arXiv subjects

Finn Lasse Buessen

Publications and source records attributed to Finn Lasse Buessen.

18 recordsLinked to original sources

arXiv2026

Fault-Tolerant Quantum Computing with Trapped Ions: The Walking Cat Architecture

We propose a fault-tolerant quantum computer architecture for trapped-ion devices, which we call the walking cat architecture. Our blueprint includes a compiler, a detailed description of all the quantum error-correction protocols, a micro-architecture, a sufficiently fast decoder, and thorough simulations. The backbone of the architecture is a cat factory, producing cat states distributed throughout the machine, which are consumed to perform logical operations. The walking cat architecture is based entirely on a modern quantum error-correction approach called low-density parity-check (LDPC) codes. We identify promising instances of the walking cat architecture, such as (1) a simple architecture based on a single LDPC code, (2) a fast architecture based on fast logical gates relying on a [[70, 6, 9]] code, equipped with Clifford-frame tracking for any 6-qubit Clifford gate, and (3) a dense architecture based on a [[102, 22, 9]]] code encoding 22 logical qubits per memory block. Our dense architecture provides a design with 110 logical qubits executing about one million T gates per day using only 2,514 physical qubits. We estimate that the quantum Hamiltonian simulation of a Heisenberg model on 100 sites can be executed within one month with 10,000 physical qubits, including all shots required to achieve chemical accuracy, suggesting that such a device could enter the regime of classically intractable physics simulations. Our design relies on hardware components that have been experimentally demonstrated on small devices. We emphasize simplicity over hypothetical performance to facilitate the practical realization of this machine. Based on this approach, we believe that a fault-tolerant quantum computer with hundreds of logical qubits capable of running millions of logical gates can be built in the near term, providing a platform to explore a broad range of applications.

quant-ph↗

arXiv2022

Simulating time evolution on distributed quantum computers

We study a variation of the Trotter-Suzuki decomposition, in which a Hamiltonian exponential is approximated by an ordered product of two-qubit operator exponentials such that the Trotter step size is enhanced for a small number of terms. Such decomposition directly reflects hardware constraints of distributed quantum computers, where operations on monolithic quantum devices are fast compared to entanglement distribution across separate nodes using interconnects. We simulate non-equilibrium dynamics of transverse-field Ising and XY spin chain models and investigate the impact of locally increased Trotter step sizes that are associated with an increasingly sparse use of the quantum interconnect. We find that the overall quality of the approximation depends smoothly on the local sparsity and that the proliferation of local errors is slow. As a consequence, we show that fast local operations on monolithic devices can be leveraged to obtain an overall improved result fidelity even on distributed quantum computers where the use of interconnects is costly.

quant-ph↗

arXiv2022

Exchange interactions and spin dynamics in the layered honeycomb ferromagnet CrI$_3$

We derive the microscopic spin Hamiltonian for rhombohedral CrI$_3$ using extensive first-principles density functional theory (DFT) calculations which incorporate spin-orbit coupling and Hubbard U. Our calculations indicate a dominant nearest-neighbor ferromagnetic Heisenberg exchange with weaker further-neighbor Heisenberg terms. In addition, we find a Dzyaloshinskii-Moriya interaction which primarily drives a topological gap in the spin-wave spectrum at the Dirac point, and uncover a non-negligible antiferromagnetic Kitaev coupling between the S=3/2 Cr moments. The out-of-plane magnetic moment is stabilized by weak symmetric bond-dependent terms and a local single-ion anisotropy. Using linear spin wave theory, we find that our exchange parameters are in reasonably good agreement with inelastic neutron scattering (INS) experiments. Employing classical Monte Carlo simulations, we study the magnetic phase transition temperature $T_c$ and its evolution with an applied in-plane magnetic field. We further demonstrate how future high-resolution INS experiments on the magnon dispersion of single crystals in an in-plane magnetic field may be used to quantitatively extract the strength of the antiferromagnetic Kitaev exchange coupling.

cond-mat.str-el↗

arXiv2022

Pre-thermalization via self-driving and external driving of extensive subsystems

We investigate the non-equilibrium states of an interacting multi-component quantum system when only an extensive subsystem is quantum-quenched or driven from the ground state. As a concrete example, we consider a system where two XXZ spin chains are coupled to a transverse field Ising (TFI) chain, and only the transverse field in the TFI chain is quantum-quenched or periodically driven in time, starting from an initially ordered state. This system is studied using density matrix renormalization group (DMRG) simulations and various entanglement entropy diagnostics. In the case of quantum quenching, when the transverse field is suddenly switched on to become the largest energy scale, the resulting internal dynamics leads to a pre-thermal steady state with persistent oscillating magnetization (`self-driving') and emergent conservation laws. Upon applying the time-dependent drive to the TFI chain (`external driving'), sufficiently fast drive gives rise to a pre-thermal steady state with finite magnetization, whereas a slow drive generates a high-temperature disordered state. We briefly discuss the experimental implementation of our protocol in organic materials with quantum-tunneling hydrogen atoms.

cond-mat.str-el↗

arXiv2021

Order by disorder in classical kagome antiferromagnets with chiral interactions

The Heisenberg antiferromagnet on the kagome lattice is an archetypal instance of how large ground state degeneracies arise, and how they may get resolved by thermal and quantum fluctuations. Augmenting the Heisenberg model by chiral spin interactions has proved to be of particular interest in the discovery of certain chiral quantum spin liquids. Here we consider the classical variant of this chiral kagome model and find that it exhibits, similar to the classical Heisenberg antiferromagnet, a remarkably large and structured ground-state manifold, which combines continuous and discrete degrees of freedom. This allows for a rich set of order-by-disorder phenomena. Degeneracy lifting occurs in a highly selective way, choosing already at the harmonic level specific triaxial states which however retain an emergent $Z_2$ degree of freedom (absent in the conventional Heisenberg model). We also study the competition of entropic and energetic ground state selection as the model interpolates between the purely chiral and Heisenberg cases. For this mixed model, we find a "proximate ordered-by-disorder" finite-temperature regime where fluctuations overcome the energetic ground state preference of the perturbation. Finally, a semiclassical route to a spin liquid is provided by quantum order by disorder in the purely chiral models, where the aforementioned $Z_2$ degrees of freedom are elevated to the role of an emergent gauge field.

cond-mat.str-el↗

arXiv2021

Dynamical Signatures of Rank-2 $U(1)$ Spin Liquids

Emergent $U(1)$ gauge theories and artificial photons in frustrated magnets are outstanding examples of many-body collective phenomena. The classical and quantum regimes of these systems provide platforms for classical and quantum spin liquids, and are the subject of current active theoretical and experimental investigations. Recently, realizations of rank-2 $U(1)$ (R2-U1) gauge theories in three-dimensional frustrated magnets have been proposed. Such systems in the quantum regime may lead to the so-called fracton ordered phases -- a new class of topological order that has been associated with quantum stabilizer codes and holography. However, there exist few distinguishing characteristics of these states for their detection in real materials. Here we focus on the classical limit, and present the dynamical spin structure factor for a R2-U1 spin liquid state on a breathing pyrochlore lattice. Remarkably, we find unique signatures of the R2-U1 state, and we contrast them with the results obtained from a more conventional $U(1)$ spin liquid. These results provide a new path of investigation for future inelastic neutron scattering experiments on candidate materials.

cond-mat.str-el↗

arXiv2021

The SpinParser software for pseudofermion functional renormalization group calculations on quantum magnets

We present the SpinParser open-source software [ https://github.com/fbuessen/SpinParser ]. The software is designed to perform pseudofermion functional renormalization group (pf-FRG) calculations for frustrated quantum magnets in two and three spatial dimensions. It aims to make such calculations readily accessible without the need to write specialized program code; instead, custom lattice graphs and microscopic spin models can be defined as plain-text input files. Underlying symmetries of the model are automatically analyzed and exploited by the numerical core written in C++ in order to optimize the performance across large-scale shared memory and/or distributed memory computing platforms.

physics.comp-ph↗

arXiv2021

Functional renormalization group study of the Kitaev-$Γ$ model on the honeycomb lattice and emergent incommensurate magnetic correlations

The theoretical inception of the Kitaev honeycomb model has had defining influence on the experimental hunt for quantum spin liquids, bringing unprecedented focus onto the synthesis of materials with bond-directional interactions. Numerous Kitaev materials, which are believed to harbor ground states parametrically close to the Kitaev spin liquid, have been investigated since. Yet, in these materials the Kitaev interaction often comes hand in hand with off-diagonal $Γ$ interactions -- with the competition of the two potentially giving rise to a magnetically ordered ground state. In an attempt to aid future material investigations, we study the phase diagram of the spin-1/2 Kitaev-$Γ$ model on the honeycomb lattice. Employing a pseudofermion functional renormalization group approach which directly operates in the thermodynamic limit and captures the joint effect of thermal and quantum fluctuations, we unveil the existence of extended parameter regimes with emergent incommensurate magnetic correlations at finite temperature. We supplement our results with additional calculations on a finite cylinder geometry to investigate the impact of periodic boundary conditions on the incommensurate order, thereby providing a perspective on previous numerical studies on finite systems.

cond-mat.str-el↗

arXiv2021

Molecular dipoles in designer honeycomb lattices

Recent advances in ultracold atoms in optical lattices and developments in surface science have allowed for the creation of artificial lattices as well as the control of many-body interactions. Such systems provide new settings to investigate interaction-driven instabilities and non-trivial topology. In this paper, we explore the interplay between molecular electric dipoles on a two-dimensional triangular lattice with fermions hopping on the dual decorated honeycomb lattice which hosts Dirac and flat band states. We show that short-range dipole-dipole interaction can lead to ordering into various stripe and vortex crystal ground states. We study these ordered states and their thermal transitions as a function of the interaction range using simulated annealing and Monte Carlo methods. For the special case of zero wave vector ferrodipolar order, incorporating dipole-electron interactions and integrating out the electrons leads to a six-state clock model for the dipole ordering. Finally, we discuss the impact of the various dipole orders on the electronic band structure and the local tunneling density of states. Our work may be relevant to studies of "molecular graphene" -- CO molecules arranged on the Cu(111) surface -- which have been explored using scanning tunneling spectroscopy, as well as ultracold molecule-fermion mixtures in optical lattices.

cond-mat.str-el↗

arXiv2021

Nematic order driven by superconducting correlations

The interplay of nematicity and superconductivity has been observed in a wide variety of quantum materials. To explore this interplay, we consider a two-dimensional (2D) array of nematogens, local droplets with $Z_3$ nematicity, coupled to a network of Josephson junction wires. Using finite temperature classical Monte Carlo simulations, we elucidate the phase diagram of this model and show that the development of superconducting correlations and the directional delocalization of Cooper pairs can promote nematogen ordering, resulting in long-range nematic order. We obtain the transport properties of our model within an effective resistor network picture. We discuss these ideas in the context of the 2D electron gas at the (111) KTaO$_3$ interface and the doped topological insulators Nb$_x$Bi$_2$Se$_3$ and Cu$_x$Bi$_2$Se$_3$. Our work makes contact with Phil Anderson's numerous contributions to broken symmetries driven by the saving of kinetic energy, including double exchange ferromagnetism and the interlayer tunneling theory of high $T_c$ superconductivity.

cond-mat.supr-con↗

arXiv2020

Magnetic vortex liquid and anomalous thermal Hall conductivity in frustrated magnets with bond-dependent interactions

Recently, the observation of large thermal Hall conductivities in correlated insulators with no apparent broken symmetry have generated immense interest and debates on the underlying ground states. Here, considering frustrated magnets with bond-dependent interactions, which are realized in the so-called Kitaev materials, we theoretically demonstrate that a large thermal Hall conductivity can originate from a classical ground state without any magnetic order. We discover a novel liquid state of magnetic vortices, which are inhomogeneous spin textures embedded in the background of polarized spins, under out-of-plane magnetic fields. In the classical regime, different configurations of vortices form a degenerate manifold. We study the static and dynamical properties of the magnetic vortex liquid state at zero and finite temperatures. In particular, we show that the spin excitation spectrum resembles a continuum of nearly flat Chern bands, which ultimately leads to a large thermal Hall conductivity. Possible connections to experiments are discussed.

cond-mat.str-el↗

arXiv2020

Domes of $T_c$ in single-band and multiband superconductors with finite-range attractive interactions

The rise and fall of the superconducting transition temperature $T_c$ upon tuning carrier density or external parameters, such as pressure or magnetic field, is ubiquitously observed in a wide range of quantum materials. In order to investigate such domes of $T_c$, we go beyond the prototypical attractive Hubbard model, and consider a lattice model of electrons coupled via instantaneous, spatially extended, attractive interactions. By numerically solving the mean-field equations, as well as going beyond mean field theory using a functional renormalization group approach, we find that for a characteristic interaction range $\ell$, there exists a dome in $T_c$ around $k_F \ell \! \sim \! {\mathcal{O}}(1)$. For multiband systems, our mean field theory shows the presence of additional domes in the vicinity of Lifshitz transitions. Our results hold in both two and three dimensions and can be intuitively understood from the geometric relation between the Fermi surface and the interaction range. Our model may be relevant for domes of $T_c$ in dilute weakly coupled superconductors or in engineered cold atom systems.

cond-mat.supr-con↗

arXiv2019

Functional renormalization group for frustrated magnets with nondiagonal spin interactions

In the field of quantum magnetism, the advent of numerous spin-orbit assisted Mott insulating compounds, such as the family of Kitaev materials, has led to a growing interest in studying general spin models with non-diagonal interactions that do not retain the SU(2) invariance of the underlying spin degrees of freedom. However, the exchange frustration arising from these non-diagonal and often bond-directional interactions for two- and three-dimensional lattice geometries poses a serious challenge for numerical many-body simulation techniques. In this paper, we present an extended formulation of the pseudo-fermion functional renormalization group that is capable of capturing the physics of frustrated quantum magnets with generic (diagonal and off-diagonal) two-spin interaction terms. Based on a careful symmetry analysis of the underlying flow equations, we reveal that the computational complexity grows only moderately, as compared to models with only diagonal interaction terms. We apply the formalism to a kagome antiferromagnet which is augmented by general in-plane and out-of-plane Dzyaloshinskii-Moriya (DM) interactions, as argued to be present in the spin liquid candidate material herbertsmithite. We calculate the complete ground state phase diagram in the strength of in-plane and out-of-plane DM couplings, and discuss the extended stability of the spin liquid of the unperturbed kagome antiferromagnet in the presence of these couplings.

cond-mat.str-el↗

arXiv2019

Emergence and stability of spin-valley entangled quantum liquids in moiré heterostructures

Twisting moiré heterostructures to the flatband regime allows for the formation of strongly correlated quantum states, since the dramatic reduction of the bandwidth can cause the residual electronic interactions to set the principal energy scale. An effective description for such correlated moiré heterostructures, derived in the strong-coupling limit at integer filling, generically leads to spin-valley Heisenberg models. Here we explore the emergence and stability of spin liquid behavior in an SU(2)$^{\mathrm{spin}}\otimes$SU(2)$^{\mathrm{valley}}$ Heisenberg model upon inclusion of Hund's-induced and longer-ranged exchange couplings, employing a pseudofermion functional renormalization group approach. We consider two lattice geometries, triangular and honeycomb (relevant to different moiré heterostructures), and find, for both cases, an extended parameter regime surrounding the SU(4) symmetric point where no long-range order occurs, indicating a stable realm of quantum spin liquid behavior. For large Hund's coupling, we identify the adjacent magnetic orders, with both antiferromagnetic and ferromagnetic ground states emerging in the separate spin and valley degrees of freedom. For both lattice geometries the inclusion of longer-ranged exchange couplings is found to have both stabilizing and destabilizing effects on the spin liquid regime depending on the sign of the additional couplings.

cond-mat.str-el↗

arXiv2018

Quantum spin liquids in frustrated spin-1 diamond antiferromagnets

Motivated by the recent synthesis of the spin-1 A-site spinel NiRh$_{\text 2}$O$_{\text 4}$, we investigate the classical to quantum crossover of a frustrated $J_1$-$J_2$ Heisenberg model on the diamond lattice upon varying the spin length $S$. Applying a recently developed pseudospin functional renormalization group (pf-FRG) approach for arbitrary spin-$S$ magnets, we find that systems with $S \geq 3/2$ reside in the classical regime where the low-temperature physics is dominated by the formation of coplanar spirals and a thermal (order-by-disorder) transition. For smaller local moments $S$=1 or $S$=1/2 we find that the system evades a thermal ordering transition and forms a quantum spiral spin liquid where the fluctuations are restricted to characteristic momentum-space surfaces. For the tetragonal phase of NiRh$_{\text 2}$O$_{\text 4}$, a modified $J_1$-$J_2^-$-$J_2^\perp$ exchange model is found to favor a conventionally ordered Néel state (for arbitrary spin $S$) even in the presence of a strong local single-ion spin anisotropy and it requires additional sources of frustration to explain the experimentally observed absence of a thermal ordering transition.

cond-mat.str-el↗

arXiv2017

Functional renormalization group approach to SU(N) Heisenberg models: Real-space RG at arbitrary N

The pseudofermion functional renormalization group (pf-FRG) is one of the few numerical approaches that has been demonstrated to quantitatively determine the ordering tendencies of frustrated quantum magnets in two and three spatial dimensions. The approach, however, relies on a number of presumptions and approximations, in particular the choice of pseudofermion decomposition and the truncation of an infinite number of flow equations to a finite set. Here we generalize the pf-FRG approach to SU(N)-spin systems with arbitrary N and demonstrate that the scheme becomes exact in the large-N limit. Numerically solving the generalized real-space renormalization group equations for arbitrary N, we can make a stringent connection between the physically most significant case of SU(2)-spins and more accessible SU(N) models. In a case study of the square-lattice SU(N) Heisenberg antiferromagnet, we explicitly demonstrate that the generalized pf-FRG approach is capable of identifying the instability indicating the transition into a staggered flux spin liquid ground state in these models for large, but finite values of N. In a companion paper (arXiv:1711.02183) we formulate a momentum-space pf-FRG approach for SU(N) spin models that allows us to explicitly study the large-N limit and access the low-temperature spin liquid phase.

cond-mat.str-el↗

arXiv2017

Functional renormalization group approach to SU(N) Heisenberg models: Momentum-space RG for the large-N limit

In frustrated magnetism, making a stringent connection between microscopic spin models and macroscopic properties of spin liquids remains an important challenge. A recent step towards this goal has been the development of the pseudofermion functional renormalization group approach (pf-FRG) which, building on a fermionic parton construction, enables the numerical detection of the onset of spin liquid states as temperature is lowered. In this work, focusing on the SU(N) Heisenberg model at large N, we extend this approach in a way that allows us to directly enter the low-temperature spin liquid phase, and to probe its character. Our approach proceeds in momentum space, making it possible to keep the truncation minimalistic, while also avoiding the bias introduced by an explicit decoupling of the fermionic parton interactions into a given channel. We benchmark our findings against exact mean-field results in the large-N limit, and show that even without prior knowledge the pf-FRG approach identifies the correct mean-field decoupling channel. On a technical level, we introduce an alternative finite temperature regularization scheme that is necessitated to access the spin liquid ordered phase. In a companion paper arXiv:1711.02182 we present a different set of modifications of the pf-FRG scheme that allow us to study SU(N) Heisenberg models (using a real-space RG approach) for arbitrary values of N, albeit only up to the phase transition towards spin liquid physics.

cond-mat.str-el↗

arXiv2016

Competing magnetic orders and spin liquids in two- and three-dimensional kagome systems: A pseudo-fermion functional renormalization group perspective

Quantum magnets on kagome lattice geometries in two and three spatial dimensions are archetypal examples of spin systems in which geometric frustration inhibits conventional magnetic ordering and instead benefits the emergence of long-range entangled spin liquids at low temperature. Here we employ a recently developed pseudo-fermion functional renormalization group (pf-FRG) approach to study the low-temperature quantum magnetism of kagome and hyperkagome spin systems with exchange interactions beyond the nearest neighbor coupling. We find that next-nearest neighbor couplings stabilize a variety of magnetic orders as well as induce additional spin liquid regimes giving rise to rather rich phase diagrams, which we characterize in detail. On a technical level, we find that the pf-FRG approach is in excellent quantitative agreement with high-temperature series expansions over their range of validity and it exhibits a systematic finite-size convergence in the temperature regime below. We discuss notable advantages and some current limitations of the pf-FRG approach in the ongoing search for unconventional forms of quantum magnetism.

cond-mat.str-el↗