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Götz Seibold

Publications and source records attributed to Götz Seibold.

6 recordsLinked to original sources

Influence of electronic correlations on disorder-induced loop currents in high-Tc superconductors

Time-reversal symmetry breaking in superconducting systems can manifest itself in the form of currents which are induced by inhomogeneities in the charge and order parameter distribution. With regard to cuprates such states have been theoretically studied in the overdoped region of the phase diagram where the inhomogeneities are related to out-of plane dopants. In this paper we will extend previous work by including local correlations within the unrestricted Gutzwiller approximation in order to study its impact on the induced loop currents. In addition, we investigate the effect of next-nearest neighbor hopping which extends the TRSB phase towards half-filling. We find that in general correlations lead to a suppression of loop currents, however, the Gutzwiller approach can sustain such states to larger values of the local on-site repulsion as compared to the Hartree-Fock approximation. Our investigations allow for an estimation of the local magnetic moment emerging from impurity-induced loop currents for cuprate superconductors.

cond-mat.supr-con↗

The charge density fluctuations and the Shrinking Fermi Liquid scenario for strange metallicity in cuprates

We interpret the strange metal (SM) properties of slightly overdoped cuprates in terms of the recently proposed Shrinking Fermi Liquid theory. This is based on the pervading presence in the cuprate phase diagram of charge density fluctuations (CDF), which have been identified and characterized in RIXS. These fluctuations are abundant and have a low energy due to the proximity of the charge density wave quantum critical point hidden under the superconducting dome of cuprates, but have a short range and non-critical character with a finite energy M/γ~10 meV as measured above Tc. Here M~ ξ^-2 is determined by the short correlation length ξ, while γencodes the Landau damping ruling the lifetime of the charge fluctuations. Besides these low energy CDF, cuprates also display phonons and a broad continuum of particle-hole excitations, mostly due to spin paramagnons arising from their strongly correlated character. With these experimentally characterized ingredients we show that above Tc the SM properties in transport are well described in terms of fermionic Landau quasiparticles scattering with CDF and phonons. The optical properties can instead be interpreted by the combined effect of low energy CDF determining the temperature dependence, and of the paramagnon continuum determining a linear in frequency scattering rate. Remarkably, the combined effect of these simple ingredients also induces ω/T scaling properties for frequencies larger than M/γ. When superconductivity is suppressed by strong magnetic fields the SM properties extend down to a few Kelvin. By assuming that the CDF dissipation parameter γgrows logarithmically by lowering T, we account for all anomalous transport and thermodynamic properties of cuprates (specific heat, Seebeck, heat transport, resistivity, and magnetoresistance) thereby providing a consistent scenario for the SM phase of cuprates.

cond-mat.str-el↗

Unveiling the Interplay of Charge and Magnetic Excitations in HgBa$_2$Ca$_2$Cu$_3$O$_{8+δ}$

Unraveling the mechanism that binds electrons into Cooper pairs in cuprate high-temperature superconductors remains one of the most fundamental challenges in condensed-matter physics. While both magnetic interactions and lattice vibrations are known to govern key electronic properties, their possible cooperation has never been directly observed. We investigate HgBa$_2$Ca$_2$Cu$_3$O$_{8+δ}$ (Hg1223) - the cuprate with the highest $T_{\mathrm{c}}$ at ambient pressure - as a magnifying glass to probe the possible entwining of the excitations at the core of the pairing. Using resonant inelastic X-ray scattering, we find that the charge response is dominated by dynamic charge density fluctuations (CDF) extending up to several hundred meV, where magnetic excitations reside. At the same momentum where CDF are most intense, the paramagnon energy exhibits a pronounced softening, revealing a strong interplay among charge, lattice, and spin excitations. Our results point to a cooperative mechanism in which dynamic charge fluctuations mediate the coupling between lattice, charge and spin degrees of freedom-shedding new light on the fundamental origin of high-$T_{\mathrm{c}}$ superconductivity.

cond-mat.supr-con↗

Boosting superconductivity in ultrathin YBa$_2$Cu$_3$O$_{7-δ}$ films via nanofaceted substrates

In cuprate high-temperature superconductors the doping level is fixed during synthesis, hence the charge carrier density per CuO$_2$ plane cannot be easily tuned by conventional gating, unlike in 2D materials. Strain engineering has recently emerged as a powerful tuning knob for manipulating the properties of cuprates, in particular charge and spin orders, and their delicate interplay with superconductivity. In thin films, additional tunability can be introduced by the substrate surface morphology, particularly nanofacets formed by substrate surface reconstruction. Here we show a remarkable enhancement of the superconducting onset temperature $T_{\mathrm{c}}^{\mathrm{on}}$ and the upper critical magnetic field $H_{c,2}$ in nanometer-thin YBa$_2$Cu$_3$O$_{7-δ}$ films grown on a substrate with a nanofaceted surface. We theoretically show that the enhancement is driven by electronic nematicity and unidirectional charge density waves, where both elements are captured by an additional effective potential at the interface between the film and the uniquely textured substrate. Our findings show a new paradigm in which substrate engineering can effectively enhance the superconducting properties of cuprates. This approach opens an exciting frontier in the design and optimization of high-performance superconducting materials.

cond-mat.supr-con↗

Phase separation and proximity effects in itinerant ferromagnet-superconductor heterostructures

Heterostructures made of itinerant ferromagnets and superconductors are studied. In contrast to most previous models, ferromagnetism is not enforced as an external Zeeman field but induced in a correlated single-band model (CSBM) that displays itinerant ferromagnetism as a mean-field ground state. This allows us to investigate the influence of an adjacent superconducting layer on the properties of the ferromagnet in a self-consistent Bogoliubov-de Gennes approach. The CSBM displays a variety features not present in the Zeeman exchange model that influence the behavior of order parameters close to the interface, as e.g. phase separation and the competition between magnetism and superconducting orders.

cond-mat.supr-con↗

Charge and pairing dynamics in the attractive Hubbard model: mode coupling and the validity of linear-response theory

Pump-probe experiments have turned out as a powerful tool in order to study the dynamics of competing orders in a large variety of materials. The corresponding analysis of the data often relies on standard linear-response theory generalized to non-equilibrium situations. Here we examine the validity of such an approach within the attractive Hubbard model for which the dynamics of pairing and charge-density wave orders is computed using the time-dependent Hartree-Fock approximation (TDHF). Our calculations reveal that the `linear-response assumption' is justified for small to moderate non-equilibrium situations (i.e., pump pulses) when the symmetry of the pump-induced state differs from that of the external field. This is the case, when we consider the pairing response in a charge-ordered state or the charge-order response in a superconducting state. The situation is very different when the non-equilibrium state and the external probe field have the same symmetry. In this case, we observe significant changes of the response in magnitude but also due to mode coupling when moving away from an equilibrium state, indicating the failure of the linear-response assumption.

cond-mat.str-el↗