arXiv subjects

François Debontridder

Publications and source records attributed to François Debontridder.

10 recordsLinked to original sources

arXiv2026

Multigap superconductivity in Ising superconductors: The case of (LaSe)1.14(NbSe2)m misfit layer compounds

Strong spin-orbit coupling and broken inversion symmetry in transition metal dichalcogenides give rise to Ising superconductivity, a spin-protected pairing state first identified in monolayer NbSe$_2$ through in-plane critical fields far exceeding the Pauli limit. More recently, Ising superconductivity has been proposed as a potential route to unconventional and even topological superconductivity in bulk misfit compounds. Here, we investigate the superconducting order parameter of layered misfit compounds composed of alternating transition metal dichalcogenide and rocksalt layers, which host extremely doped, electronically decoupled NbSe$_2$ sheets within a three-dimensional crystal. Using directional scanning tunneling spectroscopy on the misfit superconductors (LaSe)$_{1.14}$(NbSe$_2$) and (LaSe)$_{1.14}$(NbSe$_2$)$_2$, we uncover a strongly anisotropic multigap superconducting state: a fragile gap on the $Γ$-centered Fermi-surface pocket coexists with a robust, intrinsic gap on the K and K$'$ pockets. These features are in quantitative agreement with momentum-resolved gaps $Δ(\mathbf{k})$ obtained from anisotropic Migdal-Eliashberg calculations. The marked fragility of the $Γ$-centered gap, combined with the strong sensitivity of the critical temperature to non-magnetic disorder, points to pairing beyond conventional $s$-wave symmetry, potentially involving a topological order parameter. These results establish NbSe$_2$-based misfit compounds as a tunable bulk platform for multigap, unconventional superconductivity, with Ising protection offering a promising route toward topological pairing.

cond-mat.supr-con↗

arXiv2025

Moiré pattern multiplicity driven by electronic effects in two-dimensional CrCl3/Au heterostructures

Moiré patterns are a central motif in van der Waals heterostructures arising from the superposition of two-dimensional (2D) incommensurate lattices. These patterns reveal a wealth of correlated effects, influencing electronic, magnetic, and structural phenomena. While diffraction techniques typically resolve multiple moiré wave-vectors corresponding to the incommensurate nature of the underlying lattices, Scanning Tunneling Microscopy (STM) often reveals only a dominant superperiod. In this work, we address this apparent discrepancy through an STM study of a twisted monolayer of CrCl3 on Au(111). We observe the coexistence of several moiré patterns at a fixed twist angle, whose relative intensity depends on the tunneling bias. Fourier analysis of STM data uncovers hidden higher-order moiré components not visible in STM topographic images, while spectroscopy maps reveal that the spectral weight of each pattern varies with electron energy. Our results establish that STM selectively probes on the same area distinct moiré modulations depending on electronic confinement, providing a unified framework that reconciles real space and reciprocal space observations of complex moiré superstructures.

cond-mat.other↗

arXiv2025

Anderson transition symmetries at the band-edge of a correlated Sn/Si monolayer

Anderson localization is predicted to enhance the critical temperature of disordered superconductors. Despite a huge body of theoretical work based on non-linear sigma models, experiments are lacking to understand correlated electrons in disordered potentials. In this study, we investigate a tin monolayer on silicon, a material known for its likely antiferromagnetic Mott-correlated groundstate. We analyze the statistical properties of tunneling conductance maps of increasingly localized states as we approach the edge of the valence band. Using multifractal analysis, we show that the system follows an exact symmetry relation based on the algebraic structure of nonlinear sigma-models (NLsMs). We anticipate that this symmetry may be broken in specific - e.g. chiral electronic phases. Finally, we point out that multifractal analysis can equally be applied to universal conductance fluctuations in magneto-transport experiments, thus providing a powerful tool to probe the underlying symmetries of disordered electronic phases.

cond-mat.mes-hall↗

arXiv2020

Misfit layer compounds: a platform for heavily-doped two-dimensional transition metal dichalcogenides

Transition metal dichalcogenides (TMDs) display a rich variety of instabilities such as spin and charge orders, Ising superconductivity and topological properties. Their physical properties can be controlled by doping in electric double-layer field-effect transistors (FET). However, for the case of single layer NbSe$_2$, FET doping is limited to $\approx 1\times 10^{14}$ cm$^{-2}$, while a somewhat larger charge injection can be obtained via deposition of K atoms. Here, by performing ARPES, STM, quasiparticle interference measurements, and first principles calculations we show that a misfit compound formed by sandwiching NbSe$_2$ and LaSe layers behaves as a NbSe$_2$ single layer with a rigid doping of $0.55-0.6$ electrons per Nb atom or $\approx 6\times 10^{14}$ cm$^{-2}$. Due to this huge doping, the $3\times3$ charge density wave is replaced by a $2\times2$ order with very short coherence length. As a tremendous number of different misfit compounds can be obtained by sandwiching TMDs layers with rock salt or other layers, our work paves the way to the exploration of heavily doped 2D TMDs over an unprecedented wide range of doping.

cond-mat.mtrl-sci↗

arXiv2018

Isolated pairs of Majorana zero modes in a disordered superconducting lead monolayer

Majorana zero modes are fractional quantum excitations appearing in pairs, each pair being a building block for quantum computation . Some possible signatures of these excitations have been reported as zero bias peaks at endpoints of one-dimensional semiconducting wires and magnetic chains. However, 1D systems are by nature fragile to a small amount of disorder that induces low-energy excitations, hence obtaining Majorana zero modes well isolated in a hard gap requires extremely clean systems. Two-dimensional systems offer an alternative route to get robust Majorana zero modes. Indeed, it was shown recently that Pb/Co/Si(111) could be used as a platform for generating 2D topological superconductivity with a strong immunity to local disorder. While 2D systems exhibit dispersive chiral edge states, they can also host Majorana zero modes located on local topological defects. According to predictions, if an odd number of zero modes are located in a topological domain an additional zero mode should appear all around the domain's edge. Here we use scanning tunneling spectroscopy to characterize a disordered superconducting monolayer of Pb coupled to underlying Co-Si magnetic islands meant to induce a topological transition. We show that pairs of zero modes are stabilized: one zero mode positioned at a point in the middle of the magnetic domain and its zero mode partner extended all around the domain. The zero mode pair is remarkably robust, it is isolated within a hard superconducting energy gap and it appears totally immune to the strong disorder present in the Pb monolayer. Our theoretical scenario supports the protected Majorana nature of this zero mode pair, highlighting the role of magnetic or spin-orbit coupling textures. This robust pair of Majorana zero modes offers a new platform for theoretical and experimental study of quantum computing.

cond-mat.supr-con↗

arXiv2018

Yu-Shiba-Rusinov bound states versus topological edge states in Pb/Si(111)

There is presently a tremendous activity around the field of topological superconductivity and Majorana fermions. Among the many questions raised, it has become increasingly important to establish the topological or non-topological origin of features associated with Majorana fermions such as zero-bias peaks. Here, we compare in-gap features associated either with isolated magnetic impurities or with magnetic clusters strongly coupled to the atomically thin superconductor Pb/Si(111). We study this system by means of scanning tunneling microscopy and spectroscopy (STM/STS). We take advantage of the fact that the Pb/Si(111) monolayer can exist either in a crystal-ordered phase or in an incommensurate disordered phase to compare the observed spectroscopic features in both phases. This allows us to demonstrate that the strongly resolved in-gap states we found around the magnetic clusters in the disordered phase of Pb have a clear topological origin.

cond-mat.supr-con↗

arXiv2017

Two-dimensional topological superconductivity in Pb/Co/Si(111)

Just like insulators can host topological Dirac states at their edges, superconductors can also exhibit topological phases characterized by Majorana edge states. Remarkable zero-energy states have been recently observed at the two ends of proximity induced superconducting wires, and were interpreted as localized Majorana end states in one-dimensional (1D) topological superconductor. By contrast, propagating Majorana states should exist at the 1D edges of two-dimensional (2D) topological superconductors. Here we report the direct observation of dispersive in-gap states surrounding topological superconducting domains made of a single atomic layer of Pb covering magnetic islands of Co/Si(111). We interpret the observed continuous dispersion across the superconducting gap in terms of a spatial topological transition accompanied by a chiral edge mode and residual gaped helical edge states. Our experimental approach enables the engineering and control of a large variety of novel quantum phases. This opens new horizons in the field of quantum materials and quantum electronics where the magnetization of the domains could be used as a control parameter for the manipulation of topological states.

cond-mat.supr-con↗

arXiv2015

Long range coherent magnetic bound states in superconductors

The quantum coherent coupling of completely different degrees of freedom is a challenging path towards creating new functionalities for quantum electronics. Usually the antagonistic coupling between spins of magnetic impurities and superconductivity leads to the destruction of the superconducting order. Here we show that a localized classical spin of an iron atom immersed in a superconducting condensate can give rise to new kind of long range coherent magnetic quantum state. In addition to the well-known Shiba bound state present on top of an impurity we reveal the existence of a star shaped pattern which extends as far as 12 nm from the impurity location. This large spatial dispersion turns out to be related, in a non-trivial way, to the superconducting coherence length. Inside star branches we observed short scale interference fringes with a particle-hole asymmetry. Our theoretical approach captures these features and relates them to the electronic band structure and the Fermi wave length of the superconductor. The discovery of a directional long range effect implies that distant magnetic atoms could coherently interact leading to new topological superconducting phases with fascinating properties.

cond-mat.supr-con↗

arXiv2013

Electric pulse induced electronic patchwork in the Mott insulator GaTa$_{4}$Se$_{8}$

Following a recent discovery of the Insulator-to-Metal Transition induced by electric field in GaTa$_{4}$Se$_{8}$, we performed a detailed Scanning Tunneling Microscopy/Spectroscopy study of both pristine (insulating) and transited (conducting) crystals of this narrow gap Mott insulator. The spectroscopic maps show that pristine samples are spatially homogeneous insulators while the transited samples reveal at nanometer scale a complex electronic pattern that consists of metallic and super-insulating patches immersed in the pristine insulating matrix. Surprisingly, both kinds of patches are accompanied by a strong local topographic inflation, thus evidencing for a strong electron-lattice coupling involved in this metal-insulator transition. Finally, using a strong electric field generated across the STM tunneling junction, we demonstrate the possibility to trig the metal-insulator transition locally even at room temperature.

cond-mat.str-el↗

arXiv2009

Electric field effects, Mott insulator, Surface patterning, Scanning tunneling microscopy, Transition metal chalcogenides

We report the first experimental evidence for a strong electromechanical coupling in the Mott insulator GaTa4Se8 allowing a highly reproducible nano-writing with a Scanning Tunneling Microscope (STM). The local electric field across the STM junction is observed to have a threshold value above which the clean (100) surface of GaTa4Se8 becomes mechanically instable: At voltage biases V > 1.1V the surface suddenly inflates and comes in contact with the STM tip, resulting in nanometer size craters. The formed pattern can be indestructibly "read" by STM at lower voltage bias, thus allowing a 5 Tdots/inch2 dense writing/reading at room temperature. The discovery of the electromechanical coupling in GaTa4Se8 might give new clues in the understanding of the Electric Pulse Induced Resistive Switching recently observed in this stoechiometric Mott insulator.

cond-mat.mtrl-sci↗