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Francesco Piazza

Publications and source records attributed to Francesco Piazza.

At least 19 recordsLinked to original sources

Cavity-enhanced superconducting response in an underdoped cuprate

Superconductors carry electrical current without resistance when paired electrons condense into a coherent macroscopic quantum state. In underdoped cuprates, evidence suggests that pairing-related correlations and superconducting fluctuations can survive above the temperature at which global coherence is lost, pointing to phase fluctuations as a key limitation on superconductivity in this regime. Motivated by recent demonstrations of cavity-modified collective states in quantum materials, we investigate whether superconducting coherence can be stabilized by engineering the electromagnetic environment of the superconductor. We study an underdoped YBa$_2$Cu$_3$O$_{7-\delta}$ thin film in a tunable terahertz cavity formed with a semi-transparent gold mirror. From temperature-dependent terahertz transmission measurements, we find that the cavity enhances the superconducting response below the critical temperature, with an increase of the inferred superfluid weight. The effect becomes more pronounced at smaller cavity lengths and is accompanied by an upward shift of the superconducting onset temperature. Calculations based on a cavity-coupled model for phase-fluctuating superconductors capture these trends and support an interpretation in terms of cavity-enhanced phase stiffness. These results showcase the potential of cavity engineering for designing emergent functionalities in correlated systems.

cond-mat.supr-con

Physical Properties of Dextran Solutions as Model Crowding Media

The role of macromolecular crowding in living systems is widely appreciated, but artificial crowders used to model these effects in vitro are often inadequately characterized. In this work, we examine density, viscosity, polymer self-diffusion and water diffusion in crowded dextran systems. Dextran viscosity and self-diffusion follow size-dependent trends, collectively described by universal functions of the overlap concentration corresponding to a Flory exponent of 0.44, characteristic of branched polymers. Viscosity increases with concentration as a power law, with a crossover from dilute to semi-dilute behaviors. Dextran self-diffusion decays exponentially: this can be interpreted in light of Rosenfeld's excess entropy scaling hypothesis. Water self-diffusivity and specific volume decrease with concentration, but show no dependence on polymer size. We show how these results can be used to construct the true volume fraction of crowders, which takes into account bound water. Overall, our findings showcase the power of polymer physics concepts in macromolecular crowding studies in vitro.

cond-mat.soft

Non-thermal pairing glue of electrons in the steady state

The study of mechanisms for enhancing superconductivity has been a central topic in condensed matter physics due to the combination of fundamental and technological interests. One promising route is to exploit non-equilibrium effects in the steady state. Efforts in this direction have so far focused on enhancing the pairing mechanism known from thermal equilibrium through modified distributions for the electrons or the bosons mediating the electron-electron interaction. In this work, we identify an additional pairing mechanism that is active only outside thermal equilibrium. By generalizing Eliashberg theory to non-equilibrium steady states using the Keldysh formalism, we derive a set of Eliashberg equations that capture the effect of this genuinely non-thermal pairing glue even in the weak-coupling regime. We discuss two examples where this mechanism has a major impact. First, in a temperature-bias setup, we find that superconductivity is enhanced when the boson mediator is colder than the electrons. Second, we find that an incoherent drive of the boson mediator at energies much greater than the temperature pushes the system far from thermal equilibrium but leaves the critical coupling essentially unchanged, owing to a competition between electron heating and the enhancement of pairing by the non-thermal glue.

cond-mat.supr-con

Formation of Cavity-Polaritons via High-Order Van Hove Singularities

We consider polaritons formed by hybridizing particle-hole excitations of an insulating phase with a cavity photon at sub-gap frequencies, where absorption is suppressed. The strength of the hybridization is driven by the Van Hove singularity in the joint density of states (JDOS) at the band gap: the stronger the singularity, the more a photon is hybridized with the interband transitions. In order to increase the singularity and thus the polariton hybridization without absorption, we propose to engineer a non-parabolic momentum dispersion of the bands around the gap in order to implement a high-order Van Hove singularity (HOVHS) in the JDOS. Ultracold atoms in tunable optical lattices are an ideal platform to engineer two-dimensional gapped phases with non-trivial band dispersions at the gap. Moreover, the intrinsic non-interacting nature of polarized fermionic atoms prevents the emergence of sub-gap excitations, which are common in solid-state systems and could otherwise spoil the absence of absorption below the gap. Our findings identify band-engineering at the gap edge as a promising route for polariton control with applications in quantum-nonlinear optics.

cond-mat.quant-gas

Cavity-induced Eliashberg effect: superconductivity vs charge density wave

Recent experiments have shown that non-equilibrium effects can play a key role in cavity-based control of material phases, notably in systems with charge-density-wave order. Motivated by this, we extend the theory of the Eliashberg effect, originally developed for superconducting phases, to charge-density-wave phases. Starting from a minimal electronic model where superconductivity and charge-density-wave order are equivalent at equilibrium, we introduce coupling to cavity photons, which are in turn coupled to an environment at a temperature different from the one of the electronic environment. This drives the system into a non-thermal steady state, which breaks the equivalence between superconductivity and charge-density-wave order. In the superconducting case, we recover the known behavior: a shift from continuous to discontinuous phase transitions with bistability. In contrast, the charge-density-wave case displays richer behavior: tuning the cavity frequency induces both continuous and discontinuous transitions, two distinct ordered phases, and a bistable regime ending at a critical point. These findings demonstrate that the scope of cavity-based non-thermal control of quantum materials is broader than at thermal equilibrium, and strongly depends on the targeted phases.

cond-mat.str-el

Cavity-control of the Ginzburg-Landau stiffness in superconductors

Confining light around solids via cavities enhances the coupling between the electromagnetic fluctuations and the matter. We predict that in superconductors this cavity-enhanced coupling enables the control of the order-parameter stiffness, which governs key length scales such as the coherence length of Cooper pairs and the magnetic penetration depth. We explain this as a renormalization of the Cooper-pair kinetic mass caused by photon-mediated repulsive interactions between the electrons building the pair. This effect is generic for Bardeen-Cooper-Schriffer superconductors and is most pronounced in low-$T_c$ materials. The strength of this effect can be tuned via the length of the cavity and we estimate it to be sizable for cavities in the infrared range.

cond-mat.supr-con

The fate of the Fermi surface coupled to a single-wave-vector cavity mode

The electromagnetic field of standing-wave or ring cavities induces a spatially modulated, infinite-range interaction between atoms in an ultracold Fermi gas, with a single wavelength comparable to the Fermi length. This interaction has no analog in other systems of itinerant particles and has so far been studied only in the regime where it is attractive at zero distance. Here, we fully solve the problem of competing instabilities of the Fermi surface induced by single-wavelength interactions. We find that while the density-wave (superradiant) instability dominates on the attractive side, it is absent for repulsive interactions, where the competition is instead won by non-superradiant superfluid phases at low temperatures, with Fermion pairs forming at both vanishing and finite center-of-mass momentum. Moreover, even in the absence of such symmetry-breaking instabilities, we find the Fermi surface to be always nontrivially deformed from an isotropic shape. We estimate this full phenomenology to be within reach of dedicated state-of-the-art experimental setups.

cond-mat.quant-gas

Effective diffusion along the backbone of combs with finite-span 1D and 2D fingers

Diffusion in complex heterogeneous media such as biological tissues or porous materials typically involves constrained displacements in tortuous structures and {\em sticky} environments. Therefore, diffusing particles experience both entropic (excluded-volume) forces and the presence of complex energy landscapes. In this situation, one may describe transport through an effective diffusion coefficient. In this paper, we examine comb structures with finite-length 1D and finite-area 2D fingers, which act as purely diffusive traps. We find that there exists a critical width of 2D fingers above which the effective diffusion along the backbone is faster than for an equivalent arrangement of 1D fingers. Moreover, we show that the effective diffusion coefficient is described by a general analytical form for both 1D and 2D fingers, provided the correct scaling variable is identified as a function of the structural parameters. Interestingly, this formula corresponds to the well-known general situation of diffusion in a medium with fast reversible adsorption. Finally, we show that the same formula describes diffusion in the presence of dilute potential energy traps, e.g. through a landscape of square wells. While diffusion is ultimately always the results of microscopic interactions (with particles in the fluid, other solutes and the environment), effective representations are often of great practical use. The results reported in this paper help clarify the microscopic origins and the applicability of global, integrated descriptions of diffusion in complex media.

cond-mat.soft

Low energy excitations in bosonic quantum quasicrystals

We present the first principles construction of the low-energy effective action for bosonic self-organized quantum quasicrystals. Our generalized elasticity approach retains the appropriate number of phase- and corresponding conjugate density- degrees-of-freedom required for a proper description of the Goldstone modes. For the dodecagonal and decagonal quasicrystal structures we obtain collective longitudinal and transversal excitations with an isotropic speed of sound. Meanwhile, for the octagonal structure, the coupling between phononic and phasonic degrees of freedom leads in turn to hybridization of the latter with the condensate sound mode, producing collective excitations with a longitudinal and transversal component, and an anisotropic speed of sound. Finally, we discuss the fate of each excitation mode at the low and high density phase transitions limiting the quantum quasicrystal phase.

cond-mat.stat-mech

Laser-painted cavity-mediated interactions in a quantum gas

Experimental platforms based on ultracold atomic gases have significantly advanced the quantum simulation of complex systems, yet the exploration of phenomena driven by long-range interactions remains a formidable challenge. Currently available methods utilizing dipolar quantum gases or multi-mode cavities allow to implement long-range interactions with a $1/r^3$ character or with a spatial profile fixed by the mode-structure of the vacuum electromagnetic field surrounding the atoms, respectively. Here we propose an experimental scheme employing laser-painted cavity-mediated interactions, which enables the realization of atom-atom interactions that are fully tunable in range, shape, and sign. Our approach combines the versatility of cavity quantum electrodynamics with the precision of laser manipulation, thus providing a highly flexible platform for simulating and understanding long-range interactions in quantum many-body systems. Our analytical predictions are supported by numerical simulations describing the full dynamics of atoms, laser, and cavity. The latter demonstrate that there is a wide and experimentally accessible parameter regime where our protocol optimally works. The methodology not only paves the way for exploring new territories in quantum simulation but also enhances the understanding of fundamental physics, potentially leading to the discovery of novel quantum states and phases.

cond-mat.quant-gas

Nonthermal electron-photon steady states in open cavity quantum materials

Coupling a system to two different baths can lead to novel phenomena escaping the constraints of thermal equilibrium. In quantum materials inside optical cavities, this feature can be exploited as electrons and cavity-photons are easily pulled away from their mutual equilibrium, even in the steady state. This offers new routes for a non-invasive control of material properties and functionalities. We show that the absence of thermal equilibrium between electrons and photons leads to reduced symmetries of the steady-state electronic distribution function. Moreover, by defining an effective temperature from the on-shell distribution function, we find a non-monotonic behaviour as a function of cavity frequency, consistent with recent experimental findings. Finally, we show that, the non-thermal behaviour leads to qualitative modifications of the material's properties, as the standard Sommerfeld expansion for observables is modified by a leading-order correction linearly proportional to the temperature difference between the two baths and to the frequency-derivative of the electron damping.

cond-mat.str-el

Integrability, multifractality, and two-photon dynamics in disordered Tavis-Cummings models

The Tavis-Cummings model is a paradigmatic central-mode model where a set of two-level quantum emitters (spins) are coupled to a collective cavity mode. Here we study the eigenstate spectrum, its localization properties and the effect on dynamics, focusing on the two-excitation sector relevant for nonlinear photonics. These models admit two sources of disorder: in the coupling between the spins and the cavity and in the energy shifts of the individual spins. While this model was known to be exactly solvable in the limit of a homogeneous coupling and inhomogeneous energy shifts, we here establish the solvability in the opposite limit of a homogeneous energy shift and inhomogeneous coupling, presenting the exact solution and corresponding conserved quantities. We identify three different classes of eigenstates, exhibiting different degrees of multifractality and semilocalization closely tied to the integrable points, and study their stability to perturbations away from these solvable points. The dynamics of the cavity occupation number away from equilibrium, exhibiting boson bunching and a two-photon blockade, is explicitly related to the localization properties of the eigenstates and illustrates how these models support a collective spin description despite the presence of disorder.

cond-mat.dis-nn

The role of atomic interactions in cavity-induced continuous time crystals

We consider continuous time-crystalline phases in dissipative many-body systems of atoms in cavities, focusing on the role of short-range interatomic interactions. First, we show that the latter can alter the nature of the time crystal by changing the type of the underlying critical bifurcation. Second, we characterize the heating mechanism and dynamics resulting from the short-range interactions and demonstrate that they make the time crystal inherently metastable. We argue that this is generic for the broader class of dissipative time crystals in atom-cavity systems whenever the cavity loss rate is comparable to the atomic recoil energy. We observe that such a scenario for heating resembles the one proposed for preheating of the early universe, where the oscillating coherent inflation field decays into a cascade of exponentially growing fluctuations. By extending approaches for dissipative dynamical systems to our many-body problem, we obtain analytical predictions for the parameters describing the phase transition and the heating rate inside the time-crystalline phase. We underpin and extend the analytical predictions of the heating rates with numerical simulations.

cond-mat.quant-gas

The physics of boundary conditions in reaction-diffusion problems

The use of fully or partially absorbing boundary conditions for diffusion-based problems has become paradigmatic in physical chemistry and biochemistry to describe reactions occurring in solutions or in living media. However, as chemical states may indeed disappear, particles cannot, unless such degradation happens physically and should thus be accounted for explicitly. Here, we introduce a simple, yet general idea that allows one to derive the appropriate boundary conditions self-consistently from the chemical reaction scheme and the geometry of the physical reaction boundaries. As an illustration, we consider two paradigmatic examples, where the known results are recovered by taking specific physical limits. More generally, we demonstrate that our mathematical analysis delivers physical insight that cannot be accessed through standard treatments.

cond-mat.stat-mech

Non-Fermi-Liquid Behavior from Cavity Electromagnetic Vacuum Fluctuations at the Superradiant Transition

We study two-dimensional materials where electrons are coupled to the vacuum electromagnetic field of a cavity. We show that, at the onset of the superradiant phase transition towards a macroscopic photon occupation of the cavity, the critical electromagnetic fluctuations, consisting of photons strongly overdamped by their interaction with electrons, can in turn lead to the absence of electronic quasiparticles. Since transverse photons couple to the electronic current, the appearance of non-Fermi-Liquid behavior strongly depends on the lattice. In particular, we find that in a square lattice the phase space for electron-photon scattering is reduced in such a way to preserve the quasiparticles, while in a honeycomb lattice the latter are removed due to a non-analytical frequency dependence of the damping $\propto |\omega|^{2/3}$. Standard cavity probes could allow to measure the characteristic frequency spectrum of the overdamped critical electromagnetic modes responsible for the non-Fermi-liquid behavior.

cond-mat.str-el

Controlling Collective Phenomena Via the Quantum State of Interaction-Mediators: Changing the Criticality of Photon-Mediated Superconductivity Via Fock States of Light

How are two-body scattering and the resulting collective phenomena affected by preparing the mediator of interactions in different quantum states? This question has recently become experimentally relevant in a specific non-relativistic version of QED implemented within materials, where standard techniques of quantum optics are available for the preparation of desired quantum states of the photon mediating interactions between matter's constituents. We develop the necessary non-equilibrium approach for computing the vertex function and find that, in addition to the energy and momentum structure of the scattering, a further structure emerges which reflects the Hilbert-space distribution of the mediator's quantum state. This emergent structure becomes non-trivial for non-Gaussian quantum states of the mediator, and can dramatically affect scattering and collective phenomena. As a first application, we show that by preparing photons in pure Fock states one can enhance pair correlations, and even modify the criticality of the superconducting phase transition. Our results also reveal that the thermal mixture of Fock states regularises the strong pair correlations present in each of its components, yielding the standard Bardeen-Cooper-Schrieffer criticality. Besides the above QED platform, ultracold atomic mixtures are among the most promising candidates for the experimental implementation of these ideas.

quant-ph

Decoherence and momentum relaxation in Fermi-polaron Rabi dynamics: a kinetic equation approach

Despite the paradigmatic nature of the Fermi-polaron model, the theoretical description of its nonlinear dynamics poses challenges. Here, we apply a quantum kinetic theory of driven polarons to recent experiments with ultracold atoms, where Rabi oscillations between a Fermi-polaron state and a non-interacting level were reported. The resulting equations separate decoherence from momentum relaxation, with the corresponding rates showing a different dependence on microscopic scattering processes and quasi-particle properties. We describe both the polaron ground state and the excited repulsive-polaron state and we find a good quantitative agreement between our predictions and the available experimental data without any fitting parameter. Our approach not only takes into account collisional phenomena, but also it can be used to study the different roles played by decoherence and the collisional integral in the strongly interacting highly-imbalanced mixture of Fermi gases.

cond-mat.quant-gas

Fermi polaron laser in two-dimensional semiconductors

We study the relaxation dynamics of driven, two-dimensional semiconductors, where itinerant electrons dress optically pumped excitons to form two Fermi-polaron branches. Repulsive polarons excited around zero momentum quickly decay to the attractive branch at high momentum. Collisions with electrons subsequently lead to a slower relaxation of attractive polarons, which accumulate at the edge of the light-cone around zero momentum where the radiative loss dominates. The bosonic nature of exciton polarons enables stimulated scattering, which results in a lasing transition at higher pump power. The latter is characterized by a superlinear increase of light emission as well as extended spatiotemporal coherence. As the coherent peak is at the edge of the light-cone and not at the center, the many-body dressing of excitons can reduce the linewidth below the limit set by the exciton nonradiative lifetime.

cond-mat.mes-hall