arXiv subjects

Francisco J. García-Vidal

Publications and source records attributed to Francisco J. García-Vidal.

At least 19 recordsLinked to original sources

arXiv2026

Fluctuational Quantum Electrodynamics of Dispersive Time-Varying Media

We present the theoretical framework of fluctuational quantum electrodynamics in frequency-dispersive and dissipative time-varying media. Our theory accounts for dispersion and losses in the temporal modulation, which is treated in an exact manner, without relying on perturbative methods. Thus, our work constitutes the first consistent quantization of the electromagnetic field in time-modulated material bodies. We derive a Fermi Golden Rule for time-varying media and use it to define the local density of states for these time-dependent systems, which includes both loss and gain contributions. Additionally, we prove the equivalence between the quantum Fermi Golden Rule and the power emitted by a classical harmonic point dipole. Moreover, we show that neglecting the dispersive and dissipative nature of the time modulation leads to erroneous predictions for both slow and fast modulations. Furthermore, we analyze the thermal radiation emitted by a time-varying material body, revealing new features in the enhancement of thermal emission in time-varying media. Finally, we study the dynamical Casimir effect, showing how the time modulation amplifies vacuum fluctuations and generates entangled pairs of polaritons exhibiting non-local spatial correlations.

physics.optics↗

arXiv2026

Close encounters between periodic light and periodic arrays of quantum emitters

We introduce crystal polaritons, hybrid excitations formed when the collective excitations of a periodic quantum-emitter array strongly couple to the resonant Bloch modes of a metasurface. This realizes a cavity-QED platform in which periodic light and periodic matter are treated on the same footing, allowing strong collective light-matter coupling in an extended, lossy, and dispersive nanophotonic structure. To describe this regime, we develop a reciprocal-space few-mode quantization based on macroscopic quantum electrodynamics, which maps the metasurface resonances seen by the emitter array onto a cavity-QED Hamiltonian at each in-plane momentum. We show that both plasmonic surface-lattice resonances and dielectric bound states in the continuum can enter the strong-coupling regime with a single emitter per unit cell. As a consequence of the resonant nonlinearities of the resulting crystal polaritons, the platform enables quantum light generation with efficiencies orders of magnitude higher than those achieved in conventional nonlinear metasurfaces.

quant-ph↗

arXiv2026

Broadband Dipole Absorption in Dispersive Photonic Time Crystals

Photonic media modulated periodically in time, termed photonic time crystals (PTCs), have attracted considerable attention for their ability to open momentum bandgaps hosting amplifying modes. These momentum gaps, however, generally appear only at the system's parametric resonance condition which constrain many features derived from amplification to a narrow frequency band. Moreover, they are accompanied by exceptional points (EPs) and may drive the system into an instability, which render their analysis more intricate. Here, we show that a careful consideration of dispersion and absorption can overcome these issues. By investigating the dissipated power of a point-dipole embedded in a dispersive and absorptive PTC, we unveil that temporal modulation enables the conversion of dipole emission into dipole absorption within a broadband frequency window free of EPs. We demonstrate that this effect is general, emerging in both the stable and unstable regimes, and occurs from weak modulation strength to low modulations frequencies that could be achieved for various material platforms.

physics.optics↗

arXiv2025

Casimir-Lifshitz Theory for Cavity Modification of Ground-State Energy

A theory for ground-state modifications of matter embedded in a Fabry-Perot cavity and whose excitations are described as harmonic oscillators is presented. Based on Lifshitz's theory for vacuum energy and employing a Lorentz model for the material permittivity, a nonperturbative macroscopic QED model that accounts for the infinite number of cavity modes with a continuum of their wavevectors was built. Differences from the commonly used single-mode Hopfield Hamiltonian are revealed. The nonresonant role of polaritons in the ground-state energy shift is also demonstrated, showing that the cavity effect is mainly caused by static screening occurring at very low frequencies. The theory allows for a straightforward incorporation of losses and temperature effects.

quant-ph↗

arXiv2025

Magnetic order tuning of excitons in the magnetic semiconductor CrCl$_3$ through strain

Magnon-exciton coupling provides an unprecedented opportunity for the optical tunability of spin information and, viceversa, for the magnetic control of the optical response. Few-layered magnets are an ideal platform for the experimental study of this coupling, in part due to the strong excitonic character of the optical response in (quasi-)two dimensions. Here, we demonstrate a strong dependence of the excitonic oscillator strength on the magnetic order in a monolayer of chromium trichloride CrCl$_3$. Solving an effective Bethe-Salpeter equation, we evaluate the changes in the excitonic response as the magnetic order switches from the ferromagnetic state to the antiferromagnetic state when strain is applied. Our results reveal an abrupt change in the spatial localization of the excitons across the transition, which translates into a strong shift and a change of the oscillator strength of the excitonic peaks. This suggests the possibility of using strain as a binary switch of the optical response in this material.

cond-mat.mtrl-sci↗

arXiv2025

Near-Field Gain and Far-Field Control via a Plasmonic Time Crystal Slab

Light matter interactions can be substantially altered in the presence of time varying media. We study the interaction between a harmonic electric dipole and a plasmonic time crystal slab. Temporal modulation of the plasma frequency enables near field gain, allowing the dipole to absorb rather than emit energy, suppressing nonradiative losses. At the parametric resonance condition, the slab radiates strongly to the far field, producing hundred per cent oscillations in the radiated power at distances up to a thousand times the epsilon near zero wavelength. These findings reveal a new mechanism for controlling light matter interaction in time varying plasmonic systems

physics.optics↗

arXiv2025

Directional Flow of Confined Polaritons in CrSBr

Nanoscale control of energy transport is a central challenge in modern photonics. Utilization of exciton-polaritons hybrid light-matter quasiparticles is one viable approach, but it typically demands complex device engineering to enable directional transport. Here, we demonstrate that the van der Waals magnet CrSBr offers an inherent avenue for steering polariton transport leveraging a unique combination of intrinsic optical anisotropy, high refractive index, and excitons dressed by photons. This combination enables low-loss guided modes that propagate tens of microns along the crystal $a$-axis, while simultaneously inducing strong one-dimensional confinement along the orthogonal $b$-axis. By embedding CrSBr flakes in a microcavity, we further enhance the confinement, as evidenced by energy modes that are discretized along the $b$-axis but continuous along the $a$-axis. Moreover, the magneto-exciton coupling characteristic of CrSBr allows unprecedented control over both unidirectional propagation and confinement. Our results establish CrSBr as a versatile polaritonic platform for integrated optoelectronic device applications, including energy-efficient optical modulators and switches.

physics.optics↗

arXiv2025

Squeezing and quantum control of antiferromagnetic magnon pseudospin

Antiferromagnets have been shown to harbor strong magnon squeezing in equilibrium, making them a potential resource for quantum correlations and entanglement. Recent experiments have also found them to host coherently coupled magnonic excitations forming a magnon pseudospin, in analogy to electronic spin. Here, we delineate the quantum properties of antiferromagnetic magnon pseudospin by accounting for spin non-conserving interactions and going beyond the rotating wave approximation. Employing concrete examples of nickel oxide and hematite, we find strong squeezing of the magnon pseudospin highlighting its important role in determining the eigenmode quantum properties. Via ground state quantum fluctuations engineering, this pseudospin squeezing enables an enhancement and control of coupling between the magnonic modes and other excitations. Finally, we evaluate the quantum superpositions that comprise a squeezed pseudospin ground state and delineate a qubit spectroscopy protocol to detect them. Our results are applicable to any system of coupled bosons and thus introduce quantum fluctuations engineering of a general bosonic pseudospin.

cond-mat.mtrl-sci↗

arXiv2025

Generation and optimization of entanglement between atoms chirally coupled to spin cavities

We explore the generation and optimization of entanglement between atoms chirally coupled to finite 1D spin chains, functioning as {\it spin cavities}. By diagonalizing the spin cavity Hamiltonian, we identify a parity effect that influences entanglement, with small even-sized cavities chirally coupled to atoms expediting entanglement generation by approximately $50\%$ faster than non-chiral coupling. Applying a classical driving field to the atoms reveals oscillations in concurrence, with resonant dips at specific driving strengths due to the resonances between the driven atom and the spin cavity. Extending our study to systems with energetic disorder, we find that high concurrence can be achieved regardless of disorder strength when the inverse participation ratio of the resulting eigenstates is favorable. Finally, we demonstrate that controlled disorder within the cavity significantly enhances and expedites entanglement generation, achieving higher concurrences up to four times faster than those attained in ordered systems.

quant-ph↗

arXiv2024

Spatially resolved photon statistics of general nanophotonic systems

While experimental measurements of photon correlations have become routine in laboratories, theoretical access to these quantities for the light generated in complex nanophotonic devices remains a major challenge. Current methods are limited to specific simplified cases and lack generality. Here we present a novel method that provides access to photon statistics resolved in space and frequency in arbitrary electromagnetic environments. Within the macroscopic QED framework, we develop a practical tool to compute electric field correlations for complex quantum systems by including lossy two-level systems that act as field detectors within the system. To make the implementation feasible, we use a recently developed multi-emitter few-mode quantization method to correctly account for fully retarded light propagation to the detectors. We demonstrate the effectiveness and robustness of the proposed technique by studying the photon correlations of one and two emitters in close proximity to a plasmonic nanoparticle. The simulations show that even in these relatively simple configurations, the light statistics exhibit a strong angular dependence. These results highlight the importance of going beyond conventional quantum-optical approaches to fully capture the analyzed physical effects and enable the study of the quantum light generation in realistic nanophotonic devices.

quant-ph↗

arXiv2024

General theory of cavity-mediated interactions between low-energy matter excitations

The manipulation of low-energy matter properties such as superconductivity, ferromagnetism and ferroelectricity via cavity quantum electrodynamics engineering has been suggested as a way to enhance these many-body collective phenomena. In this work, we investigate the effective interactions between low-energy matter excitations induced by the off-resonant coupling with cavity electromagnetic modes. We extend previous work by going beyond the dipole approximation accounting for the full polarization and magnetization densities of matter. We further include the often neglected diamagnetic interaction and, for the cavity, we consider general linear absorbing media with possibly non-local and non-reciprocal response. We demonstrate that, even in this general scenario, the effective cavity-induced interactions between the matter degrees of freedom are of electrostatic and magnetostatic nature. This confirms the necessity of a multimode description for cavity engineering of matter systems where the low-energy assumption holds. Our findings provide a theoretical framework for studying the influence of general optical environments on extended low-energy matter excitations.

quant-ph↗

arXiv2024

Magneto-optics in a van der Waals magnet tuned by self-hybridized polaritons

Controlling quantum materials with light is of fundamental and technological importance. By utilizing the strong coupling of light and matter in optical cavities (1-3), recent studies were able to modify some of their most defining features (4-6). In this work, we study the magneto-optical properties of a van der Waals magnet that supports strong coupling of photons and excitons even in the absence of external cavity mirrors. In this material - the layered magnetic semiconductor CrSBr - emergent light-matter hybrids called polaritons are shown to significantly increase the spectral bandwidth of correlations between the magnetic, electronic, and optical properties, enabling largely tunable optical responses to applied magnetic fields and magnons. Our results highlight the importance of exciton-photon self-hybridization in van der Waals magnets and motivate novel directions for the manipulation of quantum material properties by strong light-matter coupling.

cond-mat.mes-hall↗

arXiv2024

Unconventional magnetism mediated by spin-phonon-photon coupling

Magnetic order typically emerges due to the short-range exchange interaction between the constituent electronic spins. Recent discoveries have found a crucial role for spin-phonon coupling in various phenomena from optical ultrafast magnetization switching to dynamical control of the magnetic state. Here, we demonstrate theoretically the emergence of a biquadratic long-range interaction between spins mediated by their coupling to phonons hybridized with vacuum photons into polaritons. The resulting ordered state enabled by the exchange of virtual polaritons between spins is reminiscent of superconductivity mediated by the exchange of virtual phonons. The biquadratic nature of the spin-spin interaction promotes ordering without favoring ferro- or antiferromagnetism. It further makes the phase transition to magnetic order a first-order transition, unlike in conventional magnets. Consequently, a large magnetization develops abruptly on lowering the temperature which \aknew{could} enable magnetic memories admitting ultralow-power thermally-assisted writing while maintaining a high data stability. The role of photons in the phenomenon further enables an in-situ static control over the magnetism. These unique features make our predicted spin-spin interaction and magnetism highly unconventional paving the way for novel scientific and technological opportunities.

cond-mat.mes-hall↗

arXiv2024

Photon Squeezing in Photonic Time Crystals

Time-varying media offer a platform to realize novel and exotic wave effects, including photonic time crystals characterized by momentum band gaps with exponential wave amplification. Here we focus on the quantum electrodynamical properties of time-varying media, in particular vacuum amplification and squeezing. For that purpose, we present a theory of photon pair generation in photonic time crystals that unveils the link between the classical and quantum electrodynamical properties of these systems, that is, a direct relation between reflectivity and pair generation through the squeezing parameter. By working within an Hermitian framework, we are able to characterize quantum pair generation processes in photonic time crystals, showing how momentum bandgaps result in a non-resonant exponential enhancement of dynamical Casimir processes.

physics.optics↗

arXiv2024

A mixed perturbative-nonperturbative treatment for strong light-matter interactions

The full information about the interaction between a quantum emitter and an arbitrary electromagnetic environment is encoded in the so-called spectral density. We present an approach for describing such interaction in any coupling regime, providing a Lindblad-like master equation for the emitter dynamics when coupled to a general nanophotonic structure. Our framework is based on the splitting of the spectral density into two terms. On the one hand, a spectral density responsible for the non-Markovian and strong-coupling-based dynamics of the quantum emitter. On the other hand, a residual spectral density including the remaining weak-coupling terms. The former is treated nonperturbatively with a collection of lossy interacting discrete modes whose parameters are determined by a fit to the original spectral density in a frequency region encompassing the quantum emitter transition frequencies. The latter is treated perturbatively under a Markovian approximation. We illustrate the power and validity of our approach through numerical simulations in three different setups, thus offering a variety of scenarios for a full test, including the ultra-strong coupling regime.

quant-ph↗

arXiv2023

Electrostatic nature of cavity-mediated interactions between low-energy matter excitations

The use of cavity quantum electrodynamical effects, i.e., of vacuum electromagnetic fields, to modify material properties in cavities has rapidly gained popularity and interest in the last few years. However, there is still a scarcity of general results that provide guidelines for intuitive understanding and limitations of what kind of effects can be achieved. We provide such a result for the effective interactions between low-energy matter excitations induced either directly by their mutual coupling to the cavity electromagnetic (EM) field or indirectly through coupling to mediator modes that couple to the EM field. We demonstrate that the induced interactions are purely electrostatic in nature and are thus fully described by the EM Green's function evaluated at zero frequency. Our findings imply that reduced models with one or a few cavity modes can easily give misleading results.

quant-ph↗

arXiv2023

A Lindblad master equation capable of describing hybrid quantum systems in the ultra-strong coupling regime

Despite significant theoretical efforts devoted to studying the interaction between quantized light modes and matter, the so-called ultra-strong coupling regime still presents significant challenges for theoretical treatments and prevents the use of many common approximations. Here we demonstrate an approach that can describe the dynamics of hybrid quantum systems in any regime of interaction for an arbitrary electromagnetic (EM) environment. We extend a previous method developed for few-mode quantization of arbitrary systems to the case of ultrastrong light-matter coupling, and show that even such systems can be treated using a Lindblad master equation where decay operators act only on the photonic modes by ensuring that the effective spectral density of the EM environment is sufficiently suppressed at negative frequencies. We demonstrate the validity of our framework and show that it outperforms current state-of-the-art master equations for a simple model system, and then study a realistic nanoplasmonic setup where existing approaches cannot be applied.

quant-ph↗

arXiv2022

A theoretical perspective on molecular polaritonics

In the last decade, much theoretical research has focused on studying the strong coupling between organic molecules (or quantum emitters, in general) and light modes. The description and prediction of polaritonic phenomena emerging in this light-matter interaction regime have proven to be difficult tasks. The challenge originates from the enormous number of degrees of freedom that need to be taken into account, both in the organic molecules and in their photonic environment. On the one hand, the accurate treatment of the vibrational spectrum of the former is key, and simplified quantum models are not valid in many cases. On the other hand, most photonic setups have complex geometric and material characteristics, with the result that photon fields corresponding to more than just a single electromagnetic mode contribute to the light-matter interaction in these platforms. Moreover, loss and dissipation, in the form of absorption or radiation, must also be included in the theoretical description of polaritons. Here, we review and offer our own perspective on some of the work recently done in the modelling of interacting molecular and optical states with increasing complexity.

quant-ph↗