arXiv subjects

Francesco Di Colandrea

Publications and source records attributed to Francesco Di Colandrea.

At least 19 recordsLinked to original sources

arXiv2026

Evidence for Counterfactual Violation of Local Conservation Laws in Quantum Events

Physical conservation laws, such as those of energy and momentum, are generally believed to hold exactly and locally in spacetime, including in quantum phenomena. Yet Aharonov, Popescu, and Rohrlich (APR) recently argued, on the basis of a thought experiment, that individual quantum events, unlike ensemble averages, may occasionally violate local conservation laws. Their argument relies on the wave phenomenon known as "superoscillations", which APR themselves discovered more than 30 years ago. Here we provide experimental evidence for such a violation. We extract photons from a small superoscillatory region near the core of an optical vortex and show that their mean transverse momentum is statistically incompatible with a general bound implied by local momentum conservation. The derivation of this bound requires only the theoretically well-supported assumption that the extraction mechanism does not alter the photons' mean transverse momentum. We also detect photons with high transverse momentum at a rate significantly exceeding that predicted by a model assuming local momentum conservation. Because this violation can be established only counterfactually and through postselection, it does not conflict with relativistic causality. Our results may represent the first example of a distinct form of quantum nonlocality that does not explicitly rely on entanglement.

quant-ph↗

arXiv2026

Single-acquisition tomography of photonic qubits with structured media

Quantum state tomography is an essential tool for characterizing quantum systems and underpins nearly every experimental realization of quantum technologies. Conventional tomography relies on performing a sequence of projective measurements on many identical copies of a quantum state, requiring the measurement apparatus to be reconfigured between successive acquisitions. As the Hilbert-space dimension increases, the number of required measurements grows rapidly; in practice, additional overcomplete measurements are often performed to improve robustness to experimental imperfections. Here, we introduce a tomography platform based on structured anisotropic media that performs informationally complete measurements of photonic polarization qubits within a single acquisition. The approach employs three liquid-crystal metasurfaces with spatially varying optic-axis orientations that transform the input polarization into a far-field distribution of discrete transverse-momentum modes. Each diffraction pattern uniquely determines the polarization state, enabling its reconstruction without sequential changes to the measurement apparatus. Unlike previous implementations, our scheme is intrinsically photon-number independent: the same optical device operates identically for arbitrary photon numbers, while the desired photon-number sector can be selected afterwards through post-selection of the corresponding $n$-fold coincidence events. We experimentally demonstrate single-frame quantum state tomography of both single- and two-photon polarization states, providing a simple and scalable route toward efficient quantum-state characterization.

quant-ph↗

arXiv2026

Universal free-space photonic circuits for polarized structured light

Traditional linear-optical schemes for implementing discrete unitary transformations rely on multi-channel interferometers, typically composed of regular meshes of beam splitters and phase shifters. These architectures are well-suited to integrated photonics, where scalability and miniaturization are central requirements. In free space, universal transformations of optical modes have often been pursued through propagation in structured or inverse-designed optical systems, offering advantages in terms of addressable optical modes, reconfigurability, and flexible detection schemes. Here, we present a complementary approach: a collinear free-space photonic circuit that implements the standard interferometric paradigm in a Hilbert space of polarized structured-light modes. The circuit exploits spin-orbit coupling between circular polarization and optical modes carrying quantized transverse momentum, so that conventional beam splitters and phase shifters are replaced by structured optical materials acting directly on selected spin-orbit modes. In our demonstration, liquid-crystal metasurfaces serve as mode beam splitters and phase shifters, and we experimentally realize representative gates in a four-mode space. We further show how the architecture generalizes to larger numbers of modes, providing a scalable route to arbitrary unitary transformations in free space. Numerical optimization over random target unitaries supports the universality of the proposed scheme. These results establish a framework for universal free-space photonic circuits encoded in structured light and structured matter.

physics.optics↗

arXiv2026

Tunable Quantum Interference in Free Space with a Liquid-Crystal Metagrating

Structured optical materials provide a promising platform for photonic quantum information processing in free space. Beam splitters, a fundamental building block of photonic circuits, have recently been demonstrated in free space using geometric-phase optical elements. These devices coherently mix circularly-polarized transverse modes of freely-propagating optical fields, including modes carrying orbital angular momentum. In this work, we investigate liquid-crystal metagratings as electrically tunable beam splitters for transverse-momentum optical modes. By exploiting the voltage-controlled birefringence of liquid-crystal metasurfaces, we experimentally tune the splitting ratio of the device and thereby control the degree of two-photon interference between indistinguishable photons. At the output, photons are spatially resolved on different regions of a time-resolved single-photon-sensitive detector, enabling the reconstruction of coincidence maps in the Fourier plane. This approach is readily scalable and enables highly parallel coincidence measurements across a large number of optical modes.

physics.optics↗

arXiv2025

Tomographic characterization of non-Hermitian Hamiltonians in reciprocal space

Non-Hermitian Hamiltonians enrich quantum physics by extending conventional phase diagrams, enabling novel topological phenomena, and realizing exceptional points with potential applications in quantum sensing. Here, we present an experimental photonic platform capable of simulating a non-unitary quantum walk generated by a peculiar type of non-Hermitian Hamiltonian, largely unexplored in the literature. The novelty of this platform lies in its direct access to the reciprocal space, which enables us to scan the quasi-momentum across the entire Brillouin zone and thus achieve a precise tomographic reconstruction of the underlying non-Hermitian Hamiltonian, indicated by the comparison between theoretical predictions and experimental measurements. From the inferred Hamiltonian, it is possible to retrieve complex-valued band structures, resolve exceptional points in momentum space, and detect the associated parity-time symmetry breaking through eigenvector coalescence. Our results, presented entirely in quasi-momentum space, represent a substantial shift in perspective in the study of non-Hermitian phenomena.

quant-ph↗

arXiv2025

Skyrmionic polarization textures in structured dielectric planar media

Skyrmionic patterns of optical fields have recently emerged across diverse photonic platforms. Here, we show that such textures also arise in the polarization eigenstates of light propagation through flat dielectric devices with an engineered, space-dependent optic-axis orientation. We focus on two-dimensional periodic structures, where propagation through multiple devices maps onto quantum dynamics on a synthetic optical lattice. Adopting the condensed-matter framework, a spatial period defines an effective Brillouin zone, and polarization eigenstates can be grouped in two bands, with the role of energy played by the opposite phase delay. When such eigenstates exhibit skyrmionic textures, the corresponding lattice model shows the topology of a Chern insulator. These structures result from the interaction between the optical field and the medium and do not reflect a topological structure of the medium itself. We validate these concepts in a system of three tunable liquid-crystal metasurfaces. Using quantum process tomography based on supervised machine learning, we reconstruct the polarization eigenmodes over one spatial period. We identify configurations of the devices' parameters that lead to topologically non-trivial bands, where we directly observe skyrmionic eigenpolarization textures. Along the analogy with condensed matter, we also extract local observables of lattice models, such as the Berry curvature and the quantum metric. We finally report a numerical simulation of an all-optical quantum Hall effect emerging when light propagates through a sequence of such devices, arranged so as to mimic the effect of an external force on the lattice.

physics.optics↗

arXiv2025

Compact and programmable large-scale optical processor in free space

Photonic circuits are central to classical and quantum information processing. While integrated technologies dominate, free-space architectures are emerging as attractive alternatives, offering broad bandwidth and direct manipulation of optical modes without confinement in waveguides. A key challenge for scalability lies in circuit depth, as the number of layers manipulating the optical field typically grows with the system size. Here, we introduce a programmable free-space photonic platform that performs high-dimensional unitary transformations using only three layers. Information is encoded in structured light modes defined by circular polarization and quantized transverse momenta, and processed with spatial light modulators interleaved with half-wave plates. We implement unitaries that are equivalent to quantum walks over up to 30 time steps, in one- and two-dimensional lattices, distributing a single input mode across more than 7,000 outputs, where conventional approaches would require tens or hundreds of layers. Despite being restricted to translationally-invariant systems, the platform supports diverse quantum walk dynamics, including disorder, synthetic gauge fields, and topological effects, previously explored only in separate experiments. Using coincidence detection with a time-tagging camera, we show compatibility with quantum optics protocols and provide examples of quantum walks of heralded single photons. These results contribute to establish free-space optical processors as promising resources for high-dimensional quantum simulation and scalable optical information processing.

physics.optics↗

arXiv2025

Nonlocal transfer of high-dimensional unitary operations

Highly correlated biphoton states are powerful resources in quantum optics, both for fundamental tests of the theory and practical applications. In particular, high-dimensional spatial correlation has been used in several quantum information processing and sensing tasks, for instance, in ghost imaging experiments along with several quantum key distribution protocols. Here, we introduce a technique that exploits spatial correlations, whereby one can nonlocally access the result of an arbitrary unitary operator on an arbitrary input state without the need to perform any operation themselves. The method is experimentally validated on a set of spatially periodic unitary operations in one-dimensional and two-dimensional spaces. Our findings pave the way for efficiently distributing quantum simulations and computations in future instances of quantum networks where users with limited resources can nonlocally access the results of complex unitary transformations via a centrally located quantum processor.

quant-ph↗

arXiv2025

Investigating the Performance of Adaptive Optics on Different Bases of Spatial Modes in Turbulent Channels

Quantum key distribution (QKD) allows secure key exchange based on the principles of quantum mechanics, with higher-dimensional photonic states offering enhanced channel capacity and resilience to noise. Free-space QKD is crucial for global networks where fibres are impractical, but atmospheric turbulence introduces severe states distortions, particularly for spatial modes. Adaptive optics (AO) provides a pathway to correct these errors, though its effectiveness depends on the encoding basis. Here, we experimentally evaluate a high-speed AO system for orbital angular momentum (OAM) modes, mutually unbiased bases (MUB), and symmetric, informationally complete, positive operator-valued measures (SIC-POVM) up to dimension $d=8$ in a turbulent free-space channel. While OAM states are strongly distorted, their cylindrical symmetry makes them optimally corrected by AO, yielding error rates below QKD security thresholds. MUB and SIC-POVM exhibit greater intrinsic robustness to turbulence but are less precisely corrected, though their performance remains within protocol tolerances. These results establish AO as a key enabler of secure, high-dimensional QKD and highlight the role of basis choice in optimizing resilience and correction.

quant-ph↗

arXiv2025

Programmable photonic quantum walks on lattices with cyclic, toroidal, and cylindrical topology

Photonic implementations of unitary processes on lattice structures, such as quantum walks, have been demonstrated across various architectures. However, few platforms offer the combined advantages of scalability, reconfigurability, and the ability to simulate dynamics on lattices with periodic boundary conditions, such as cyclic or toroidal geometries. Here, we employ a recently developed platform that enables the implementation of arbitrary translationally invariant unitary operations on one- and two-dimensional lattices, and demonstrate a natural mechanism for introducing periodic boundary conditions. Our approach leverages direct access to the reciprocal lattice, where discrete sampling of the unitary evolution effectively enforces the desired topology. We program our platform to realize quantum walks on 1D cyclic lattices and 2D lattices with cylindrical or toroidal topologies. The lattice size can be readily tuned by adjusting the sampling density in reciprocal space. By controlling reciprocal-space occupancy, we investigate the dynamics of localized states and wavepackets, observing refocusing behavior, breathing modes modulated by reciprocal-space discretizations, and wavepacket trajectories that reflect the underlying topology. We further demonstrate a form of dimensional reduction by mapping a 2D quantum walk on a cylinder to a 1D walk with a high-dimensional coin. These results establish a versatile platform for realizing a broad class of optical mode transformations within bounded Hilbert spaces.

quant-ph↗

arXiv2025

High-Dimensional Quantum Key Distribution with Qubit-like States

Quantum key distribution (QKD) protocols most often use two conjugate bases in order to verify the security of the quantum channel. In the majority of protocols, these bases are mutually unbiased to one another, which is to say they are formed from balanced superpositions of the entire set of states in the opposing basis. Here, we introduce a high-dimensional QKD protocol using qubit-like states, referred to as Fourier-qubits (or $\textit{F}$-qubits). In our scheme, each $\textit{F}$-qubit is a superposition of only two computational basis states with a relative phase that can take $d$ distinct values, where $d$ is the dimension of the computational basis. This non-mutually unbiased approach allows us to bound the information leaked to an eavesdropper, maintaining security in high-dimensional quantum systems despite the states' seemingly two-dimensional nature. By simplifying state preparation and measurement, our protocol offers a practical alternative for secure high-dimensional quantum communications. We experimentally demonstrate this protocol for a noisy high-dimensional QKD channel using the orbital angular momentum degree of freedom of light and discuss the potential benefits for encoding in other degrees of freedom.

quant-ph↗

arXiv2025

Programmable non-Hermitian photonic quantum walks via dichroic metasurfaces

The evolution of a closed quantum system is described by a unitary operator generated by a Hermitian Hamiltonian. However, when certain degrees of freedom are coupled to an environment, the relevant dynamics can be captured by non-unitary evolution operators, arising from non-Hermitian Hamiltonians. Here we introduce a photonic platform that implements non-unitary quantum walks, commonly used to emulate open-system dynamics, in the synthetic space of light transverse momentum. These walks are realized by propagating light through a series of dichroic liquid-crystal metasurfaces, that impart polarization-dependent momentum shifts. The non-unitary behavior stems from dichroic dye molecules with polarization-dependent absorption, whose orientation is coupled to that of the liquid crystals. We demonstrate multiple walks up to five time steps, with adjustable levels of dichroism set by the metasurface voltage, which is controlled remotely. This discrete-time process maps onto two-band tight-binding models with reciprocal yet non-Hermitian nearest-neighbor couplings, corresponding to a less-studied class of non-Hermitian systems. Our platform broadens the range of optical simulators for controlled investigations of non-Hermitian quantum dynamics.

quant-ph↗

arXiv2025

Large-scale free-space photonic circuits in two dimensions

Photonic circuits, engineered to couple optical modes according to a specific map, serve as processors for classical and quantum light. The number of components typically scales with that of processed modes, thus correlating system size, circuit complexity, and optical losses. Here we present a photonic-circuit technology implementing large-scale unitary maps in free space, coupling a single input to hundreds of output modes in a two-dimensional compact layout. The map corresponds to a quantum walk of structured photons, realized through light propagation in three liquid-crystal metasurfaces, having their optic axes artificially patterned. Theoretically, the walk length and the number of connected modes can be arbitrary, while keeping losses constant. The patterns can be designed to replicate multiple unitary maps. We also discuss limited reconfigurability by adjusting the overall birefringence and the relative displacement of the optical elements. These results lay the basis for the design of low-loss non-integrated photonic circuits, primarily for manipulating multi-photon states in quantum regimes.

physics.optics↗

arXiv2025

Electrically tunable liquid-crystal metasurfaces with patterned birefringence and dichroism

Light propagation through artificially patterned anisotropic materials, such as dielectric metasurfaces, enables precise control of the spatio-vectorial properties of optical fields using highly transparent, thin, and flat optical elements. Liquid-crystal cells are a common realization of such devices. Optical losses are typically assumed to be polarization-independent and are therefore often overlooked in modeling these systems. In this work, we introduce electrically tunable liquid-crystal metasurfaces with patterned birefringence and dichroism, achieved by incorporating dichroic dye molecules into the liquid-crystal mixture. These dye molecules align with the liquid crystal, effectively coupling birefringence and dichroism effects. The behavior of these metasurfaces is described using non-unitary Jones matrices, validated through polarimetric measurements. In the case of devices that are patterned to form polarization gratings, we also characterize the diffraction efficiency as a function of the dichroism and birefringence parameters, which can be tuned jointly by applying an electric field across the cell. This study not only introduces a new class of optical components but also deepens our understanding of light propagation through anisotropic materials, where dichroism can naturally arise from bulk material properties or from reflection and transmission laws at their interfaces.

physics.optics↗

arXiv2024

Generation of the Complete Bell Basis via Hong-Ou-Mandel Interference

Optical vector modes (VMs), characterized by spatially varying polarization distributions, have become essential tools across microscopy, metrology, optical trapping, nanophotonics, and optical communications. The Hong-Ou-Mandel (HOM) effect, a fundamental two-photon interference phenomenon in quantum optics, offers significant potential to extend the applications of VMs beyond the classical regime. Here, we demonstrate the simultaneous generation of all four Bell states by exploiting the HOM interference of VMs. The resulting Bell states exhibit spatially tailored distributions that are determined by the input modes. These results represent a significant step in manipulating HOM interference within structured photons, offering promising avenues for high-dimensional quantum information processing and in particular high-dimensional quantum communication, quantum sensing, and advanced photonic technologies reliant on tailored quantum states of light.

quant-ph↗

arXiv2024

Engineering qubit dynamics in open systems with photonic synthetic lattices

The evolution of a quantum system interacting with an environment can be described as a unitary process acting on both the system and the environment. In this framework, the system's evolution can be predicted by tracing out the environmental degrees of freedom. Here, we establish a precise mapping between the global unitary dynamics and the quantum operation involving the system, wherein the system is a single qubit, and the environment is modeled as a discrete lattice space. This approach enables the implementation of arbitrary noise operations on single-polarization qubits using a minimal set of three liquid-crystal metasurfaces, whose transverse distribution of the optic axes can be patterned to reproduce the target process. We experimentally validate this method by simulating common noise processes, such as phase errors and depolarization.

quant-ph↗

arXiv2024

Predicting atmospheric turbulence for secure quantum communications in free space

Atmospheric turbulence is the main barrier to large-scale free-space quantum communication networks. Aberrations distort optical information carriers, thus limiting or preventing the possibility of establishing a secure link between two parties. For this reason, forecasting the turbulence strength within an optical channel is highly desirable, as it allows for knowing the optimal timing to establish a secure link in advance. Here, we train a Recurrent Neural Network, TAROCCO, to predict the turbulence strength within a free-space channel. The training is based on weather and turbulence data collected over 9 months for a 5.4 km intra-city free-space link across the City of Ottawa. The implications of accurate predictions from our network are demonstrated in a simulated high-dimensional Quantum Key Distribution protocol based on orbital angular momentum states of light across different turbulence regimes. TAROCCO will be crucial in validating a free-space channel to optimally route the key exchange for secure communications in real experimental scenarios.

quant-ph↗

arXiv2024

Biphoton State Reconstruction via Phase Retrieval Methods

The complete measurement of the quantum state of two correlated photons requires reconstructing the amplitude and phase of the biphoton wavefunction. We show how, by means of spatially resolved single photon detection, one can infer the spatial structure of bi-photons generated by spontaneous parametric down conversion. In particular, a spatially resolved analysis of the second-order correlations allows us to isolate the moduli of the pump and phasematching contributions to the two-photon states. When carrying this analysis on different propagation planes, the free space propagation of pump and phasematching is observed. This result allows, in principle, to gain enough information to reconstruct also the phase of pump and phasematching, and thus the full biphoton wavefunction. We show this in different examples where the pump is shaped as a superposition of orbital angular momentum modes or as a smooth amplitude with a phase structure with no singularities. The corresponding phase structure is retrieved employing maximum likelihood or genetic algorithms. These findings have potential applications in fast, efficient quantum state characterisation that does not require any control over the source.

quant-ph↗