arXiv subjects

Florian Kaiser

Publications and source records attributed to Florian Kaiser.

At least 37 records · Page 2Linked to original sources

arXiv2021

Narrow inhomogeneous distribution of spin-active emitters in silicon carbide

Optically active solid-state spin registers have demonstrated their unique potential in quantum computing, communication and sensing. Realizing scalability and increasing application complexity requires entangling multiple individual systems, e.g. via photon interference in an optical network. However, most solid-state emitters show relatively broad spectral distributions, which hinders optical interference experiments. Here, we demonstrate that silicon vacancy centres in semiconductor silicon carbide (SiC) provide a remarkably small natural distribution of their optical absorption/emission lines despite an elevated defect concentration of $\approx 0.43\,\rm μm^{-3}$. In particular, without any external tuning mechanism, we show that only 13 defects have to be investigated until at least two optical lines overlap within the lifetime-limited linewidth. Moreover, we identify emitters with overlapping emission profiles within diffraction limited excitation spots, for which we introduce simplified schemes for generation of computationally-relevant Greenberger-Horne-Zeilinger (GHZ) and cluster states. Our results underline the potential of the CMOS-compatible SiC platform toward realizing networked quantum technology applications.

quant-ph↗

arXiv2020

Spectrally reconfigurable quantum emitters enabled by optimized fast modulation

The ability to shape photon emission facilitates strong photon-mediated interactions between disparate physical systems, thereby enabling applications in quantum information processing, simulation and communication. Spectral control in solid state platforms such as color centers, rare earth ions, and quantum dots is particularly attractive for realizing such applications on-chip. Here we propose the use of frequency-modulated optical transitions for spectral engineering of single photon emission. Using a scattering-matrix formalism, we find that a two-level system, when modulated faster than its optical lifetime, can be treated as a single-photon source with a widely reconfigurable photon spectrum that is amenable to standard numerical optimization techniques. To enable the experimental demonstration of this spectral control scheme, we investigate the Stark tuning properties of the silicon vacancy in silicon carbide, a color center with promise for optical quantum information processing technologies. We find that the silicon vacancy possesses excellent spectral stability and tuning characteristics, allowing us to probe its fast modulation regime, observe the theoretically-predicted two-photon correlations, and demonstrate spectral engineering. Our results suggest that frequency modulation is a powerful technique for the generation of new light states with unprecedented control over the spectral and temporal properties of single photons.

quant-ph↗

arXiv2020

Two-photon phase-sensing with single-photon detection

Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realising this experimentally is technologically demanding, as it requires coincident single-photon detection proportional to the number of photons involved, which represents a severe challenge for achieving a practical quantum advantage over classical methods. Here, we exploit advanced quantum state engineering based on superposing two photon-pair creation events to realise a new approach that bypasses this issue. In particular, optical phase shifts are probed with a two-photon quantum state whose information is subsequently effectively transferred to a single-photon state. Notably, without any multiphoton detection, we infer phase shifts by measuring the average intensity of the single-photon beam on a photodiode, in analogy to standard classical measurements. Importantly, our approach maintains the quantum advantage: twice as many interference fringes are observed for the same phase shift, corresponding to N=2 path-entangled photons. Our results demonstrate that the advantages of quantum-enhanced phase-sensing can be fully exploited in standard intensity measurements, paving the way towards resource-efficient and practical quantum optical metrology.

quant-ph↗

arXiv2020

A universal, plug-and-play synchronisation scheme for practical quantum networks

We propose and experimentally demonstrate a plug-and-play, practical, and enabling method allowing to synchronize the building blocks of a quantum network in an all-optical way. Our scheme relies on mature and reliable classical telecommunication and non-linear optical technologies and can be implemented in a universal way with off-the-shelf components. Compared to already reported solutions, it allows achieving high-quality synchronization compatible with high network-operation rate and is free from opto-electronic jitters affecting servo-loop based configurations. We test our scheme with a genuine quantum optical method in terms of the interference between two photons coming from two remotely synchronized sources spaced by distances of up to 100 km. Measured visibilities well above 90% confirm the validity of our approach. Due its simplicity and high-quality performance, our scheme paves the way for the synchronization of long-distance quantum networks based on fibre, free-space, as well as hybrid solutions.

quant-ph↗

arXiv2020

Vibronic states and their effect on the temperature and strain dependence of silicon-vacancy qubits in 4H silicon carbide

Silicon-vacancy qubits in silicon carbide (SiC) are emerging tools in quantum technology applications due to their excellent optical and spin properties. In this paper, we explore the effect of temperature and strain on these properties by focusing on the two silicon-vacancy qubits, V1 and V2, in 4H SiC. We apply density functional theory beyond the Born-Oppenheimer approximation to describe the temperature dependent mixing of electronic excited states assisted by phonons. We obtain polaronic gap around 5 and 22~meV for V1 and V2 centers, respectively, that results in significant difference in the temperature dependent dephasing and zero-field splitting of the excited states, which explains recent experimental findings. We also compute how crystal deformations affect the zero-phonon-line of these emitters. Our predictions are important ingredients in any quantum applications of these qubits sensitive to these effects.

quant-ph↗

arXiv2020

Spin-controlled generation of indistinguishable and distinguishable photons from silicon vacancy centres in silicon carbide

Quantum systems combining indistinguishable photon generation and spin-based quantum information processing are essential for remote quantum applications and networking. However, identification of suitable systems in scalable platforms remains a challenge. Here, we investigate the silicon vacancy centre in silicon carbide and demonstrate controlled emission of indistinguishable and distinguishable photons via coherent spin manipulation. Using strong off-resonant excitation and collecting photons from the ultra-stable zero-phonon line optical transitions, we show a two-photon interference contrast close to 90% in Hong-Ou-Mandel type experiments. Further, we exploit the system's intimate spin-photon relation to spin-control the colour and indistinguishability of consecutively emitted photons. Our results provide a deep insight into the system's spin-phonon-photon physics and underline the potential of the industrially compatible silicon carbide platform for measurement-based entanglement distribution and photonic cluster state generation. Additional coupling to quantum registers based on recently demonstrated coupled individual nuclear spins would further allow for high-level network-relevant quantum information processing, such as error correction and entanglement purification.

quant-ph↗

arXiv2019

Fibre based hyperentanglement generation for dense wavelength division multiplexing

Entanglement is a key resource in quantum information science and associated emerging technologies. Photonic systems offer a large range of exploitable entanglement degrees of freedom such as frequency, time, polarization, and spatial modes. Hyperentangled photons exploit multiple degrees of freedom simultaneously to enhance the performance of quantum information protocols. Here, we report a fully guided-wave approach for generating polarization and energy-time hyperentangled photons at telecom wavelengths. Moreover, by demultiplexing the broadband emission spectrum of the source into five standard telecom channel pairs, we demonstrate compliance with fibre network standards and improve the effective bit rate capacity of the quantum channel up to one order of magnitude. In all channel pairs, we observe a violation of a generalised Bell inequality by more than 27 standard deviations, underlining the relevance of our approach.

quant-ph↗

arXiv2019

Quantum optical frequency up-conversion for polarisation entangled qubits: towards interconnected quantum information devices

Realising a global quantum network requires combining individual strengths of different quantum systems to perform universal tasks, notably using flying and stationary qubits. However, transferring coherently quantum information between different systems is challenging as they usually feature different properties, notably in terms of operation wavelength and wavepacket. To circumvent this problem for quantum photonics systems, we demonstrate a polarisation-preserving quantum frequency conversion device in which telecom wavelength photons are converted to the near infrared, at which a variety of quantum memories operate. Our device is essentially free of noise which we demonstrate through near perfect single photon state transfer tomography and observation of high-fidelity entanglement after conversion. In addition, our guided-wave setup is robust, compact, and easily adaptable to other wavelengths. This approach therefore represents a major building block towards advantageously connecting quantum information systems based on light and matter.

quant-ph↗

arXiv2019

Spectrally stable defect qubits with no inversion symmetry for robust spin-to-photon interface

Scalable spin-to-photon interfaces require quantum emitters with strong optical transition dipole moment and low coupling to phonons and stray electric fields. It is known that particularly for coupling to stray electric fields, these conditions can be simultaneously satisfied for emitters that show inversion symmetry. Here, we show that inversion symmetry is not a prerequisite criterion for a spectrally stable quantum emitter. We find that identical electron density in ground and excited states can eliminate the coupling to the stray electric fields. Further, a strong optical transition dipole moment is achieved in systems with altering sign of the ground and excited wavefunctions. We use density functional perturbation theory to investigate an optical center that lacks of inversion symmetry. Our results show that this system close to ideally satisfies the criteria for an ideal quantum emitter. Our study opens a novel rationale in seeking promising materials and point defects towards the realisation of robust spin-to-photon interfaces.

quant-ph↗

arXiv2018

Laser writing of scalable single colour centre in silicon carbide

Single photon emitters in silicon carbide (SiC) are attracting attention as quantum photonic systems. However, to achieve scalable devices it is essential to generate single photon emitters at desired locations on demand. Here we report the controlled creation of single silicon vacancy ($V_{Si}$) centres in 4H-SiC using laser writing without any post-annealing process. Due to the aberration correction in the writing apparatus and the non-annealing process, we generate single $V_{Si}$ centres with yields up to 30%, located within about 80 nm of the desired position in the transverse plane. We also investigated the photophysics of the laser writing $V_{Si}$ centres and conclude that there are about 16 photons involved in the laser writing $V_{Si}$ centres process. Our results represent a powerful tool in fabrication of single $V_{Si}$ centres in SiC for quantum technologies and provide further insights into laser writing defects in dielectric materials.

cond-mat.mes-hall↗

arXiv2018

High-fidelity spin and optical control of single silicon vacancy centres in silicon carbide

Optically interfaced spins in the solid promise scalable quantum networks. Robust and reliable optical properties have so far been restricted to systems with inversion symmetry. Here, we release this stringent constraint by demonstrating outstanding optical and spin properties of single silicon vacancy centres in silicon carbide. Despite the lack of inversion symmetry, the system's particular wave function symmetry decouples its optical properties from magnetic and electric fields, as well as from local strain. This provides a high-fidelity spin-to-photon interface with exceptionally stable and narrow optical transitions, low inhomogeneous broadening, and a large fraction of resonantly emitted photons. Further, the weak spin-phonon coupling results in electron spin coherence times comparable with nitrogen-vacancy centres in diamond. This allows us to demonstrate coherent hyperfine coupling to single nuclear spins, which can be exploited as qubit memories. Our findings promise quantum network applications using integrated semiconductor-based spin-to-photon interfaces.

quant-ph↗

arXiv2018

Non-classical measurement statistics induced by a coherent spin environment

We demonstrate the role of measurement back-action of a coherent spin environment on the dynamics of a spin (qubit) coupled to it, by inducing non-classical (Quantum Random Walk like) statistics on its measurement trajectory. We show how the long-life time of the spin-bath allows it to correlate measurements of the qubit over many repetitions. We have used Nitrogen Vacancy centers in diamond as a model system, and the projective single-shot readout of the electron spin at low temperatures to simulate these effects. We show that the proposed theoretical model, explains the experimentally observed statistics and their application for quantum state engineering of spin ensembles towards desired states.

quant-ph↗

arXiv2017

Quantum enhancement of accuracy and precision in optical interferometry

White-light interferometry is one of today's most precise tools for determining optical material properties. Achievable precision and accuracy are typically limited by systematic errors due to a high number of interdependent data fitting parameters. Here, we introduce spectrally-resolved quantum white-light interferometry as a novel tool for optical property measurements, notably chromatic dispersion in optical fibres. By exploiting both spectral and photon-number correlations of energy-time entangled photon pairs, the number of fitting parameters is significantly reduced which eliminates systematic errors and leads to an absolute determination of the material parameter. By comparing the quantum method to state-of-the-art approaches, we demonstrate the quantum advantage through 2.4 times better measurement precision, despite involving 62 times less photons. The improved results are due to conceptual advantages enabled by quantum optics which are likely to define new standards in experimental methods for characterising optical materials.

quant-ph↗

arXiv2017

Fully guided-wave photon pair source for quantum applications

We report a fully guided-wave source of polarisation entangled photons based on a periodically poled lithium niobate waveguide mounted in a Sagnac interferometer. We demonstrate the source's quality by converting polarisation entanglement to postselection-free energy-time entanglement for which we obtain a near-optimal $S$-parameter of $2.75 \pm 0.02$, i.e. a violation of the Bell inequality by more than 35 standard deviations. The exclusive use of guided-wave components makes our source compact and stable which is a prerequisite for increasingly complex quantum applications. Additionally, our source offers a great versatility in terms of photon pair emission spectrum and generated quantum state, making it suitable for a broad range of quantum applications such as cryptography and metrology. In this sense, we show how to use our source for chromatic dispersion measurements in optical fibres which opens new avenues in the field of quantum metrology.

quant-ph↗

arXiv2017

High-quality photonic entanglement for wavelength-multiplexed quantum communication based on a silicon chip

We report an efficient energy-time entangled photon-pair source based on four-wave mixing in a CMOS-compatible silicon photonics ring resonator. Thanks to suitable optimization, the source shows a large spectral brightness of 400\,pairs of entangled photons /s/MHz for $\rm 500\,μW$ pump power. Additionally, the resonator has been engineered so as to generate a frequency comb structure compatible with standard telecom dense wavelength division multiplexers. We demonstrate high-purity energy-time entanglement, i.e., free of photonic noise, with near perfect raw visibilities ($>$~98\%) between various channel pairs in the telecom C-band. Such a compact source stands as a path towards more complex quantum photonic circuits dedicated to quantum communication systems.

quant-ph↗

arXiv2016

Quantum photonics at telecom wavelengths based on lithium niobate waveguides

Integrated optical components on lithium niobate play a major role in standard high-speed communication systems. Over the last two decades, after the birth and positioning of quantum information science, lithium niobate waveguide architectures have emerged as one of the key platforms for enabling photonics quantum technologies. Due to mature technological processes for waveguide structure integration, as well as inherent and efficient properties for nonlinear optical effects, lithium niobate devices are nowadays at the heart of many photon-pair or triplet sources, single-photon detectors, coherent wavelength-conversion interfaces, and quantum memories. Consequently, they find applications in advanced and complex quantum communication systems, where compactness, stability, efficiency, and interconnectability with other guided-wave technologies are required. In this review paper, we first introduce the material aspects of lithium niobate, and subsequently discuss all of the above mentioned quantum components, ranging from standard photon-pair sources to more complex and advanced circuits.

quant-ph↗

arXiv2016

Optimal analysis of ultra broadband energy-time entanglement for high bit-rate dense wavelength division multiplexed quantum networks

We demonstrate an experimental method for measuring energy-time entanglement over almost 80 nm spectral bandwidth in a single shot with a quantum bit error rate below 0.5%. Our scheme is extremely cost-effective and efficient in terms of resources as it employs only one source of entangled photons and one fixed unbalanced interferometer per phase-coded analysis basis. We show that the maximum analysis spectral bandwidth is obtained when the analysis interferometers are properly unbalanced, a strategy which can be straightforwardly applied to most of today's experiments based on energy-time and time-bin entanglement. Our scheme has therefore a great potential for boosting bit rates and reducing the resource overhead of future entanglement-based quantum key distribution systems.

quant-ph↗

arXiv2016

Entanglement distribution over 150 km in wavelength division multiplexed channels for quantum cryptography

Granting information privacy is of crucial importance in our society, notably in fiber communication networks. Quantum cryptography provides a unique means to establish, at remote locations, identical strings of genuine random bits, with a level of secrecy unattainable using classical resources. However, several constraints, such as non-optimized photon number statistics and resources, detectors' noise, and optical losses, currently limit the performances in terms of both achievable secret key rates and distances. Here, these issues are addressed using an approach that combines both fundamental and off-the-shelves technological resources. High-quality bipartite photonic entanglement is distributed over a 150 km fiber link, exploiting a wavelength demultiplexing strategy implemented at the end-user locations. It is shown how coincidence rates scale linearly with the number of employed telecommunication channels, with values outperforming previous realizations by almost one order of magnitude. Thanks to its potential of scalability and compliance with device-independent strategies, this system is ready for real quantum applications, notably entanglement-based quantum cryptography.

quant-ph↗