arXiv subjects

Florent Lecocq

Publications and source records attributed to Florent Lecocq.

13 recordsLinked to original sources

arXiv2026

Magnetic flux distribution, quasiparticle spectroscopy, and quality factors in Nb films for superconducting qubits

Niobium is a practical material platform for superconducting microwave circuits; however, device-level performance can vary significantly depending on film growth and processing conditions. We compare three epitaxial Nb films grown on $c-$plane sapphire substrates under nominally identical conditions, except for the deposition temperature. To correlate internal quality factors, $Q_{\mathrm {i}}$, with material properties, we combine magneto-optical imaging of magnetic flux distribution with quasiparticle spectroscopy via measurements of the London penetration depth, $\lambda(T)$. In the low-$Q_{\mathrm i}$ film, there is a lesser ability to screen the magnetic field and an irregular temperature variation of $\lambda(T)$, implying the existence of localized in-gap states. High $Q_{\mathrm i}$ films show the opposite trend. We conclude that our measurements provide an efficient method for characterizing and optimizing superconducting films for quantum informatics applications.

cond-mat.supr-con↗

arXiv2026

Quasiparticle spectroscopy in tantalum films with different Ta/sapphire interfaces

One of the crucial aspects of current research in quantum information science is the identification and control of loss mechanisms in superconducting circuits. Although microwave measurements directly quantify device performance, additional techniques that probe quasiparticle excitations in superconducting films are needed to understand the microscopic mechanisms underlying dissipation and decoherence. Here, we present results from quasiparticle spectroscopy of Ta/sapphire films by measuring the Meissner-state magnetic susceptibility using a precision frequency-domain resonator specifically designed for thin films. We find direct evidence for additional low-energy excitations in samples with lower internal quality factors. These excitations are consistent with deep subgap states due to two-level systems, Yu-Shiba-Rusinov states near the gap edge, and perhaps other pair-breaking mechanisms. The developed non-destructive frequency-domain quasiparticle spectroscopy is a valuable addition to the quantum materials toolbox.

cond-mat.supr-con↗

arXiv2024

Cryogenic photonic link using an extended-InGaAs photodiode and short pulse illumination towards high-fidelity drive of superconducting qubits

We investigate short pulse illumination of a high-speed extended-InGaAs photodiode at cryogenic temperatures towards its use in control and readout of superconducting qubits. First, we demonstrate high detector responsivity at 1550 nm illumination at 20 mK, a wavelength band unavailable to cryogenic standard InGaAs detectors due to the temperature-dependent bandgap shift. Second, we demonstrate an improved signal-to-noise ratio (SNR) at the shot noise limit for cryogenic short optical pulse detection when compared to conventional modulated continuous-wave laser detection. At 40 uA of photocurrent and a detector temperature of 4 K, short pulse detection yields an SNR improvement of 20 dB and 3 dB for phase and amplitude quadratures, respectively. Lastly, we discuss how short pulse detection offers a path for signal multiplexing, with a demonstration of simultaneous production of microwave pulses at two different carrier frequencies. Together, these advancements establish a path towards low noise and power efficient multiplexed photonic links for quantum computing with a large number of superconducting qubits.

physics.optics↗

arXiv2024

Interface-sensitive microwave loss in superconducting tantalum films sputtered on c-plane sapphire

Quantum coherence in superconducting circuits has increased steadily over the last decades as a result of a growing understanding of the various loss mechanisms. Recently, tantalum (Ta) emerged as a promising material to address microscopic sources of loss found on niobium (Nb) or aluminum (Al) surfaces. However, the effects of film and interface microstructure on low-temperature microwave loss are still not well understood. Here we present a systematic study of the structural and electrical properties of Ta and Nb films sputtered on c-plane sapphire at varying growth temperatures. As growth temperature is increased, our results show that the onset of epitaxial growth of alpha-phase Ta correlates with lower Ta surface roughness, higher critical temperature, and higher residual resistivity ratio, but surprisingly also correlates with a significant increase in loss at microwave frequency. Notably, this high level of loss is not observed in Nb films prepared in the same way and having very similar structure. By experimentally controlling the surface on which the Ta film is nucleated, we determine that the source of loss is only present in samples having an epitaxial Ta/sapphire interface and show that it is apparently mitigated by either growing a thin, epitaxial Nb inter-layer between the Ta film and the substrate or by intentionally treating, and effectively damaging, the sapphire surface with an in-situ argon plasma before Ta growth. In addition to elucidating this interfacial microwave loss, this work provides adequate process details to aid reproducible growth of low-loss Ta films across fabrication facilities.

quant-ph↗

arXiv2024

Fabrication and characterization of low-loss Al/Si/Al parallel plate capacitors for superconducting quantum information applications

Increasing the density of superconducting circuits requires compact components, however, superconductor-based capacitors typically perform worse as dimensions are reduced due to loss at surfaces and interfaces. Here, parallel plate capacitors composed of aluminum-contacted, crystalline silicon fins are shown to be a promising technology for use in superconducting circuits by evaluating the performance of lumped element resonators and transmon qubits. High aspect ratio Si-fin capacitors having widths below $300nm$ with an approximate total height of 3$\mu$m are fabricated using anisotropic wet etching of Si(110) substrates followed by aluminum metallization. The single-crystal Si capacitors are incorporated in lumped element resonators and transmons by shunting them with lithographically patterned aluminum inductors and conventional $Al/AlO_x/Al$ Josephson junctions respectively. Microwave characterization of these devices suggests state-of-the-art performance for superconducting parallel plate capacitors with low power internal quality factor of lumped element resonators greater than 500k and qubit $T_1$ times greater than 25$\mu$s. These results suggest that Si-Fins are a promising technology for applications that require low loss, compact, superconductor-based capacitors with minimal stray capacitance.

quant-ph↗

arXiv2022

Deepest sensitivity to wavelike dark photon dark matter with superconducting radio frequency cavities

Wavelike, bosonic dark matter candidates like axions and dark photons can be detected using microwave cavities known as haloscopes. Traditionally, haloscopes consist of tunable copper cavities operating in the TM$_{010}$ mode, but ohmic losses have limited their performance. In contrast, superconducting radio frequency (SRF) cavities can achieve quality factors of $\sim 10^{10}$, perhaps five orders of magnitude better than copper cavities, leading to more sensitive dark matter detectors. In this paper, we first derive that the scan rate of a haloscope experiment is proportional to the loaded quality factor $Q_L$, even if the cavity bandwidth is much narrower than the dark matter halo line shape. We then present a proof-of-concept search for dark photon dark matter using a nontunable ultrahigh quality SRF cavity. We exclude dark photon dark matter with kinetic mixing strengths of $\chi > 1.5\times 10^{-16}$ for a dark photon mass of $m_{A^{\prime}} = 5.35\mu$eV, achieving the deepest exclusion to wavelike dark photons by almost an order of magnitude.

hep-ex↗

arXiv2022

Observation of two-mode squeezing in a traveling wave parametric amplifier

Traveling wave parametric amplifiers (TWPAs) have recently emerged as essential tools for broadband near quantum-limited amplification. However, their use to generate microwave quantum states still misses an experimental demonstration. In this letter, we report operation of a TWPA as a source of two-mode squeezed microwave radiation. We demonstrate broadband entanglement generation between two modes separated by up to 400 MHz by measuring logarithmic negativity between 0.27 and 0.51 and collective quadrature squeezing below the vacuum limit between 1.5 and 2.1 dB. This work opens interesting perspectives for the exploration of novel microwave photonics experiments with possible applications in quantum sensing and continuous variable quantum computing.

quant-ph↗

arXiv2021

Direct observation of deterministic macroscopic entanglement

Quantum entanglement of mechanical systems emerges when distinct objects move with such a high degree of correlation that they can no longer be described separately. Although quantum mechanics presumably applies to objects of all sizes, directly observing entanglement becomes challenging as masses increase, requiring measurement and control with a vanishingly small error. Here, using pulsed electromechanics, we deterministically entangle two mechanical drumheads with masses of 70 pg. Through nearly quantum-limited measurements of the position and momentum quadratures of both drums, we perform quantum state tomography and thereby directly observe entanglement. Such entangled macroscopic systems are uniquely poised to serve in fundamental tests of quantum mechanics, enable sensing beyond the standard quantum limit, and function as long-lived nodes of future quantum networks.

quant-ph↗

arXiv2016

Sideband Cooling Beyond the Quantum Limit with Squeezed Light

Quantum fluctuations of the electromagnetic vacuum impose an observable quantum limit to the lowest temperatures that can be reached with conventional laser cooling techniques. As laser cooling experiments continue to bring massive mechanical systems to unprecedented temperatures, this quantum limit takes on increasingly greater practical importance in the laboratory. Fortunately, vacuum fluctuations are not immutable, and can be "squeezed" through the generation of entangled photon pairs. Here we propose and experimentally demonstrate that squeezed light can be used to sideband cool the motion of a macroscopic mechanical object below the quantum limit. To do so, we first cool a microwave cavity optomechanical system with a coherent state of light to within 15% of this limit. We then cool by more than 2 dB below the quantum limit using a squeezed microwave field generated by a Josephson Parametric Amplifier (JPA). From heterodyne spectroscopy of the mechanical sidebands, we measure a minimum thermal occupancy of 0.19 phonons. With this novel technique, even low frequency mechanical oscillators can in principle be cooled arbitrarily close to the motional ground state, enabling the exploration of quantum physics in larger, more massive systems.

quant-ph↗

arXiv2016

Observation of Strong Radiation Pressure Forces from Squeezed Light on a Mechanical Oscillator

Quantum enhanced sensing is a powerful technique in which nonclassical states are used to improve the sensitivity of a measurement. For enhanced mechanical displacement sensing, squeezed states of light have been shown to reduce the photon counting noise that limits the measurement noise floor. It has long been predicted, however, that suppressing the noise floor with squeezed light should produce an unavoidable increase in radiation pressure noise that drives the mechanical system. Such nonclassical radiation pressure forces have thus far been hidden by insufficient measurement strengths and residual thermal mechanical motion. Since the ultimate measurement sensitivity relies on the delicate balance between these two noise sources, the limits of the quantum enhancement have not been observed. Using a microwave cavity optomechanical system, we observe the nonclassical radiation pressure noise that necessarily accompanies any quantum enhancement of the measurement precision. By varying both the magnitude and phase of the squeezing, we optimize the fundamental trade-off between mechanical imprecision and backaction noise in accordance with the Heisenberg uncertainty principle. As the strength of the measurement is further increased, radiation pressure forces eventually dominate the mechanical motion. In this regime, the optomechanical interaction can be exploited as an efficient quantum nondemolition (QND) measurement of the amplitude fluctuations of the light field. By overwhelming mechanical thermal noise with radiation pressure by two orders of magnitude, we demonstrate a mechanically-mediated measurement of the squeezing with an effective homodyne efficiency of 94%. Thus, with strong radiation pressures forces, mechanical motion enhances the measurement of nonclassical light, just as nonclassical light enhances the measurement of the motion.

quant-ph↗

arXiv2012

Coherent frequency conversion in a superconducting artificial atom with two internal degrees of freedom

By adding a large inductance in a dc-SQUID phase qubit loop, one decouples the junctions' dynamics and creates a superconducting artificial atom with two internal degrees of freedom. In addition to the usual symmetric plasma mode ({\it s}-mode) which gives rise to the phase qubit, an anti-symmetric mode ({\it a}-mode) appears. These two modes can be described by two anharmonic oscillators with eigenstates $\ket{n_{s}}$ and $\ket{n_{a}}$ for the {\it s} and {\it a}-mode, respectively. We show that a strong nonlinear coupling between the modes leads to a large energy splitting between states $\ket{0_{s},1_{a}}$ and $\ket{2_{s},0_{a}}$. Finally, coherent frequency conversion is observed via free oscillations between the states $\ket{0_{s},1_{a}}$ and $\ket{2_{s},0_{a}}$.

cond-mat.mes-hall↗

arXiv2011

Non-linear coupling between the two oscillation modes of a dc-SQUID

We make a detailed theoretical description of the two-dimensional nature of a dc-SQUID, analyzing the coupling between its two orthogonal phase oscillation modes. While it has been shown that the mode defined as "longitudinal" can be initialized, manipulated and measured, so as to encode a quantum bit of information, the mode defined as "transverse" is usually repelled at high frequency and does not interfere in the dynamics. We show that, using typical parameters of existing devices, the transverse mode energy can be made of the order of the longitudinal one. In this regime, we can observe a strong coupling between these modes, described by an Hamiltonian providing a wide range of interesting effects, such as conditional quantum operations and entanglement. This coupling also creates an atomic-like structure for the combined two mode states, with a V-like scheme.

cond-mat.mes-hall↗

arXiv2011

Novel E-beam lithography technique for in-situ junction fabrication: the controlled undercut

We present a novel shadow evaporation technique for the realization of junctions and capacitors. The design by E-beam lithography of strongly asymmetric undercuts on a bilayer resist enables in-situ fabrication of junctions and capacitors without the use of the well-known suspended bridge[1]. The absence of bridges increases the mechanical robustness of the resist mask as well as the accessible range of the junction size, from 0.01 to more than 10000 micron square. We have fabricated Al/AlOx/Al Josephson junctions, phase qubit and capacitors using a 100kV E- beam writer. Although this high voltage enables a precise control of the undercut, implementation using a conventional 20kV E-beam is also discussed. The phase qubit coherence times, extracted from spectroscopy resonance width, Rabi and Ramsey oscillations decay and energy relaxation measurements, are longer than the ones obtained in our previous samples realized by standard techniques. These results demonstrate the high quality of the junction obtained by this controlled undercut technique.

cond-mat.mes-hall↗