arXiv subjects

Florian Büscher

Publications and source records attributed to Florian Büscher.

3 recordsLinked to original sources

arXiv2022

Discrimination of Chiral and Helical Contributions to Raman Scattering of Liquid Crystals using Vortex Beams

We use vortex photon fields with orbital and spin angular momentum to probe chiral fluctuations within liquid crystals. In the regime of iridescence with a well-defined pitch length of chirality, we find low energy Raman scattering that can be decomposed into helical and chiral components depending on the scattering vector and the topological charge of the incident photon field. Based on the observation of an anomalous dispersion we attribute quasi-elastic scattering to a transfer of angular momenta to roton-like quasiparticles. The latter are due to a competition of short-range repulsive and long-range dipolar interactions. Our approach using a transfer of orbital angular momentum opens up an avenue for the advanced characterization of chiral and optically active devices and materials.

cond-mat.soft↗

arXiv2021

Raman scattering of plane-wave and twisted light off chiral molecular liquids

We present an experimental study of the quasi-elastic Raman scattering (QES) of plane-wave and twisted light by liquid crystals. Depending on their temperature, these crystals can exhibit isotropic, nematic and chiral nematic phases. The question is addressed of how the phase of a crystal and the state of incident light can affect the quasi-elastic energy spectra of the scattered radiation, whose shape is usually described by the combination of Lorentzian and Gaussian components. Special attention is paid to the \textit{chiral phase}, for which the Raman QES spectrum is dominated by a Lorentzian with reduced linewidth, pointing to diminished disorder and configurational entropy. Moreover, this phase is also known for a regime of iridescence (selective backscattering) which arises when the wavelength of incident light becomes comparable with the chiral pitch length. Detailed measurements, performed in this \textit{resonant} regime and by employing twisted light, carrying various projections of the orbital angular momentum (OAM), have indicated a low-energy scattering surplus depending on OAM. We argue that this observation might indicate a transfer of angular momentum between light and the liquid crystal.

physics.optics↗

arXiv2020

Effect of topology on quasi-particle interactions in the Weyl semimetal WP$_2$

We compare two crystallographic phases of the low-dimensional WP$_2$ to better understand features of electron-electron and electron-phonon interactions in topological systems. The topological $β$-phase, a Weyl semimetal with a giant magneto-resistance, shows a larger intensity of electronic Raman scattering compared to the topologically trivial $α$-phase. This intensity sharply drops for $T < T^* = 20$ K which evidences a crossover in the topological phase from marginal quasiparticles to a coherent low temperature regime. In contrast, the non-topological $α$-phase shows more pronounced signatures of electron-phonon interaction. Here there exist generally enlarged phonon linewidths and deviations from conventional anharmonicity in an intermediate temperature regime. These effects provide evidence for an interesting interplay of electronic correlations and electron-phonon coupling. Both interband and intraband electronic fluctuations are involved in these effects. Their dependence on symmetry as well as momentum conservation are critical ingredients to understand this interplay.

cond-mat.str-el↗