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G. A. Souliotis

Publications and source records attributed to G. A. Souliotis.

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Heavy Residue Isoscaling as a Probe of the Process of N/Z Equilibration

The isotopic and isobaric scaling behavior of the yield ratios of heavy projectile residues from the collisions of 25 MeV/nucleon 86Kr projectiles on 124Sn and 112Sn targets is investigated and shown to provide information on the process of N/Z equilibration occurring between the projectile and the target. The logarithmic slopes $α$ and $β^{'}$ of the residue yield ratios with respect to residue neutron number N and neutron excess N--Z are obtained as a function of the atomic number Z and mass number A, respectively, whereas excitation energies are deduced from velocities. The relation of the isoscaling parameters $α$ and $β^{'}$ with the N/Z of the primary (excited) projectile fragments is employed to gain access to the degree of N/Z equilibration prior to fragmentation as a function of excitation energy. A monotonic relation between the N/Z difference of fragmenting quasiprojectiles and their excitation energy is obtained indicating that N/Z equilibrium is approached at the highest observed excitation energies. Simulations with a deep-inelastic transfer model are in overall agreement with the isoscaling conclusions. The present residue isoscaling approach to N/Z equilibration offers an attractive tool of isospin and reaction dynamics studies in collisions involving beams of stable or rare isotopes.

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Isoscaling in Peripheral Nuclear Collisions around the Fermi Energy and a Signal of Chemical Separation from its Excitation Energy Dependence

The isoscaling is investigated using the fragment yield data from fully reconstructed quasi-projectiles observed in peripheral collisions of 28Si with 124,112Sn at projectile energies 30 and 50 MeV/nucleon. The excitation energy dependence of the isoscaling parameter beta_prime is observed which is independent of beam energy. For a given quasi-projectile produced in reactions with different targets no isoscaling is observed. The isoscaling thus reflects the level of N/Z-equilibration in reactions with different targets represented by the initial quasi-projectile samples. The excitation energy dependence of the isoscaling parameter beta_prime, corrected for the trivial 1/T temperature dependence, does not follow the trend of the homogeneous system above 4 MeV/nucleon thus possibly signaling the onset of separation into isospin asymmetric dilute and isospin symmetric dense phase.

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Effect of neutron composition and excitation energy of primary fragments on isospin observables in multifragmentation

The isospin properties of primary and secondary fragments produced in multifragmentation of Fe + Ni and Fe + Fe systems with respect to Ni + Ni system are analyzed within the statistical multifragmentation model framework. The reduced neutron and proton densities show an asymmetry in the primary fragments, that is lessened after secondary decay. with increasing isospin (N/Z) this effect increases, while the sensitivity of fragment isospin towards excitation energy and N/Z of the primary fragments remains unchanged.

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Effect of Shell Structure on Fission Isoscaling

Recently, the fragment yield ratios were investigated in the fission of 238,233U targets induced by 14 MeV neutrons [1]. The effect of the deformed shell structure around N=64 on the dynamics of scission was suggested as an explanation of the observed breakdown of the isoscaling behavior. As an alternative explanation, the effect of binding energy of final fragments, in particular the neutron shell closure of the complementary fragment around N=82, was suggested by Friedman [2]. When applying that concept consistently, the observed two breakdowns of the isoscaling behavior around N=62 and N=80 signal the effect of two shell closures (N=82 and N=64) on the dynamics of scission. To separate the two effects, we examine the isoscaling plots obtained using fission fragment yield data from the spontaneous fission of the heavier nuclei 248,244Cm and find that the breakdown of isoscaling around N=64 persists even if it can not be related to shell closure of the complementary fragment and thus it manifests the effect of the deformed shell structure in the scission configuration.

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Isotopic Scaling of Heavy Projectile Residues from the collisions of 25 MeV/nucleon 86Kr with 124Sn, 112Sn and 64Ni, 58Ni

The scaling of the yields of heavy projectile residues from the reactions of 25 MeV/nucleon 86Kr projectiles with 124Sn,112Sn and 64Ni, 58Nitargets is studied. Isotopically resolved yield distributions of projectile fragments in the range Z=10-36 from these reaction pairs were measured with the MARS recoil separator in the angular range 2.7-5.3 degrees. The velocities of the residues, monotonically decreasing with Z down to Z~26-28, are employed to characterize the excitation energy. The yield ratios R21(N,Z) for each pair of systems are found to exhibit isotopic scaling (isoscaling), namely, an exponential dependence on the fragment atomic number Z and neutron number N. The isoscaling is found to occur in the residue Z range corresponding to the maximum observed excitation energies. The corresponding isoscaling parameters are alpha=0.43 and beta=-0.50 for the Kr+Sn system and alpha=0.27 and beta=-0.34 for the Kr+Ni system. For the Kr+Sn system, for which the experimental angular acceptance range lies inside the grazing angle, isoscaling was found to occur for Z<26 and N<34. For heavier fragments from Kr+Sn, the parameters vary monotonically, alpha decreasing with Z and beta increasing with N. This variation is found to be related to the evolution towards isospin equilibration and, as such, it can serve as a tracer of the N/Z equilibration process. The present heavy-residue data extend the observation of isotopic scaling from the intermediate mass fragment region to the heavy-residue region. Such high-resolution mass spectrometric data can provide important information on the role of isospin in peripheral and mid-peripheral collisions, complementary to that accessible from modern large-acceptance multidetector devices.

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Heavy Residues with A<90 in the Asymmetric Reaction of 20 AMeV 124Sn+27Al as a Sensitive Probe of the Onset of Multifragmentation

The cross sections and velocity distributions of heavy residues from the reaction of 20 AMeV 124Sn + 27Al have been measured at forward angles using the MARS recoil separator at Texas A&M in a wide mass range. A consistent overall description of the measured cross sections and velocity distributions was achieved using a model calculation employing the concept of deep-inelastic transfer for the primary stage of peripheral collisions, pre-equilibrium emission and incomplete fusion for the primary stage of more violent central collisions and the statistical model of multifragmentation (SMM code) for the deexcitation stage. An alternative calculation employing the sequential binary decay (GEMINI code) could not reproduce the observed yields of the residues from violent collisions (A<90) due to different kinematic properties. The success of SMM demonstrates that the heavy residues originate from events where a competition of thermally equilibrated fragment partitions takes place rather than a sequence of binary decays.

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Enhanced Production of Neutron-Rich Rare Isotopes in Peripheral Collisions at Fermi Energies

A large enhancement in the production of neutron-rich projectile residues is observed in the reactions of a 25 MeV/nucleon 86Kr beam with the neutron rich 124Sn and 64Ni targets relative to the predictions of the EPAX parametrization of high-energy fragmentation, as well as relative to the reaction with the less neutron-rich 112Sn target. The data demonstrate the significant effect of the target neutron-to-proton ratio (N/Z) in peripheral collisions at Fermi energies. A hybrid model based on a deep-inelastic transfer code (DIT) followed by a statistical de-excitation code appears to account for part of the observed large cross sections. The DIT simulation indicates that the production of the neutron-rich nuclides in these reactions is associated with peripheral nucleon exchange. In such peripheral encounters, the neutron skins of the neutron-rich 124Sn and 64Ni target nuclei may play an important role. From a practical viewpoint, such reactions between massive neutron-rich nuclei offer a novel and attractive synthetic avenue to access extremely neutron-rich rare isotopes towards the neutron-drip line.

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Enhanced Production of Neutron-Rich Rare Isotopes in the Reaction of 25 MeV/nucleon Kr-86 on Ni-64

The cross sections and velocity distributions of projectile-like fragments from the reaction of 25 MeV/nucleon 86Kr + 64Ni have been measured using the MARS recoil separator at Texas A&M, with special emphasis on the neutron rich isotopes. Proton-removal and neutron pick-up isotopes have been observed with large cross sections. A model of deep-inelastic transfer (DIT) for the primary interaction stage and the statistical evaporation code GEMINI for the deexcitation stage have been used to describe the properties of the product distributions. The results have also been compared with the EPAX parametrization of high-energy fragmentation yields. The experimental data show an enhancement in the production of neutron-rich isotopes close to the projectile, relative to the predictions of DIT/GEMINI and the expectations of EPAX. We attribute this enhancement mainly to the effect of the extended neutron distribution (neutron ``skin'') of the 64Ni target in peripheral interactions of 86Kr with 64Ni. The large cross sections of such reactions near the Fermi energy, involving peripheral nucleon exchange, suggest that, not only the N/Z of the projectile and the target, but also the N/Z distribution at the nuclear surface may properly be exploited in the production of neutron-rich rare isotopes. This synthesis approach may offer a fruitful pathway to extremely neutron-rich nuclei, towards the neutron-drip line.

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Studies of reaction dynamics in the Fermi energy domain

An overview of recent results on reaction dynamics in the energy region 20 - 50 A.MeV is given. The results of the study of projectile multifragmentation using the detector array FAUST are presented. Reaction mechanism is determined and thermodynamical properties of the hot quasiprojectile are investigated. Preliminary results on fragment isospin asymmetry obtained using the 4$π$ detector array NIMROD are given. Procedure for selecting centrality in two-dimensional multiplicity histograms is described. Possibility to extract thermodynamical temperature from systematics of isotope ratios is investigated. Reaction mechanism leading to production of hot sources is discussed. Furthermore, the possibilities for production of rare isotopes are discussed and recent experimental results obtained using recoil separator MARS are presented.

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Heavy Residue Formation in 20 MeV/nucleon 197Au + 90Zr collisions

The yields and velocity distributions of heavy residues and fission fragments from the reaction of 20 MeV/nucleon 197Au + 90Zr have been measured using the MSU A1200 fragment separator. A bimodal distribution of residues is observed, with one group, resulting from peripheral collisions, having fragment mass numbers A=160-200, while the other group, resulting from ``hard'' collisions, has A=120-160. This latter group of residues can be distinguished from fission fragments by their lower velocities. A model combining deep-inelastic transfer and incomplete fusion for the primary interaction stage and a statistical evaporation code for the deexcitation stage has been used to describe the properties of the product distributions.

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