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Feng Ding

Publications and source records attributed to Feng Ding.

At least 91 records · Page 5Linked to original sources

The Phase-curve Signature of Condensible Water-rich Atmospheres on Slowly Rotating Tidally Locked Exoplanets

We use an idealized three-dimensional general circulation model to study condensible-rich atmospheres with an ineffective cold trap on slowly rotating tidally locked terrestrial planets. In particular, we show the climate dynamics in a thin and temperate atmosphere with condensible water vapor. The similarities between our thin and temperate atmosphere and the warm and thick atmosphere approaching the water vapor runaway greenhouse in previous works are discussed, including the reversal of the thermal emission between the day and night hemispheres. Different from the transit spectroscopy of water vapor that depends on the absolute amount of atmospheric water vapor, the contrast between the dayside and nightside thermal emission provides information regarding the relative ratio of water vapor to the background atmosphere as well as the atmospheric pressure near the substellar tropopause and the emission level on the nightside on potentially habitable worlds.

astro-ph.EP↗

Comet-like tails of disintegrating exoplanets explained by escaping outflows emanated from the permanent nightside: day-side versus night-side escape

Ultra-hot disintegrating exoplanets have been detected with tails trailing behind and/or shooting ahead of them. These tails are believed to be made of dusts that are carried upward by the supersonic flow escaping the planet's gravity field from the fiercely heated permanent day-side. Conserving angular momentum, this day-side escape flux would lead the planet in orbit. In order to explain the trailing tails in observation, radiation pressure, a repulsive force pushing the escape flow away from the host star is considered to be necessary. We here investigate whether escape could occur on the night-side as the escape flow is deflected by the pressure gradient force. We demonstrate in an idealized framework that escape flux from the night-side could dominate that from the day-side; and the former may naturally explain the commonly-observed trailing tails based on angular momentum conservation, without the need to invoke radiation pressure, which has previously been thought to be the key. We also find analytical approximations for both dayside and nightside escape fluxes, which may be applied to study planetary evolution of disintegrating planets and to infer planetary sizes from observations of the properties of their dusty tails.

astro-ph.EP↗

Stabilization of dayside surface liquid water via tropopause cold trapping on arid slowly rotating tidally locked planets

Terrestrial-type exoplanets orbiting nearby red dwarf stars (M-dwarfs) are among the best targets for atmospheric characterization and biosignature searches in the near future. Recent evolutionary studies have suggested that terrestrial planets in the habitable zone of M-dwarfs are probably tidally locked and have limited surface water inventories as a result of their host stars' high early luminosities. Several previous climate simulations of such planets have indicated that their remaining water would be transported to the planet's permanent nightside and become trapped as surface ice, leaving the dayside devoid of water. Here we use a three-dimensional general circulation model with a water cycle and accurate radiative transfer scheme to investigate the surface water evolution on slowly rotating tidally locked terrestrial planets with limited surface water inventories. We show that there is a competition for water trapping between the nightside surface and the substellar tropopause in this type of climate system. Although under some conditions the surface water remains trapped on the nightside as an ice sheet, in other cases liquid water stabilizes in a circular area in the substellar region as a wetland. Planets with 1 bar N$_2$ and atmospheric CO$_2$ levels greater than 0.1 bar retain stable dayside liquid water, even with very small surface water inventories. Our results reveal the diversity of possible climate states on terrestrial-type exoplanets and highlight the importance of surface liquid water detection techniques for future characterization efforts.

astro-ph.EP↗

Atmospheric Evolution on Low-gravity Waterworlds

Low-gravity waterworlds ($M\lesssim 0.1 M_{\oplus}$) are of interest for their potential habitability. The weakly bound atmospheres of such worlds have proportionally larger radiative surfaces and are more susceptible to escape. We conduct a unified investigation into these phenomena, combining analytical energy balance and hydrodynamic escape with line-by-line radiative transfer calculations. Because outgoing radiation is forced to increase with surface temperature by the expansion of the radiative surface, we find that these worlds do not experience a runaway greenhouse. Furthermore, we show that a long-lived liquid water habitable zone is possible for low-gravity waterworlds of sufficient mass. Its inner edge is set by the rate of atmospheric escape, because a short-lived atmosphere limits the time available for life to evolve. In describing the physics of the parameter space transition from "planet-like" to "comet-like", our model produces a lower bound for habitability in terms of gravity. These results provide valuable insights in the context of the ongoing hunt for habitable exoplanets and exomoons.

astro-ph.EP↗

A New Line-By-Line General Circulation Model for Simulations of Diverse Planetary Atmospheres: Initial Validation and Application to the Exoplanet GJ 1132b

Exploring diverse planetary atmospheres requires modeling tools that are both accurate and flexible. Here, we develop a three-dimensional general circulation model (3D GCM) that for the first time uses a line-by-line approach to describe the radiative transfer. We validate our GCM by comparing with published results done by different 1D and 3D models. To demonstrate the versatility of the model, we apply the GCM to the hot Earth-sized exoplanet GJ 1132b and study its climate and circulation assuming an atmosphere dominated by abiotic oxygen (O$_2$). Our simulations show that a minor CO$_2$ composition can change the circulation pattern substantially, intensifying the equatorial superrotation in particular. Computation of the phase-resolved spectroscopy indicates that the vertical profile of the superrotating jet could be inferred in future spectro-photometric observations by the phase shift of the hotspot in the CO$_2$ principle absorption band centered at 667 cm$^{-1}$. We also show that atmospheric mass could potentially be constrained by the phase amplitude in the O$_2$ vibrational fundamental band for planets with O$_2$-rich atmospheres, although further experimental and/or theoretical O$_2$-O$_2$ collision-induced absorption data at high temperatures is needed to confirm this. More physical schemes such as moist dynamics will be implemented in the GCM in the future so that it can be used to tackle a wide variety of planetary climate problems.

astro-ph.EP↗

The Strength of Mechanically-Exfoliated Monolayer Graphene

The deformation and fracture behaviour of one-atom-thick mechanically exfoliated graphene has been studied in detail. Monolayer graphene flakes with different lengths, widths and shapes were successfully prepared by mechanical exfoliation and deposited onto poly(methyl methacrylate) (PMMA) beams. The fracture behaviour of the monolayer graphene was followed by deforming the PMMA beams. Through in-situ Raman mapping at different strain levels, the distributions of strain over the graphene flakes were determined from the shift of the graphene Raman 2D band. The failure mechanisms of the exfoliated graphene were either by flake fracture or failure of the graphene/polymer interface. The fracture of the flakes was observed from the formation of cracks identified from the appearance of lines of zero strain in the strain contour maps. It was found that the strength of the monolayer graphene flakes decreased with increasing flake width. The strength dropped to less than 10 GPa for large flakes, much lower than the reported value of 130 GPa for monolayer graphene, thought to be due to the presence of defects. It is shown that a pair of topological defects in monolayer graphene will form a pseudo crack and the effect of such defects upon the strength of monolayer graphene has been modelled using molecular mechanical simulations.

cond-mat.mtrl-sci↗

Chemically Induced Transformation of CVD-Grown Bilayer Graphene into Single Layer Diamond

Notwithstanding numerous density functional studies on the chemically induced transformation of multilayer graphene into a diamond-like film, a comprehensive convincing experimental proof of such a conversion is still lacking. We show that the fluorination of graphene sheets in Bernal (AB)-stacked bilayer graphene (AB-BLG) grown by chemical vapor deposition on a single crystal CuNi(111) surface triggers the formation of interlayer carbon-carbon bonds, resulting in a fluorinated diamond monolayer (F-diamane). Induced by fluorine chemisorption, the phase transition from AB-BLG to single layer diamond was studied and verified by X-ray photoelectron, ultraviolet photoelectron, Raman, UV-Vis, electron energy loss spectroscopies, transmission electron microscopy, and DFT calculations.

cond-mat.mtrl-sci↗

Grain Boundaries in Chemical Vapor Deposited Atomically Thin Hexagonal Boron Nitride

Large-area two-dimensional (2D) materials for technical applications can now be produced by chemical vapor deposition (CVD). Unfortunately, grain boundaries (GBs) are ubiquitously introduced as a result of the coalescence of grains with different crystallographic orientations. It is well known that the properties of materials largely depend on GB structures. Here, we carried out a systematic study on the GB structures in CVD-grown polycrystalline h-BN monolayer films by transmission electron microscope. Interestingly, most of these GBs are revealed to be formed via overlapping between neighboring grains, which are distinct from the covalently bonded GBs as commonly observed in other 2D materials. Further density functional theory (DFT) calculations show that the hydrogen plays an essential role in overlapping GB formation. This work provides an in-depth understanding of the microstructures and formation mechanisms of GBs in CVD-grown h-BN films, which should be informative in guiding the precisely controlled synthesis of large area single crystalline h-BN and other 2D materials.

cond-mat.mtrl-sci↗

Towards the growth of single-crystal boron nitride monolayer on Cu

Atom-layered hexagonal boron nitride (hBN), with excellent stability, flat surface and large bandgap, has been reported to be the best 2D insulator to open up the great possibilities for exciting potential applications in electronics, optoelectronics and photovoltaics. The ability to grow high-quality large single crystals of hBN is at the heart for those applications, but the size of single-crystal 2D BN is less than a millimetre till now. Here, we report the first epitaxial growth of a 10*10 cm2 single-crystal hBN monolayer on a low symmetry Cu(110) "vicinal surface". The growth kinetics, unidirectional alignment and seamless stitching of hBN domains are unambiguously illustrated using centimetre- to the atomic-scale characterization techniques. The findings in this work are expected to significantly boost the massive applications of 2D materials-based devices, and also pave the way for the epitaxial growth of broad non-centrosymmetric 2D materials.

cond-mat.mtrl-sci↗

Global or Local Pure-Condensible Atmospheres: Importance of Horizontal Latent Heat Transport

The distribution of a pure condensible planetary atmosphere in equilibrium with a surface reservoir is revisited employing the energy budget of the climate system, emphasizing the atmospheric horizontal latent heat transport. This configuration is applicable to icy Solar System bodies such as Triton as well as a range of possible exoplanet atmospheres, including water or $\mathrm{CO_2}$ iceballs or ocean worlds, and lava planets with mineral vapor atmospheres. Climate regimes for slowly rotating planets with the hot-spot near the substellar point, and for rapidly rotating planets with a warm equatorial belt, are both treated. A non-dimensional parameter controlling the fractional variation of the surface pressure is derived; it measures whether the pure condensible atmosphere is global or localized. The global pure condensible atmosphere with the non-dimensional parameter much less than order of unity is maintained by the strong horizontal latent heat transport associated with an "evaporation/sublimation-driven flow" from warm to cold places that compensates for the incoming differential radiative forcing. We show that the variation of surface temperature can be estimated in terms of this non-dimensional parameter if it is not too large. In the case of a pure water-vapor atmosphere with an ice or liquid surface, we show that the atmosphere is thick enough to maintain nearly isothermal surface conditions even when the substellar surface temperature is around the freezing point. Finally, it is proposed that the evaporation/sublimation-driven flow regime for global atmospheres could be detected via its effect on the inhomogeneous distribution of minor non-condensible components in the atmosphere.

astro-ph.EP↗

Abrupt climate transition of icy worlds from snowball to moist or runaway greenhouse

Ongoing and future space missions aim to identify potentially habitable planets in our Solar System and beyond. Planetary habitability is determined not only by a planet's current stellar insolation and atmospheric properties, but also by the evolutionary history of its climate. It has been suggested that icy planets and moons become habitable after their initial ice shield melts as their host stars brighten. Here we show from global climate model simulations that a habitable state is not achieved in the climatic evolution of those icy planets and moons that possess an inactive carbonate-silicate cycle and low concentrations of greenhouse gases. Examples for such planetary bodies are the icy moons Europa and Enceladus, and certain icy exoplanets orbiting G and F stars. We find that the stellar fluxes that are required to overcome a planet's initial snowball state are so large that they lead to significant water loss and preclude a habitable planet. Specifically, they exceed the moist greenhouse limit, at which water vapour accumulates at high altitudes where it can readily escape, or the runaway greenhouse limit, at which the strength of the greenhouse increases until the oceans boil away. We suggest that some icy planetary bodies may transition directly to a moist or runaway greenhouse without passing through a habitable Earth-like state.

astro-ph.EP↗

Differences in water vapor radiative transfer among 1D models can significantly affect the inner edge of the habitable zone

An accurate estimate of the inner edge of the habitable zone is critical for determining which exoplanets are potentially habitable and for designing future telescopes to observe them. Here, we explore differences in estimating the inner edge among seven one-dimensional (1D) radiative transfer models: two line-by-line codes (SMART and LBLRTM) as well as five band codes (CAM3, CAM4_Wolf, LMDG, SBDART, and AM2) that are currently being used in global climate models. We compare radiative fluxes and spectra in clear-sky conditions around G- and M-stars, with fixed moist adiabatic profiles for surface temperatures from 250 to 360 K. We find that divergences among the models arise mainly from large uncertainties in water vapor absorption in the window region (10 um) and in the region between 0.2 and 1.5 um. Differences in outgoing longwave radiation increase with surface temperature and reach 10-20 Wm^-2; differences in shortwave reach up to 60 Wm^-2, especially at the surface and in the troposphere, and are larger for an M-dwarf spectrum than a solar spectrum. Differences between the two line-by-line models are significant, although smaller than among the band models. Our results imply that the uncertainty in estimating the insolation threshold of the inner edge (the runaway greenhouse limit) due only to clear-sky radiative transfer is ~10% of modern Earth's solar constant (i.e., ~34 Wm^-2 in global mean) among band models and ~3% between the two line-by-line models. These comparisons show that future work is needed focusing on improving water vapor absorption coefficients in both shortwave and longwave, as well as on increasing the resolution of stellar spectra in broadband models.

astro-ph.EP↗

Size dependence of the Graphene Islands Moving on Cu (111) Surface during the CVD Growth

The graphene islands, formed as different sizes, are crucial for the final quality of the formed graphene during the CVD growth either as the nucleation seeds or as the build blocks for larger graphene domains. Extensive efforts had been devoted to the size or the morphology control while fewer works were reported on the moving dynamics of these graphene islands as well as the associate influences to their coalescence during the CVD Growth of graphene. In this study, based on the self-developed C-Cu empirical potential, we performed systematic molecular dynamics simulations on the surface moving of three typical graphene islands CN (N = 24, 54 and 96) on the Cu (111) surface and discovered their different behaviors in sinking, lateral translation and rotation at the atomic scale owning to their different sizes, which were proved to bring forth significant impacts to their coalescences and the final quality of the as-formed larger domains of graphene. This study would deepen our atomistic insights into the mechanisms of the graphene CVD growth and provide significant theoretical guidelines to its controlled synthesis.

physics.comp-ph↗

Magic Graphene Clusters Formation in the graphene CVD growth process on Ru and Rh

To improve atomically controlled chemical vapor deposition (CVD) growth of graphene, understanding the evolution from various carbon species to a graphene nuclei on various catalyst surfaces is essential. Experimentally, an ultra-stable carbon cluster on Ru(0001), Rh(111) surfaces was observed, while its structure and formation process were still under highly debate. Using ab initio calculations and kinetic analyses, we disclosed a specific type of carbon clusters, composed of a C21 core and a few dangling C atoms around, were exceptional stable in the size range from 21 to 27. The most stable one of them, an isomer of C24 characterized as three dangling C atoms attached to the C21 (denoted as C21-3C), is the most promising candidate for the experimental observation. The ultra-stability of C21-3C originates from both the stable core and the appropriate passivation of dangling carbon atoms by the catalyst surface.

cond-mat.mtrl-sci↗

Ultrafast Epitaxial Growth of Metre-Sized Single-Crystal Graphene on Industrial Cu Foil

A foundation of the modern technology that uses single-crystal silicon has been the growth of high-quality single-crystal Si ingots with diameters up to 12 inches or larger. For many applications of graphene, large-area high-quality (ideally of single-crystal) material will be enabling. Since the first growth on copper foil a decade ago, inch-sized single-crystal graphene has been achieved. We present here the growth, in 20 minutes, of a graphene film of 5 x 50 cm2 dimension with > 99% ultra-highly oriented grains. This growth was achieved by: (i) synthesis of sub-metre-sized single-crystal Cu(111) foil as substrate; (ii) epitaxial growth of graphene islands on the Cu(111) surface; (iii) seamless merging of such graphene islands into a graphene film with high single crystallinity and (iv) the ultrafast growth of graphene film. These achievements were realized by a temperature-driven annealing technique to produce single-crystal Cu(111) from industrial polycrystalline Cu foil and the marvellous effects of a continuous oxygen supply from an adjacent oxide. The as-synthesized graphene film, with very few misoriented grains (if any), has a mobility up to ~ 23,000 cm2V-1s-1 at 4 K and room temperature sheet resistance of ~ 230 ohm/square. It is very likely that this approach can be scaled up to achieve exceptionally large and high-quality graphene films with single crystallinity, and thus realize various industrial-level applications at a low cost.

cond-mat.mtrl-sci↗

Dynamics of atmospheres with a non-dilute condensible component

The diversity of characteristics for the host of recently discovered exoplanets opens up a great deal of fertile new territory for geophysical fluid dynamics, particularly when the fluid flow is coupled to novel thermodynamics, radiative transfer or chemistry. In this paper, we survey one of these new areas-the climate dynamics of atmospheres with a non-dilute condensible component, defined as the situation in which a condensible component of the atmosphere makes up a substantial fraction of the atmospheric mass within some layer. Non-dilute dynamics can occur for a wide range of condensibles, generically applying near both the inner and the outer edges of the conventional habitable zone and in connection with runaway greenhouse phenomena. It also applies in a wide variety of other planetary circumstances. We first present a number of analytical results developing some key features of non-dilute atmospheres, and then show how some of these features are manifest in simulations with a general circulation model adapted to handle non-dilute atmospheres. We find that non-dilute atmospheres have weak horizontal temperature gradients even for rapidly rotating planets, and that their circulations are largely barotropic. The relative humidity of the condensible component tends towards 100% as the atmosphere becomes more non-dilute, which has important implications for runaway greenhouse thresholds. Non-dilute atmospheres exhibit a number of interesting organized convection features, for which there is not yet any adequate theoretical understanding.

astro-ph.EP↗

Convection in Condensible-rich Atmospheres

Condensible substances are nearly ubiquitous in planetary atmospheres. For the most familiar case-water vapor in Earth's present climate-the condensible gas is dilute, in the sense that its concentration is everywhere small relative to the noncondensible background gases. A wide variety of important planetary climate problems involve nondilute condensible substances. These include planets near or undergoing a water vapor runaway and planets near the outer edge of the conventional habitable zone, for which CO2 is the condensible. Standard representations of convection in climate models rely on several approximations appropriate only to the dilute limit, while nondilute convection differs in fundamental ways from dilute convection. In this paper, a simple parameterization of convection valid in the nondilute as well as dilute limits is derived and used to discuss the basic character of nondilute convection. The energy conservation properties of the scheme are discussed in detail and are verified in radiative-convective simulations. As a further illustration of the behavior of the scheme, results for a runaway greenhouse atmosphere for both steady instellation and seasonally varying instellation corresponding to a highly eccentric orbit are presented. The latter case illustrates that the high thermal inertia associated with latent heat in nondilute atmospheres can damp out the effects of even extreme seasonal forcing.

astro-ph.EP↗

Dynamic Modulation of the Transport Properties of the LaAlO3/SrTiO3 Interface Using Uniaxial Strain

Among the interfacial transport modulations to the LaAlO3/SrTiO3 (LAO/STO) heterostructure, mechanical strain has been proven to be an effective approach by growing the LAO/STO films on different substrates with varying lattice mismatches to STO. However, this lattice-mismatch-induced strain effect is static and biaxial, hindering the study of the strain effect in a dynamic way. In this work we realize dynamic and uniaxial strain to the LAO/STO oxide heterostructure at low temperature, through mechanical coupling from a magnetostrictive template. This anisotropic strain results in symmetry breaking at the interface and induces further splitting of the electronic band structure and therefore produces different conductivities along the x and y in-plane directions. In particular, we observe that along the strained direction the interface conductivity decreases by up to 70% under a tensile strain, while it increases by 6.8% under a compressive strain at 2 K. Also, it is revealed that the modulation on the interfacial transport property can be anisotropic, i.e., the resistance changes differently when an excitation current is parallel or perpendicular to the strain direction. This approach of strain engineering provides another degree of freedom for control of transport properties of oxide heterostructures and opens an additional way to investigate strain effects in materials science.

cond-mat.mtrl-sci↗