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Filomena M. Nunes

Publications and source records attributed to Filomena M. Nunes.

11 recordsLinked to original sources

Systematic study of the validity of the eikonal model including uncertainties

Nuclear reactions at intermediate beam energies are often interpreted using the eikonal model. In the analysis of complex reaction probes, where few-body reaction methods are needed, the eikonal method may be used as an efficient way for describing the fragment-target reaction process. In this work, we perform a systematic study to test the validity of the eikonal approximation for nucleon-nucleus reactions. We also quantify uncertainties due to the nucleon optical potential on reaction observables. We inspect the validity of the eikonal model and its semiclassical correction by comparing it to exact solutions (obtained from solving the optical model equation with a finite differences method) for a wide range of reactions. We also study the effect of relativistic corrections, both kinematic and dynamic, by effectively incorporating the relativistic effects at intermediate energies. The uncertainties from a Bayesian global optical potential (KDUQ) are propagated to the observables of interest. Our study includes neutron and proton reactions on $^{27}$Al, $^{40}$Ca, $^{90}$Zr and $^{208}$Pb, for a wide range of energies $E_{lab}=0-400$ MeV. Our results show that for the proton absorption cross section, the eikonal model can be used down to around $60$ MeV and the semiclassical correction extends its use to $30$ MeV. However, the validity of the eikonal model for the neutron total cross section only goes down to $\approx120$ MeV, a range extended to $\approx 50$ MeV when using the semiclassical correction. We find the semi-classical correction to the eikonal model to be less effective in describing the angular distributions. The $1σ$ uncertainty intervals on the observables we studied is less than $5$% for most of the energies considered, but increases rapidly for higher energies, namely energies outside the range of KDUQ ($E_{lab}>200$ MeV).

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Systematic study of the propagation of uncertainties to transfer observables

A systematic study of parametric uncertainties in transfer reactions is performed using the recently developed uncertainty quantified global optical potential (KDUQ). We consider reactions on the doubly-magic spherical nucleus $^{48}$Ca and explore the dependence of the predicted $(d,p)$ angular distribution uncertainties at different beam energies and for different properties of the final single-particle state populated by the reaction. Our results show that correlations between the uncertainties associated with the bound state potential and with the optical potentials may be important for correctly determining the uncertainty in the transfer cross sections (in our case, these do not add in quadrature). In general, we find small uncertainties in the predicted transfer observables: half-width of the 68% credible interval is roughly $5-10$%, which is comparable to the experimental error on the transfer data. Finally, our results show that the relative magnitude of the parametric uncertainty in transfer observables increases with the beam energy and does not depend strongly on the properties of the final state.

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ROSE: A reduced-order scattering emulator for optical models

A new generation of phenomenological optical potentials requires robust calibration and uncertainty quantification, motivating the use of Bayesian statistical methods. These Bayesian methods usually require calculating observables for thousands or even millions of parameter sets, making fast and accurate emulators highly desirable or even essential. Emulating scattering across different energies or with interactions such as optical potentials is challenging because of the non-affine parameter dependence, meaning the parameters do not all factorize from individual operators. Here we introduce and demonstrate the Reduced Order Scattering Emulator (ROSE) framework, a reduced basis emulator that can handle non-affine problems. ROSE is fully extensible and works within the publicly available BAND Framework software suite for calibration, model mixing, and experimental design. As a demonstration problem, we use ROSE to calibrate a realistic nucleon-target scattering model through the calculation of elastic cross sections. This problem shows the practical value of the ROSE framework for Bayesian uncertainty quantification with controlled trade-offs between emulator speed and accuracy as compared to high-fidelity solvers. Planned extensions of ROSE are discussed.

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New perspectives on spectroscopic factor quenching from reactions

The evolution of single-particle strengths as the neutron-to-proton asymmetry changes informs us of the importance of short- and long-range correlations in nuclei and has therefore been extensively studied for the last two decades. Surprisingly, the strong asymmetry dependence of these strengths and their extreme values for highly-asymmetric nuclei inferred from knockout reaction measurements on a target nucleus are not consistent with what is extracted from electron-induced, transfer, and quasi-free reaction data, constituting a two-decade old puzzle. This work presents the first consistent analysis of one-nucleon transfer and one-nucleon knockout data, in which theoretical uncertainties associated with the nucleon-nucleus effective interactions considered in the reaction models are quantified using a Bayesian analysis. Our results demonstrate that, taking into account these uncertainties, the spectroscopic strengths of loosely-bound nucleons extracted from both probes agree with each other and, although there are still discrepancies for deeply-bound nucleons, the slope of the asymmetry dependence of the single-particle strengths inferred from transfer and knockout reactions are consistent within $1σ$. Both probes are consistent with a small asymmetry dependence of these strengths. The uncertainties obtained in this work represent a lower bound and are already significantly larger than the original estimates.

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Quantifying uncertainties due to optical potentials in one-neutron knockout reactions

One-neutron knockout reactions have been widely used to extract information about the single-particle structure of nuclei from the valley of stability to the driplines. The interpretation of knockout data relies on reaction models, where the uncertainties are typically not accounted for. In this work we quantify uncertainties of optical potentials used in these reaction models and propagate them, for the first time, to knockout observables using a Bayesian analysis. We study two reactions in the present paper, the first of which involves a loosely-bound halo projectile, $^{11}$Be, and the second a tightly-bound projectile, $^{12}$C. We first quantify the parametric uncertainties associated with phenomenological optical potentials. Complementing to this approach, we also quantify the model uncertainties associated with the chiral forces that can be used to construct microscopic optical potentials. For the phenomenological study, we investigate the impact of the imaginary terms of the optical potential on the breakup and stripping components of the knockout cross sections as well as the impact of the angular range. For the $^{11}$Be case, the theoretical uncertainty from the phenomenological method is on the order of the experiment uncertainty on the knockout observables; however, for the $^{12}$C case, the theoretical uncertainty is significantly larger. The widths of the confidence intervals for the knockout observables obtained for the microscopic study and the phenomenological approach are of similar order of magnitude. Based on this work we conclude that structure information inferred from the ratio of the knockout cross sections, will carry a theoretical uncertainty of at least $20\%$ for halo nuclei and at least $40\%$ for tightly-bound nuclei.

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The complete quantification of parametric uncertainties in (d,p) transfer reactions

Previous work quantified the uncertainty associated with the optical potentials between the nucleons and the target. In this study, we extend that work by also including the parameters of the mean field associated with the overlap function of the final bound state, thus obtaining the full parametric uncertainty on transfer observables. We use Bayesian Markov Chain Monte Carlo simulations to obtain parameter posterior distributions. We use elastic-scattering cross sections to constrain the optical potential parameters and use the asymptotic normalization coefficient of the final state to constrain the bound state interaction. We then propagate these posteriors to the transfer angular distributions and obtain confidence intervals for this observable. We study (d,p) reactions on 14C, 16O, and 48Ca at energies in the range E=10-24 MeV. Our results show a strong reduction in uncertainty by using the asymptotic normalization coefficient as a constraint, particularly for those reactions most sensitive to ambiguities in the mean-field. For those reactions, the importance of constraining the bound state interaction is equal to that of constrain the optical potentials. The case of 14C is an outlier because it populates a halo state, and the observable is less sensitive to the nuclear interior. We conclude that when minimal constraints are used on the parameters of the nucleon-target interaction, the 68% confidence interval uncertainties on the differential cross sections are very large (~ 140-185%). However, if elastic-scattering data and the asymptotic normalization coefficient are used in the analysis, with an error of 10% (5%), this uncertainty reduces to ~30% (~15%).

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Uncertainty Quantification in Breakup Reactions

Breakup reactions are one of the favored probes to study loosely bound nuclei, particularly those in the limit of stability forming a halo. In order to interpret such breakup experiments, the continuum discretized coupled channel method is typically used. In this study, the first Bayesian analysis of a breakup reaction model is performed. We use a combination of statistical methods together with a three-body reaction model (the continuum discretized coupled channel method) to quantify the uncertainties on the breakup observables due to the parameters in the effective potential describing the loosely bound projectile of interest. The combination of tools we develop opens the path for a Bayesian analysis of not only breakup processes, but also a wide array of complex processes that require computationally intensive reaction models.

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Considering non-locality in the optical potentials within eikonal models

Background: For its simplicity, the eikonal method is the tool of choice to analyze nuclear reactions at high energies ($E>100$ MeV/nucleon), including knockout reactions. However, so far, the effective interactions used in this method are assumed to be fully local. Purpose: Given the recent studies on non-local optical potentials, in this work we assess whether non-locality in the optical potentials is expected to impact reactions at high energies and then explore different avenues for extending the eikonal method to include non-local interactions. Method: We compare angular distributions obtained for non-local interactions (using the exact R-matrix approach for elastic scattering and the adiabatic distorted wave approximation for transfer) with those obtained using their local-equivalent interactions. Results: Our results show that transfer observables are significantly impacted by non-locality in the high-energy regime. Because knockout reactions are dominated by stripping (transfer to inelastic channels), non-locality is expected to have a large effect on knockout observables too. Three approaches are explored for extending the eikonal method to non-local interactions, including an iterative method and a perturbation theory. Conclusions: None of the derived extensions of the eikonal model provide a good description of elastic scattering. This work suggests that non-locality removes the formal simplicity associated with the eikonal model.

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Study of Cluster Structures in Nuclei through the Ratio Method. A Tribute to Mahir Hussein

For one-neutron halo nuclei, the cross section for elastic scattering and breakup at intermediate energy exhibit similar angular dependences. The Recoil Excitation and Breakup (REB) model of reactions elegantly explains this feature. It also leads to the idea of a new reaction observable to study the structure of loosely-bound nuclear systems: the Ratio. This observable consists of the ratio of angular distributions for different reaction channels, viz. elastic scattering and breakup, which cancels most of the dependence on the reaction mechanism; in particular it is insensitive to the choice of optical potentials that simulate the projectile-target interaction. This new observable is very sensitive to the structure of the projectile. In this article, we review the Ratio Method and its extension to low beam energies and proton-halo nuclei.

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Inclusive deuteron-induced reactions and final neutron states

We present in this paper a formalism for deuteron-induced inclusive reactions. We disentangle direct elastic breakup contributions from other processes (which we generically call non-elastic breakup) implying a capture of the neutron both above and below the neutron emission threshold. The reaction is described as a two step process, namely the breakup of the deuteron followed by the propagation of the neutron-target system driven by an optical potential. The final state interaction between the neutron and the target can eventually form an excited compound nucleus. Within this context, the direct neutron transfer to a sharp bound state is a limiting case of the present formalism.

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Establishing a theory for deuteron induced surrogate reactions

The goal of this work is to establish on firm grounds a theory for deuteron induced neutron capture reactions. This includes formulating elastic and inelastic breakup in a consistent manner. We describe this process both in post and prior form distorted wave Born approximation, and we apply our method to the 53Nb(d,p)X at Ed =15 MeV and 25 MeV, obtaining a good description of the data. We look at the various partial wave contributions, as well as elastic versus inelastic contributions. We also connect our formulation with transfer to neutron bound states.

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