arXiv subjects

Fen Zou

Publications and source records attributed to Fen Zou.

At least 19 recordsLinked to original sources

arXiv2026

Frequency upconversion of infrared signals via molecular cavity optomechanical systems with gain

Molecular cavity optomechanical systems have recently emerged as a promising platform for enhancing infrared detection sensitivity, owing to their ability to up-convert low-frequency infrared (IR) photons to visible frequency range. Generally, under red-detuned pumping in such systems, the ideal conversion efficiency of the IR signal approaches 1. To overcome this efficiency constraint, we propose a scheme that incorporates gain into the infrared cavity of a molecular cavity optomechanical system comprising two cavities and an ensemble of N molecules. The upconversion process, which relies on IR absorption and Raman scattering associated with specific vibrational modes, is significantly amplified by the incorporation of gain under the red-detuned conditions. Moreover, our analysis demonstrates that the added noise is maintained near 0.5.

quant-ph↗

arXiv2026

Frequency upconversion of infrared signals via molecular optomechanical cavities

Molecular optomechanical cavities have recently emerged as a promising platform for frequency upconversion, enabling the quantum coherent conversion of infrared signal into the visible range. In a recent work [F. Zou et al., Phys. Rev. Lett. 132, 153602 (2024)], we proposed an amplification mechanism that can enhance the intensity of the upconverted infrared signals by a factor of 1000 or more within such a cavity under the ideal case without any noise. In this work, we employ the power spectrum method to investigate the noise added to the upconverted signal in a molecular optomechanical cavity along with the conversion efficiency from infrared signal into visible range. In the red-detuned regime, the anti-Stokes sideband achieves superior conversion efficiency relative to the Stokes sideband. Conversely, the Stokes sideband dominates under the blue-detuned condition, which amplifies the infrared signal. We further demonstrate the dependence of the added noise on the coupling strength and decay rates of the system. In particular, we find that when the infrared signal is amplified, the added noise approaches the quantum limit of one quantum.

quant-ph↗

arXiv2025

Enantiospecific Two-Photon Electric-Dipole Selection Rule of Chiral Molecules

Distinguishing between enantiomers is crucial in the study of chiral molecules in chemistry and pharmacology. Many optical approaches rely on enantiospecific cyclic electric-dipole transitions induced by three microwave or laser beams. However, these approaches impose stringent requirements, including phase locking, three-photon resonance, and precise control over beam intensities and operation times, which enhance the complexity and restrict the applicability. In this letter, we present a novel optical method that {\it eliminates these constraints entirely.} Specifically, we demonstrate that in the presence of a static electric field, there is a selection rule for two-photon electric-dipole transitions that differs between enantiomers. This distinction arises because the static electric field breaks the symmetry associated with the combined action of a specific rotation and time-reversal transformation. Leveraging the enantiospecific two-photon selection rule, one can selectively excite a desired enantiomer using two beams, without the need for phase locking, resonance condition, and the precise control of their intensities and operation times. Our method significantly enhances the feasibility and applicability of optical approaches for enantiomer differentiation.

quant-ph↗

arXiv2024

Enantiomer-Specific Pumping of Chiral Molecules

Enantiomer-specific state transfer (ESST), which involves transferring enantiomers with different handedness of a chiral molecule into different-energy internal states, is a challenging yet significant task. Previous ESST methods are based on dynamic processes and thus require the preparation of initial states and precise control of microwave operation times. We propose a novel ESST approach, called enantiomer-specific pumping (ESP), which is based on a {\it dissipative} process, and thereby eliminates the need for these two technical requirements. This approach utilizes a special microwave-induced dark state that appears exclusively for the enantiomer with a specific handedness. Specifically, in ESP, the enantiomer lacking the dark state can be pumped out of the subspace of relevant internal states, while the enantiomer with the dark state maintains a finite probability within this subspace, offering high efficiency in ESST. Notably, ESP facilitates enantiodetection without the need for enantiopure samples as reference.

quant-ph↗

arXiv2023

Two-mode correlated multiphoton bundle emission

The preparation of correlated multiphoton sources is an important research topic in quantum optics and quantum information science. Here, two-mode correlated multiphoton bundle emission in a nondegenerate multiphoton Jaynes-Cummings model, which is comprised of a two-level system coupled with two cavity modes is studied. The two-level system is driven by a near-resonant strong laser such that the Mollow regime dominates the physical processes in this system. Under certain resonance conditions, a perfect super-Rabi oscillation between the zero-photon state $|0\rangle_{a}|0\rangle_{b}$ and the ($n+m$)-photon state $|n\rangle_{a}|m\rangle_{b}$ of the two cavity modes can take place. Induced by the photon decay, the two-mode correlated multiphoton bundle emission occurs in this system. More importantly, the results show that there is an antibunching effect between the strongly-correlated photon bundles, so that the system behaves as an antibunched ($n+m$)-photon source. The work opens up a route towards achieving two-mode correlated multiphoton source device, which has potential applications in modern quantum technology.

quant-ph↗

arXiv2023

Amplifying Frequency Up-Converted Infrared Signals with a Molecular Optomechanical Cavity

Frequency up-conversion, enabled by molecular optomechanical coupling, has recently emerged as a promising approach for converting infrared signals into the visible range through quantum coherent conversion of signals. However, detecting these converted signals poses a significant challenge due to their inherently weak signal intensity. In this work, we propose an amplification mechanism capable of enhancing the signal intensity by a factor of 1000 or more for the frequency up-converted infrared signal in a molecular optomechanical system. The mechanism takes advantage of the strong coupling enhancement with molecular collective mode and Stokes sideband pump. This work demonstrates a feasible approach for up-converting infrared signals to the visible range.

quant-ph↗

arXiv2023

Dynamical $N$-photon bundle emission

Engineering multiphoton resources is of importance in quantum metrology, quantum lithography, and biological sensing. Here we propose a concept of dynamical emission of $N$ strongly-correlated photons. This is realized in a circuit quantum electrodynamical system driven by two Gaussian-pulse sequences. The underlying physical mechanism relies on the stimulated Raman adiabatic passage that allows efficient and selective preparation of target multiphoton states. Assisted by the photon decay, a highly pure $N$-photon bundle emission takes place in this system. In particular, the dynamical $N$-photon bundle emission can be tuned by controlling the time interval between consecutive pulses so that the device behaves as an $N$-photon gun, which can be triggered on demand. Our work opens up a route to achieve multiphoton source devices, which have wide potential applications in quantum information processing and quantum metrology.

quant-ph↗

arXiv2023

Optical-pumping enantio-conversion of chiral mixtures in presence of tunneling between chiral states

Enantio-conversion of chiral mixtures, converting the mixtures composed of left- and right-handed chiral molecules into the homochiral ensembles, has become an important research topic in chemical and biological fields. In previous studies on enantio-conversion, the tunneling interaction between the left- and right-handed chiral states was often neglected. However, for certain chiral molecules, this tunneling interaction is significant and cannot be ignored. Here we propose a scheme for enantio-conversion of chiral mixtures through optical pumping based on a four-level model of chiral molecules, comprising two chiral ground states and two achiral excited states, with a tunneling interaction between the chiral states. Under one-photon large detuning and two-photon resonance conditions, one of the achiral excited states is eliminated adiabatically. By well designing the detuning and coupling strengths of the electromagnetic fields, the tunneling interaction between two chiral states and the interaction between one of the chiral states and the remaining achiral excited state can be eliminated. Consequently, one chiral state remains unchanged, while the other can be excited to an achiral excited state, establishing chiral-state-selective excitations. By numerically calculating the populations of two chiral ground states and the enantiomeric excess, we observe that high-efficiency enantio-conversion is achieved under the combined effects of system dissipation and chiral-state-selective excitations.

quant-ph↗

arXiv2022

Multiple-photon bundle emission in the $n$-photon Jaynes-Cummings model

We study the multiple-photon bundle emission in the $n$-photon Jaynes-Cummings model composed of a two-level system coupled to a single-mode optical field via the $n$-photon exciting process. Here, the two-level system is strongly driven by a near-resonant monochromatic field, and hence the system can work in the Mollow regime, in which a super-Rabi oscillation between the zero-photon state and the $n$-photon state can take place under proper resonant conditions. We calculate the photon number populations and the standard equal-time high-order correlation functions, and find that the multiple-photon bundle emission can occur in this system. The multiple-photon bundle emission is also confirmed by investigating the quantum trajectories of the state populations and both the standard and generalized time-delay second-order correlation functions for multiple-photon bundle. Our work paves the way towards the study of multiple-photon quantum coherent devices, with potential application in quantum information sciences and technologies.

quant-ph↗

arXiv2022

Retrieval of photon blockade effect in the dispersive Jaynes-Cummings model

We propose a reliable scheme to recover the conventional photon blockade effect in the dispersive Jaynes-Cummings model, which describes a two-level atom coupled to a single-mode cavity field in the large-detuning regime. This is achieved by introducing a transversal driving to the atom and then photonic nonlinearity is obtained. The eigenenergy spectrum of the system is derived analytically and the photon blockade effect is confirmed by numerically calculating the photon-number distributions and equal-time second-order correlation function of the cavity field in the presence of system dissipations. We find that the conventional photon blockade effect can be recovered at proper atomic and cavity-field drivings. This work will provide a method to generate the conventional photon blockade effect in the dispersively coupled quantum optical systems.

quant-ph↗

arXiv2022

Enantiodiscrimination of chiral molecules via quantum correlation function

We propose a method to realize enantiodiscrimination of chiral molecules based on quantum correlation function in a driven cavity-molecule system, where the chiral molecule is coupled with a quantized cavity field and two classical light fields to form a cyclic three-level model. According to the inherent properties of electric-dipole transition moments of chiral molecules, there is a $\pi$-phase difference in the overall phase of the cyclic three-level model for the left- and right-handed chiral molecules. Thus, the correlation function depends on this overall phase and is chirality-dependent. The analytical and numerical results indicate that the left- and right-handed chiral molecules can be discriminated by detecting quantum correlation function. Our work opens up a promising route to discriminate molecular chirality, which is an extremely important task in pharmacology and biochemistry.

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arXiv2021

Dynamical emission of phonon pairs in optomechanical systems

Multiphonon state plays an important role in quantum information processing and quantum metrology. Here we propose a scheme to realize dynamical emission of phonon pairs based on the technique of stimulated Raman adiabatic passage in a single cavity optomechanical system, where the optical cavity is driven by two Gaussian pulse lasers. By exploring quantum trajectories of the state populations and the average phonon number, we find that the dynamical phonon-pair emission can be realized under the appropriate parameter conditions and is tunable by controlling the time interval between the consecutive pulses of pump lasers. In particular, the numerical results for the standard and generalized second-order correlation functions of the mechanical mode show that the system can behave as an antibunched phonon-pair emitter. Our proposal can be extended to achieve an antibunched $n$-phonon emitter, which has potential applications for on-chip quantum communications.

quant-ph↗

arXiv2021

Optical normal-mode-induced phonon-sideband splitting in photon-blockade effect

We study the photon-blockade effect in a loop-coupled optomechanical system consisting of two cavity modes and one mechanical mode. Here, the mechanical mode is optomechanically coupled to the two cavity modes, which are coupled with each other via a photon-hopping interaction. By treating the photon-hopping interaction as a perturbation, we obtain the analytical results of the eigenvalues and eigenstates of the system in the subspaces associated with zero, one, and two photons. We find a phenomenon of optical normal-mode-induced phonon-sideband splitting in the photon-blockade effect by analytically and numerically calculating the second-order correlation functions of the two cavity modes. This work not only presents a method to choose optimal driving frequency for photon blockade by tuning the photon-hopping interaction, but also provides a means to characterize the normal-mode splitting with cavity photon statistics.

quant-ph↗

arXiv2020

Multiphoton blockade in the two-photon Jaynes-Cummings model

We study multiphoton blockade and photon-induced tunneling effects in the two-photon Jaynes-Cummings model, where a single-mode cavity field and a two-level atom are coupled via a two-photon interaction. We consider both the cavity-field-driving and atom-driving cases, and find that single-photon blockade and photon-induced tunneling effects can be observed when the cavity mode is driven, while the two-photon blockade effect appears when the atom is driven. For the atom-driving case (the two-photon transition process), we present a criterion of the correlation functions for the multiphoton blockade effect. Specifically, we show that quantum interference can enhance the photon blockade effect in the single-photon cavity-field-driving case. Our results are confirmed by analytically and numerically calculating the correlation function of the cavity-field mode. Our work has potential applications in quantum information processing and paves the way for the study of multiphoton quantum coherent devices.

quant-ph↗

arXiv2020

Spectral characterization of couplings in a mixed optomechanical model

We study the spectrum of single-photon emission and scattering in a mixed optomechanical model which consists of both linear and quadratic optomechanical interactions. The spectra are calculated based on the exact long-time solutions of the single-photon emission and scattering processes in this system. We find that there exist some phonon sideband peaks in the spectra and there are some sub peaks around the phonon sideband peaks under proper parameter conditions. The correspondence between the spectral features and the optomechanical interactions is confirmed, and the optomechanical coupling strengths can be inferred by analyzing the resonance peaks and dips in the spectra.

quant-ph↗

arXiv2020

Enhancement of photon blockade effect via quantum interference

We study the photon blockade effect in a coupled cavity system, which is formed by a linear cavity coupled to a Kerr-type nonlinear cavity via a photon-hopping interaction. We explain the physical phenomenon from the viewpoint of the conventional and unconventional photon blockade effects. The corresponding physical mechanisms of the two kinds of photon blockade effects are based on the anharmonicity in the eigenenergy spectrum and the destructive quantum interference between two different transition paths, respectively. In particular, we find that the photon blockade via destructive quantum interference also exists in the conventional photon blockade regime, and that the unconventional photon blockade occurs in both the weak- and strong-Kerr nonlinearity cases. The photon blockade effect can be observed by calculating the second-order correlation function of the cavity field. This model is general and hence it can be implemented in various experimental setups such as coupled optical-cavity systems, coupled photon-magnon systems, and coupled superconducting-resonator systems. We present some discussions on the experimental feasibility.

quant-ph↗

arXiv2020

Quantum thermalization and vanishing thermal entanglement in the open Jaynes-Cummings model

The quantum thermalization of the Jaynes-Cummings (JC) model in both equilibrium and non-equilibrium open-system cases is sdudied, in which the two subsystems, a two-level system and a single-mode bosonic field, are in contact with either two individual heat baths or a common heat bath. It is found that in the individual heat-bath case, the JC model can only be thermalized when either the two heat baths have the same temperature or the coupling of the JC system to one of the two baths is turned off. In the common heat-bath case, the JC system can be thermalized irrespective of the bath temperature and the system-bath coupling strengths. The thermal entanglement in this system is also studied. A \emph{counterintuitive} phenomenon of \emph{vanishing} thermal entanglement in the JC system is found and proved.

quant-ph↗

arXiv2019

Enhancement of few-photon optomechanical effects with cross-Kerr nonlinearity

Few-photon optomechanical effects are not only important physical evidences for understanding the radiation-pressure interaction between photons and mechanical oscillation, but also have wide potential applications in modern quantum technology. Here we study the few-photon optomechanical effects including photon blockade and generation of the Schrödinger cat states under the assistance of a cross-Kerr interaction, which is an inherent interaction accompanied the optomechanical coupling in a generalized optomechanical system. By exactly diagonalizing the generalized optomechanical Hamiltonian and calculating its unitary evolution operator, we find the physical mechanism of the enhancement of photon blockade and single-photon mechanical displacement. The quantum properties in this generalized optomechanical system are studied by investigating the second-order correlation function of the cavity field and calculating the Wigner function and the probability distribution of the rotated quadrature operator for the mechanical mode. We also study the influence of the dissipations on the few-photon optomechanical effects.

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