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Florian Pilat

Publications and source records attributed to Florian Pilat.

5 recordsLinked to original sources

Microwave noise downconversion in interband cascade laser frequency combs

Chip-scale semiconductor laser frequency combs offer remarkable prospects for compact and power-efficient optical sensors. For the laser to be suitable for typical comb applications, its degree of coherence must first be assessed from a microwave self-mixing signal. Unfortunately, such measurements require scarcely available high-speed photodetectors with multi-GHz bandwidths and radio-frequency electronics. However, in this work, we demonstrate a simplified approach to comb coherence assessment for interband cascade lasers based on a relationship between easily-accessible MHz-frequency (baseband) noise and the multi-GHz-frequency intermode beat note. The downconversion of microwave noise to near-DC frequencies is found to originate intrinsically from the laser, which simultaneously acts as a frequency mixer due to electrical nonlinearities and a phase-to-amplitude noise converter due to the linewidth enhancement factor. Correlation between the electrical signals is explored in both frequency and time domains. Since this phenomenon is potentially universal in semiconductor lasers, it creates a new opportunity for frequency comb characterization, which may be particularly valuable in wavelength regions where fast photodetectors have limited availability.

physics.optics

Fast Gain Dynamics in Interband Cascade Lasers

Interband Cascade Lasers (ICL) have matured into a versatile technological platform in the mid-infrared spectral domain. To broaden their applicability even further, ongoing research pursues the emission of ultrashort pulses. The most promising approach is passive mode-locking with a fast saturable absorber. However, despite vast attempts no passive mode-locked ICL has been demonstrated up to date. In this study we perform pump-probe measurements on the ICL gain and show that its dynamics are mainly ($\sim$70%) governed by a fast recovery time of 2 ps. Our findings explain why passive mode-locking has not succeeded so far, shedding a new light on ICL dynamics as we propose strategies to overcome the current limitations.

physics.optics

Nozaki-Bekki optical solitons

Recent years witnessed rapid progress of chip-scale integrated optical frequency comb sources. Among them, two classes are particularly significant -- semiconductor Fabry-Perót lasers and passive ring Kerr microresonators. Here, we merge the two technologies in a ring semiconductor laser and demonstrate a new paradigm for free-running soliton formation, called Nozaki-Bekki soliton. These dissipative waveforms emerge in a family of traveling localized dark pulses, known within the famed complex Ginzburg-Landau equation. We show that Nozaki-Bekki solitons are structurally-stable in a ring laser and form spontaneously with tuning of the laser bias -- eliminating the need for an external optical pump. By combining conclusive experimental findings and a complementary elaborate theoretical model, we reveal the salient characteristics of these solitons and provide a guideline for their generation. Beyond the fundamental soliton circulating inside the ring laser, we demonstrate multisoliton states as well, verifying their localized nature and offering an insight into formation of soliton crystals. Our results consolidate a monolithic electrically-driven platform for direct soliton generation and open a door for a new research field at the junction of laser multimode dynamics and Kerr parametric processes.

physics.optics

Spectrally resolved linewidth enhancement factor of a semiconductor frequency comb

The linewidth enhancement factor (LEF) has recently moved into the spotlight of research on frequency comb generation in semiconductor lasers. Here we present a novel modulation experiment, which enables the direct measurement of the spectrally resolved LEF in a laser frequency comb. By utilizing a phase-sensitive technique, we are able to extract the LEF for each comb mode. We first investigate and verify this universally applicable technique using Maxwell-Bloch simulations and then present the experimental demonstration on a quantum cascade laser frequency comb.

physics.optics

Influence of Environmentally Affected Hole Transport Layers on Spatial Homogeneity and Charge Transport Dynamics of Organic Solar Cells

After the efficiency of organic photovoltaic (OPV) cells achieved more than 10%, the control of stability and degradation mechanisms of solar cells became a prominent task. The improvement of device efficiency due to incorporation of a hole-transport layer (HTL) in bulk-heterojunction solar cells has been extensively reported. However, the most widely used HTL material, PEDOT:PSS is frequently suspected to be the dominating source for devices instability under environmental conditions. Thereby effects like photooxidation and electrode corrosion are often reported to shorten device lifetime. However, often in environmental device studies, the source of degradation, whether being from the HTL, the active layer or the metal cathode are rather difficult to distinguish, because the external diffusion of oxygen and water affects all components. In this study, different HTLs, namely prepared from traditional PEDOT:PSS and also two types of molybdenum trioxide (MoO3), are exposed to different environments such as oxygen, light or humidity, prior to device finalization under inert conditions. This allows investigating any effects within the HTL and from reactions at its interface to the indium-tin-oxide electrode or the active layer. The surface and bulk chemistry of the exposed HTL has been monitored and discussed in context to the observed device physics, dynamic charge transport and spatial performance homogeneity of the according OPV device. The results show that merely humidity-exposure of the HTL leads to decreased device performance for PEDOT:PSS, but also for one type of the tested MoO3. The losses are related to the amount of absorbed water in the HTL, inducing loss of active area in terms of interfacial contact. The device with PEDOT:PSS HTL after humid air exposure showed seriously decreased photocurrent by micro-delamination of swelling/shrinkage of the hygroscopic layer.

physics.app-ph