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Frederik Schröder

Publications and source records attributed to Frederik Schröder.

4 recordsLinked to original sources

Integrated on-chip quantum light sources on a van der Waals platform

Scalable photonic quantum information technologies require a platform combining quantum light sources, waveguides, and detectors on a single chip. Here, we introduce a van der Waals platform comprising strain-engineered bilayer WSe$_2$ quantum emitters, integrated on multimode WS$_2$ waveguides with grating couplers, enabling efficient on-chip quantum light sources. The emitters exhibit bright, highly polarised emission that couples efficiently into WS$_2$ waveguides. Under discrete-state excitation, we observe high-purity, waveguide-coupled single-photon emission, measured using both single-port and cross-correlated, multi-port photon streams, yielding $g^{(2)}(0) = 0.003^{+0.030}_{-0.003}$ and $g^{(2)}(0) = 0.076\pm0.023$, respectively. For a single output, the out-coupled single-photon count rate at the first lens reaches approximately 357 kHz under continuous-wave discrete-state excitation, corresponding to an estimated minimum waveguide-coupled rate of 1.68 MHz. These results demonstrate an efficient, integrated single-photon source and establish a pathway toward scalable photonic quantum information processing centred around nanoengineered van der Waals materials.

physics.optics↗

Ultrafast control of coherent acoustic lattice dynamics in the transition metal dichalcogenide alloy WSSe

Coherent acoustic phonons (CAPs)$-$propagating strain waves that can dynamically modify the structure and symmetry of a crystal$-$offer unique opportunities for controlling material properties. We investigate CAP generation in the Janus-like layered alloy tungsten sulfide selenide (WS$_x$Se$_{1-x}$, hereafter WSSe). Employing high-fluence photoexcitation at 400 nm combined with ultrafast transient reflection spectroscopy, we capture the carrier-lattice dynamics governed by a cascade of processes including rapid exciton formation, phonon recycling, and thermoelastic deformation. These phenomena precede the emergence of a robust CAP mode at 27 GHz. Notably, the CAP amplitude in WSSe substantially exceeds that observed in the symmetric parent crystals WS$_2$ and WSe$_2$, which we attribute to an enhanced coupling mediated by a built-in out-of-plane electric field arising from the inversion asymmetry of the WSSe alloy. Furthermore, the implementation of a tailored two-pulse excitation sequence enables optical control of the CAP, underscoring the potential of WSSe and related Janus-like layered alloys as versatile building blocks in optomechanical and nanoacoustic device applications.

cond-mat.mtrl-sci↗

Confocal polarization tomography of dielectric nanocavities

We employ polarization tomography to characterize the modal properties of a dielectric nanocavity with sub-wavelength mode confinement. Our analysis of reflection spectra shows that the Fano-lineshape depends strongly on the polarization in a confocal configuration, and that the lineshape can be transformed into a Lorentzian-like peak for a certain polarization. For this polarization setting, the background is almost fully suppressed in a finite range of frequencies. This enables us to identify another resonance that has not yet been experimentally reported for these nanocavities. Lastly, we use symmetry-forbidden polarizations and show that, surprisingly, the modal resonance features of the system remain visible.

physics.optics↗

Fiber-pigtailing quantum-dot cavity-enhanced light emitting diodes

We report on a process for the fiber-coupling of electrically driven cavity-enhanced quantum dot light emitting devices. The developed technique allows for the direct and permanent coupling of p-i-n-doped quantum dot micropillar cavities to single-mode optical fibers. The coupling process, fully carried out at room temperature, involves a spatial scanning technique, where the fiber facet is positioned relative to a device with a diameter of 2 $μ$m using the fiber-coupled electroluminescence of the cavity emission as a feedback parameter. Subsequent gluing and UV curing enables a rigid and permanent coupling between micropillar and fiber core. Comparing our experimental results with finite element method simulations indicates a cavity-to-fiber mode-coupling efficiency of ~46%. Furthermore, we demonstrate pulsed current injection at a repetition rate exceeding 200 MHz as well as low-temperature operation down to 77 K of the fiber-coupled micropillar device. The technique presented in this work is an important step in the quest for efficient and practical quantum light sources for applications in quantum information.

cond-mat.mes-hall↗