arXiv subjects

Francesco Mattiotti

Publications and source records attributed to Francesco Mattiotti.

18 recordsLinked to original sources

arXiv2026

Enhanced localization length in a disordered one-dimensional band via cavity coupling to delocalized states

We investigate the localization properties of cavity-coupled electronic states in disordered systems, motivated by recent proposals of cavity-mediated hopping in quantum Hall systems. We first introduce a minimal two-band model in which localized states in a disordered one-dimensional band are coupled, through a homogeneous cavity mode, to an excited band of delocalized states. Combining perturbation theory with a transfer-matrix approach, we show that cavity-assisted hopping between localized states decays exponentially with distance, implying that the eigenstates remain localized even beyond the perturbative regime. Nevertheless, the corresponding localization length increases with the light-matter coupling strength and can extend over several lattice sites in the single-electron ultrastrong-coupling regime. We then study a disordered Landau band coupled to a cavity mode within the framework developed in Refs.[1,2]. We find that the effective cavity-mediated coupling between edge states also decays exponentially with distance, but with a localization length that can reach micrometer scales for experimentally realistic parameters. By analyzing the inverse participation ratio, we show that this enhanced coupling is predominantly mediated by the most extended states of the upper Landau band. Our results demonstrate that, while cavity-induced hopping in disordered quantum Hall systems remains exponentially localized, the associated localization length can become sufficiently large for the corresponding states to exhibit effectively delocalized behavior on mesoscopic length scales.

cond-mat.mes-hall↗

arXiv2026

Time complexity of a monitored quantum search with resetting

Searching a database is a central task in computer science and is paradigmatic of transport and optimization problems in physics. For an unstructured search, Grover's algorithm predicts a quadratic speedup, with the search time $τ(N)=Θ(\sqrt{N})$ and $N$ the database size. Numerical studies suggest that the time complexity can change in the presence of feedback, injecting information during the search. Here, we determine the time complexity of the quantum analog of a randomized algorithm, which implements feedback in a simple form. The search is a continuous-time quantum walk on a complete graph, where the target is continuously monitored by a detector. Additionally, the quantum state is reset if the detector does not click within a specified time interval. This yields a non-unitary, non-Markovian dynamics. We optimize the search time as a function of the hopping amplitude, detection rate, and resetting rate, and identify the conditions under which time complexity could outperform Grover's scaling. The overall search time does not violate Grover's optimality bound when including the time budget of the physical implementation of the measurement. For databases of finite sizes monitoring can warrant rapid convergence and provides a promising avenue for fault-tolerant quantum searches.

quant-ph↗

arXiv2025

Relation between structure and functionality in photosynthetic antenna complex of green sulfur bacteria: efficiency under natural sunlight pumping

Large-scale simulations of light-matter interaction in natural photosynthetic antenna complexes of the Chlorobium Tepidum green sulfur bacteria (GSB) containing more than one hundred thousand chlorophyll molecules, comparable with natural size, have been performed. Here we have modeled the entire process of the exciton energy transfer, from sunlight absorption to exciton trapping in the reaction centers (RCs) in presence of a thermal bath. The energy transfer has been analyzed using the radiative non-Hermitian Hamiltonian and solving the rate equations for the populations. Sunlight pumping has been modeled as black-body radiation with an attenuation factor that takes the Sun-Earth distance into account. Cylindrical structures typical of GSB antenna complexes, and the dimeric baseplate comparable to natural size have been considered. Our analysis shows that under natural sunlight, in photosynthetic antennae of GSB the number of excitations reaching the RC per unit time matches the RC closure rate and the internal efficiency shows values close to 80%. We also considered cylindrical structures where the orientation of the dipoles does not reflect the natural one. Specifically, we vary continuously the angle of the transition dipole with respect to the cylinder main axis, focusing on the case where all dipoles are parallel to the cylinder axis. We also consider the important case where the dipoles are randomly oriented. In all cases the light-harvesting efficiency is lower than in the natural structure, showing the high sensitivity of light harvesting to the specific orientation of the dipole moments. Our results allow for a better understanding of the relationship between structure and functionality in photosynthetic antennae of GSB and could drive the design of efficient light-harvesting devices.

cond-mat.mes-hall↗

arXiv2025

Scale-invariant phase transition of disordered bosons in one dimension

The disorder-induced quantum phase transition between superfluid and non-superfluid states of bosonic particles in one dimension is generally expected to be of the Berezinskii-Kosterlitz-Thouless (BKT) type. Here, we show that hard-core lattice bosons with integrable power-law hopping decaying with distance as $1/r^α$ - corresponding in spin language to a $XY$ model with power-law couplings - undergo a non-BKT continuous phase transition instead. We use exact quantum Monte-Carlo methods to determine the phase diagram for different values of the exponent $α$, focusing on the regime $α> 2$. We find that the scaling of the superfluid stiffness with the system size is scale-invariant at the transition point for any $α\leq 3$ - a behavior incompatible with the BKT scenario and typical of continuous phase transitions in higher dimension. By scaling analysis near the transition point, we find that our data are consistent with a correlation length exponent satisfying the Harris bound $ν\geq 2$ and demonstrate a new universal behavior of disordered bosons in one dimension. For $α>3$ our data are consistent with a BKT scenario where the liquid is pinned by infinitesimal disorder.

cond-mat.quant-gas↗

arXiv2024

Large scale simulations of photosynthetic antenna systems: interplay of cooperativity and disorder

Large scale simulations of light-matter interaction in natural photosynthetic antenna complexes containing more than one hundred thousands chlorophyll molecules, comparable with natural size, have been performed. Photosynthetic antenna complexes present in Green sulfur bacteria and Purple bacteria have been analyzed using a radiative non-Hermitian Hamiltonian, well known in the field of quantum optics, instead of the widely used dipole-dipole Frenkel Hamiltonian. This approach allows to study ensembles of emitters beyond the small volume limit (system size much smaller than the absorbed wavelength), where the Frenkel Hamiltonian fails. When analyzed on a large scale, such structures display superradiant states much brighter then their single components. An analysis of the robustness to static disorder and dynamical (thermal) noise, shows that exciton coherence in the whole photosynthetic complex is larger than the coherence found in its parts. This provides evidence that the photosynthetic complex as a whole has a predominant role in sustaining coherences in the system even at room temperature. Our results allow a better understanding of natural photosynthetic antennae and could drive experiments to verify how the response to the electromagnetic radiation depends on the size of the photosynthetic antenna.

cond-mat.mes-hall↗

arXiv2024

Multifractality in the interacting disordered Tavis-Cummings model

We analyze the spectral and transport properties of the interacting disordered Tavis-Cummings model at half excitation filling. We demonstrate that a Poissonian level statistics coexists with eigenfunctions that are multifractal (extended, but non-ergodic) in the Hilbert space, for all strengths of light-matter interactions. This is associated with a lack of thermalization for a local perturbation. We find that the bipartite entanglement entropy grows logarithmically with time, similarly to many-body localized systems, while the spin imbalance tends to zero for strong coupling, in analogy to ergodic phases. We show that these effects are due to the combination of finite interactions and integrability of the model. When a small integrability-breaking perturbation (nearest-neighbor hopping) is introduced, typical eigenfunctions become ergodic, seemingly turning the system into a near-perfect conductor, contrary to the single-excitation noninteracting case. We propose a realization of this model with cold atoms.

quant-ph↗

arXiv2023

Localization of light in three dimensions: a mobility edge in the imaginary axis in non-Hermitian Hamiltonians

Searching for Anderson localization of light in three dimensions has challenged experimental and theoretical research for the last decades. Here the problem is analyzed through large scale numerical simulations, using a radiative Hamiltonian i.e. a non-Hermitian long-range hopping Hamiltonian, well suited to model light-matter interaction in cold atomic clouds. Light interaction in atomic clouds is considered in presence of positional and diagonal disorder. Due to the interplay of disorder and cooperative effects (sub- and super-radiance) a novel type of localization transition is shown to emerge, differing in several aspects from standard localization transitions which occur along the real energy axis. The localization transition discussed here is characterized by a mobility edge along the imaginary energy axis of the eigenvalues which is mostly independent from the real energy value of the eigenmodes. Differently from usual mobility edges it separates extended states from hybrid localized states and it manifest itself in the large moments of the participation ratio of the eigenstates. Our prediction of a mobility edge in the imaginary axis, i.e. depending on the eigenmode lifetime, paves the way to achieve control both in the time and space domain of open quantum systems.

cond-mat.mes-hall↗

arXiv2023

Extraordinary electrical conductance through amorphous non-conducting polymers under vibrational strong coupling

Achieving electrical conductance in amorphous non-doped polymers is a challenging task. Here, we show that vibrational strong coupling of the aromatic C-H(D) out-of-plane bending modes of polystyrene, deuterated polystyrene, and poly (benzyl methacrylate) to the vacuum electromagnetic field of the cavity enhance the electrical conductivity by at least six orders of magnitude compared to the uncoupled polymers. The conductance is thermally activated at the onset of strong coupling. It becomes temperature and cavity path length independent at the highest coupling strengths, giving rise to the extraordinary electrical conductance in these polymers. The electrical characterizations are performed without external light excitation, demonstrating the role of quantum light in enhancing the long-range coherent transport even in amorphous non-conducting polymers.

cond-mat.mtrl-sci↗

arXiv2023

Anomalous diffusion in the Long-Range Haken-Strobl-Reineker model

We analyze the propagation of excitons in a $d$-dimensional lattice with power-law hopping $\propto 1/r^α$ in the presence of dephasing, described by a generalized Haken-Strobl-Reineker model. We show that in the strong dephasing (quantum Zeno) regime the dynamics is described by a classical master equation for an exclusion process with long jumps. In this limit, we analytically compute the spatial distribution, whose shape changes at a critical value of the decay exponent $α_{\rm cr} = (d+2)/2$. The exciton always diffuses anomalously: a superdiffusive motion is associated to a Lévy stable distribution with long-range algebraic tails for $α\leqα_{\rm cr}$, while for $α> α_{\rm cr}$ the distribution corresponds to a surprising mixed Gaussian profile with long-range algebraic tails, leading to the coexistence of short-range diffusion and long-range Lévy-flights. In the many-exciton case, we demonstrate that, starting from a domain-wall exciton profile, algebraic tails appear in the distributions for any $α$, which affects thermalization: the longer the hopping range, the faster equilibrium is reached. Our results are directly relevant to experiments with cold trapped ions, Rydberg atoms and supramolecular dye aggregates. They provide a way to realize an exclusion process with long jumps experimentally.

quant-ph↗

arXiv2023

Enhanced robustness and dimensional crossover of superradiance in cuboidal nanocrystal superlattices

Cooperative emission of coherent radiation from multiple emitters (known as superradiance) has been predicted and observed in various physical systems, most recently in CsPbBr$_3$ nanocrystal superlattices. Superradiant emission is coherent and occurs on timescales faster than the emission from isolated nanocrystals. Theory predicts cooperative emission being faster by a factor of up to the number of nanocrystals ($N$). However, superradiance is strongly suppressed due to the presence of energetic disorder, stemming from nanocrystal size variations and thermal decoherence. Here, we analyze superradiance from superlattices of different dimensionalities (one-, two- and three-dimensional) with variable nanocrystal aspect ratios. We predict as much as a 15-fold enhancement in robustness against realistic values of energetic disorder in three-dimensional (3D) superlattices composed of cuboid-shaped, as opposed to cube-shaped, nanocrystals. Superradiance from small $(N\lesssim 10^3)$ two-dimensional (2D) superlattices is up to ten times more robust to static disorder and up to twice as robust to thermal decoherence than 3D superlattices with the same $N$. As the number of $N$ increases, a crossover in the robustness of superradiance occurs from 2D to 3D superlattices. For large $N\ (> 10^3)$, the robustness in 3D superlattices increases with $N$, showing cooperative robustness to disorder. This opens the possibility of observing superradiance even at room temperature in large 3D superlattices, if nanocrystal size fluctuations can be kept small.

cond-mat.mes-hall↗

arXiv2022

Engineering random spin models with atoms in a high-finesse cavity

All-to-all interacting, disordered quantum many-body models have a wide range of applications across disciplines, from spin glasses in condensed-matter physics, over holographic duality in high-energy physics, to annealing algorithms in quantum computing. Typically, these models are abstractions that do not find unambiguous physical realisations in nature. Here, we realise an all-to-all interacting, disordered spin system by subjecting an atomic cloud in a cavity to a controllable light shift. Adjusting the detuning between atom resonance and cavity mode, we can tune between disordered versions of a central-mode model and a Lipkin-Meshkov-Glick model. By spectroscopically probing the low-energy excitations of the system, we explore the competition of interactions with disorder across a broad parameter range. We show how disorder in the central-mode model breaks the strong collective coupling, making the dark state manifold cross over to a random distribution of weakly-mixed light-matter, "grey", states. In the Lipkin-Meshkov-Glick model the ferromagnetic finite-size ground state evolves towards a paramagnet as disorder is increased. In that regime, semi-localised eigenstates emerge, as we observe by extracting bounds on the participation ratio. These results present significant steps towards freely programmable cavity-mediated interactions for the design of arbitrary spin Hamiltonians.

cond-mat.quant-gas↗

arXiv2022

Efficient light harvesting and photon sensing via engineered cooperative effects

Efficient devices for light harvesting and photon sensing are fundamental building blocks of basic energy science and many essential technologies. Recent efforts have turned to biomimicry to design the next generation of light-capturing devices, partially fueled by an appreciation of the fantastic efficiency of the initial stages of natural photosynthetic systems at capturing photons. In such systems extended excitonic states are thought to play a fundamental functional role, inducing cooperative coherent effects, such as superabsorption of light and supertransfer of photoexcitations. Inspired by this observation, we design an artificial light-harvesting and photodetection device that maximally harnesses cooperative effects to enhance efficiency. The design relies on separating absorption and transfer processes (energetically and spatially) in order to overcome the fundamental obstacle to exploiting cooperative effects to enhance light capture: the enhanced emission processes that accompany superabsorption. This engineered separation of processes greatly improves the efficiency and the scalability of the system.

physics.optics↗

arXiv2021

Bio-inspired natural sunlight-pumped lasers

Even though sunlight is by far the most abundant renewable energy source available to humanity, its dilute and variable nature has kept efficient ways to collect, store, and distribute this energy tantalisingly out of reach. Turning the incoherent energy supply provided by the Sun into a coherent laser beam would overcome several of the practical limitations inherent in using sunlight as a source of clean energy: laser beams travel nearly losslessly over large distances, and they are effective at driving chemical reactions which convert sunlight into chemical energy. Here we propose a bio-inspired blueprint for a novel type of laser with the aim of upgrading unconcentrated natural sunlight into a coherent laser beam. Our proposed design constitutes a novel and different path towards sunlight-pumped lasers. In order to achieve lasing with the extremely dilute power provided by natural sunlight, we here propose a laser medium comprised of molecular aggregates inspired by the architecture of natural photosynthetic complexes. Such complexes exhibit a very large internal efficiency in harvesting photons from a power source as dilute as natural sunlight. Specifically, we consider a hybrid structure, where photosynthetic complexes in purple bacteria (Rhodobacter sphaeroides) surround a suitably engineered molecular dimer composed of two strongly coupled chromophores. We show that if pumped by the surrounding photosynthetic complex, which efficiently collects and concentrates solar energy, the core dimer structure can reach population inversion, and reach the lasing threshold under natural sunlight. The design principles proposed here will also pave the way for developing other bio-inspired quantum devices.

quant-ph↗

arXiv2021

Disorder-Enhanced and Disorder-Independent Transport with Long-Range Hopping: Application to Molecular Chains in Optical Cavities

Overcoming the detrimental effect of disorder at the nanoscale is very hard since disorder induces localization and an exponential suppression of transport efficiency. Here we unveil novel and robust quantum transport regimes achievable in nanosystems by exploiting long-range hopping. We demonstrate that in a 1D disordered nanostructure in the presence of long-range hopping, transport efficiency, after decreasing exponentially with disorder at first, is then enhanced by disorder [disorder-enhanced transport (DET) regime] until, counterintuitively, it reaches a disorder-independent transport (DIT) regime, persisting over several orders of disorder magnitude in realistic systems. To enlighten the relevance of our results, we demonstrate that an ensemble of emitters in a cavity can be described by an effective long-range Hamiltonian. The specific case of a disordered molecular wire placed in an optical cavity is discussed, showing that the DIT and DET regimes can be reached with state-of-the-art experimental setups.

quant-ph↗

arXiv2019

Real and imaginary energy gaps: a comparison between single excitation Superradiance and Superconductivity and robustness to disorder

A comparison between the single particle spectrum of the discrete Bardeen-Cooper-Schrieffer (BCS) model, used for small superconducting grains, and the spectrum of a paradigmatic model of Single Excitation Superradiance (SES) is presented. They are both characterized by an equally spaced energy spectrum (Picket Fence) where all the levels are coupled between each other by a constant coupling which is real for the BCS model and purely imaginary for the SES model. While the former corresponds to the discrete BCS-model describing the coupling of Cooper pairs in momentum space and it induces a Superconductive regime, the latter describes the coupling of single particle energy levels to a common decay channel and it induces a Superradiant transition. We show that the transition to a Superradiant regime can be connected to the emergence of an imaginary energy gap, similarly to the transition to a Superconductive regime where a real energy gap emerges. Despite their different physical origin, it is possible to show that both the Superradiant and the Superconducting gaps have the same magnitude in the large gap limit. Nevertheless, some differences appear: while the critical coupling at which the Superradiant gap appears is independent of the system size $N$, for the Superconductivity gap it scales as $(\ln N)^{-1}$. The presence of a gap in the imaginary energy axis between the Superradiant and the Subradiant states shares many similarities with the "standard" gap on the real energy axis: the superradiant state is protected against disorder from the imaginary gap as well as the superconducting ground state is protected by the real energy gap. Moreover we connect the origin of the gapped phase to the long-range nature of the coupling between the energy levels.

cond-mat.supr-con↗

arXiv2018

Macroscopic coherence as an emergent property in molecular nanotubes

Nanotubular molecular self-aggregates are characterized by a high degree of symmetry and they are fundamental systems for light-harvesting and energy transport. While coherent effects are thought to be at the basis of their high efficiency, the relationship between structure, coherence and functionality is still an open problem. We analyze natural nanotubes present in Green Sulfur Bacteria. We show that they have the ability to support macroscopic coherent states, i.e. delocalized excitonic states coherently spread over many molecules, even at room temperature. Specifically, assuming a canonical thermal state, in natural structures we find a large thermal coherence length, of the order of 1000 molecules. By comparing natural structure with other mathematical models, we show that this macroscopic coherence cannot be explained either by the magnitude of the nearest-neighbour coupling between the molecules, which would induce a thermal coherence length of the order of 10 molecules, or by the presence of long-range interactions between the molecules. Indeed we prove that the existence of macroscopic coherent states is an emergent property of such structures due to the interplay between geometry and cooperativity (superradiance and super-transfer). In order to prove this, we give evidence that the lowest part of the spectrum of natural systems is determined by a cooperatively enhanced coupling (super-transfer) between the eigenstates of modular sub-units of the whole structure. Due to this enhanced coupling strength, the density of states is lowered close to the ground state, thus boosting the thermal coherence length.

cond-mat.mes-hall↗

arXiv2017

Temperature of a single chaotic eigenstate

The onset of thermalization in a closed finite system of randomly interacting bosons, at the level of a single eigenstate, is discussed. The main interest is in the emergence of the Bose-Einstein distribution of single-particle occupation numbers, establishing a global and local criterion for thermalization. We show how to define the temperature of a given eigenstate, provided that it has a chaotic structure in the basis defined by single-particle states. The analytical expression for the eigenstate temperature as a function of the inter-particle interaction and energy is complemented by numerical data.

quant-ph↗

arXiv2015

Non-Hermitian Hamiltonian approach to quantum transport in disordered networks with sinks: validity and effectiveness

We investigate the validity of the non-Hermitian Hamiltonian approach in describing quantum transport in disordered tight-binding networks connected to external environments, acting as sinks. Usually, non-Hermitian terms are added, on a phenomenological basis, to such networks to summarize the effects of the coupling to the sinks. Here we consider a paradigmatic model of open quantum network for which we derive a non-Hermitian effective model, discussing its limit of validity by a comparison with the analysis of the full Hermitian model. Specifically, we consider a ring of sites connected to a central one-dimensional lead. The lead acts as a sink which absorbs the excitation initially present in the ring. The coupling strength to the lead controls the opening of the ring system. This model has been widely discussed in literature in the context of light-harvesting systems. We analyze the effectiveness of the non-Hermitian description both in absence and in presence of static disorder on the ring. In both cases, the non-Hermitian model is valid when the energy range determined by the eigenvalues of the ring Hamiltonian is smaller than the energy band in the lead. Under such condition, we show that results about the interplay of opening and disorder, previously obtained within the non-Hermitian Hamiltonian approach, remain valid when the full Hermitian model in presence of disorder is considered. The results of our analysis can be extended to generic networks with sinks, leading to the conclusion that the non-Hermitian approach is valid when the energy dependence of the coupling to the external environments is sufficiently smooth in the energy range spanned by the eigenstates of the network.

cond-mat.mes-hall↗