arXiv subjects

Frank Setzpfandt

Publications and source records attributed to Frank Setzpfandt.

At least 19 recordsLinked to original sources

arXiv2026

Quantum scanning synthetic optical holography

Synthetic optical holography (SOH) introduced holographic reconstruction into scanning optical microscopy, enabling quantitative phase imaging with sequential acquisition and point detection. Here, we extend this concept to the quantum regime by implementing SOH within quantum imaging with undetected light (QIUL). By integrating a controlled synthetic phase carrier into a scanning QIUL implementation, we retrieve amplitude and phase images of objects probed by mid-infrared (MIR) photons while detecting only their visible partners. We demonstrate the method on binary, transparent, and biological samples, showing complex-field reconstruction in a scanning quantum imaging system. This approach decouples spatial resolution from photon-pair spatial correlations and establishes a route toward diffraction-limited, label-free MIR phase imaging with visible-wavelength detection.

physics.optics↗

arXiv2026

Generation of Tunable Entanglement from Thin-Film Lithium Niobate

Entangled photon pairs play a major role in various modern technologies such as quantum imaging, communication, and computing. Conventional photon-pair sources are often based on spontaneous parametric down-conversion in bulk nonlinear crystals. Recent advances have also shown entangled photon-pairs from transition metal dichalcogenide thin-films, however, these materials are not widely available and are not compatible with existing fabrication capabilities. We present a new thin-film lithium niobate source of polarization-entangled photon pairs at the telecom wavelength that requires no additional optical elements for entanglement generation and allows for easy application using the existing lithium niobate fabrication technologies. We demonstrate tunable entanglement generation using the three-fold rotational crystal symmetry of lithium niobate, allowing the generation of different maximally entangled Bell states or completely separable states depending on the polarization of the pump beam.

quant-ph↗

arXiv2026

Quadratic Quantum Polarimetry with Entangled Photon Pairs

Conventional polarimetry, including schemes leveraging entangled light, characterizes optical samples through linear transformations of polarization states. We introduce a two-photon probing approach in which both photons of an entangled pair interact with the same depolarizing medium simultaneously. In this regime, the transformation of the two-photon polarization correlations becomes quadratic in the Mueller matrix, enabling access to second-order polarization information beyond conventional polarimetry. We develop a theoretical framework linking the Mueller matrix to the evolution of the two-photon polarization correlation tensor and show that depolarization induces quadratic degradation of entanglement and state purity. Experiments using polarization-entangled photon pairs transmitted through controlled scattering media confirm the predicted response and reveal enhanced sensitivity to polarization scrambling compared with single-photon probing. These results establish two-photon probing as a higher-order quantum polarimetric modality for characterizing polarization channels.

quant-ph↗

arXiv2026

Toward Spectral Engineering of Squeezed Light in High-Gain PDC

We investigated the spectral properties of squeezed light generated via parametric down-conversion in the high-gain regime, considering both unapodized and apodized dispersion-engineered waveguides. The gain-dependent evolution of these states is examined starting from the low-gain regime, which includes both highly correlated and nearly uncorrelated cases. For the unapodized configuration, we observe a monotonic increase in spectral purity with gain, whereas the apodized configuration exhibits a nonmonotonic dependence, initially decreasing and then recovering at higher gain. By combining Schmidt-mode analysis with a group-velocity-based interpretation, we explain why different dispersion conditions exhibit distinct gain-dependent behavior, specifically that rapid purification occurs when the pump group velocity lies between those of the signal and idler. Our study shows that the evolution of spectral purity is governed primarily by the underlying dispersion of the waveguide. These results demonstrate that dispersion engineering and parametric gain can be jointly exploited to tailor the spectral-mode structure of squeezed-light sources, enabling their optimization for a broad range of quantum applications.

quant-ph↗

arXiv2025

Noise resilient real-time phase imaging via undetected light

Quantum imaging with undetected light has recently emerged as a technique in which quantum correlations and nonlinear interferometry are combined to decouple illumination and detection paths. This approach has been more recently extended and combined with digital phase-shifting holography and off-axis holography to extract both the amplitude and phase information of a sample relying on single-photon interference. Despite these advantages, implementing the technique in real-world scenarios where the observed system is subject to environmental noise and dynamic variations remains challenging. The primary limitation lies in the inability of quantum imaging systems to retrieve object information in real time under high-noise conditions. Here, we experimentally demonstrate real-time amplitude and phase imaging in noisy environments, building upon our previous implementation of quantum off-axis holography. Our results demonstrate real-time imaging at acquisition rates up to 4~Hz, even when the noise level exceeds the signal by an order of magnitude.

physics.optics↗

arXiv2025

Quantum Phase Gradient Imaging Using a Nonlocal Metasurface System

Quantum phase imaging enables the analysis of transparent samples with thickness and refractive index variations in scenarios requiring precise measurements under low-light conditions. Here, we present a compact quantum phase-gradient imaging system integrating a lithium niobate (LiNbO3) metasurface for generating spatially entangled photon pairs and a silicon (Si) metasurface for phase gradient extraction. By leveraging nonlocal resonances, the LiNbO3 metasurface enables efficient spontaneous parametric down-conversion (SPDC) with all-optically angularly tunable emission, while the Si metasurface provides a nearly linear optical transfer function (OTF) that differentiates the photon wavefunction and extracts phase gradients.Experimental proof-of-concept results demonstrate the imaging of up to 25~rad/mm phase gradients, achieving 89% similarity with the reference values. The pixel resolution of the system can be potentially enhanced by orders of magnitude by increasing the metasurface dimensions and resonance quality factor.Our work showcases the application of metasurfaces in both generating and detecting quantum states and establishes a new paradigm for portable quantum phase-gradient imaging, with potential applications in quantum sensing, microscopy, and LiDAR technology.

physics.optics↗

arXiv2025

Enhanced photon-pair generation from a van der Waals metasurface

Quantum photon pairs play a pivotal role in many quantum applications. Metasurfaces, two-dimensional arrays of nanostructures, have been studied intensively to enhance and control pair generation via spontaneous parametric downconversion (SPDC). Van der Waals (VdW) layered materials have emerged as promising candidates for nonlinear materials in quantum light sources, owing to their high nonlinear susceptibility and compatibility with on-chip integration. In this work, we present the first demonstration of SPDC from a metasurface composed of the VdW material 3R-MoS2. The nanoresonators support quasi-bound states in the continuum (qBIC) with a quality factor of up to 120, enhancing light-matter interactions. This design achieves a 20-fold increase in SPDC rate compared to an unstructured film and significantly higher brightness, resulting in enhanced quantum photon-pair generation. This work establishes a new approach for utilizing van der Waals metasurfaces in the generation of quantum photon pairs, opening avenues for advanced quantum applications.

physics.optics↗

arXiv2025

Mid-infrared quantum scanning microscopy via visible light beyond spatial correlations

The mid-infrared (MIR) region of the electromagnetic spectrum spans from 2- to 25-$\mu \mathrm{m}$, serving as a valuable tool for accessing rich chemical information. Functional groups, lipids, and other complex molecules can be analyzed by optical absorption measurements due to their vibrational modes in the MIR spectral region. Over the past few decades, this field has faced challenges due to difficulties in generating MIR light and the limited maturity of detection systems in this spectral range. Quantum imaging with undetected light (QIUL) provides a spectrally tuneable photon-pair source, in which the sample can be illuminated with MIR light while visible (VIS) light is employed for detection and image reconstruction, overcoming the detection limitations and benefiting from the rich chemical information of the MIR spectral region. All previous QIUL implementations are based on spatial correlations, which are never perfect and thus hindered the imaging performance. In this work, we implement a raster-scanning QIUL method that is independent of the strength of the spatial correlations and achieves a spatial resolution beyond the limitations of these correlations.

physics.optics↗

arXiv2025

Broadband bright biphotons from periodically poled triple-resonance metasurface

Biphotons from spontaneous parametric down conversion with broad bandwidth are highly wanted in many quantum technologies. However, achieving broad bandwidth in both frequency and momentum while keeping a high rate remains a challenge for both conventional nonlinear crystals and recently emerging nonlinear metasurfaces. Here, we address this challenge by introducing a periodically poled triple-resonance metasurface (PPTM) incorporating a nano-grating atop a periodically poled LiNbO$_3$ thin film. PPTM supports high-Q guided mode resonances at pump, signal, and idler wavelengths meanwhile enabling quasi-phase matching between three guided modes in a broad frequency/momentum range. The predicted biphoton rate is over 100 MHz/mW with a frequency bandwidth of 165 nm around 1550 nm and a momentum bandwidth of $13^\circ \times 6^\circ$, improving the state-of-the-art by over three orders of magnitude in rate and one order of magnitude in bandwidths. This ultrathin broadband bright biphoton source could stimulate system-level miniaturization of various free-space quantum photonic technologies.

physics.optics↗

arXiv2024

Bridging classical and quantum approaches in optical polarimetry: Predicting polarization-entangled photon behavior in scattering environments

We explore quantum-based optical polarimetry as a potential diagnostic tool for biological tissues by developing a theoretical and experimental framework to understand polarization-entangled photon behavior in scattering media. We investigate the mathematical relationship between Wolf's coherency matrix in classical optics and the density matrix formalism of quantum mechanics which allows for the extension of classical Monte Carlo method to quantum states. The developed generalized Monte Carlo approach uniquely integrates the Bethe-Salpeter equation for classical scattering, the Jones vector formalism for polarization, and the density matrix approach for quantum state representation. Therefore, this unified framework can model both classical and quantum polarization states, handle multi-photon states, and account for varying degrees of entanglement. Additionally, it facilitates the prediction of quantum state evolution in scattering media based on classical optical principles. The validity of the computational model is experimentally confirmed through high-fidelity agreement between predicted and measured quantum state evolution in tissue-mimicking phantoms. This work bridges the gap between classical and quantum optical polarimetry by developing and validating a comprehensive theoretical framework that unifies these traditionally distinct domains, paving the way for future quantum-enhanced diagnostics of tissues and other turbid environments.

physics.optics↗

arXiv2024

Generation of tunable quantum entanglement via nonlinearity symmetry breaking in semiconductor metasurfaces

Tunable biphoton quantum entanglement generated from nonlinear processes is highly desirable for cutting-edge quantum technologies, yet its tunability is substantially constrained by the symmetry of material nonlinear tensors. Here, we overcome this constraint by introducing symmetry-breaking in nonlinear polarization to generate optically tunable biphoton entanglement at picosecond speeds. Asymmetric optical responses have made breakthroughs in classical applications like non-reciprocal light transmission. We now experimentally demonstrate the nonlinear asymmetry response for biphoton entanglement using a semiconductor metasurface incorporating [110] InGaP nano-resonators with structural asymmetry. We realize continuous tuning of polarization entanglement from near-unentangled states to a Bell state. This tunability can also extend to produce tailored hyperentanglement. Furthermore, our nanoscale entanglement source features an ultra-high coincidence-to-accidental ratio of $\approx7\times10^4$, outperforming existing semiconductor flat optics by two orders of magnitude. Introducing asymmetric nonlinear response in quantum metasurfaces opens new directions for tailoring on-demand quantum states and beyond.

physics.optics↗

arXiv2024

Fabrication of low-loss lithium niobate on insulator waveguides on the wafer scale

We report on the wafer scale fabrication of single mode low-loss lithium niobate on insulator waveguides utilizing a chemically amplified resist and an optimized dry etching method. The fabricated single mode waveguides are free of residuals and re-deposition, with measured losses for straight waveguides around 2 dB/m (0.02 dB/cm). We present on a method offering advantages for large-scale production due to its cost-effectiveness, faster writing time, and simplified processes. This work holds promise for advancing integrated photonics and optical communication technologies.

physics.optics↗

arXiv2024

Entangled Photon-pair Generation in Nonlinear Thin-films

We develop a fully vectorial and non-paraxial formalism to describe spontaneous parametric down-conversion in nonlinear thin films. The formalism is capable of treating slabs with a sub-wavelength thickness, describe the associated Fabry-Pérot effects, and even treat absorptive nonlinear materials. With this formalism, we perform an in-depth study of the dynamics of entangled photon-pair generation in nonlinear thin films, to provide a needed theoretical understanding for such systems that have recently attracted much experimental attention as sources of photon pairs. As an important example, we study the far-field radiation properties of photon pairs generated from a high-refractive-index nonlinear thin-film with Zinc-Blende structure, that is deposited on a linear low-refractive-index substrate. In particular, we study the thickness-dependent effect of Fabry-Pérot interferences on the far-field radiation pattern of the photon pairs. We also pay special attention to study of entanglement generation, and find the conditions under which maximally polarization-entangled photon pairs can be generated and detected in such nonlinear thin-films.

quant-ph↗

arXiv2024

Enhancing entangled two-photon absorption of Nile Red via temperature-controlled SPDC

Entangled two-photon absorption can enable a linear scaling of fluorescence emission with the excitation power. In comparison to classical two-photon absorption with a quadratic scaling, this can allow fluorescence imaging or photolithography with high axial resolution at minimal exposure intensities. However, most experimental studies on two-photon absorption were not able to show an unambiguous proof of fluorescence emission driven by entangled photon pairs. On the other hand, existing theoretical models struggle to accurately predict the entangled two-photon absorption behavior of chemically complex dyes. In this paper, we introduce an approach to simulate entangled two-photon absorption in common fluorescence dyes considering their chemical properties. Our theoretical model allows a deeper understanding of experimental results and thus the occurrence of entangled two-photon absorption. In particular, we found a remarkable dependency of the absorption probability on the phase-matching temperature of the nonlinear material. Further, we compared results of our theoretical approach to experimental data for Nile Red.

quant-ph↗

arXiv2024

Off-axis holographic imaging with undetected light

Quantum imaging with undetected light (QIUL) can retrieve amplitude and phase information of an object by exploiting the quantum correlations of photon-pairs generated through spontaneous parametric down conversion (SPDC), where the illumination and detection can be carried at very distinct wavelength ranges. This fact allows to benefit from a mature detection technology in the visible spectral range, while probing the object at a more exotic wavelength. Here we experimentally implement a QIUL approach with Fourier off-axis holography in a hybrid-type induced-coherence non-linear interferometer. Our approach reconstructs the amplitude and phase information of an object with a single shot in a wide-field configuration, being an alternative in front of techniques that require multiple acquisition frames, such as phase-shifting holography.

physics.optics↗

arXiv2024

A hybrid source of quantum light for generation of frequency tunable Fock states

We propose a scheme for quantum-light generation in a nonlinear cavity hybridized with a 2-level system and theoretically show that, when excited by a series of controlled pump pulses, the hybrid source generates Fock states with high probabilities. E.g., 1- and 2-photon states can be generated near-on-demand, and Fock states with up to $7$ photons with a probability above $50\%$. The tailorable nature of the nonlinear cavity allows for generating Fock states with arbitrary frequencies, even with a fixed 2-level system, creating fundamentally new opportunities in all areas of quantum technologies.

quant-ph↗

arXiv2024

Robust Classical and Quantum Polarimetry with a Single Nanostructured Metagrating

We formulate a new conceptual approach for one-shot complete polarization state measurement with nanostructured metasurfaces applicable to classical light and multi-photon quantum states, by drawing on the principles of generalized quantum measurements based on positive operator-valued measures (POVMs). Accurate polarization reconstruction from a combination of photon counts or correlations from several diffraction orders is robust with respect to even strong fabrication inaccuracies, requiring only a single classical calibration of metasurface transmission. Furthermore, this approach operates with a single metagrating without interleaving, allowing for the metasurface size reduction while preserving the high transmission efficiency and output beam quality. We theoretically obtained original metasurface designs, fabricated the metasurface from amorphous silicon nanostructures deposited on glass, and experimentally confirmed accurate polarization reconstruction for laser beams. We also anticipate robust operation under changes in environmental conditions, opening new possibilities for space-based imaging and satellite optics.

physics.optics↗

arXiv2024

Nonlinear Nanoresonators for Bell State Generation

Entangled photon states are a fundamental resource for optical quantum technologies and investigating the fundamental predictions of quantum mechanics. Up to now such states are mainly generated in macroscopic nonlinear optical systems with elaborately tailored optical properties. In this theoretical work, we extend the understanding on the generation of entangled photonic states towards the nanoscale regime, by investigating the fundamental properties of photon-pair-generation in sub-wavelength nonlinear nanoresonators. Taking materials with Zinc-Blende structure as example, we reveal that such systems can naturally generate various polarization-entangled Bell states over a very broad range of wavelengths and emission directions, with little to no engineering needed. Interestingly, we uncover different regimes of operation, where polarization-entangled photons can be generated with dependence on or complete independence from the pumping wavelength and polarization, and the modal content of the nanoresonator. Our work also shows the potential of nonlinear nanoresonators as miniaturized sources of biphoton states with highly complex and tunable properties.

physics.optics↗