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Fusayoshi J. Ohkawa

Publications and source records attributed to Fusayoshi J. Ohkawa.

At least 19 recordsLinked to original sources

Resonating-valence-bond liquid in low dimensions

The Hubbard model in $D$ dimensions, with the on-site repulsion $U$ and the transfer integral between nearest neighbors $-t/\sqrt{D}$, is studied on the basis of the Kondo-lattice theory. If $U/|t| \gg 1$, $|n - 1| \lesssim |t|/(DU)$, where $n$ is the number of electrons per unit cell, and $D$ is so small that $|J|/D \gg k_{\rm B}T_c$, where $J = -4t^2/U$ and $T_c$ is $0 {\rm K}$ for $D = 1$ and is the highest critical temperature among possible ones for $D \ge 2$, a low-$T$ phase where $T_c < T \ll |J|/(k_{\rm B}D)$ is a frustrated electron liquid. Since the liquid is stabilized by the Kondo effect in conjunction with the resonating-valence-bond (RVB) mechanism, it is simply the RVB electron liquid; in one dimension, it is also the Tomonaga-Luttinger liquid. The Kondo energy of the RVB liquid is $k_{\rm B}T_{\rm K} = O(|J|/D)$; its effective Fermi energy is $O(k_{\rm B}T_{\rm K})$. A midband appears on the chemical potential between the upper and lower Hubbard bands; the Hubbard gap is a pseudogap. As regards the density of states per unit cell of the midband, its bandwidth is $O(k_{\rm B}T_{\rm K})$ or $O(|J|/D)$, its peak height is $O(1/U)$, and its spectral weight is $O[t^2/(DU^2)]$. Since the midband almost disappears in the Heisenberg limit, the RVB electron liquid in the Heisenberg limit is simply the RVB spin liquid. The RVB electron and spin liquids adiabatically continue to each other. Since local moments form in a high-$T$ phase where $T \gtrsim T_{\rm K}$, the high-$T$ phase is simply the Mott insulator.

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Adiabatic Continuation between Resonating-Valence-Bond Electron and Spin Liquids

The Hubbard model in the strong-coupling regime is studied by the Kondo-lattice theory. If no symmetry is broken at a sufficiently low temperature in sufficiently low dimensions, an electron liquid is stabilized by the Fock-type exchange effect of the superexchange interaction. Since the stabilization mechanism is none other than the resonating-valence-bond (RVB) mechanism, the electron liquid is none other than an RVB electron liquid. The RVB electron liquid in the Hubbard model is adiabatically connected to the RVB spin liquid in the Heisenberg model.

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Residual Entropy of the Mott Insulator with No Symmetry Broken

The half-filled ground state of the Hubbard model on the hypercubic lattice in D dimensions is studied by the Kondo-lattice theory, which is none other than the 1/D expansion theory, but within the constrained Hilbert subspace where no symmetry is allowed to be broken. A gap can open in the single-particle excitation spectrum if and only if the residual entropy or entropy at T=+0 K is nonzero. The Mott insulator with no symmetry broken, if it is possible, is characterized by nonzero residual entropy or nonzero entropy at T=+0 K. This conclusion is consistent with Brinkman and Rice's theory and the dynamical mean-field theory. According to the well-known argument based on the Bethe-ansatz solution, on the other hand, the half-filled ground state in one dimension is the Mott insulator although its residual entropy per unit cell is vanishing in the thermodynamic limit. Two possible explanations are given for the contradiction between the present paper and the well-known argument.

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Instability of the Mott or Lieb-Wu insulator caused by an infinitesimal perturbation

The half-filled ground state of the Hubbard model in one dimension is studied by Kondo-lattice theory. Because of the Kondo effect, any insulating ground state with a complete gap open is unstable in the presence of an infinitesimal perturbation. This fact casts doubt on the claim by E. H. Lieb and F. Y. Wu, Phys. Rev. Lett. 20, 1445 (1968) that the half-filled ground state is the Mott insulator. Though the claim is based on a rigorous result given by the Bethe-ansatz solution, the rigorous result is simply a necessary condition for the ground state being an insulator.

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Itinerant-Electron Magnetism in the Heisenberg Limit

The Hubbard model in the Heisenberg limit is studied by Kondo-lattice theory. The Kondo temperature T_K or k_BT_K, which is an energy scale of low-energy local quantum spin fluctuations, is enhanced by the resonating valence bond (RVB) mechanism, so that T_K\simeq T_MF/(2D), where T_MF is the Neel temperature in the mean-field approximation of the corresponding Heisenberg model and D is the spatial dimensionality. Electrons certainly behave as localized spins at T\gg T_K, but they are still itinerant at T\ll T_K unless an antiferromagnetic complete gap opens. When the Neel temperature T_N is so high that T_N\gg T_MF/(2D), magnetism is prototypic local-moment magnetism. When T_N is so low that T_N \ll T_MF/(2D) because of low dimensionality or frustration, magnetism is itinerant-electron magnetism of an almost spin liquid, i.e., a normal Fermi liquid or a Tomonaga-Luttinger liquid in which the spectral weight of single-particle excitations is almost vanishing. The spin susceptibility has a temperature and wave-number dependence characteristic of itinerant-electron magnetism. This type of itinerant-electron magnetism must also be possible in the Heisenberg model.

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Frustrated electron liquids in the Hubbard model

The ground state of the Hubbard model is studied within the constrained Hilbert space where no order parameter exists. The self-energy of electrons is decomposed into the single-site and multisite self-energies. The calculation of the single-site self-energy is mapped to a problem of self-consistently determining and solving the Anderson model. When an electron reservoir is explicitly considered, it is proved that the single-site self-energy is that of a normal Fermi liquid even if the multisite self-energy is anomalous. Thus, the ground state is a normal Fermi liquid in the supreme single-site approximation (S^3A). In the strong-coupling regime, the Fermi liquid is stabilized by the Kondo effect in the S^3A and is further stabilized by the Fock-type term of the superexchange interaction or the resonating-valence-bond (RVB) mechanism beyond the S^3A. The stabilized Fermi liquid is frustrated as much as an RVB spin liquid in the Heisenberg model. It is a relevant unperturbed state that can be used to study a normal or anomalous Fermi liquid and an ordered state in the whole Hilbert space by Kondo lattice theory. Even if higher-order multisite terms than the Fock-type term are considered, the ground state cannot be a Mott insulator. It can be merely a gapless semiconductor even if the multisite self-energy is so anomalous that it is divergent at the chemical potential. A Mott insulator is only possible as a high temperature phase.

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Strong-coupling Superconductivity in the Cuprate Oxide

Superconductivity in the cuprate oxide is studied by Kondo-lattice theory based on the t-J model with the el-ph interaction arising from the modulation of the superexchange interaction by phonons. The self-energy of electrons is decomposed into the single-site and multisite ones. It is proved by using the mapping of the single-site one in the t-J model to its corresponding one in the Anderson model that the single-site self-energy is that of a normal Fermi liquid, even if a superconducting (SC) order parameter appears or the multisite one is anomalous. The electron liquid characterized by the single-site self-energy is a normal Fermi liquid. The Fermi liquid is further stabilized by the RVB mechanism. The stabilized Fermi liquid is a relevant unperturbed state that can be used to study superconductivity and anomalous Fermi-liquid behaviors. The so-called spin-fluctuation-mediated exchange interaction, which includes the superexchange interaction as a part, is the attractive interaction that binds d-wave Cooper pairs. An analysis of the spin susceptibility implies that, because of the el-ph interaction, the imaginary part of the exchange interaction has a sharp peak or dip at \pmω^*, where ω^*\simeq ω_ph in the normal state and ε_G/2 \lessim ω^* \lessim ε_G /2+ ω_ph in the SC state, where ω_ph is the energy of relevant phonons and ε_G is the SC gap. If the imaginary part has a sharp peak or dip at \pmω^*, the dispersion relation of quasi-particles has kink structures near \pmω^* above and below the chemical potential, the density of states has dip-and-hump structures near \pm ω^* outside the coherence peaks in the SC state, and the anisotropy of the gap deviates from the simple d-wave anisotropy.

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Fermi liquid in the Hubbard Model with an electron reservoir: Normal state of cuprate superconductors

It is proved that the ground state under the supreme single-site approximation (S^3A), the dynamical mean-field theory (DMFT), or the dynamical coherent potential approximation (DCPA) is the normal Fermi liquid in the presence of an infinitesimally weak hybridization with an electron reservoir, except for the just half filling of electrons and the infinite on-site repulsion. In the strong-coupling regime, in particular, the Fermi liquid is stabilized under S^3A, DMFT, or DCPA by the Kondo effect, which stabilizes a local singlet on each unit cell, and is further stabilized beyond it by the Fock-type term of the superexchange interaction or a resonating valence bond (RVB) mechanism, which stabilizes a local singlet on each pair of nearest neighbors. The Fermi liquid is a relevant normal state to study possible lower-temperature phases or the true ground state. It is proposed that the Fermi liquid stabilized by the Kondo effect and the RVB mechanism is the normal state of cuprate high-temperature superconductors.

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Kondo-lattice theory of anisotropic singlet superconductivity

Kondo-lattice theory for the t-J model and a phenomenological theory based on it are developed to study superconductivity in the vicinity of the Mott metal-insulator transition. Since the quenching of magnetic moments by single-site quantum spin fluctuations or the Kondo effect is reduced by the opening of a superconducting gap, spin density wave (SDW) can appear in a superconducting state and the Knight shift can deviate from the Yosida function to be small. The electron-phonon interaction, which arises from the modulation of the superexchange interaction by phonons, is crucial in the coexistence of superconductivity and SDW. It is proposed that the coexistence of superconductivity, a double-Q SDW, a double-Q lattice distortion, and a double-Q charge density wave induced by the SDW rather than the lattice distortion, is responsible for the checkerboard structure and the zero-temperature pseudo-gap observed in under-doped cuprate superconductors.

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Mott metal-insulator transition in the Hubbard model

The Hubbard model in the strong-coupling regime is mainly studied by Kondo-lattice theory or 1/d expansion theory, with d the spatial dimensionality. In two dimensions and higher, the ground state within the Hilbert subspace with no order parameter is a normal Fermi liquid except for n=1 and U/W=+infinity, with n the electron density per unit cell, U the on-site repulsion, and W the bandwidth; the cooperation between the Kondo effect, which favors a local singlet on each unit cell, and a resonating-valence-bond effect, which favors a local singlet on each pair of nearest-neighbor unit cells, stabilizes the Fermi liquid, whose ground state is a singlet as a whole, in the strong-coupling regime. In the whole Hilbert space with no restriction, the normal Fermi liquid is unstable at least against a magnetic or superconducting state. This analysis confirms an early Fermi-liquid theory of high-temperature superconductivity, F. J. Ohkawa, Jpn. J. Appl. Phys. 26, L652 (1987). The ground state for n=1 and U/W=+infinity is a Mott insulator. Actual metal-insulator transitions cannot be explained within the Hubbard model. In order to explain them, the electron-phonon interaction, multi-band or multi-orbital effects, and effects of disorder should be considered beyond the Hubbard model. The crossover between local-moment magnetism and itinerant-electron magnetism corresponds to that between a localized spin and a normal Fermi liquid in the Kondo effect and it is simply a Mott metal-insulator crossover.

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Mott metal-insulator transition in the Hubbard model

The ground state of the Hubbard model is studied within the single-site approximation (SSA) and beyond the SSA. Within the SSA, the ground state is a typical Mott insulator at the critical point n=1 and U/W=+infty, with n being the electron density per unit cell, W the bandwidth of electrons, and U the on-site repulsion, and is a normal Fermi liquid except for the critical point. Beyond the SSA, the normal Fermi liquid is unstable against a non-normal Fermi liquid state except for a trivial case of U=0 such as a magnetic or superconducting state in two and higher dimensions. In order to explain actual observed metal-insulator transitions, one or several effects among the electron-phonon interaction, multi-band or multi-orbital effects, and effects of disorder should be considered beyond the Hubbard model.

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Origin and roles of a strong electron-phonon interaction in cuprate oxide superconductors

A strong electron-phonon interaction arises from the modulation of the superexchange interaction by lattice vibrations. It is responsible for the softening of the half-breathing modes around (pm pi/a,0) and (0, pm pi/a) in the two-dimensional Brillouin zone, with a being the lattice constant of CuO_2 planes, as is studied in Phys. Rev. B70, 184514 (2004). Provided that antiferromagnetic spin fluctuations are developed around Q=(pm 3 pi/4a, pm pi/a) and (pm pi/a, pm 3 pi/4a), the electron-phonon interaction can also cause the softening of Cu-O bond stretching modes around 2Q, or around (pm pi/2a,0) and (0, pm pi/2a). The softening around 2Q is accompanied by the development of charge fluctuations corresponding to the so called 4a-period stripe or 4a*4a-period checker-board state. However, an observation that the 4a-period modulating part or the 2Q part of the density of states is almost symmetric with respect to the chemical potential contradicts a scenario that the stabilization of a single-2Q or double-2Q charge density wave following the complete softening of the 2Q bond stretching modes is responsible for the ordered stripe or checker-board state. It is proposed that the stripe or checker-board state is simply a single-Q or double-Q spin density wave, whose second-harmonic effects can explain the observed almost symmetric 2Q part of the density of states. The strong electron-phonon interaction can play no or only a minor role in the occurrence of d gamma-wave superconductivity in cuprate oxides.

cond-mat.supr-con↗

Origin and roles of a strong electron-phonon interaction in cuprate oxide superconductors

A strong electron-phonon interaction arises from the modulation of the superexchange interaction by phonons. As is studied in Phys. Rev. B 70, 184514 (2004), Cu-O bond stretching modes can be soft around (pm pi/a, 0) and (0, pm pi/a), with a the lattice constant of CuO_2 planes. In the critical region of SDW, where antiferromagnetic spin fluctuations are developed around nesting wave numbers Q of the Fermi surface, the stretching modes can also be soft around 2Q. Almost symmetric energy dependences of the 2Q component of the density of states, which are observed in the so called stripe and checker-board states, cannot be explained by CDW with 2Q following the complete softening of the 2Q modes, but they can be explained by a second-harmonic effect of SDW with Q. The strong electron-phonon interaction can play no or only a minor role in the occurrence of superconductivity.

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Opening of a pseudogap in a quasi-two dimensional superconductor due to critical thermal fluctuations

We examine the role of the anisotropy of superconducting critical thermal fluctuations in the opening of a pseudogap in a quasi-two dimensional superconductor such as a cuprate-oxide high-temperature superconductor. When the anisotropy between planes and their perpendicular axis is large enough and its superconducting critical temperature T_c is high enough, the fluctuations are much developed in its critical region so that lifetime widths of quasiparticles are large and the energy dependence of the selfenergy deviates from that of Landau's normal Fermi liquids. A pseudogap opens in such a critical region because quasiparticle spectra around the chemical potential are swept away due to the large lifetime widths. The pseudogap never smoothly evolves into a superconducting gap; it starts to open at a temperature higher than T_c while the superconducting gap starts to open just at T_c. When T_c is rather low but the ratio of varepsilon_G(0)/k_BT_c, with varepsilon_G(0) the superconducting gap at T=0K and k_B the Boltzmann constant, is much larger than a value about 4 according to the mean-field theory, the pseudogap must be closing as temperature T approaches to the low T_c because thermal fluctuations become less developed as T decreases. Critical thermal fluctuations cannot cause the opening of a prominent pseudogap in an almost isotropic three dimensional superconductor, even if its T_c is high.

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Coexistence of double-Q spin density wave and multi-Q pair density wave in cuprate oxide superconductors

Spatial 4a x 4a modulations, with a the lattice constant of CuO_2 planes, or the so called checkerboards can arise from double-Q spin density wave (SDW) with Q_1 = (pm pi/a, pm 3 pi/4a) and Q_2 = (pm 3 pi/4a, pm pi/a). When multi-Q pair density wave, that is, the condensation of d gamma-wave Cooper pairs with zero total momenta, pm 2Q_1, pm 2Q_2, pm 4Q_1, pm 4Q_2, and so on is induced by the SDW, gaps can have fine structures similar to those of the so called zero-temperature pseudogaps.

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Crossover between local-moment magnetism and itinerant-electron magnetism in the t-J model

A Kondo-lattice theory is applied to the crossover between local-moment magnetism for almost half fillings of electrons and itinerant-electron magnetism away from the half filling. In clean systems with no disorder, the bandwidth W^* of quasiparticles is non-zero and of the order of |J| at T=0K even in the limit of the half filling, with J the superexchange interaction constant between nearest neighbors. The so called Gutzwiller's term also contributes to W^* away from the half filling; it is approximately proportional to doping concentrations measured from the half filling. Magnetism is enhanced by disorder because the renormalization of W^* by J is reduced by disorder. The asymmetry of disorder between electron-doped and hole-doped cuprate oxide superconductors must be, at least partly, responsible for that of antiferromagnetic phases between them. The so called Kumagai phase is characterized as an SDW state in a disordered system rather than a spin glass. The Neel temperature T_N about 300K of non-doped cuprate oxides can be explained by the reduction of T_N by critical thermal antiferromagnetic fluctuations in quasi-two dimensions.

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Opening of pseudogaps due to superconducting critical fluctuations in quasi-two dimensions

We examine the role of the anisotropy of superconducting thermal critical fluctuations in the opening of pseudogaps in quasi-two dimensions. When the anisotropy of coherence or correlation lengths of the fluctuations is large enough and critical temperatures T_c are high enough, the energy dependence of the selfenergy deviates from that of Landau's normal Fermi liquid in critical regions; its imaginary part has no minimum at the chemical potential. Prominent pseudogaps open in such a non-Fermi liquid phase. Pseudogaps must be absent or subtle in quasi-two dimensional superconductors with low T_c and almost isotropic three dimensional superconductors.

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Application of Kondo-lattice theory to Mott-Hubbard metal-insulator crossover in disordered cuprate-oxide superconductors

A theory of Kondo lattices is applied to the crossover between local-moment magnetism and itinerant-electron magnetism in the t-J model on a quasi-two dimensional lattice. The Kondo temperature T_K is defined as a characteristic temperature or energy scale of local quantum spin fluctuations. Magnetism with T_N >> T_K, where T_N is the N\eel temperature, is characterized as local-moment one, while magnetism with T_N << T_K is characterized as itinerant-electron one. The Kondo temperature, which also gives a measure of the strength of the quenching of magnetic moments, is renormalized by the Fock term of the superexchange interaction. Because the renormalization depends on life-time widths γof quasiparticles in such a way that T_K is higher for smaller γ, T_N can be controlled by disorder. The asymmetry of T_N between electron-doped and hole-doped cuprates must mainly arise from that of disorder; an almost symmetric behavior of T_N must be restored if we can prepare hole-doped and electron-doped cuprates with similar degree of disorder to each other. Because effective disorder is enhanced by magnetic fields in Kondo lattices, antiferromagnetic ordering must be induced by magnetic fields in cuprates that exhibit large magnetoresistance.

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