arXiv subjects

Fulong Dong

Publications and source records attributed to Fulong Dong.

8 recordsLinked to original sources

arXiv2026

All-optical reconstruction of valley polarization through helicity-resolved high-harmonic generation

We theoretically investigate valley-resolved high-order harmonic generation in gapped graphene driven by elliptically polarized laser fields. Using two-band density-matrix simulations and an electron-hole recombination trajectory model, we find that the two inequivalent valleys emit harmonics with opposite helicities. Under an elliptically polarized field, these emissions occur predominantly in different half cycles of the laser field. Time-dependent density functional theory calculations for monolayer MoS$_2$ show the same temporal separation of harmonic emissions with opposite helicities, supporting the generality of this valley-dependent chiral response. We further propose an all-optical scheme to reconstruct valley polarization from helicity-resolved harmonic signals. A circularly polarized pulse first prepares a valley population imbalance. A subsequent elliptically polarized laser induces different changes in the harmonic intensities of opposite helicities through Pauli blocking. The ratio of these intensity changes provides a direct measure of the valley polarization. Our results demonstrate that chiral high-harmonic emission can serve as an all-optical probe of ultrafast valley-dependent carrier dynamics.

physics.optics↗

arXiv2026

Attosecond Reconstruction of Strain Tensors via Electronic Fingerprints

We demonstrate an attosecond transient absorption spectroscopy (ATAS) scheme for reconstructing strain tensors in two-dimensional materials. Using strained graphene as a prototype system, we show that the fishbone structures in ATAS serve as distinctive spectral fingerprints of strain, where strain-induced shifts and splittings of van Hove singularities encode the magnitude and orientation of the strain tensor, respectively. By combining density-matrix simulations with analytical modeling, we establish a direct mapping between transient absorption spectra and strain tensors, enabling accurate retrieval of lattice deformation from ultrafast electronic responses. Our work introduces an attosecond spectroscopic paradigm for ultrafast strain metrology, where electronic fingerprints replace conventional structural probes for sensing lattice deformation in quantum materials.

cond-mat.mtrl-sci↗

arXiv2025

Effect of Berry connection on attosecond transient absorption spectroscopy in gapped graphene

We investigate the attosecond transient absorption spectroscopy (ATAS) in gapped graphene by numerically solving the four-band density matrix equations. Our results reveal that, in contrast to pristine graphene, whose fishbone-shaped spectra oscillate at twice the pump laser frequency, the ATAS of gapped graphene exhibits an additional component oscillating at the pump laser frequency, induced by the Berry connection. To gain insight into these interesting results, we employ a simplified model to derive an analytical expression for the spectral component stemming from the Berry connection. Our analytical results qualitatively reproduce the key features observed in the numerical simulations, revealing that the intensity of the fundamental-frequency spectral component depends not only on the Berry connection but also on the energy shifts associated with the effective mass of electrons at the van Hove singularities. These results shed light on the complex generation mechanism of the ATAS in symmetry-broken materials.

cond-mat.mes-hall↗

arXiv2025

Attosecond transient absorption spectroscopy in monolayer hexagonal boron nitride

We simulate the attosecond transient absorption spectroscopy (ATAS) of monolayer hexagonal boron nitride (hBN) using the time-dependent density functional theory and two-band density-matrix equations within the tight-binding approximation. The simulation results from the two methods are qualitatively consistent. We focus on the fishbone structure around the gap energy of the M point, which exhibits a temporal period equal to that of the pump laser. To gain deeper insight into this structure, we simplify the two-band model to a single-electron model located at the M point, allowing us to derive an analytical expression that can qualitatively reproduce the numerical results. By isolating the influence of the Berry connection on the ATAS, our analytical results reveal that both the interband transition dipole moments and the Berry connection play important roles in the fishbone structure of the ATAS. Moreover, we also have investigated the dependence of ATAS on the gap energy based the tight-binding approximation. The results demonstrate that the ATAS intensity is enhanced as the gap energy increases, in agreement with our analytical prediction. Our study may shed light on the generation mechanism of the fishbone structure of the ATAS in hBN.

physics.atom-ph↗

arXiv2025

Isolated elliptically-polarized attosecond pulse generation in gapped graphene driven by linearly polarized laser fields

We theoretically investigate high-order harmonic generation (HHG) and its ellipticity in gapped graphene, driven by a femtosecond short-pulse laser at various orientation angles, employing the two-band density-matrix equations within the tight-binding approximation. The orientation-dependent harmonic spectra exhibit pronounced enhancement of specific harmonics, which we attribute to the caustic effect. Using the recombination trajectory model, we reveal that the orientation dependence of these enhanced harmonics originates from the distinct band structures encountered by electrons ionized from the two inequivalent $\textrm{K}$ points. Moreover, we focus on the ellipticity of the enhanced harmonics at specific angles and demonstrate that it primarily depends on the phase difference between the parallel and perpendicular components, which can be accurately predicted by our recombination trajectory model. Based on these insights, we propose a two-color (fundamental plus second-harmonic) field scheme to generate isolated elliptically polarized attosecond pulses (IEAPs) in gapped graphene. Our findings may provide a promising pathway toward the generation of IEAPs in gapped graphene or transition metal dichalcogenides.

physics.atom-ph↗

arXiv2023

Caustic effects on the high-order harmonic generation in graphene

We employ the two-band density-matrix equations and time-dependent density functional theory to calculate high-order harmonic generation (HOHG) in graphene under a femtosecond laser irradiation. Our investigation uncovers a striking harmonic enhancement structure (HES) within a specific energy range of the HOHG spectrum. In this regime, we find the convergence of multiple interband electron-hole recombination trajectories, leading to the zero determinant of the Hessian matrix of the semiclassical action. This trajectory convergence exhibits the characteristics akin to the focusing behavior of light rays, commonly known as caustic effects. In contrast to atom situation, where caustic effects are confined to a narrow energy regime around the HOHG cut-off energy and the enhancement due to caustic trajectory convergence is less apparent, the two-dimensional nature of graphene results in a broad energy region for HOHG enhancement that the caustic trajectories can even dominate the entire interband harmonic generation regime. The magnitude of enhancement is significant and can be estimated to be on the order of $\sim N^{2/3}$, with $N$ representing the harmonic order, according to the catastrophe theory. These mechanisms have broad applicability and hold significant implications for other two-dimensional materials, as well as bulk materials, providing crucial insights into the understanding of HOHG phenomena in diverse material systems.

physics.atom-ph↗

arXiv2022

Fishbone resonance structure in the attosecond transient absorption spectroscopy of graphene

We investigate the attosecond transient absorption spectroscopy (ATAS) of graphene by numerically solving four-band density-matrix equations, which demonstrates apparent fish bone resonance structures. To gain insight into these interesting structures, we exploit a simplified model that only considers the electrons of $Γ$ and M points in the Brillouin zone. With the help of this model, we can analytically express the ATAS spectrum as the sum of zeroth- and first-order Bessel functions in the variables of the strength and frequency of the infrared pump field as well as the effective mass of electrons at the $Γ$ and M points. Lorentzian and Fano line shapes in the absorption spectrum are addressed. The fish bone structure consists of periodic V-shaped structure that can be explained by first-order Bessel functions and its tilt angle is solely determined by the frequency of the pump laser. The periodicity of the V-shaped structure in the fish bone originates from the periodic dependence of the Lorentzian and Fano line shapes of the absorption spectrum on the time delay between the pump and probe lasers. Compared with the numerical results, our analytical theory can qualitatively or even quantitatively predict the zeroth- and first-order fringes in the fish bone structures of the ATAS spectrum. The gauge issues in the numerical simulations are also discussed.

cond-mat.mes-hall↗

arXiv2022

Knee structure in the laser intensity dependence of high-order harmonic generations for graphene

We investigate the high-order harmonic generations (HHGs) of graphene irradiated by linearly polarized lasers with intensities in a wide range from $10^{8}$ W/cm$^2$ to $10^{13}$ W/cm$^2$. We find a striking knee structure in the laser intensity dependence of HHGs, which consists of a linear growth regime, followed by a plateau of the saturated HHGs, and then a transition to a nonlinear growth. The knee structure is rather universal for the varied harmonic orders and has been certificated by the calculations of two-band density-matrix equations as well as the \textit{ab initio} calculations of time-dependent density functional theory. Based on the two-band model, we reveal the underlying mechanisms: The behavior of linear growth can be depicted analytically by the perturbative theory of optical conductivity; While, the plateau of saturated HHGs and the transition to a nonlinear growth are caused by the quantum destructive interference and constructive interference of harmonics generated by the electrons corresponding to the lattice momentums around Dirac points and M points in Brillouin zone, respectively. In particular, we find that tuning Fermi energy can effectively alter the knee structure while the profile of the knee structure is not sensitive to the temperature. Our calculations of the third-order harmonic vs. tuning Fermi energy are compared with recent experiment showing a good agreement. Our predicted knee structure and its associated properties are observable with the current experimental techniques.

physics.atom-ph↗