arXiv subjects

Frédéric Bouchard

Publications and source records attributed to Frédéric Bouchard.

At least 19 recordsLinked to original sources

arXiv2026

High-Dimensional Quantum Photonics: Roadmap

The field of high-dimensional quantum photonics involves the use of multimode photonic degrees-of-freedom such as the spatial, temporal, or spectral structure of light to encode multi-level quantum states. Recent years have seen rapid progress in the development of methods to generate, manipulate, and distribute such quantum states of light and their use in a range of quantum technology applications that offer practical advantages over conventional qubit-based approaches. High-dimensional quantum states of light encoded in photonic time-bins, frequency-bins, transverse-spatial modes, waveguide paths, and temporal modes have enabled noise-robust fundamental tests of quantum mechanics, error-resilient and high-capacity quantum communication protocols, andas well as efficient approaches for quantum information processing, to name just a few examples. However, research in this field has progressed fairly independently, with little exchange across different photonic degrees-of-freedom or between experiment and theory and no comprehensive comparison between degrees-of-freedom. This roadmap aims to bridge this gap by surveying progress in each area and identifying shared challenges and opportunities that cut across two or more photonic degrees-of-freedoms. We review early work and state-of-the-art experimental techniques under development for high-dimensional quantum states encoded in single and entangled photons, as well as theoretical tools for their measurement and certification. We outline the main outstanding challenges for theory and each experimental degree-of-freedom, identifying promising future directions of research that may enable these to be overcome. We end by discussing interconnections and shared challenges centered around their distribution, measurement, and manipulation, with a view towards their integration into next-generation quantum technology platforms and applications.

quant-ph↗

arXiv2026

Simultaneous amplitude and phase spectroscopy using two-photon interference

Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin beams of light to reduce the noise sources inherent to absorption spectroscopy. However, measurements of the phase shift imparted by the chemical sample, which provides complementary information to the absorption, continue to be a challenge. Here, we propose and demonstrate a scheme using entangled photon pairs that can simultaneously measure both the absorption and phase shift of a sample with extremely low optical intensities and with relatively fast few-minute acquisition times. This method combines the previous use of intensity correlations with a broadband quantum interferometer utilizing two-photon interference to measure the complete linear optical response of the sample. Our work shows that precise measurements of absorption can also be made phase-sensitive using suitable choices of probe beam and detection scheme. This enables a new class of quantum spectroscopy schemes which measure absorption and phase with a single probe. Our technique is relevant to the characterization of a wide array of chemical and biological samples, such as quantum dots and organic fluorophores, and may be useful for spectroscopic measurements that are otherwise constrained in intensity.

quant-ph↗

arXiv2025

Ultrafast switching of telecom photon-number states

A crucial component of photonic quantum information processing platforms is the ability to modulate, route, convert, and switch quantum states of light noiselessly with low insertion loss. For instance, a high-speed, low-loss optical switch is crucial for scaling quantum photonic systems that rely on measurement-based feed-forward approaches. Such a device will also ideally be capable of operating on photon-number states, which can act as non-Gaussian resources. Here, we demonstrate ultrafast all-optical switching of heralded photon-number states, of up to 6 photons, using the optical Kerr effect in a single-mode fiber. A local birefringence is created by a high-intensity pump pulse at a center wavelength of 1030 nm which overlaps temporally with the 1550 nm photons in the fiber. A switching efficiency of $>$99 % is reached with a resolution of 2.3 ps, an insertion loss of $2.27\pm0.08$ dB, and a signal-to-noise ratio of 32,000.

quant-ph↗

arXiv2025

Broadband spectral manipulation of single photons using cross-phase modulation

Manipulating the frequency and bandwidth of light is crucial in classical and quantum applications including communication, spectroscopy, imaging, and signal processing. Such capabilities also offer potential for interfacing disparate quantum systems in quantum networking and for quantum information processing. We experimentally demonstrate deterministic, broadband frequency control of heralded telecom-band single photons via cross-phase modulation in a short length of single-mode fiber. An intense, ultrafast pump pulse imposes a transient, intensity-dependent refractive-index gradient which imparts a tunable phase shift on the single photons. We present absolute frequency shifts of up to $+6.46\pm0.01$\,THz and $-5.74\pm0.01$\,THz, and bandwidth manipulation ranging from a factor of $0.66\pm0.03$ to $8.4\pm0.3$ times that of the input. Spectral measurements are acquired with a time-of-flight spectrometer and superconducting nanowire detectors. Our scheme offers a compact and scalable route to spectral routing and bandwidth engineering for ultrafast quantum networking and quantum information processing.

quant-ph↗

arXiv2025

Imaging at the quantum limit with convolutional neural networks

Deep neural networks have been shown to achieve exceptional performance for computer vision tasks like image recognition, segmentation, and reconstruction or denoising. Here, we evaluate the ultimate performance limits of deep convolutional neural network models for image reconstruction, by comparing them against the standard quantum limit set by shot-noise and the Heisenberg limit on precision. We train U-Net models on images of natural objects illuminated with coherent states of light, and find that the average mean-squared error of the reconstructions can surpass the standard quantum limit, and in some cases reaches the Heisenberg limit. Further, we train models on well-parameterized images for which we can calculate the quantum Cramér-Rao bound to determine the minimum possible measurable variance of an estimated parameter for a given probe state. We find the mean-squared error of the model predictions reaches these bounds calculated for the parameters, across a variety of parameterized images. These results suggest that deep convolutional neural networks can learn to become the optimal estimators allowed by the laws of physics, performing parameter estimation and image reconstruction at the ultimate possible limits of precision for the case of classical illumination of the object.

cs.LG↗

arXiv2025

Ultrafast all-optical modulation of spatially structured photons

Manipulating the structure of single photons in the ultrafast domain is enabling new quantum information processing technologies. At the picosecond timescale, quantum information can be processed before decoherence can occur. In this work, we study the capabilities of few-mode cross-phase modulation via the optical Kerr effect, using ultrafast pulses. We observe a significant modulation in the spatial mode of structured photons on timescales $\leq 1.3$~ps.

quant-ph↗

arXiv2025

High-Dimensional Quantum Key Distribution with Qubit-like States

Quantum key distribution (QKD) protocols most often use two conjugate bases in order to verify the security of the quantum channel. In the majority of protocols, these bases are mutually unbiased to one another, which is to say they are formed from balanced superpositions of the entire set of states in the opposing basis. Here, we introduce a high-dimensional QKD protocol using qubit-like states, referred to as Fourier-qubits (or $\textit{F}$-qubits). In our scheme, each $\textit{F}$-qubit is a superposition of only two computational basis states with a relative phase that can take $d$ distinct values, where $d$ is the dimension of the computational basis. This non-mutually unbiased approach allows us to bound the information leaked to an eavesdropper, maintaining security in high-dimensional quantum systems despite the states' seemingly two-dimensional nature. By simplifying state preparation and measurement, our protocol offers a practical alternative for secure high-dimensional quantum communications. We experimentally demonstrate this protocol for a noisy high-dimensional QKD channel using the orbital angular momentum degree of freedom of light and discuss the potential benefits for encoding in other degrees of freedom.

quant-ph↗

arXiv2025

Terahertz electro-optic modulation of single photons

The manipulation of visible and near-infrared light at the single-photon level plays a key role in quantum communication systems where information is encoded into photonic degrees of freedom. In practical implementations, it is important to achieve this manipulation with high speeds, low loss, and low noise. In this work, we propose the use of terahertz~(THz) electric fields as a pump source for electro-optic modulation of single photons in bulk media. We demonstrate spectral modulations of single photons in the form of frequency translation and bandwidth manipulations as the terahertz field imparts linear and quadratic phases on the photons at various time delays within 1~ps. Our results show frequency translations exceeding 500~GHz at multi-THz modulation speeds and loss levels of $\approx$1~dB, complementing the current state-of-the-art electro-optic modulation techniques limited to speeds up to 100~GHz. The proposed approach leverages recent developments in terahertz generation techniques, introducing new avenues to manipulate non-classical light in an unexplored regime for quantum photonics.

quant-ph↗

arXiv2024

Gain-induced group delay in spontaneous parametric down-conversion

Strongly-driven nonlinear optical processes such as spontaneous parametric down-conversion and spontaneous four-wave mixing can produce multiphoton nonclassical beams of light which have applications in quantum information processing and sensing. In contrast to the low-gain regime, new physical effects arise in a high-gain regime due to the interactions between the nonclassical light and the strong pump driving the nonlinear process. Here, we describe and experimentally observe a gain-induced group delay between the multiphoton pulses generated in a high-gain type-II spontaneous parametric down-conversion source. Since the group delay introduces distinguishability between the generated photons, it will be important to compensate for it when designing quantum interference devices in which strong optical nonlinearities are required.

quant-ph↗

arXiv2024

Multiphoton interference in a single-spatial-mode quantum walk

Multiphoton interference is crucial to many photonic quantum technologies. In particular, interference forms the basis of optical quantum information processing platforms and can lead to significant computational advantages. It is therefore interesting to study the interference arising from various states of light in large interferometric networks. Here, we implement a quantum walk in a highly stable, low-loss, multiport interferometer with up to 24 ultrafast time bins. This time-bin interferometer comprises a sequence of birefringent crystals which produce pulses separated by 4.3\,ps, all along a single optical axis. Ultrafast Kerr gating in an optical fiber is employed to time-demultiplex the output from the quantum walk. We measure one-, two-, and three-photon interference arising from various input state combinations, including a heralded single-photon state, a thermal state, and an attenuated coherent state at one or more input ports. Our results demonstrate that ultrafast time bins are a promising platform to observe large-scale multiphoton interference.

quant-ph↗

arXiv2024

Predicting atmospheric turbulence for secure quantum communications in free space

Atmospheric turbulence is the main barrier to large-scale free-space quantum communication networks. Aberrations distort optical information carriers, thus limiting or preventing the possibility of establishing a secure link between two parties. For this reason, forecasting the turbulence strength within an optical channel is highly desirable, as it allows for knowing the optimal timing to establish a secure link in advance. Here, we train a Recurrent Neural Network, TAROCCO, to predict the turbulence strength within a free-space channel. The training is based on weather and turbulence data collected over 9 months for a 5.4 km intra-city free-space link across the City of Ottawa. The implications of accurate predictions from our network are demonstrated in a simulated high-dimensional Quantum Key Distribution protocol based on orbital angular momentum states of light across different turbulence regimes. TAROCCO will be crucial in validating a free-space channel to optimally route the key exchange for secure communications in real experimental scenarios.

quant-ph↗

arXiv2024

Programmable Photonic Quantum Circuits with Ultrafast Time-bin Encoding

We propose a quantum information processing platform that utilizes the ultrafast time-bin encoding of photons. This approach offers a pathway to scalability by leveraging the inherent phase stability of collinear temporal interferometric networks at the femtosecond-to-picosecond timescale. The proposed architecture encodes information in ultrafast temporal bins processed using optically induced nonlinearities and birefringent materials while keeping photons in a single spatial mode. We demonstrate the potential for scalable photonic quantum information processing through two independent experiments that showcase the platform's programmability and scalability, respectively. The scheme's programmability is demonstrated in the first experiment, where we successfully program 362 different unitary transformations in up to 8 dimensions in a temporal circuit. In the second experiment, we show the scalability of ultrafast time-bin encoding by building a passive optical network, with increasing circuit depth, of up to 36 optical modes. In each experiment, fidelities exceed 97\%, while the interferometric phase remains passively stable for several days.

quant-ph↗

arXiv2024

Photonic quantum walk with ultrafast time-bin encoding

The quantum walk (QW) has proven to be a valuable testbed for fundamental inquiries in quantum technology applications such as quantum simulation and quantum search algorithms. Many benefits have been found by exploring implementations of QWs in various physical systems, including photonic platforms. Here, we propose a novel platform to perform quantum walks using an ultrafast time-bin encoding (UTBE) scheme. This platform supports the scalability of quantum walks to a large number of steps while retaining a significant degree of programmability. More importantly, ultrafast time bins are encoded at the picosecond time scale, far away from mechanical fluctuations. This enables the scalability of our platform to many modes while preserving excellent interferometric phase stability over extremely long periods of time without requiring active phase stabilization. Our 18-step QW is shown to preserve interferometric phase stability over a period of 50 hours, with an overall walk fidelity maintained above $95\%$

quant-ph↗

arXiv2024

3D-2D Neural Nets for Phase Retrieval in Noisy Interferometric Imaging

In recent years, neural networks have been used to solve phase retrieval problems in imaging with superior accuracy and speed than traditional techniques, especially in the presence of noise. However, in the context of interferometric imaging, phase noise has been largely unaddressed by existing neural network architectures. Such noise arises naturally in an interferometer due to mechanical instabilities or atmospheric turbulence, limiting measurement acquisition times and posing a challenge in scenarios with limited light intensity, such as remote sensing. Here, we introduce a 3D-2D Phase Retrieval U-Net (PRUNe) that takes noisy and randomly phase-shifted interferograms as inputs, and outputs a single 2D phase image. A 3D downsampling convolutional encoder captures correlations within and between frames to produce a 2D latent space, which is upsampled by a 2D decoder into a phase image. We test our model against a state-of-the-art singular value decomposition algorithm and find PRUNe reconstructions consistently show more accurate and smooth reconstructions, with a x2.5 - 4 lower mean squared error at multiple signal-to-noise ratios for interferograms with low (< 1 photon/pixel) and high (~100 photons/pixel) signal intensity. Our model presents a faster and more accurate approach to perform phase retrieval in extremely low light intensity interferometry in presence of phase noise, and will find application in other multi-frame noisy imaging techniques.

physics.optics↗

arXiv2023

High-dimensional Encoding in the Round-Robin Differential-Phase-Shift Protocol

In quantum key distribution (QKD), protocols are tailored to adopt desirable experimental attributes, including high key rates, operation in high noise levels, and practical security considerations. The round-robin differential phase shift protocol (RRDPS), falling in the family of differential phase shift protocols, was introduced to remove restrictions on the security analysis, such as the requirement to monitor signal disturbances, improving its practicality in implementations. While the RRDPS protocol requires the encoding of single photons in high-dimensional quantum states, at most, only one bit of secret key is distributed per sifted photon. However, another family of protocols, namely high-dimensional (HD) QKD, enlarges the encoding alphabet, allowing single photons to carry more than one bit of secret key each. The high-dimensional BB84 protocol exemplifies the potential benefits of such an encoding scheme, such as larger key rates and higher noise tolerance. Here, we devise an approach to extend the RRDPS QKD to an arbitrarily large encoding alphabet and explore the security consequences. We demonstrate our new framework with a proof-of-concept experiment and show that it can adapt to various experimental conditions by optimizing the protocol parameters. Our approach offers insight into bridging the gap between seemingly incompatible quantum communication schemes by leveraging the unique approaches to information encoding of both HD and DPS QKD.

quant-ph↗

arXiv2023

Measuring ultrafast time-bin qudits

Time-bin qudits have emerged as a promising encoding platform in many quantum photonic applications. However, the requirement for efficient single-shot measurement of time-bin qudits instead of reconstructive detection has restricted their widespread use in experiments. Here, we propose an efficient method to measure arbitrary superposition states of time-bin qudits and confirm it up to dimension 4. This method is based on encoding time bins at the picosecond time scale, also known as ultrafast time bins. By doing so, we enable the use of robust and phase-stable single spatial mode temporal interferometers to measure time-bin qudit in different measurement bases.

quant-ph↗

arXiv2021

Quantum communication with ultrafast time-bin qubits

The photonic temporal degree of freedom is one of the most promising platforms for quantum communication over fiber networks and free-space channels. In particular, time-bin states of photons are robust to environmental disturbances, support high-rate communication, and can be used in high-dimensional schemes. However, the detection of photonic time-bin states remains a challenging task, particularly for the case of photons that are in a superposition of different time-bins. Here, we experimentally demonstrate the feasibility of picosecond time-bin states of light, known as ultrafast time-bins, for applications in quantum communications. With the ability to measure time-bin superpositions with excellent phase stability, we enable the use of temporal states in efficient quantum key distribution protocols such as the BB84 protocol.

quant-ph↗

arXiv2021

Photonic angular super-resolution using twisted N00N states

The increased phase sensitivity of N00N states has been used in many experiments, often involving photon paths or polarization. Here we experimentally combine the phase sensitivity of N00N states with the orbital angular momentum (OAM) of photons up to 100$\,\hslash$, to resolve rotations of a light field around its optical axis. The results show that both a higher photon number and larger OAM increase the resolution and achievable sensitivity. The presented method opens a viable path to unconditional angular super-sensitivity and accessible generation of N00N states between any transverse light fields.

quant-ph↗