arXiv subjects

Götz S. Uhrig

Publications and source records attributed to Götz S. Uhrig.

At least 55 records · Page 3Linked to original sources

arXiv2022

Dynamic mean-field theory for dense spin systems at infinite temperature

A dynamic mean-field theory for spin ensembles (spinDMFT) at infinite temperatures on arbitrary lattices is established. The approach is introduced for an isotropic Heisenberg model with $S = \tfrac12$ and external field. For large coordination numbers, it is shown that the effect of the environment of each spin is captured by a classical time-dependent random mean-field which is normally distributed. Expectation values are calculated by averaging over these mean-fields, i.e., by a path integral over the normal distributions. A self-consistency condition is derived by linking the moments defining the normal distributions to spin autocorrelations. In this framework, we explicitly show how the rotating wave approximation becomes a valid description for increasing magnetic field. We also demonstrate that the approach can easily be extended. Exemplarily, we employ it to reach a quantitative understanding of a dense ensemble of spins with dipolar interaction which are distributed randomly on a plane including static Gaussian noise as well.

cond-mat.stat-mech↗

arXiv2022

Simulation of nonequilibrium spin dynamics in quantum dots subjected to periodic laser pulses

Large-scale simulations of the spin dynamics in quantum dots subjected to trains of periodic laser pulses enable us to describe and understand related experiments. By comparing the data for different models to experimental results, we gain an improved understanding of the relevant physical mechanisms. Using sophisticated numerical approaches and an efficient implementation combined with extrapolation arguments, nonequilibrium stationary states are reached for parameter ranges close to the ones in real experiments. With the help of high performance computing, we can tune the experimental parameters to guide future experimental research. Importantly, our simulations reveal the possibility of resonant spin amplification in Faraday geometry, i.e., when a longitudinal magnetic field is applied to the quantum dots.

cond-mat.mes-hall↗

arXiv2021

Double-Exchange Enhanced Magnetic Blue-Shift of Mott Gaps

A substantial energy gap of charge excitations induced by strong correlations is the characteristic feature of Mott insulators. We study how the Mott gap is affected by long-range antiferromagnetic order. Our key finding is that the Mott gap is increased by the magnetic ordering: a magnetic blue-shift (MBS) occurs. Thus, the effect is proportional to the exchange coupling in the leading order in the Hubbard model. In systems with additional localized spins the double-exchange mechanism induces an additional contribution to the MBS which is proportional to the hopping in the leading order. The coupling between spin and charge degrees of freedom bears the potential to enable spin-to-charge conversion in Mott systems on extreme time scales determined by hopping and exchange only, since a spin-orbit mediated transfer of angular momentum is not involved in the process. In view of spintronic and magnonic applications, it is highly promising to observe that several entire classes of compounds show exchange and double-exchange effects. Exemplarily, we show that the magnetic contribution to the band-gap blue-shift observed in the optical conductivity of $α$-MnTe is correctly interpreted as the MBS of a Mott gap.

cond-mat.str-el↗

arXiv2021

Lattice-driven femtosecond magnon dynamics in $α$-MnTe

The light-induced femtosecond dynamics of the sublattice magnetizations in the antiferromagnetically ordered phase of the semiconductor $α$-MnTe is investigated theoretically as function of an external driving field. The electromagnetic field is coupled to optical modes and the concomitant atomic displacements modulate the Heisenberg exchange couplings. We derive the equations of motion for the time-dependent sublattice magnetization in spin wave theory and analyze the contributions from the driven magnon modes. The antiferromagnetic order parameter exhibits coherent longitudinal oscillations determined by the external driving frequency which decay due to dephasing. Including a phenomenological dissipative term to mimic spin-lattice relaxation processes leads to relaxation back to thermal equilibrium. We provide approximate analytic solutions of the resulting differential equations which allow us to understand the effect of the driving light pulse on the amplitude, frequency, and lifetime of the coherent spin dynamics.

cond-mat.str-el↗

arXiv2021

Charge dynamics in magnetically disordered Mott insulators

With the aid of both a semi-analytical and a numerically exact method we investigate the charge dynamics in the vicinity of half-filling in the one- and two-dimensional $t$-$J$ model derived from a Fermi-Hubbard model in the limit of large interaction $U$ and hence small exchange coupling $J$. The spin degrees of freedom are taken to be disordered. So we consider the limit $0 < J \ll T \ll W$ where $W$ is the band width. We focus on evaluating the spectral density of a single hole excitation and the charge gap which separates the upper and the lower Hubbard band. One of the key findings is the evidence for the absence of sharp edges of the Hubbard band, instead Gaussian tails appear.

cond-mat.str-el↗

arXiv2020

Interplay of spin mode locking and nuclei-induced frequency focusing in quantum dots

We study the influence of nuclei-induced frequency focusing on the mode locking of spin coherence in quantum dots subjected to a periodic train of optical pulses. In particular, we address the question whether or not nuclei-induced frequency focusing always enhances the effect of spin mode locking. We combine two advanced semiclassical approaches and extend the resulting model by including the full dynamics of the optically excited trion state. In order to reduce the discrepancy to a full quantum model, we establish a nondeterministic pulse description by interpreting each pump pulse as a measurement. Both extensions lead to significant qualitative changes of the physics. Their combination improves the description of the corresponding experiments. Importantly, we observe the emergence of dynamic nuclear polarization, i.e., the formation of a nonzero average polarization of the nuclear spin bath, leading to a certain increase of the coherence time.

cond-mat.mes-hall↗

arXiv2020

Probing thermalization in quenched (non-)integrable Fermi-Hubbard models

Using numerically exact methods we examine the Fermi-Hubbard model on arbitrary cluster topology. We focus on the question which systems eventually equilibrate or even thermalize after an interaction quench when initially prepared in a state highly entangled between system and bath. We find that constants of motion in integrable clusters prevent equilibration to the thermal state. We discuss the size of fluctuations during equilibration and thermalization and the influence of integrability. The influence of real space topology and in particular of infinite-range graphs on equilibration and thermalization is studied.

cond-mat.str-el↗

arXiv2020

Topological superconductivity induced by a triple-Q magnetic structure

We demonstrate that the recently discovered triple-Q (3Q) magnetic structure, when embedded in a magnet-superconductor hybrid (MSH) system, gives rise to the emergence of topological superconductivity. We investigate the structure of chiral Majorana edge modes at domain walls, and show that they can be distinguished from trivial in-gap modes through the spatial distribution of the induced supercurrents. Finally, we show that topological superconductivity in 3Q MSH systems is a robust phenomenon that does not depend on the relative alignment of the magnetic and superconducting layers, or on the presence of electronic degrees of freedom in the magnetic layer.

cond-mat.supr-con↗

arXiv2019

Spin inertia and polarization recovery in quantum dots: Role of pumping strength and resonant spin amplification

Spin inertia measurements are a novel experimental tool to study long-time spin relaxation processes in semiconductor nanostructures. We develop a theory of the spin inertia effect for resident electrons and holes localized in quantum dots. We consider the spin orientation by short optical pulses with arbitrary pulse area and detuning from the trion resonance. The interaction with an external longitudinal magnetic field and the hyperfine interaction with the nuclear spin bath is considered in both the ground and excited (trion) states of the quantum dots. We analyze how the spin inertia signal depends on the magnetic field (polarization recovery) and on the modulation frequency of the helicity of the pump pulses as well as on their power and detuning. In particular, we elaborate how approaching the saturation limit of the spin polarization influences the measurements. The quantitative description of spin inertia measurements will enable the determination of the parameters of spin dynamics such as the spin relaxation times in the ground and excited states and the parameters of the hyperfine interaction. Finally, we predict the emergence of resonant spin amplification due to the transverse components of the nuclear spin fluctuations, which manifests itself as oscillations of the spin polarization as a function of the longitudinal magnetic field.

cond-mat.mes-hall↗

arXiv2018

Magnetic field dependence of the electron spin revival amplitude in periodically pulsed quantum dots

Periodic laser pulsing of singly charged semiconductor quantum dots in an external magnetic field leads to a synchronization of the spin dynamics with the optical excitation. The pumped electron spins partially rephase prior to each laser pulse, causing a revival of electron spin polarization with its maximum at the incidence time of a laser pulse. The amplitude of this revival is amplified by the frequency focusing of the surrounding nuclear spins. Two complementary theoretical approaches for simulating up to 20 million laser pulses are developed and employed that are able to bridge between 11 orders of magnitude in time: a fully quantum mechanical description limited to small nuclear bath sizes and a technique based on the classical equations of motion applicable for a large number of nuclear spins. We present experimental data of the nonmonotonic revival amplitude as function of the magnetic field applied perpendicular to the optical axis. The dependence of the revival amplitude on the external field with a profound minimum at $4\;$T is reproduced by both of our theoretical approaches and is ascribed to the nuclear Zeeman effect. Since the nuclear Larmor precession determines the electronic resonance condition, it also defines the number of electron spin revolutions between pump pulses, the orientation of the electron spin at the incidence time of a pump pulse, and the resulting revival amplitude. The magnetic field of $4\;$T, for example, corresponds to half a revolution of nuclear spins between two laser pulses.

cond-mat.mes-hall↗

arXiv2018

Non-trivial topology of the quasi-one-dimensional triplons in the quantum antiferromagnet ${\text{BiCu}}_{2}{\text{PO}}_{6}$

Topological properties of physical systems are attracting tremendous interest. Recently, magnetic solid state compounds with and without magnetic order have become a focus. We show that ${\text{BiCu}}_{2}{\text{PO}}_{6}$ is the first gapful quantum antiferromagnet with a finite Zak phase, which characterises one-dimensional systems, and only the second with topological non-trivial triplon excitations. Surprisingly, in spite of the bulk-boundary correspondence no localised edge mode occurs. This unexpected behaviour is explained by the distinction between direct and indirect gaps among the triplon bands.

cond-mat.str-el↗

arXiv2018

Positivity of the spectral densities of retarded Floquet Green functions

Periodically driven nonequilibrium many-body systems are interesting because they have a quasi-energy spectra, which can be tailored by controlling the external driving fields. We derive the general spectral representation of retarded Green functions in the Floquet regime, thereby generalizing the well-known Lehmann representation from equilibrium many-body physics. The derived spectral Floquet representation allows us to prove the nonnegativity of spectral densities and to determine exact spectral sum rules, which can be employed to benchmark the accuracy of approximations to the exact Floquet many-body Green functions.

cond-mat.str-el↗

arXiv2018

Emergence of Floquet Behavior for Lattice Fermions Driven by Light Pulses

As many-body Floquet theory becomes more popular, it is important to find ways to connect theory with experiment. Theoretical calculations can have a periodic driving field that is always on, but experiment cannot. Hence, we need to know how long a driving field is needed before the system starts to look like the periodically driven Floquet system. We answer this question here for noninteracting band electrons in the infinite-dimensional limit by studying the properties of the system under pulsed driving fields and illustrating how they approach the Floquet limit. Our focus is on determining the minimal pulse lengths needed to recover the qualitative and semiquantitative Floquet theory results.

cond-mat.str-el↗

arXiv2018

Comparison of the Iterated Equation of Motion Approach and the Density Matrix Formalism for the Quantum Rabi Model

The density matrix formalism and the equation of motion approach are two semi-analytical methods that can be used to compute the non-equilibrium dynamics of correlated systems. While for a bilinear Hamiltonian both formalisms yield the exact result, for any non-bilinear Hamiltonian a truncation is necessary. Due to the fact that the commonly used truncation schemes differ for these two methods, the accuracy of the obtained results depends significantly on the chosen approach. In this paper, both formalisms are applied to the quantum Rabi model. This allows us to compare the approximate results and the exact dynamics of the system and enables us to discuss the accuracy of the approximations as well as the advantages and the disadvantages of both methods. It is shown to which extent the results fulfill physical requirements for the observables and which properties of the methods lead to unphysical results.

cond-mat.str-el↗

arXiv2018

Nuclear frequency focusing in periodically pulsed semiconductor quantum dots described by infinite classical central spin models

The coherence of an electronic spin in a semiconductor quantum dot decays due to its interaction with the bath of nuclear spins in the surrounding isotopes. This effect can be reduced by subjecting the system to an external magnetic field and by applying optical pulses. By repeated pulses in long trains the spin precession can be synchronized to the pulse period $T_\text{R}$. This drives the nuclear spin bath into states far from equilibrium leading to nuclear frequency focusing. In this paper, we use an efficient classical approach introduced in Phys. Rev. B $\textbf{96}$, 054415 (2017) to describe and to analyze this nuclear focusing. Its dependence on the effective bath size and on the external magnetic field is elucidated in a comprehensive study. We find that the characteristics of the pulse as well as the nuclear Zeeman effect influence the behavior decisively.

cond-mat.mes-hall↗

arXiv2018

Quantum mechanical treatment of large spin baths

The electronic spin in quantum dots can be described by central spin models (CSMs) with a very large number $N_\mathrm{eff} \approx 10^4$ to $10^6$ of bath spins posing a tremendous challenge to theoretical simulations. Here, a fully quantum mechanical theory is developed for the limit $N_\mathrm{eff} \to \infty$ by means of iterated equations of motion (iEoM). We find that the CSM can be mapped to a four-dimensional impurity coupled to a non-interacting bosonic bath in this limit. Remarkably, even for infinite bath the CSM does not become completely classical. The data obtained by the proposed iEoM approach is tested successfully against data from other, established approaches. Thus, the iEoM mapping extends the set of theoretical tools which can be used to understand the spin dynamics in large CSMs.

quant-ph↗

arXiv2018

Strong quenches in the one-dimensional Fermi-Hubbard model

The one-dimensional Fermi-Hubbard model is used as testbed for strong global parameter quenches. With the aid of iterated equations of motion in combination with a suitable scalar product for operators we describe the dynamics and the long-term behavior in particular of the system after interaction quenches. This becomes possible because the employed approximation allows for oscillatory dynamics avoiding spurious divergences. The infinite-time behavior is captured by an analytical approach based on stationary phases; no numerical averages over long times need to be computed. We study the most relevant frequencies in the dynamics after the quench and find that the local interaction $U$ as well as the band width $W$ dominate. In contrast to former studies a crossover instead of a sharp dynamical transition depending on the strength of the quench is identified. For weak quenches the band width is more important while for strong quenches the local interaction $U$ dominates.

cond-mat.str-el↗

arXiv2017

Quantum model for mode locking in pulsed semiconductor quantum dots

Quantum dots in GaAs/InGaAs structures have been proposed as a candidate system for realizing quantum computing. The short coherence time of the electronic quantum state that arises from coupling to the nuclei of the substrate is dramatically increased if the system is subjected to a magnetic field and to repeated optical pulsing. This enhancement is due to mode locking: Oscillation frequencies resonant with the pulsing frequencies are enhanced, while off-resonant oscillations eventually die out. Because the resonant frequencies are determined by the pulsing frequency only, the system becomes immune to frequency shifts caused by the nuclear coupling and by slight variations between individual quantum dots. The effects remain even after the optical pulsing is terminated. In this work, we explore the phenomenon of mode locking from a quantum mechanical perspective. We treat the dynamics using the central spin model, which includes coupling to 10-20 nuclei and incoherent decay of the excited electronic state, in a perturbative framework. Using scaling arguments, we extrapolate our results to realistic system parameters. We find that the synchronization to the pulsing frequency needs time scales in the order of 1 s.

cond-mat.mes-hall↗