arXiv subjects

Francesco Graffitti

Publications and source records attributed to Francesco Graffitti.

At least 19 recordsLinked to original sources

arXiv2026

Optimised spectral purity of unfiltered photons via pump and nonlinearity shaping

Photonic quantum technologies rely on the efficient generation and interference of indistinguishable photons. Exceptional achievements in this respect have been obtained by domain engineering of quasi-phase-matched parametric down-conversion sources, demonstrating high two-photon interference visibility using only moderate bandpass spectral filtering. Here, we optimised the spectral purity and indistinguishability of photons from telecom-wavelength sources by combining Gaussian quasi-phase-matching with Gaussian pump spectral shaping. Without spectral filtering, we used time-of-flight spectrometry to estimate an upper bound spectral purity of 99.9272(6)%, and achieved visibilities of up to 98.5(8)% in two-photon interference experiments with independent sources.

quant-ph↗

arXiv2026

Twist-Engineered Nonlinearity in Two-Dimensional Crystals for Tailored Quantum Light

Van der Waals (vdW) materials enable nonlinear-optical engineering with unprecedented resolution: their strong second-order susceptibilities ($χ^{(2)}$) and twist-tunable interlayer symmetry allow the effective nonlinearity to be shaped continuously, rather than through binary $\pmχ^{(2)}$ domain inversion as in bulk ferroelectrics. Here, we show that twist-angle domain engineering exploits this continuous degree of freedom to reconstruct target longitudinal nonlinearity profiles with high fidelity. Using spontaneous parametric down-conversion (SPDC) as a benchmark, we demonstrate that twist-engineered vdW crystals yield significantly improved approximations of target phase-matching functions and correspondingly higher single-photon purities, particularly in compact devices where fabrication constraints limit conventional approaches. We further show that this framework remains effective in experimentally relevant vdW materials and demanding non-degenerate wavelength regimes involving mid-infrared photons. More broadly, the ability to continuously and locally program $χ^{(2)}$ establishes a general framework for tailoring a wide range of SPDC properties, including absolute brightness, joint spectral amplitude structure, signal-idler frequency separation, and temporal wavepacket shape beyond what is accessible in conventional nonlinear crystals. These results position vdW heterostructures as a powerful platform for engineered quantum light sources and open new opportunities for nonlinear-optical devices shaped with monolayer thickness scale.

physics.optics↗

arXiv2025

Decoy-state quantum key distribution over 227 km with a frequency-converted telecom single-photon source

We implement a decoy-state quantum key distribution scheme using a telecom C-band single-emitter source. The decoy states are created by varying the optical excitation of the quantum emitter to modulate the photon number distribution. We provide an analysis of our scheme based on existing security proofs, allowing the calculation of secret key rates including finite key effects. This enables us to demonstrate, with a realistic single-photon source, positive secret key rates using our scheme over 227 km of optical fiber, equivalent to a loss tolerance one order of magnitude greater than non-decoy schemes. This work broadens the scope of single-photon sources in future quantum networks by enabling long-distance QKD with realistic levels of single-photon purity.

quant-ph↗

arXiv2025

A Large-Scale Reconfigurable Multiplexed Quantum Photonic Network

Entanglement distribution in quantum networks will enable next-generation technologies for quantum-secured communications, distributed quantum computing and sensing. Future quantum networks will require dense connectivity, allowing multiple users to share entanglement in a reconfigurable and multiplexed manner, while long-distance connections are established through the teleportation of entanglement, or entanglement swapping. While several recent works have demonstrated fully connected, local multi-user networks based on multiplexing, extending this to a global network architecture of interconnected local networks remains an outstanding challenge. Here we demonstrate the next stage in the evolution of multiplexed quantum networks: a prototype global reconfigurable network where entanglement is routed and teleported in a flexible and multiplexed manner between two local multi-user networks composed of four users each. At the heart of our network is a programmable 8x8-dimensional multi-port circuit that harnesses the natural mode-mixing process inside a multi-mode fibre to implement on-demand high-dimensional operations on two independent photons carrying eight transverse-spatial modes. Our circuit design allows us to break away from the limited planar geometry and bypass the control and fabrication challenges of conventional integrated photonic platforms. Our demonstration showcases the potential of this architecture for enabling large-scale, global quantum networks that offer versatile connectivity while being fully compatible with an existing communications infrastructure.

quant-ph↗

arXiv2023

Conference key agreement in a quantum network

Quantum conference key agreement (QCKA) allows multiple users to establish a secure key from a shared multi-partite entangled state. In a quantum network, this protocol can be efficiently implemented using a single copy of a N-qubit Greenberger-Horne-Zeilinger (GHZ) state to distil a secure N-user conference key bit, whereas up to N-1 entanglement pairs are consumed in the traditional pair-wise protocol. We demonstrate the advantage provided by GHZ states in a testbed consisting of a photonic six-user quantum network, where four users can distil either a GHZ state or the required number of Bell pairs for QCKA using network routing techniques. In the asymptotic limit, we report a more than two-fold enhancement of the conference key rate when comparing the two protocols. We extrapolate our data set to show that the resource advantage for the GHZ protocol persists when taking into account finite-key effects.

quant-ph↗

arXiv2023

Engineering quantum states from a spatially structured quantum eraser

Quantum interference is a central resource in many quantum-enhanced tasks, from computation to communication protocols. While it usually occurs between identical input photons, quantum interference can be enabled by projecting the quantum state onto ambiguous properties that render the photons indistinguishable, a process known as a quantum erasing. Structured light, on the other hand, is another hallmark of photonics: it is achieved by manipulating the degrees of freedom of light at the most basic level and enables a multitude of applications in both classical and quantum regimes. By combining these ideas, here we design and experimentally demonstrate a simple and robust scheme that tailors quantum interference to engineer photonic states with spatially structured coalescence along the transverse profile, a type of quantum mode with no classical counterpart. To achieve this, we locally tune the distinguishability of a photon pair via spatial structuring of their polarisation, creating a structured quantum eraser. We believe these spatially-engineered multi-photon quantum states may be of significance in fields such as quantum metrology, microscopy, and communications.

quant-ph↗

arXiv2023

Hyper-entanglement between pulse modes and frequency bins

Hyper-entanglement between two or more photonic degrees of freedom (DOF) can enhance and enable new quantum protocols by allowing each DOF to perform the task it is optimally suited for. Here we demonstrate the generation of photon pairs hyper-entangled between pulse modes and frequency bins. The pulse modes are generated via parametric downconversion in a domain-engineered crystal and subsequently entangled to two frequency bins via a spectral mapping technique. The resulting hyper-entangled state is characterized and verified via measurement of its joint spectral intensity and non-classical two-photon interference patterns from which we infer its spectral phase. The protocol combines the robustness to loss, intrinsic high dimensionality and compatibility with standard fiber-optic networks of the energy-time DOF with the ability of hyper-entanglement to increase the capacity and efficiency of the quantum channel, already exploited in recent experimental applications in both quantum information and quantum computation.

quant-ph↗

arXiv2022

Single-emitter quantum key distribution over 175 km of fiber with optimised finite key rates

Quantum key distribution with solid-state single-photon emitters is gaining traction due to their rapidly improving performance and compatibility with future quantum network architectures. In this work, we perform fibre-based quantum key distribution with a quantum dot frequency-converted to telecom wavelength, achieving count rates of 1.6 MHz with $g^{\left(2\right)}\left(0\right) = 3.6 \%$. We demonstrate positive key rates up to 175 km in the asymptotic regime. We then show that the community standard analysis for non-decoy state QKD drastically overestimates the acquisition time required to generate secure finite keys. Our improved analysis using the multiplicative Chernoff bound reduces the required number of received signals by a factor of $10^8$ over existing work, with the finite key rate approaching the asymptotic limit at all achievable distances for acquisition times of one hour. Over a practical distance of 100 km we achieve a finite key rate of 13 kbps after one minute of integration time. This result represents major progress towards the feasibility of long-distance single-emitter QKD networks.

quant-ph↗

arXiv2022

Frequency-bin entanglement from domain-engineered down-conversion

Frequency encoding is quickly becoming an attractive prospect for quantum information protocols owing to larger Hilbert spaces and increased resilience to noise compared to other photonic degrees of freedom. To fully make use of frequency encoding as a practical paradigm for QIP, an efficient and simple source of frequency entanglement is required. Here we present a single-pass source of discrete frequency-bin entanglement which does not use filtering or a resonant cavity. We use a domain-engineered nonlinear crystal to generate an eight-mode frequency-bin entangled source at telecommunication wavelengths. Our approach leverages the high heralding efficient and simplicity associated with bulk crystal sources.

quant-ph↗

arXiv2021

Quantum communication complexity beyond Bell nonlocality

Efficient distributed computing offers a scalable strategy for solving resource-demanding tasks such as parallel computation and circuit optimisation. Crucially, the communication overhead introduced by the allotment process should be minimised -- a key motivation behind the communication complexity problem (CCP). Quantum resources are well-suited to this task, offering clear strategies that can outperform classical counterparts. Furthermore, the connection between quantum CCPs and nonlocality provides an information-theoretic insights into fundamental quantum mechanics. Here we connect quantum CCPs with a generalised nonlocality framework -- beyond the paradigmatic Bell's theorem -- by incorporating the underlying causal structure, which governs the distributed task, into a so-called nonlocal hidden variable model. We prove that a new class of communication complexity tasks can be associated to Bell-like inequalities, whose violation is both necessary and sufficient for a quantum gain. We experimentally implement a multipartite CCP akin to the guess-your-neighbour-input scenario, and demonstrate a quantum advantage when multipartite Greenberger-Horne-Zeilinger (GHZ) states are shared among three users.

quant-ph↗

arXiv2021

A Bright Source of Telecom Single Photons Based on Quantum Frequency Conversion

On-demand indistinguishable single photon sources are essential for quantum networking and communication. Semiconductor quantum dots are among the most promising candidates, but their typical emission wavelength renders them unsuitable for use in fibre networks. Here, we present quantum frequency conversion of near-infrared photons from a bright quantum dot to the telecommunication C-band, allowing integration with existing fibre architectures. We use a custom-built, tunable 2400 nm seed laser to convert single photons from 942 nm to 1550 nm in a difference frequency generation process. We achieve an end-to-end conversion efficiency of $\sim$35%, demonstrate count rates approaching 1 MHz at 1550 nm with $g^{\left(2\right)}\left(0\right) = 0.04$, and achieve Hong-Ou-Mandel visibilities of 60%. We expect this scheme to be preferable to quantum dot sources directly emitting at telecom wavelengths for fibre based quantum networking.

quant-ph↗

arXiv2021

Optimised Domain-engineered Crystals for Pure Telecom Photon Sources

The ideal photon-pair source for building up multi-qubit states needs to produce indistinguishable photons with high efficiency. Indistinguishability is crucial for minimising errors in two-photon interference, central to building larger states, while high heralding rates will be needed to overcome unfavourable loss scaling. Domain engineering in parametric down-conversion sources negates the need for lossy spectral filtering allowing one to satisfy these conditions inherently within the source design. Here, we present a telecom-wavelength parametric down-conversion photon source that operates on the achievable limit of domain engineering. We generate photons from independent sources which achieve two-photon interference visibilities of up to $98.6\pm1.1\%$ without narrow-band filtering. As a consequence, we reach net heralding efficiencies of up to $67.5\%$, which corresponds to collection efficiencies exceeding $90\%$.

quant-ph↗

arXiv2020

Hyperentanglement in structured quantum light

Entanglement in high-dimensional quantum systems, where one or more degrees of freedom of light are involved, offers increased information capacities and enables new quantum protocols. Here, we demonstrate a functional source of high-dimensional, noise-resilient hyperentangled states encoded in time-frequency and vector-vortex structured modes, which in turn carry single-particle entanglement between polarisation and orbital angular momentum. Pairing nonlinearity-engineered parametric downconversion in an interferometric scheme with spin-to-orbital-angular-momentum conversion, we generate highly entangled photon pairs at telecom wavelength that we characterise via two-photon interference and quantum state tomography, achieving near-unity visibilities and fidelities. While hyperentanglement has been demonstrated before in photonic qubits, this is the first instance of such a rich entanglement structure involving spectrally and spatially structured light, where three different forms of entanglement coexist in the same biphoton state.

quant-ph↗

arXiv2020

Reconfigurable single photon sources based on functional materials

The future of quantum photonic technology depends on the realization of efficient sources of single photons, the ideal carriers of quantum information. Parametric downconversion (PDC) is a promising route to create highly coherent, spectrally pure single photons for quantum photonics using versatile group-velocity matching (GVM) and tailored nonlinearities. However, the functionality to actively control the poling period of nonlinear crystals used in PDC is currently missing, yet would enable to dynamically modify the wavelength of single photons produced in the PDC process. Here a detailed GVM study is presented for functional PMN-0.38PT material which can be dynamically repolled at ambient conditions with fields as low as 0.4 kV/mm. Our study reveals phase-matching conditions for spectrally pure single photon creation at 5-6 microns. Further, a practical approach is proposed for on-flight wavelength switching of the created single photons. The reported reconfigurable functionality benefits a wide range of emerging quantum-enhanced applications in the mid-IR spectral region where the choice of single photon sources is currently limited.

physics.optics↗

arXiv2019

Assisted Macroscopic Quantumness

It is commonly expected that quantum theory is universal, in that it describes the world at all scales. Yet, quantum effects at the macroscopic scale continue to elude our experimental observation. This fact is commonly attributed to decoherence processes affecting systems of sufficiently large number of constituent subsystems leading to an effective macro-scale beyond which a quantum description of the whole system becomes superfluous. Here, we show both theoretically and experimentally that the existence of such a scale is unjustifiable from an information-theoretic perspective. We introduce a variant of the Wigner's friend experiment in which a multiparticle quantum system is observed by the friend. The friend undergoes rapid decoherence through her interactions with the environment. In the usual version of this thought experiment, decoherence removes the need for Wigner to treat her as a quantum system. However, for our variant we prove theoretically and observe experimentally that there exist partitions of the subsystems in which the friend is entangled with one of the particles in assistance with the other particle, as observed by Wigner. Importantly, we show that the friend is indispensable for the entanglement to be observed. Hence Wigner is compelled to treat the friend as part of a larger quantum system. By analyzing our scenario in the context of a quantum key distribution protocol, we show that a semi-classical description of the experiment is suboptimal for security analysis, highlighting the significance of the quantum description of the friend.

quant-ph↗

arXiv2019

Experimental test of local observer-independence

The scientific method relies on facts, established through repeated measurements and agreed upon universally, independently of who observed them. In quantum mechanics, the objectivity of observations is not so clear, most dramatically exposed in Eugene Wigner's eponymous thought experiment where two observers can experience seemingly different realities. The question whether these realities can be reconciled in an observer-independent way has long remained inaccessible to empirical investigation, until recent no-go-theorems constructed an extended Wigner's friend scenario with four observers that allows us to put it to the test. In a state-of-the-art 6-photon experiment, we realise this extended Wigner's friend scenario, experimentally violating the associated Bell-type inequality by 5 standard deviations. If one holds fast to the assumptions of locality and free-choice, this result implies that quantum theory should be interpreted in an observer-dependent way.

quant-ph↗

arXiv2019

Direct generation of tailored pulse-mode entanglement

Photonic quantum technology increasingly uses frequency encoding to enable higher quantum information density and noise resilience. Pulsed time-frequency modes (TFM) represent a unique class of spectrally encoded quantum states of light that enable a complete framework for quantum information processing. Here, we demonstrate a technique for direct generation of entangled TFM-encoded states in single-pass, tailored downconversion processes. We achieve unprecedented quality in state generation---high rates, heralding efficiency and state fidelity---as characterised via highly resolved time-of-flight fibre spectroscopy and two-photon interference. We employ this technique in a four-photon entanglement swapping scheme as a primitive for TFM-encoded quantum protocols.

quant-ph↗

arXiv2019

Measurement Device Independent Verification of Quantum Channels

The capability to reliably transmit and store quantum information is an essential building block for future quantum networks and processors. Gauging the ability of a communication link or quantum memory to preserve quantum correlations is therefore vital for their technological application. Here, we experimentally demonstrate a measurement-device-independent protocol for certifying that an unknown channel acts as an entanglement-preserving channel. Our results show that, even under realistic experimental conditions, including imperfect single-photon sources and the various kinds of noise---in the channel or in detection---where other verification means would fail or become inefficient, the present verification protocol is still capable of affirming the quantum behaviour in a faithful manner without requiring any trust on the measurement device.

quant-ph↗