arXiv subjects

Ferdinand Schmidt-Kaler

Publications and source records attributed to Ferdinand Schmidt-Kaler.

At least 73 records · Page 4Linked to original sources

arXiv2019

Excitation of E1-forbidden Atomic Transitions with Electric, Magnetic or Mixed Multipolarity in Light Fields Carrying Orbital and Spin Angular Momentum

Photons carrying a well-defined orbital angular momentum have been proven to modify spectroscopic selection rules in atomic matter. Excitation profiles of electric quadrupole transitions have been measured with single trapped $^{40}$Ca$^+$ ions for varying polarizations. We further develop the photo-absorption formalism to study the case of arbitrary alignment of the beam's optical axis with respect to the ion's quantization axis and mixed multipolarity. Thus, predictions for M1-dominated $^{40}Ar^{13+}$, E3-driven $^{171}Yb^+$ and $^{172}Yb^+$, and B-like $^{20}Ne^{5+}$ are presented. The latter case displays novel effects, coming from the presence of a strong photon -- magnetic dipole coupling.

quant-ph↗

arXiv2018

Trapping and sympathetic cooling of single thorium ions for spectroscopy

Precision optical spectroscopy of exotic ions reveals accurate information about nuclear properties such as charge radii and magnetic and quadrupole moments. Thorium ions exhibit unique nuclear properties with high relevance for testing symmetries of nature. We report loading and trapping of single $^{232}$Th$^+$ ions in a linear Paul trap, embedded into and sympathetically cooled by small crystals of trapped $^{40}$Ca$^+$ ions. Trapped Th ions are identified in a non-destructive manner from the voids in the laser-induced Ca fluorescence pattern emitted by the crystal, and alternatively, by means of a time-of-flight signal when extracting ions from the Paul trap and steering them into an external detector. We have loaded and handled a total of 231 individual Th ions. We reach a time-of-flight detection efficiency of $\gtrsim 95\, \%$, consistent with the quantum efficiency of the detector. The sympathetic cooling technique is expected to be applicable for other isotopes and various charge states of Th e.g., for future studies of $^{229m}$Th.

physics.atom-ph↗

arXiv2017

Efficient and robust photo-ionization loading of beryllium ions

We demonstrate the efficient generation of Be$^+$ ions with a 60 ns and 150 nJ laser pulse near 235 nm for two-step photo-ionization, proven by subsequent counting the number of ions loaded into a linear Paul trap. The bandwidth and power of the laser pulse are chosen in such a way that a first, resonant step fully saturates the entire velocity distribution of beryllium atoms effusing from a thermal oven. The second excitation step is driven by the same light field causing efficient non-resonant ionization. Our ion-loading scheme is more than 15 times more efficient as compared to former pathways using two-photon continuous wave laser excitation.

physics.atom-ph↗

arXiv2017

Experimental Verification of Position-Dependent Angular-Momentum Selection Rules for Absorption of Twisted Light by a Bound Electron

We analyze the multipole excitation of atoms with twisted light, i.e., by a vortex light field that carries orbital angular momentum. A single trapped $^{40}$Ca$^+$ ion serves as a localized and positioned probe of the exciting field. We drive the $S_{1/2} \to D_{5/2}$ transition and observe the relative strengths of different transitions, depending on the ion's transversal position with respect to the center of the vortex light field. On the other hand, transition amplitudes are calculated for a twisted light field in form of a Bessel beam, a Bessel-Gauss and a Gauss-Laguerre mode. Analyzing experimental obtained transition amplitudes we find agreement with the theoretical predictions at a level of better than 3\%. Finally, we propose measurement schemes with two-ion crystals to enhance the sensing accuracy of vortex modes in future experiments.

quant-ph↗

arXiv2017

Twisted-ligth--ion interaction: the role of longitudinal fields

The propagation of light beams is well described using the paraxial approximation, where field components along the propagation direction are usually neglected. For strongly inhomogeneous or shaped light fields, however, this approximation may fail, leading to intriguing variations of the light-matter interaction. This is the case of twisted light having opposite orbital and spin angular momenta. We compare experimental data for the excitation of a quadrupole transition in a single trapped $^{40}$Ca$^+$ ion by Schmiegelow et al, Nat.\ Comm.\ 7, 12998 (2016), with a complete model where longitudinal components of the electric field are taken into account. Our model matches the experimental data and excludes by 11 standard deviations the approximation of complete transverse field. This demonstrates the importance of all field components in the interaction of twisted light with matter.

physics.optics↗

arXiv2016

Investigation of two-frequency Paul traps for antihydrogen production

Radio-frequency (rf) Paul traps operated with multifrequency rf trapping potentials provide the ability to independently confine charged particle species with widely different charge-to-mass ratios. In particular, these traps may find use in the field of antihydrogen recombination, allowing antiproton and positron clouds to be trapped and confined in the same volume without the use of large superconducting magnets. We explore the stability regions of two-frequency Paul traps and perform numerical simulations of small, multispecies charged-particle mixtures that indicate the promise of these traps for antihydrogen recombination.

physics.atom-ph↗

arXiv2016

Fast ion swapping for quantum information processing

We demonstrate a SWAP gate between laser-cooled ions in a segmented microtrap via fast physical swapping of the ion positions. This operation is used in conjunction with qubit initialization, manipulation and readout, and with other types of shuttling operations such as linear transport and crystal separation and merging. Combining these operations, we perform quantum process tomography of the SWAP gate, obtaining a mean process fidelity of 99.5(5)\%. The swap operation is demonstrated with motional excitations below 0.05(1)~quanta for all six collective modes of a two-ion crystal, for a process duration of 42~$μ$s. Extending these techniques to three ions, we reverse the order of a three-ion crystal and reconstruct the truth table for this operation, resulting in a mean process fidelity of 99.96(13)\% in the logical basis.

quant-ph↗

arXiv2016

A long-lived Zeeman trapped-ion qubit

We demonstrate a coherence time of 2.1(1)~s for electron spin superposition states of a single trapped $^{40}$Ca$^+$ ion. The coherence time, measured with a spin-echo experiment, corresponds to residual rms magnetic field fluctuations $\leq$~2.7$\times$10$^{-12}$~T. The suppression of decoherence induced by fluctuating magnetic fields is achieved by combining a two-layer $μ$-metal shield, which reduces external magnetic noise by 20 to 30~dB for frequencies of 50~Hz to 100~kHz, with Sm$_2$Co$_{17}$ permanent magnets for generating a quantizing magnetic field of 0.37~mT. Our results extend the coherence time of the simple-to-operate spin qubit to ultralong coherence times which so far have been observed only for magnetic insensitive transitions in atomic qubits with hyperfine structure.

quant-ph↗

arXiv2016

Maximizing the information gain of a single ion microscope using bayes experimental design

We show nanoscopic transmission microscopy, using a deterministic single particle source and compare the resulting images in terms of signal-to-noise ratio, with those of conventional Poissonian sources. Our source is realized by deterministic extraction of laser-cooled calcium ions from a Paul trap. Gating by the extraction event allows for the suppression of detector dark counts by six orders of magnitude. Using the Bayes experimental design method, the deterministic characteristics of this source are harnessed to maximize information gain, when imaging structures with a parametrizable transmission function. We demonstrate such optimized imaging by determining parameter values of one and two dimensional transmissive structures.

quant-ph↗

arXiv2016

A Quantum Repeater Node with Trapped Ions: A Realistic Case Example

We evaluate the feasibility of the implementation of two quantum repeater protocols with an existing experimental platform based on a $^{40}$Ca$^+$-ion in a segmented micro trap, and a third one that requires small changes to the platform. A fiber cavity serves as an ion-light interface. Its small mode volume allows for a large coupling strength of $g_c = 2 π20$ MHz despite comparatively large losses $κ= 2 π36.6$ MHz. With a fiber diameter of 125 mu m, the cavity is integrated into the microstructured ion trap, which in turn is used to transport single ions in and out of the interaction zone in the fiber cavity. We evaluate the entanglement generation rate for a given fidelity using parameters from the experimental setup. The DLCZ protocol (Duan et al, Nature, 2001, 414, 413-418) and the hybrid protocol (van Loock et al, Phys. Rev. Lett., 2006, 96, 240501) outperform the EPR protocol (Sanguard et al, New J. Phys., 2013, 15, 085004). We calculate rates of more than than 35 s$^{-1}$ for non-local Bell state fidelities larger than 0.9 with the existing platform. We identify parameters which mainly limit the attainable rates, and conclude that entanglement generation rates of 740 s$^{-1}$ at fidelities of 0.9 are within reach with current technology.

quant-ph↗

arXiv2016

Visibility of Young's interference fringes: Scattered light from small ion crystals

We observe interference in the light scattered from trapped $^{40}$Ca$^+$ ion crystals. By varying the intensity of the excitation laser, we study the influence of elastic and inelastic scattering on the visibility of the fringe pattern and discriminate its effect from that of the ion temperature and wave-packet localization. In this way we determine the complex degree of coherence and the mutual coherence of light fields produced by individual atoms. We obtain interference fringes from crystals consisting of two, three and four ions in a harmonic trap. Control of the trapping potential allows for the adjustment of the interatomic distances and thus the formation of linear arrays of atoms serving as a regular grating of microscopic scatterers.

quant-ph↗

arXiv2015

Microscopy with a Deterministic Single Ion Source

We realize a single particle microscope by using deterministically extracted laser cooled $^{40}$Ca$^+$ ions from a Paul trap as probe particles for transmission imaging. We demonstrate focusing of the ions with a resolution of 5.8$\;\pm\;$1.0$\,$nm and a minimum two-sample deviation of the beam position of 1.5$\,$nm in the focal plane. The deterministic source, even when used in combination with an imperfect detector, gives rise to much higher signal to noise ratios as compared with conventional Poissonian sources. Gating of the detector signal by the extraction event suppresses dark counts by 6 orders of magnitude. We implement a Bayes experimental design approach to microscopy in order to maximize the gain in spatial information. We demonstrate this method by determining the position of a 1$\,μ$m circular hole structure to an accuracy of 2.7$\,$nm using only 579 probe particles.

physics.atom-ph↗

arXiv2015

Excitation of an Atomic Transition with a Vortex Laser Beam

Photons carry one unit of angular momentum associated with their spin~\cite{Beth1936}. Structured vortex beams carry additional orbital angular momentum which can also be transferred to matter~\cite{Allen1992}. This extra twist has been used for example to drive motion of microscopic particles in optical tweezers as well as to create vortices in degenerate quantum gases~\cite{He1995,Andersen2006}. Here we demonstrate the transfer of optical orbital angular momentum from the transverse spatial structure of the beam to the internal (electronic) degrees of freedom of an atom. Probing a quadrupole transition of a single trapped $^{40}$Ca$^+$ ion localized at the center of the vortex, we observe strongly modified selection rules, accounting for both the photon spin and the vorticity of the field. In particular, we show that an atom can absorb two quanta of angular momentum from a single photon even when rotational symmetry is conserved. In contrast to previous findings~\cite{Araoka2005,Loeffler2011a,Mathevet2013}, our experiment allows for conditions where the vorticity of the laser beam determines the optical excitation, contributing to the long-standing discussion on whether the orbital angular momentum of photons can be transferred to atomic internal degrees of freedom~\cite{VanEnk1994,Babiker2002,Jauregui2004, Schmiegelow2012, Mondal2014, Scholz-Marggraf2014} and paves the way for its use to tailor light-matter interactions.

quant-ph↗

arXiv2015

A single-atom heat engine

We report the experimental realization of a single-atom heat engine. An ion is confined in a linear Paul trap with tapered geometry and driven thermally by coupling it alternately to hot and cold reservoirs. The output power of the engine is used to drive a harmonic oscillation. From direct measurements of the ion dynamics, we determine the thermodynamic cycles for various temperature differences of the reservoirs. We use these cycles to evaluate power $P$ and efficiency $η$ of the engine, obtaining up to $P=342\,$yJ and $η=0.28 \,\%$, consistent with analytical estimations. Our results demonstrate that thermal machines can be reduced to the ultimate limit of single atoms.

cond-mat.stat-mech↗

arXiv2015

Phase-stable free-space optical lattices for trapped ions

We demonstrate control of the absolute phase of an optical lattice with respect to a single trapped ion. The lattice is generated by off-resonant free-space laser beams, we actively stabilize its phase by measuring its ac-Stark shift on a trapped ion. The ion is localized within the standing wave to better than 2\% of its period. The locked lattice allows us to apply displacement operations via resonant optical forces with a controlled direction in phase space. Moreover, we observe the lattice-induced phase evolution of spin superposition states in order to analyze the relevant decoherence mechanisms. Finally, we employ lattice-induced phase shifts for inferring the variation of the ion position over 157~$μ$m range along the trap axis at accuracies of better than 6~nm.

quant-ph↗

arXiv2015

Optimal Phonon-to-Spin Mapping in a system of a trapped ion

We propose a protocol for measurement of the phonon number distribution of a harmonic oscillator based on selective mapping to a discrete spin-1/2 degree of freedom. We consider a system of a harmonically trapped ion, where a transition between two long lived states can be driven with resolved motional sidebands. The required unitary transforms are generated by amplitude-modulated polychromatic radiation fields, where the time-domain ramps are obtained from numerical optimization by application of the Chopped RAndom Basis (CRAB) algorithm. We provide a detailed analysis of the scaling behavior of the attainable fidelities and required times for the mapping transform with respect to the size of the Hilbert space. As one application we show how the mapping can be employed as a building block for experiments which require measurement of the work distribution of a quantum process.

quant-ph↗

arXiv2015

Fast thermometry for trapped ions using dark resonances

We experimentally demonstrate a method to determine the temperature of trapped ions which is suitable for monitoring fast thermalization processes. We show that observing and analyzing the lineshape of dark resonances in the fluorescence spectrum provides a temperature measurement which accurate over a large dynamic range, applied to single ions and small ion crystals. Laser induced fluorescence is detected over a time of only $20\,μ$s allowing for rapid determination of the ion temperature. In the measurement range of $10^{-1}-10^{+2}\,$mK we reach better than $15\,\%$ accuracy. Tuning the cooling laser to selected resonance features allows for controlling the ion temperatures between $0.7\,$mK and more than $10\,$mK. Experimental work is supported by a solution of the 8-level optical Bloch equations when including the ions classical motion. This technique paves the way for many experiments comprising heat transport in ion strings, heat engines, non-equilibrium thermodynamics or thermometry of large ion crystals.

quant-ph↗

arXiv2015

Hexagonal Plaquette Spin-spin Interactions and Quantum Magnetism in a Two-dimensional Ion Crystal

We propose a trapped ion scheme en route to realize spin Hamiltonians on a Kagome lattice which, at low energies, are described by emergent Z2 gauge fields, and support a topological quantum spin liquid ground state. The enabling element in our scheme is the hexagonal plaquette spin-spin interactions in a 2D ion crystal. For this, the phonon-mode spectrum of the crystal is engineered by standing-wave optical potentials or by using Rydberg excited ions, thus generating localized phonon-modes around a hexagon of ions selected out of the entire two-dimensional crystal. These tailored modes can mediate spin-spin interactions between ion-qubits on a hexagonal plaquette when subject to state-dependent optical dipole forces. We discuss how these interactions can be employed to emulate a generalized Balents-Fisher-Girvin model in minimal instances of one and two plaquettes. This model is an archetypical Hamiltonian in which gauge fields are the emergent degrees of freedom on top of the classical ground state manifold. Under realistic situations, we show the emergence of a discrete Gauss's law as well as the dynamics of a deconfined charge excitation on a gauge-invariant background using the two-plaquettes trapped ions spin-system. The proposed scheme in principle allows further scaling in a future trapped ion quantum simulator, and we conclude that our work will pave the way towards the simulation of emergent gauge theories and quantum spin liquids in trapped ion systems.

cond-mat.quant-gas↗