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G. Álvarez-Pérez

Publications and source records attributed to G. Álvarez-Pérez.

4 recordsLinked to original sources

Ultraconfined THz Phonon Polaritons in Hafnium Dichalcogenides

The confinement of electromagnetic radiation to subwavelength scales relies on strong light-matter interactions. In the infrared (IR) and terahertz (THz) spectral ranges, phonon polaritons are commonly employed to achieve extremely subdiffractional light confinement, with much lower losses as compared to plasmon polaritons. Among these, hyperbolic phonon polaritons in anisotropic materials offer a highly promising platform for light confinement, which, however, typically plateaus at values of λ0/100, with λ0 being the free-space incident wavelength. In this study, we report on ultraconfined phonon polaritons in hafnium-based dichalcogenides with confinement factors exceeding λ0/250 in the terahertz spectral range. This extreme light compression within deeply sub-wavelength thin films is enabled by the unprecedented magnitude of the light-matter coupling strength in these compounds, and the natural hyperbolicity of HfSe2 in particular. Our findings emphasize the critical role of light-matter coupling for polariton confinement, which for phonon polaritons in polar dielectrics is dictated by the transverse-longitudinal optic phonon energy splitting. Our results demonstrate transition metal dichalcogenides as an enabling platform for THz nanophotonic applications that push the limits of light control.

physics.optics↗

Unidirectional Ray Polaritons in Twisted Asymmetric Stacks

The vast repository of van der Waals (vdW) materials supporting polaritons offers numerous possibilities to tailor electromagnetic waves at the nanoscale. The development of twistoptics - the modulation of the optical properties by twisting stacks of vdW materials - enables directional propagation of phonon polaritons (PhPs) along a single spatial direction, known as canalization. Here we demonstrate a complementary type of directional propagation of polaritons by reporting the visualization of unidirectional ray polaritons (URPs). They arise naturally in twisted hyperbolic stacks with very different thicknesses of their constituents, demonstrated for homostructures of $α$-MoO$_3$ and heterostructures of $α$-MoO$_3$ and $β$-Ga$_2$O$_3$. Importantly, their ray-like propagation, characterized by large momenta and constant phase, is tunable by both the twist angle and the illumination frequency. Apart from their fundamental importance, our findings introduce twisted asymmetric stacks as efficient platforms for nanoscale directional polariton propagation, opening the door for applications in nanoimaging, (bio)-sensing or polaritonic thermal management.

physics.optics↗

Multiple and spectrally robust photonic magic angles in reconfigurable α-MoO3 trilayers

The assembling of twisted stacks of van der Waals (vdW) materials had led to the discovery of a profusion of remarkable physical phenomena in recent years, as it provides a means to accurately control and harness electronic band structures. This has given birth to the so-called field of twistronics. An analogous concept has been developed for highly confined polaritons, or nanolight, in twisted bilayers of strongly anisotropic vdW materials, extending the field to the twistoptics realm. In this case, the emergence of a topological transition of the polaritonic dispersion at a given twist angle (photonic magic angle) results in the propagation of nanolight along one specific direction (canalization regime), holding promises for unprecedented control of the flow of energy at the nanoscale. However, there is a fundamental limitation in twistoptics that critically impedes such control: there is only one photonic magic angle (and thus canalization direction) in a twisted bilayer and it is fixed for each incident frequency. Here, we overcome this limitation by demonstrating the existence of multiple spectrally robust photonic magic angles in reconfigurable twisted vdW trilayers. As a result, we show that canalization of nanolight can be programmed at will along any desired in-plane direction in a single device, and, importantly, within broad spectral ranges of up to 70 cm-1. Our findings lay the foundation for robust and widely tunable twistoptics, opening the door for applications in nanophotonics where on-demand control of energy at the nanoscale is crucial, such as thermal management, nanoimaging or entanglement of quantum emitters.

physics.optics↗

Planar nano-optics in anisotropic media: anomalous refraction and diffraction-free lensing of highly confined polaritons

As one of the most fundamental optical phenomena, refraction between isotropic media is characterized by light bending towards the normal to the boundary when passing from a low- to a high-refractive-index medium. However, in anisotropic media, refraction is a much more exotic phenomenon. The most general case of refraction between two anisotropic media remains unexplored, particularly in natural media and at the nanoscale. Here, we visualize and comprehensively study refraction of electromagnetic waves between two strongly anisotropic (hyperbolic) media, and, importantly, we do it with the use of polaritons confined to the nanoscale in a low-loss natural medium, alpha-MoO3. Our images show refraction of polaritons under the general case in which both the direction of propagation and the wavevector are not collinear. As they traverse planar nanoprisms tailored in alpha-MoO3, refracted polaritons exhibit non-intuitive directions of propagation, enabling us to unveil an exotic optical effect: bending-free refraction. Furthermore, we succeed in developing the first in-plane refractive hyperlens, which yields foci as small as lamdap/6, being lamdap the polariton wavelength (lamda0/50 with respect to the wavelength of light in free space). Our results set the grounds for planar nano-optics in strongly anisotropic media, with potential for unprecedented control of the flow of energy at the nanoscale.

physics.optics↗