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Feng Jin

Publications and source records attributed to Feng Jin.

At least 19 recordsLinked to original sources

Thermally enhanced magnon-phonon resonance in van der Waals antiferromagnet FePS3

Strong coupling between collective excitations provides a route to controlling quantum states of matter, yet its evolution under thermal fluctuations remains poorly understood. In the van der Waals antiferromagnet FePS3, strong magnon-phonon coupling is established at low temperatures. At the same time, recent terahertz experiments revealed the counterintuitive stabilization of a long-lived metastable magnetic state with an exceedingly long lifetime of 5 msec at the antiferromagnetic transition, not at the base temperature. This was attributed to a strongly coupled spin-lattice scenario, challenging the conventional wisdom that increased magnetic and thermal fluctuations near TN should be detrimental to the coherent control of a metastable phase. Thus it requires an independent examination for correct understanding. Using high-field Raman spectroscopy, we systematically investigate the temperature evolution of magnon-phonon coupling in FePS3. We observe a pronounced avoided crossing between magnon and phonon modes across a wide range of temperatures and find that the coupling strength remains remarkably robust with increasing temperatures. The zero-field magnon-phonon detuning decreases progressively with warming, driving the system toward resonance and thereby enhancing their hybridization near the transition temperature. This anomalous thermal evolution provides the crucial key to understanding the unusual terahertz-driven states recently reported in FePS3. More broadly, our results highlight van der Waals magnets as a promising platform for strong coupling among collective excitations and for controlling magnetic states through light-matter interactions.

cond-mat.mtrl-sci↗

Intrinsic Raman Modes and Crystal Symmetry of Altermagnetic $α$-MnTe

Crystal symmetry governs the physical properties of materials and provides the framework for interpreting their microscopic excitations and macroscopic responses. In altermagnets, the crystal symmetries that relate opposite-spin sublattices give rise to momentum-dependent spin splitting despite compensated magnetization. Determining the real crystal symmetry is therefore essential for understanding the intrinsic electronic and magnetic properties. For the altermagnetic semiconductor $α$-MnTe, conflicting Raman assignments have left both its intrinsic lattice excitations and its crystal symmetry unresolved. Here we combine high-resolution Raman and second-harmonic generation (SHG) spectroscopy with first-principles calculations to distinguish intrinsic lattice excitations from Te-derived spectral contributions and to examine bulk inversion symmetry of $α$-MnTe. We show that several prominent Raman features previously assigned to $α$-MnTe instead originate from segregated Te clusters or precipitates. The remaining intrinsic Raman response consists of a single Raman-active mode assigned to the calculated $E_{2g}$ phonon, consistent with the centrosymmetric $D_{6h}$ symmetry. The SHG response agrees with surface electric-dipole and bulk electric-quadrupole contributions expected for a centrosymmetric $D_{6h}$ crystal, supporting the preservation of bulk inversion symmetry in $α$-MnTe. Our findings revise the Raman assignments in $α$-MnTe and provide a basis for interpreting its altermagnetic properties within the appropriate crystal-symmetry framework.

cond-mat.mtrl-sci↗

AlignPred: Error-Controlled KV Cache Compression via Alignment and Predictive Coding

Long-running agents retain KV caches across turns and sessions for hours or days. Compressing these persistent caches requires reducing storage while controlling reconstruction error. We present AlignPred, a codec that combines local alignment with predictive coding under a configurable KV reconstruction-error budget. Local orthogonal transforms align related heads or layers into a common coordinate frame, allowing AlignPred to combine token-wise prediction with same-token prediction across heads or layers. Residuals are quantized on an error-bounded lattice and entropy-coded, without learned predictors, encoder-side mode search, or large joint transforms. Across three attention mechanisms, AlignPred requires less storage than the evaluated baselines at comparable measured reconstruction error. Against the evaluated CPU codec implementations, it decodes at least 1.6 times faster while matching or improving encode time. AlignPred achieves near-native task scores at substantially compressed operating points on LongBench-Pro at 128K context. AlignPred's SGLang HiCache integration reduces persistent target-KV storage by 42-72% relative to native HiCache, with comparable latency.

cs.PF↗

Self-Indexing Attention for Compression-Compatible Sparse Long-Context LLM Inference

Sparse long-context inference requires efficient token retrieval in both prefill and decode. Existing methods often use different retrieval strategies for the two stages, preventing one retrieval representation from being reused throughout inference. We propose Self-Indexing Attention, a training-free framework built on a shared transform-domain sign-magnitude representation. The key signs provide a reusable token-level index for grouped prefill selection and decode retrieval, while the same representation remains compatible with external KV-cache compression without separate indexer metadata. This 1-bit index enables efficient retrieval through bitwise operations widely supported by modern accelerators. At 5% attention density, Self-Indexing Attention remains close to dense attention on LongBench and RULER and achieves up to 6.1x prefill and 10.3x decode attention-operator speedups. Experiments with TurboQuant and DeepSeekV4-Flash further demonstrate compatibility with low-bit KV-cache compression and pretrained sparse-attention indexers.

cs.IR↗

Temperature-driven sodium-ion dynamical-to-static crossover in the zig-zag ordered phase of Na$_{0.5}$CoO$_2$

We employ polarization-resolved Raman spectroscopy combined with first-principles calculations to study the sodium-ion lattice dynamics in a sodium zig-zag ordered cobaltate compound Na$_{0.5}$CoO$_2$. We detect two sodium phonon modes for the first time, and their mode frequencies are consistent with first-principles phonon calculations based on an orthorhombic unit cell. We find that they appear below around $T^*\sim300\pm50$K with large linewidth broadening, much lower than the sodium zig-zag ordering temperature $T_\text{S}\sim460$K, and then narrow at lower temperatures. We interpret the sodium-phonon anomalies occurring at $T^*$ as a dynamical-to-static crossover involving mainly the motion of sodium ions. Our results suggest that the gradual freezing of the sodium ions and the well-defined static sodium-zigzag order below $T^*$ set the stage for the emergent electronic and magnetic orders in the CoO$_2$ layer of Na$_{0.5}$CoO$_2$.

cond-mat.mtrl-sci↗

Field-induced multipolar character in the dipolar ground state of the honeycomb rare-earth chalcohalide NdOF

Field-tunable reconstruction of crystalline electric field (CEF) doublets offers a promising avenue for inducing multipolar character, while its observation in real materials has been little explored so far. Here we establish the honeycomb rare-earth chalcohalide NdOF as such a platform. Raman spectroscopy identifies four CEF excitations at 1.7, 15.6, 19.2, and 80.9~meV, and a Zeeman--CEF analysis reproduces their nonlinear field splitting into seven branches. Magnetization and susceptibility over 0.1--9~T are well described by a CEF model for the total angular momentum $J = 9/2$ manifold, confirming the robustness of the extracted CEF scheme. These results demonstrate a field-driven continuous evolution of the ground-state doublet from dipolar to dipolar-multipolar character, with pressure providing a complementary tuning knob, establishing NdOF as a model system for exploring the controlled induction of multipolar components in rare-earth magnets.

cond-mat.str-el↗

Emergent Dispersive Multipolar Excitations in NaErSe$_{2}$

In most condensed-matter systems, local and collective excitations remain decoupled due to their distinct energy scales. Here, we identify coupled local-collective excitations in the triangular antiferromagnet NaErSe$_2$ by combining neutron spectroscopy with total angular momentum modeling. The low-lying crystalline electric field (CEF) doublets include a dipolar $Γ_4$ ground state forming stripe-$x$ order and a $Γ_{5,6}$ excited state with dipole-octupole character. High-resolution spectra reveal emergent symmetry-selected dispersions, where magnon branches from the ground state are replicated on higher $Γ_4$ levels but couple with the $Γ_{5,6}$ levels to form a distinct multipolar band. An applied magnetic field reconstructs the CEF wavefunctions and polarizes the system into a multipolar ferromagnet, further reshaping the spectra. This study demonstrates the emergent coupling of local and collective excitations driven by strong spin-orbit coupling and establishes NaErSe$_2$ as a platform for field-tunable multipolar excitations in frustrated magnets.

cond-mat.str-el↗

MultiPath Memory Access: Breaking Host-GPU Bandwidth Bottlenecks in LLM Services

Host-GPU data movement has become a latency-critical bottleneck in LLM serving, surfacing in common paths such as model-weight movement and KV cache offload/fetch. Today, each host-GPU copy is effectively confined to the PCIe path of the target GPU, even though modern multi-GPU servers contain additional PCIe links on peer GPUs and high bandwidth GPU interconnects. This leaves substantial intra-server I/O capacity unused. To address this issue, we present Multipath Memory Access (MMA), a software-defined multipath memory access system for host--GPU data transfer. To the best of our knowledge, MMA is the first software-defined system to enable efficient multipath host--GPU data transfer within a single multi-GPU server. MMA expands a single host--GPU copy across available direct and relay paths without hardware, driver, or application changes. It preserves CUDA stream semantics with a dependency-preserving Dummy Task, coordinates distributed micro-transfer completion through a lightweight synchronization mechanism, and uses queue backpressure to route traffic without explicit link-state feedback. On an 8-GPU NVIDIA H20 server, MMA achieves 245 GB/s peak host-to-GPU bandwidth, a 4.62x improvement over native CUDA copies, and reduces TTFT for KV cache fetching by 1.14-2.38x and model wake-up/switching latency by 1.12-2.48x.

cs.DC↗

Beam canalization by a non-Abelian gauge field

Hyperbolic and quasi-flat isofrequency contours (IFCs) are used for beam canalization and can be created by tilted Dirac points in photonic systems. Dirac points in microcavities are generated by the combination of transverse-electric/transverse-magnetic splitting and linear birefringence. We show that the canalization is here strongly assisted by the coupling between the spatial dynamics and polarization pseudospin precession. This dynamics is well described analytically and numerically as the action of a non-Abelian gauge field on emergent charges (spin current). We demonstrate a ten-fold enhancement of the canalization for a Gaussian beam by the gauge field, as compared to a description based solely on the group velocity associated with the IFCs.

cond-mat.mes-hall↗

Bragg-Williams order competes with superconductivity

Orderings in charge and spin have been extensively studied to unravel their correlation to emergent superconductivity over the past decades. Bragg-Williams order (BWO), a classical structural order parameter describing site occupancy in alloys, has long been speculated to influence superconducting behavior. Yet, its role still remains ambiguous, largely due to the difficulty of isolating BWO from concomitant charge doping or competing electronic instabilities. Here, we establish In2/3PSe3 as a platform wherein indium vacancies are reversibly configurable between ordered and disordered states via thermal treatment. We show that the disordered phase undergoes a pressure-induced superconducting transition with a Tc of 11 K, significantly higher than the 7 K observed in its ordered counterpart. This constitutes a rare instance in which pure BWO variation drives a substantial shift in Tc. By combining a Ginzburg-Landau phenomenological analysis with a BCS-McMillan microscopic description, we demonstrate that BWO naturally suppresses superconductivity through electron-phonon interactions, a mechanism supported by ultra-low-wavenumber Raman measurements. Our findings support BWO as an independent order parameter that competes directly with superconductivity, extending the concept of competing orders beyond conventional electronic and magnetic degrees of freedom.

cond-mat.supr-con↗

Excitations across the equilibrium and photoinduced `hidden' states of magnetoresistive manganites

"Hidden" phases, generated using ultrafast laser pulses (few hundred femtoseconds), with properties distinct from thermodynamic equilibrium, are appealing for technologies because they can be long-lived, with lifetimes of hours or weeks, and reversible with temperature sweeping or extra pulses. In this regard, La$_{2/3}$Ca$_{1/3}$MnO$_3$ (LCMO) stands out due to its tunability through epitaxial strain, which can drive the bulk ferromagnetic metal (FMM) into an antiferromagnetic insulator (AFI), and its susceptibility to photo-induced transitions. Indeed, AFI LCMO displays a long-lived photo-induced transition into a putative 'hidden' phase whose exact nature and excitations are still largely unknown. Here, we combine ultrafast photo-excitation in the near infrared with in situ transport, x-ray absorption (XAS), and Resonant Inelastic X-ray Scattering (RIXS) to investigate the excitations (polarons, phonons, and orbital) of the photo-excited phase of LCMO and contrast them with the thermodynamic phases achieved through strain and temperature. In the thermodynamic regime, we establish the correlation between polarons and transport, placing them in the 'strong coupling' regime of the Holstein model. Upon photo-excitation of LCMO-AFI, we uncover a long-lived phase characterized by the softening of the polaron excitations, the partial suppression of the Jahn-Teller distortion, and nearly unchanged phonons, showing the emergence of a photo-excited state absent in the equilibrium phase diagram. Finally, by varying temperature, epitaxial strain, and photo-excitation fluence, we construct a polaron phase diagram and identify the key spectroscopic signatures of each phase. Our laser-RIXS approach establishes a versatile platform for exploring photo-induced 'hidden' phases in quantum materials in non-stroboscopic conditions.

cond-mat.str-el↗

Dynamic topological exciton-polaritons enabling ultrafast logic operations

Topological active materials have emerged as powerful paradigm bridging the discovery of exotic topological phases of matter with the development of functional topological devices. The recent extension of these material systems into dynamic regime, where topological properties can be actively manipulated at ultrafast timescales, promises unprecedented control over topological states and their functionalities. However, translating the static topological lasing signals into high-performance logic functions remain highly challenging, which imposes a far more stringent set of materials attributes. Here, leveraging the strong nonlinearity and pronounced spectral isolation of perovskite exciton-polaritons embedded in a Dirac vortex microcavity, we experimentally demonstrate the dynamic topological Majorana-like state polariton condensation with its ultrafast logic operations at room temperature. By actively coordinating pump and control beams in both spectral and temporal domain, we dynamically steer the topological polariton condensation process and demonstrate AND and NOT logic operations, achieving record extinction ratio (~20 dB), extremely low control fluence (~0.2 nJ/cm2) and sub-picosecond response time (~500 fs). Our results expand the frontier of dynamic topology and establish a novel pathway towards robust, ultrafast, and reconfigurable on-chip polaritonic logic circuits.

physics.optics↗

Optically reconfigurable canalization of exciton-polaritons in a non-hyperbolic perovskite

The ability to steer polariton flow on-demand holds significant promise towards nanophotonic applications and photonic circuitry. Polariton canalization, exhibiting intrinsic collimation and diffractionless transport, emerges as a promising solution without guiding structures. However, earlier demonstrations have been restricted to certain crystal surfaces with intrinsic hyperbolic responses and operated in the linear regime. Here, we experimentally demonstrate canalization of nonlinear exciton polariton condensates with optical reconfigurability in a birefringent CsPbBr3 perovskite crystal without intrinsic hyperbolic response. By embedding the birefringent perovskite crystal into a planar microcavity, the interplay between cavity transverse-electric-transverse-magnetic splitting and crystalline birefringence produces an anisotropic band geometry with a hyperbolic-flat-parabolic evolution of polaritonic isofrequency contours (IFCs). Nonresonant pumping drives exciton polariton condensation onto flat far-field contours with nonlinear emission amplification, leading to coherent canalized flows with over twentyfold collimation with respect to arc-shaped contours. Reconfiguring the optical pumping-spot size allows switching the nonlinear polariton condensates into hyperbolic and parabolic IFC regimes, leading to divergent propagation behaviour with collimating reconfiguration. Our study reveals a distinct canalization framework for shaping the nonlinear exciton-polariton condensate flows, opening opportunities for all-optical polaritonic logic circuits based on stabilized nonlinear quantum interconnects.

physics.optics↗

Tunable spin-phonon polarons in a chiral molecular qubit framework

Chiral structures that produce asymmetric spin-phonon coupling can theoretically generate spin-phonon polarons -- quasiparticles exhibiting non-degenerate spin states with phonon displacements. These quasiparticles are speculated to be the origin of chirality-induced spin selectivity and presumably can display exotic dynamic behaviors. However, direct experimental evidence of spin-phonon polarons has been lacking. Using a chiral molecular qubit framework embedding stable semiquinone-like radicals, we report spin dynamic signatures that indicate the formation of spin-phonon polarons for the first time. Our non-adiabatic model reveals that these quasiparticles introduce an active spin relaxation channel when polaron reorganization energy approaches Zeeman splitting. This new channel manifests itself as anomalous, temperature-independent spin relaxation, which can be suppressed by high magnetic fields or pore-filling solvents (e.g. CH2Cl2, CS2). Such field- and guest-tunable relaxation is unattainable in conventional spin systems. Harnessing this mechanism could boost repetition rates in spin-based quantum information technologies without compromising coherence or quantum sensing performance.

cond-mat.mes-hall↗

Symmetry-engineered and electrically tunable in-plane anomalous Hall effect in oxide heterostructures

The family of Hall effects has long served as a premier probe of how symmetry, magnetic order, and topology intertwine in solids. Recently, the in-plane anomalous Hall effect (IP-AHE), a transverse Hall response driven by in-plane magnetization, has emerged as a distinct member of this family, offering innovative spintronic functionalities and illuminating intricate interplay between mirror-symmetry breaking and in-plane magnetic order. However, practical routes to deterministically and reversibly control IP-AHE remain limited. Here, we establish a symmetry-engineered IP-AHE platform, CaRuO3/La2/3Ca1/3MnO3/CaRuO3 heterostructure on NdGaO3(110), that turns strict mirror-symmetry breaking constraints into effective tuning knobs. IP-AHE in these epitaxial trilayers unambiguously couples to the CaRuO3-buffer-induced mirror-symmetry breaking and faithfully reproduces the ferromagnetic hysteresis. Ionic liquid gating further enables reversible reconfigurations of the symmetry breaking, thereby achieving electrical modulation and ON/OFF switching of IP-AHE. This highly tunable IP-AHE platform opens pathways for exploring nontrivial magnetic order and developing programmable Hall functionalities in planar geometries.

cond-mat.str-el↗

Quantum fluctuations associated with first-order magnetic transition in a frustrated kagome lattice antiferromagnet

Intense quantum fluctuations arising from geometrical frustrations in kagome-lattice magnets provide a feasible approach to exotic quantum states. Here, we document an unexpected isosymmetric first-order magnetic transition in the recently synthesized frustrated kagome-lattice antiferromagnet Nd3ScBi5, which is characterized by significant latent heat and a pronounced magnetocaloric effect, as well as discontinuous Raman shifts and negligible hysteresis. Employing the magnetocaloric effect as a detection method, in conjunction with systematical field-dependent physical properties, we uncover a distinctive 1/2 magnetization plateau phase with significant quantum fluctuations. Our study unveils Nd3ScBi5 as a prototypical model with an emerging phase of enhanced quantum fluctuations triggered by first-order magnetic transitions.

cond-mat.str-el↗

Anomalous enhancement of magnetism by nonmagnetic doping in the honeycomb-lattice antiferromagnet ErOCl

Tuning magnetic anisotropy through chemical doping is a powerful strategy for designing functional materials with enhanced magnetic properties. Here, we report an enhanced Er^3+ magnetic moment resulting from nonmagnetic Lu^3+ substitution in the honeycomb-lattice antiferromagnet ErOCl. Unlike the Curie-Weiss type divergence typically observed in diluted magnetic systems, our findings reveal a distinct enhancement of magnetization per Er^3+ ion under high magnetic fields, suggesting an unconventional mechanism. Structural analysis reveals that Lu^3+ doping leads to a pronounced contraction of the c axis, which is attributed to chemical pressure effects, while preserving the layered SmSI-type crystal structure with space group R-3m. High-resolution Raman spectroscopy reveals a systematic blueshift of the first and seventh crystalline electric field (CEF) excitations, indicating an increase in the axial CEF parameter B_2^0. This modification enhances the magnetic anisotropy along the c axis, leading to a significant increase in magnetization at low temperatures and under high magnetic fields, contrary to conventional expectations for magnetic dilution. Our work not only clarifies the intimate connection between magnetism and CEF in rare-earth compounds, but more importantly, it reveals a physical pathway to effectively tune magnetic anisotropy via anisotropic lattice distortion induced by chemical pressure.

cond-mat.mtrl-sci↗

Hidden phonon-assisted charge density wave transition in BaFe2Al9 revealed by ultrafast optical spectroscopy

The interplay between electronic and lattice degrees of freedom is fundamental to charge density wave (CDW) formation, yet the microscopic origin often remains elusive. Here, we investigate the transient optical response of the intermetallic compound BaFe2Al9 using polarization-resolved ultrafast optical spectroscopy. We identify a discontinuous sign reversal in the transient reflectivity at Tc ~ 110 K, providing unambiguous evidence for the first-order transition. The anisotropic quasiparticle relaxation establishes the three-dimensional nature of the ordered state. Below Tc, a single coherent 1.6 THz oscillation appears abruptly and remains confined to the CDW phase. This mode exhibits weak temperature dependence with negligible softening and is absent in Raman spectra. First-principles calculations imply that it is a precursor phonon at the CDW wave vector with strong electron-phonon coupling. Our results indicate that the CDW in BaFe2Al9 arises from intertwined electronic and lattice instabilities, assisted by a displacive mechanism mediated by a hidden strongly coupled phonon, distinct from conventional amplitude-mode softening scenarios.

cond-mat.str-el↗