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Filippo De Luca

Publications and source records attributed to Filippo De Luca.

4 recordsLinked to original sources

Generic nonlocal statistics of the stationary measure in conserved active systems

The stationary measure of equilibrium systems with detailed balance follows a Boltzmann distribution, so that for short-ranged interactions the measure is local, meaning that distant spatial domains are statistically independent. In contrast, active systems break detailed balance, and can have nonlocal stationary measure even for fully local dynamics. Here, by expanding in nonlinearity about a Gaussian-model limit, we construct the measure perturbatively deep in the disordered phase for a class of models that includes Active Model A, Active Model B+, Model AB, the Nonreciprocal Cahn--Hilliard model, and the Toner--Tu model. In this regime, nonlocality is linked to a dynamical conservation law. Our results generically preclude construction of a Landau--Ginzburg expansion of the stationary measure (as opposed to the dynamical equations) for conserved active field theories.

cond-mat.stat-mech

Active Cahn-Hilliard theory for nonequilibrium phase separation: quantitative macroscopic predictions and a microscopic derivation

Phase-separating active systems can display phenomenology that is impossible in equilibrium. The binodal densities are not solely determined by a bulk (effective) free energy, but also affected by gradient terms, while capillary waves and Ostwald processes are determined by three distinct interfacial tensions. These and related phenomena were so far explained at continuum level using a top-down minimal theory (Active Model B+). This theory, by Taylor-expanding in the scalar order parameter (or density), effectively assumes that phase separation is weak, which is not true across most of the phase diagram. Here, we develop a quantitative account of active phase separation, by introducing an active counterpart of Cahn-Hilliard theory, constructing the density current from all possible terms with up to four spatial derivatives without Taylor-expanding in the density. From this O(grad^4) theory, we show how to compute binodals and interfacial tensions for arbitrary choices of the five density-dependent 'coefficient functions' that specify the theory (replacing the four constant coefficients of Active Model B+). We further consider a particle model composed of thermal quorum-sensing active particles (tQSAPs) yielding a fully specified example of the O(grad^4) theory upon coarse-graining. We find that to coarse-grain consistently at O(grad^4) requires a systematic procedure, based on multiple-scale analysis, to eliminate fast-evolving orientational moments. Using this, we calculate from microscopic physics all five coefficient functions of the active Cahn-Hilliard theory for tQSAPs. We identify contributions that were missed in previous continuum theories, and show how neglecting them becomes justified only in the limit of large quorum-sensing range parameter. Comparison with particle simulations of tQSAPs shows that our O(grad^4) theory improves on previous continuum models [...]

cond-mat.stat-mech

Hyperuniformity in phase ordering: the roles of activity, noise, and non-constant mobility

Hyperuniformity emerges generically in the coarsening regime of phase-separating fluids. Numerical studies of active and passive systems have shown that the structure factor $S(q)$ behaves as $q^ς$ for $q\to 0$, with hyperuniformity exponent $ς= 4$. For passive systems, this result was explained in 1991 by a qualitative scaling analysis of Tomita, exploiting isotropy at scales much larger than the coarsening length $\ell$. Here we reconsider and extend Tomita's argument to address cases of active phase separation and of non-constant mobility, again finding $ς=4$. We further show that dynamical noise of variance $D$ creates a transient $ς= 2$ regime for $\hat q\ll \hat{q}_\ast \sim \sqrt{D} t^{[1-(d+2)ν]/2}$, crossing over to $ς= 4$ at larger $\hat{q}$. Here, $ν$ is the coarsening exponent, with $\ell\sim t^ν$, and $\hat{q} \propto q \ell$ is the rescaled wavenumber. In diffusive coarsening, $ν=1/3$, so the rescaled crossover wavevector $\hat{q}_\ast$ vanishes at large times when $d\geq 2$. The slowness of this decay suggests a natural explanation for experiments that observe a long-lived $ς= 2$ scaling in phase-separating active fluids (where noise is typically large). Conversely, in $d=1$, we demonstrate that with noise the $ς= 2$ regime survives as $t\to\infty$, with $\hat{q}_\ast\sim D^{5/6}$. (The structure factor is not then determined by the zero-temperature fixed point.) We confirm our analytical predictions by numerical simulations of active and passive continuum theories in the deterministic case and of Model B for the stochastic case. We also compare them with related findings for a system near an absorbing-state transition rather than undergoing phase separation. A central role is played throughout by the presence or absence of a conservation law for the centre of mass position of the order parameter field.

cond-mat.soft

Supramolecular assemblies in active motor-filament systems: micelles, bilayers, and foams

Active matter systems evade the constraints of thermal equilibrium, leading to the emergence of intriguing collective behavior. A paradigmatic example is given by motor-filament mixtures, where the motion of motor proteins drives alignment and sliding interactions between filaments and their self-organization into macroscopic structures. After defining a microscopic model for these systems, we derive continuum equations, exhibiting the formation of active supramolecular assemblies such as micelles, bilayers and foams. The transition between these structures is driven by a branching instability, which destabilizes the orientational order within the micelles, leading to the growth of bilayers at high microtubule densities. Additionally, we identify a fingering instability, modulating the shape of the micelle interface at high motor densities. We study the role of various mechanisms in these two instabilities, such as contractility, active splay, and anchoring, allowing for generalization beyond the system considered here.

cond-mat.soft