorbed on Pb(111). We show that both asymmetries originate in interfering tunneling paths via a spin-carrying orbital and the highest occupied molecular orbital (HOMO). Strong evidence for this model comes from nodal planes of the HOMO, where tunneling reveals symmetric Kondo and YSR resonances. Our results establish an important mechanism for the asymmetries of Kondo and YSR lineshapes.

cond-mat.mes-hall↗

arXiv2020

Long distance coherence of Majorana wires

Theoretically, a pair of Majorana bound states in a topological superconductor forms a single fermionic level even at large separations, implying that the parity information is stored nonlocally. The nonlocality leads to a long-distance coherence for electrons tunneling through a Coulomb blockaded Majorana wire [Fu, Phys. Rev. Lett. 104, 056402 (2010)], an effect that can be observed, e.g., in an interferometer. Here, we examine theoretically the coherent electron transfer, taking into account that tunneling implies the long-distance transfer of charge, which is carried by one-dimensional plasmons. We show that the charge dynamics does not affect the coherence of the electron tunneling process in a topological superconductor consisting of a semiconductor wire proximitized by a single bulk superconductor. The coherence may be strongly suppressed, however, if the topological superconductivity derives from a semiconductor wire proximitized by a granular superconductor.

cond-mat.mes-hall↗