arXiv subjects

Francesco Ancilotto

Publications and source records attributed to Francesco Ancilotto.

At least 37 records · Page 2Linked to original sources

arXiv2020

Rotating mixed $^3$He-$^4$He nanodroplets

Mixed $^3$He-$^4$He droplets created by hydrodynamic instability of a cryogenic fluid-jet may acquire angular momentum during their passage through the nozzle of the experimental apparatus. These free-standing droplets cool down to very low temperatures undergoing isotopic segregation, developing a nearly pure $^3$He crust surrounding a very $^4$He-rich superfluid core. Here, the stability and appearance of rotating mixed helium droplets are investigated using Density Functional Theory for an isotopic composition that highlights, with some marked exceptions related to the existence of the superfluid inner core, the analogies with viscous rotating droplets.

cond-mat.quant-gas↗

arXiv2019

Rotating He-3 droplets

Motivated by recent experiments, we study normal-phase rotating He-3 droplets within Density Functional Theory in a semi-classical approach. The sequence of rotating droplet shapes as a function of angular momentum are found to agree with those of rotating classical droplets, evolving from axisymmetric oblate to triaxial prolate to two-lobed shapes as the angular momentum of the droplet increases. Our results, which are obtained for droplets of nanoscopic size, are rescaled to the mesoscopic size characterizing ongoing experimental measurements, allowing for a direct comparison of shapes. The stability curve in the angular velocity-angular momentum plane shows small deviations from the classical rotating drop model predictions, whose magnitude increases with angular momentum. We attribute these deviations to effects not included in the simplified classical model description of a rotating fluid held together by surface tension, i.e. to surface diffuseness, curvature and finite compressibility, and to quantum effects associated with deformation of the He-3 Fermi surface. The influence of all these effects is expected to diminish as the droplet size increases, making the classical rotating droplet model a quite accurate representation of He-3 rotation.

cond-mat.other↗

arXiv2019

Angular momentum in rotating superfluid droplets

The angular momentum of rotating superfluid droplets originates from quantized vortices and capillary waves, the interplay between which remains to be uncovered. Here, the rotation of isolated sub-micrometer superfluid 4He droplets is studied by ultrafast x-ray diffraction using a free electron laser. The diffraction patterns provide simultaneous access to the morphology of the droplets and the vortex arrays they host. In capsule-shaped droplets, vortices form a distorted triangular lattice, whereas they arrange along elliptical contours in ellipsoidal droplets. The combined action of vortices and capillary waves results in droplet shapes close to those of classical droplets rotating with the same angular velocity. The findings are corroborated by density functional theory calculations describing the velocity fields and shape deformations of a rotating superfluid cylinder.

cond-mat.other↗

arXiv2019

Vorticity and quantum turbulence in the merging of superfluid Helium nanodroplets

We have studied the merging of two $^4$He droplets at zero temperature, caused by their Van der Waals mutual attraction. During the early stages of the merging, density structures appear which closely match the experimental observations by Vicente et al. [J. Low Temp. Phys. 121, 627 (2000)]. When the droplets are merging, quantized vortex-antivortex ring pairs nucleate at the surface and annihilate inside the merged droplet producing a roton burst. We also observe the nucleation of quantized vortex-antivortex rings that wrap the droplet surface and remain localized on the surface until they eventually decay into short-wavelength surface waves. Analysis of the kinetic energy spectrum discloses the existence of a regime where turbulence caused by vortex interaction and annihilation is characterized by a Kolmogorov power law. This is followed by another regime where roton radiation (produced by vortex-antivortex annihilation) dominates, whose hallmark is a weak, turbulent surface dynamics. We suggest that similar processes might appear in superfluid helium droplets after they capture impurities or if they are produced by hydrodynamic instability of a liquid jet. Experiments on collisions between recently-discovered self-bound Bose-Einstein condensates should display a similar phenomenology.

cond-mat.mes-hall↗

arXiv2019

Supersolid behaviour of a dipolar Bose-Einstein condensate confined in a tube

Motivated by a recent experiment [L.Chomaz et al., Nature Physics 14, 442 (2018)], we perform numerical simulations of a dipolar Bose-Einstein Condensate (BEC) in a tubular confinement at T=0 within Density Functional Theory, where the beyond-mean-field correction to the ground state energy is included in the Local Density Approximation. We study the excitation spectrum of the system by solving the corresponding Bogoliubov-de Gennes equations. The calculated spectrum shows a roton minimum, and the roton gap decreases by reducing the effective scattering length. As the roton gap disappears, the system spontaneously develops in its ground-state a periodic, linear structure formed by denser clusters of atomic dipoles immersed in a dilute superfluid background. This structure shows the hallmarks of a supersolid system, i.e. (i) a finite non-classical translational inertia along the tube axis and (ii) the appearance, besides the phonon mode, of the Nambu-Goldstone gapless mode corresponding to phase fluctuations, and related to the spontaneous breaking of the gauge symmetry. A further decrease in the scattering length eventually leads to the formation of a periodic linear array of self-bound droplets.

cond-mat.quant-gas↗

arXiv2019

Prediction for two spatially modulated superfluids: $^4$He on fluorographene and on hexagonal BN

We have derived the adsorption potential of $^4$He atoms on fluorographene (GF), on graphane and on hexagonal boron nitride (hBN) by a recently developed ab initio method that incorporates the van der Waals interaction. The $^4$He monolayer on GF and on hBN is studied by state-of-the-art quantum simulations at T=0 K. With our adsorption potentials we find that in both cases the ground state of $^4$He monolayer is a fluid and not an ordered state with localized atoms as on graphite and on graphene. In the case of GF the present result is in qualitative agreement with the superfluid phase that was obtained using an empirical adsorption potential [M. Nava et al., Phys. Rev. B 86, 174509 (2012)]. This fluid state of $^4$He on GF and on hBN is characterized by a very large density modulation and at the equilibrium density the ratio $Γ$ between the largest and the smallest local density along the direction of two neighboring adsorption sites and averaged over the perpendicular direction is $Γ$ = 1.91 for GF and $Γ$ = 1.65 for hBN. Recent experiments [J. Nyeki et al., Nature Physics 13, 455 (2017)] have discovered a superfluid phase in the second layer $^4$He. This is a spatially modulated superfluid that turns out to have anomalous thermal properties. This gives a strong motivation for an experimental study of monolayer $^4$He on GF and on hBN that we predict to be a superfluid with a much stronger spatial modulation.

cond-mat.mes-hall↗

arXiv2018

Self-bound ultra dilute Bose mixtures within Local Density Approximation

We have investigated self-bound binary ultra dilute bosonic mixtures at zero temperature within Density Functional Theory using a Local Density Approximation. We provide the explicit expression of the Lee-Huang-Yang correction in the general case of heteronuclear mixtures, and investigate the general thermodynamic conditions which lead to the formation of self-bound systems. We have determined the conditions for stability against the evaporation of one component, as well as the mechanical and diffusive spinodal lines. We have also calculated the surface tension of the self-bound state as a function of the inter-species interaction strength. We find that relatively modest changes of the latter result in order-of-magnitude changes in the calculated surface tension. We suggest experimental realizations which might display the metastability and phase separation of the mixture when entering regions of the phase diagram characterized by negative pressures. Finally, we show that these droplets may sustain stable vortex and vortex dimers.

cond-mat.quant-gas↗

arXiv2018

Spinning superfluid helium-4 nanodroplets

We have studied spinning superfluid $^4$He nanodroplets at zero temperature using Density Functional theory. Due to the irrotational character of the superfluid flow, the shapes of the spinning nanodroplets are very different from those of a viscous normal fluid drop in steady rotation. We show that when vortices are nucleated inside the superfluid droplets, their morphology, which evolves from axisymmetric oblate to triaxial prolate to two-lobed shapes, is in good agreement with experiments. The presence of vortex arrays confers to the superfluid droplets the rigid-body behavior of a normal fluid in steady rotation, and this is the ultimate reason of the surprising good agreement between recent experiments and the classical models used for their description.

cond-mat.mes-hall↗

arXiv2018

Out-of-equilibrium dynamics of repulsive Fermi gases in quasi-periodic potentials: a Density Functional Theory study

The dynamics of a one-dimensional two-component Fermi gas in the presence of a quasi-periodic optical lattice (OL) is investigated by means of a Density Functional Theory approach. Inspired by the protocol implemented in recent cold-atom experiments, designed to identify the many-body localization transition, we analyze the relaxation of an initially prepared imbalance between the occupation number of odd and of even sites. For quasi-disorder strength beyond the Anderson localization transition, the imbalance survives for long times, indicating the inability of the system to reach local equilibrium. The late time value diminishes for increasing interaction strength. Close to the critical quasi-disorder strength corresponding to the noninteracting (Anderson) transition, the interacting system displays an extremely slow relaxation dynamics, consistent with sub-diffusive behavior. The amplitude of the imbalance fluctuations around its running average is found to decrease with time, and such damping is more effective with increasing interaction strengths. While our study addresses the setup with two equally intense OLs, very similar effects due to interactions have been observed also in recent cold-atom experiments performed in the tight-binding regime, i.e. where one of the two OLs is very deep and the other is much weaker.

cond-mat.quant-gas↗

arXiv2018

First observation of bright solitons in bulk superfluid He-4

The existence of bright solitons in bulk superfluid He-4 is demonstrated by time-resolved shadowgraph i maging experiments and density functional theory (DFT) calculations. The initial liquid compression that leads to the creation of non-linear waves is produced by rapidly expanding plasma from laser ablation. Af ter the leading dissipative period, these waves transform into bright solitons, which exhibit three chara cteristic features: dispersionless propagation, negligible interaction in two-wave collision, and direct dependence between soliton amplitude and the propagation velocity. The experimental observations are supp orted by DFT calculations, which show rapid evolution of the initially compressed liquid into bright soli tons. At high amplitudes, solitons become unstable and break down into dispersive shock waves.

cond-mat.other↗

arXiv2017

Density Functional Theory of doped superfluid liquid helium and nanodroplets

During the last decade, density function theory (DFT) in its static and dynamic time dependent forms, has emerged as a powerful tool to describe the structure and dynamics of doped liquid helium and droplets. In this review, we summarize the activity carried out in this field within the DFT framework since the publication of the previous review article on this subject [M. Barranco et al., J. Low Temp. Phys. 142, 1 (2006)]. Furthermore, a comprehensive presentation of the actual implementations of helium DFT is given, which have not been discussed in the individual articles or are scattered in the existing literature. This is an Accepted Manuscript of an article published on August 2, 2017 by Taylor & Francis Group in Int. Rev. Phys. Chem. 36, 621 (2017), available online: http://dx.doi.org/10.1080/0144235X.2017.1351672

physics.chem-ph↗

arXiv2017

The onset of nanoscale dissipation in superfluid He-4 at zero temperature: the role of vortex shedding and cavitation

Two-dimensional flow past an infinitely long cylinder of nanoscopic radius in superfluid He-4 at zero temperature is studied by time-dependent density functional theory. The calculations reveal two distinct critical phenomena for the onset of dissipation: 1) vortex-antivortex pair shedding from the periphery of the moving cylinder and 2) appearance of cavitation in the wake, which possesses similar geometry as observed experimentally for fast moving micrometer-scale particles in superfluid He-4. Vortex pairs with the same circulation are occasionally emitted in the form of dimers, which constitute the building blocks for the Benard-von Karman vortex street structure observed in classical turbulent fluids and Bose-Einstein condensates. The cavitation induced dissipation mechanism should be common to all superfluids that are self-bound and have a finite surface tension, which include the recently discovered self-bound droplets in ultracold Bose gases.

cond-mat.mes-hall↗

arXiv2016

Superfluid behavior of quasi-1D p-H$_2$ inside carbon nanotube

We perform ab-initio Quantum Monte Carlo simulations of para-hydrogen (pH$_2$) at $T=0$ K confined in carbon nanotubes (CNT) of different radii. The radial density profiles show a strong layering of the pH$_2$ molecules which grow, with increasing number of molecules, in solid concentric cylindrical shells and eventually a central column. The central column can be considered an effective one-dimensional (1D) fluid whose properties are well captured by the Tomonaga-Luttinger liquid theory. The Luttinger parameter is explicitly computed and interestingly it shows a non-monotonic behavior with the linear density similar to what found for pure 1D $^3$He. Remarkably, for the central column in a (10,10) CNT, we found an ample linear density range in which the Luttinger liquid is (i) superfluid and (ii) stable against a weak disordered external potential, as the one expected inside realistic pores. This superfluid behavior could be experimentally revealed in bundles of carbon nanotubes, where deviations from classical inertial values associated with superfluid density could be measured via torsional oscillator techniques. In summary, our results suggest that pH$_2$ within carbon nanopores could be a practical realization of the long sought-after, elusive superfluid phase of parahydrogen.

cond-mat.other↗

arXiv2016

Kohn-Sham approach to Fermi gas superfluidity: the bilayer of fermionic polar molecules

By using a well established 'ab initio' theoretical approach developed in the past to quantitatively study the superconductivity of condensed matter systems, which is based on the Kohn-Sham Density Functional theory, I study the superfluid properties and the BCS-BEC crossover of two parallel bi-dimensional layers of fermionic dipolar molecules, where the pairing mechanism leading to superfluidity is provided by the inter-layer coupling between dipoles. The finite temperature superfluid properties of both the homogeneous system and one were the fermions in each layer are confined by a square optical lattice are studied at half filling conditions, and for different values of the strength of the confining optical potential. The T=0 results for the homogeneous system are found to be in excellent agreement with Diffusion Monte Carlo results. The superfluid transition temperature in the BCS region is found to increase, for a given inter-layer coupling, with the strength of the confining optical potential. A transition occurs at sufficiently small interlayer distances, where the fermions becomes localized within the optical lattice sites in a square geometry with an increased effective lattice constant, forming a system of localized composite bosons. This transition should be signalled by a sudden drop in the superfluid fraction of the system.

cond-mat.quant-gas↗

arXiv2015

Kohn-Sham theory of rotating dipolar Fermi gas in two dimensions

A two-dimensional dipolar Fermi gas in harmonic trap under rotation is studied by solving "ab initio" Kohn-Sham equations. The physical parameters used match those of ultracold gas of fermionic $^{23}Na^{40}K$ molecules, a prototype system of strongly interacting dipolar quantum matter, which has been created very recently. We find that, as the critical rotational frequency is approached and the system collapses into the lowest Landau level, an array of tightly packed quantum vortices develops, in spite of the non-superfluid character of the system. In this state the system looses axial symmetry, and the fermionic cloud boundaries assume an almost perfect square shape. At higher values of the filling factor the vortex lattice disappears, while the system still exhibits square-shaped boundaries. At lower values of the filling factor the fermions become instead localized in a "Wigner cluster" structure.

cond-mat.quant-gas↗

arXiv2015

Quenched dynamics of the momentum distribution of the unitary Bose gas

We study the quenched dynamics of the momentum distribution of a unitary Bose gas under isotropic harmonic confinement within a time-dependent density functional approach based on our recently calculated Monte Carlo (MC) bulk equation of state. In our calculations the inter-atomic s-wave scattering length of the trapped bosons is suddenly increased to a very large value and the real-time evolution of the system is studied. Prompted by the very recent experimental data of $^{85}$Rb atoms at unitarity [Nature Phys. 10, 116 (2014)] we focus on the momentum distribution as a function of time. Our results suggest that at low momenta, a quasi-stationary momentum distribution is reached after a long transient, contrary to what found experimentally for large momenta which equilibrate on a time scale shorter than the one for three body losses.

cond-mat.quant-gas↗

arXiv2015

Vortex arrays in nanoscopic superfluid helium droplets

We have studied the appearance of vortex arrays in a rotating helium-4 nanodroplet at zero temperature within density functional theory. Our results are compared with those for classical rotating fluid drops used to analyze the shape and vorticity in recent experiments [L.F. Gomez et al., Science 345, 906 (2014)], where vortices have been directly seen in superfluid droplets for the first time. In agreement with the experiments, we have found that the shape of the droplet changes from pseudo-spheroid, oblate-like for a small number of vortices to a peculiar "wheel-like" shape, delimited by nearly flat upper and lower surfaces, when the number of vortices is large. Also in agreement with the experiments, we have found that the droplet remains stable well above the stability limit predicted by classical theories.

cond-mat.mes-hall↗

arXiv2014

Vortex arrays in a rotating superfluid He-4 nanocylinder

Within Density Functional theory, we investigate stationary many-vortex structures in a rotating $^4$He nanocylinder at zero temperature. We compute the stability diagram and compare our results with the classical model of vortical lines in an inviscid and incompressible fluid. Scaling the results to millimeter-size buckets, they can be compared with experiments on vortex arrays conducted in the past. Motivated by recent experiments that have used atomic impurities as a means of visualizing vortices in superfluid $^4$He droplets, we have also considered the formation of chains of xenon atoms along a vortex line and the interaction between xenon atoms inside the same vortex and on different neighboring vortex lines.

cond-mat.mes-hall↗