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Francesc Pérez-Murano

Publications and source records attributed to Francesc Pérez-Murano.

3 recordsLinked to original sources

Dichroism of coupled multipolar plasmonic modes in twisted triskelion stacks

We present a systematic investigation of the optical response to circularly polarized illumination in twisted stacked plasmonic nanostructures. The system consissts in two identical, parallel gold triskelia centrally aligned and rotated at a central angle relative to each other. Sample fabrication was acomplished through a double electron beam lithograpy process. This stack holds two plasmonic modes of multipolar character in the near-infrared range, showing a strong dependence of their excitation intensities on the handedness of the circularly polarized incident light. This translates in a large circular dicrhoism which can be modulated by adjusting the twist angle of the stack. Fourier-transform infrared spectroscopy and numerical simulations were employed to characterize the spectral features of the modes. Remarkable, in contrast to previous results in other stacked nanostructures, the system's response exhibits a behavious analogous to that of two interacting dipoles only at small angles. As the angle approaches 15 degrees, where the maximum dichroism is observed, more complex modes of the stack emerge. These modes evolve towards two in-phase multipolar excitations of the two triskelia as the angle increases uo to 60 degrees. Finally, simulations for a triangular array of such stacked elements show a sharp mode arising from the hybridization of a surface lattice resonance with the low-energy mode of the stack.

physics.optics↗

Roadmap for focused ion beam technologies

The focused ion beam (FIB) is a powerful tool for the fabrication, modification and characterization of materials down to the nanoscale. Starting with the gallium FIB, which was originally intended for photomask repair in the semiconductor industry, there are now many different types of FIB that are commercially available. These instruments use a range of ion species and are applied broadly in materials science, physics, chemistry, biology, medicine, and even archaeology. The goal of this roadmap is to provide an overview of FIB instrumentation, theory, techniques and applications. By viewing FIB developments through the lens of the various research communities, we aim to identify future pathways for ion source and instrumentation development as well as emerging applications, and the scope for improved understanding of the complex interplay of ion-solid interactions. We intend to provide a guide for all scientists in the field that identifies common research interests and will support future fruitful interactions connecting tool development, experiment and theory. While a comprehensive overview of the field is sought, it is not possible to cover all research related to FIB technologies in detail. We give examples of specific projects within the broader context, referencing original works and previous review articles throughout.

physics.ins-det↗

Stiffening graphene by controlled defect creation

Graphene extraordinary strength, stiffness and lightness have generated great expectations towards its application in flexible electronics and as mechanical reinforcement agent. However, the presence of lattice defects, unavoidable in sheets obtained by scalable routes, might degrade its mechanical properties. Here we report a systematic study on the elastic modulus and strength of graphene with controlled density of defects. Counter intuitively, the in-plane Young modulus increases with increasing defect density up to almost twice the initial value for vacancy content of ~0.2%, turning it into the stiffest material ever reported. For higher density of vacancies, elastic modulus decreases with defect inclusion. The initial increase in Young modulus is explained in terms of a dependence of the elastic coefficients with the momentum of flexural modes predicted for 2D membranes. In contrast, the fracture strength decreases with defect density according to standard fracture continuum models. These quantitative structure-property relationships, measured in atmospheric conditions, are of fundamental and technological relevance and provide guidance for applications in which graphene mechanics represents a disruptive improvement.

cond-mat.mtrl-sci↗