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G. D. Gu

Publications and source records attributed to G. D. Gu.

At least 145 records · Page 8Linked to original sources

FeTe$_{0.55}$Se$_{0.45}$: a multiband superconductor in the clean and dirty limit

The detailed optical properties of the multiband iron-chalcogenide superconductor FeTe$_{0.55}$Se$_{0.45}$ have been reexamined for a large number of temperatures above and below the critical temperature $T_c=14$ K for light polarized in the a-b planes. Instead of the simple Drude model that assumes a single band, above $T_c$ the normal-state optical properties are best described by the two-Drude model that considers two separate electronic subsystems; we observe a weak response ($ω_{p,D;1}\simeq 3000$ cm$^{-1}$) where the scattering rate has a strong temperature dependence ($1/τ_{D,1}\simeq 32$ cm$^{-1}$ for $T \gtrsim T_c$), and a strong response ($ω_{p,D;2}\simeq 14\,500$ cm$^{-1}$) with a large scattering rate ($1/τ_{D,2}\simeq 1720$ cm$^{-1}$) that is essentially temperature independent. The multiband nature of this material precludes the use of the popular generalized-Drude approach commonly applied to single-band materials, implying that any structure observed in the frequency dependent scattering rate $1/τ(ω)$ is spurious and it cannot be used as the foundation for optical inversion techniques to determine an electron-boson spectral function $α^2 F(ω)$. Below $T_c$ the optical conductivity is best described using two superconducting optical gaps of $2Δ_1\simeq 45$ and $2Δ_2 \simeq 90$ cm$^{-1}$ applied to the strong and weak responses, respectively. The scattering rates for these two bands are vastly different at low temperature, placing this material simultaneously in both clean and dirty limit. Interestingly, this material falls on the universal scaling line initially observed for the cuprate superconductors.

cond-mat.supr-con↗

Dependence of superconductivity in CuxBi2Se3 on quenching conditions

Topological superconductivity, implying gapless protected surface states, has recently been proposed to exist in the compound CuxBi2Se3. Unfortunately, low diamagnetic shielding fractions and considerable inhomogeneity have been reported in this compound. In an attempt to understand and improve on the finite superconducting volume fractions, we have investigated the effects of various growth and post-annealing conditions. With a melt-growth (MG) method, diamagnetic shielding fractions of up to 56% in Cu0.3Bi2Se3 have been obtained, the highest value reported for this method. We investigate the efficacy of various quenching and annealing conditions, finding that quenching from temperatures above 560C is essential for superconductivity, whereas quenching from lower temperatures or not quenching at all is detrimental. A modified floating zone (FZ) method yielded large single crystals but little superconductivity. Even after annealing and quenching, FZ-grown samples had much less chance of being superconducting than MG-grown samples. From the low shielding fractions in FZ-grown samples and the quenching dependence, we suggest that a metastable secondary phase having a small volume fraction in most of the samples may be responsible for the superconductivity.

cond-mat.supr-con↗

Melting of Charge Stripes in Vibrationally Driven La1.875Ba0.125CuO4: Assessing the Respective Roles of Electronic and Lattice Order in Frustrated Superconductors

We report femtosecond resonant soft X-ray diffraction measurements of the dynamics of the charge order and of the crystal lattice in non-superconducting, stripe-ordered La1.875Ba0.125CuO4. Excitation of the in-plane Cu-O stretching phonon with a mid-infrared pulse has been previously shown to induce a transient superconducting state in the closely related compound La1.675Eu0.2Sr0.125CuO4. In La1.875Ba0.125CuO4, we find that the charge stripe order melts promptly on a sub-picosecond time scale. Surprisingly, the low temperature tetragonal distortion is only weakly reduced, reacting on significantly longer time scales that do not correlate with light-induced superconductivity. This experiment suggests that charge modulations alone, and not the LTT distortion, prevent superconductivity in equilibrium.

cond-mat.supr-con↗

Observation of the chiral magnetic effect in ZrTe5

The chiral magnetic effect is the generation of electric current induced by chirality imbalance in the presence of magnetic field. It is a macroscopic manifestation of the quantum anomaly in relativistic field theory of chiral fermions (massless spin $1/2$ particles with a definite projection of spin on momentum) -- a dramatic phenomenon arising from a collective motion of particles and antiparticles in the Dirac sea. The recent discovery of Dirac semimetals with chiral quasi-particles opens a fascinating possibility to study this phenomenon in condensed matter experiments. Here we report on the first observation of chiral magnetic effect through the measurement of magneto-transport in zirconium pentatelluride, ZrTe_5. Our angle-resolved photoemission spectroscopy experiments show that this material's electronic structure is consistent with a 3D Dirac semimetal. We observe a large negative magnetoresistance when magnetic field is parallel with the current. The measured quadratic field dependence of the magnetoconductance is a clear indication of the chiral magnetic effect. The observed phenomenon stems from the effective transmutation of Dirac semimetal into a Weyl semimetal induced by the parallel electric and magnetic fields that represent a topologically nontrivial gauge field background.

cond-mat.str-el↗

Evidence for a New Excitation at the Interface Between a High-Tc Superconductor and a Topological Insulator

High-temperature superconductors exhibit a wide variety of novel excitations. If contacted with a topological insulator, the lifting of spin rotation symmetry in the surface states can lead to the emergence of unconventional superconductivity and novel particles. In pursuit of this possibility, we fabricated high critical-temperature (Tc ~ 85 K) superconductor/topological insulator (Bi2Sr2CaCu2O8+delta/Bi2Te2Se) junctions. Below 75 K, a zero-bias conductance peak (ZBCP) emerges in the differential conductance spectra of this junction. The magnitude of the ZBCP is suppressed at the same rate for magnetic fields applied parallel or perpendicular to the junction. Furthermore, it can still be observed and does not split up to at least 8.5 T. The temperature and magnetic field dependence of the excitation we observe appears to fall outside the known paradigms for a ZBCP.

cond-mat.supr-con↗

Imaging Dirac-Mass Disorder from Magnetic Dopant-Atoms in the Ferromagnetic Topological Insulator Cr$_x$(Bi$_{0.1}$Sb$_{0.9}$)$_{2-x}$Te$_3$

To achieve and utilize the most exotic electronic phenomena predicted for the surface states of 3D topological insulators (TI),it is necessary to open a "Dirac-mass gap" in their spectrum by breaking time-reversal symmetry. Use of magnetic dopant atoms to generate a ferromagnetic state is the most widely used approach. But it is unknown how the spatial arrangements of the magnetic dopant atoms influence the Dirac-mass gap at the atomic scale or, conversely, whether the ferromagnetic interactions between dopant atoms are influenced by the topological surface states. Here we image the locations of the magnetic (Cr) dopant atoms in the ferromagnetic TI Cr$_{0.08}$(Bi$_{0.1}$Sb$_{0.9}$)$_{1.92}$Te$_3$. Simultaneous visualization of the Dirac-mass gap $Δ(r)$ reveals its intense disorder, which we demonstrate directly is related to fluctuations in $n(r)$, the Cr atom areal density in the termination layer. We find the relationship of surface-state Fermi wavevectors to the anisotropic structure of $Δ(r)$ consistent with predictions for surface ferromagnetism mediated by those states. Moreover, despite the intense Dirac-mass disorder, the anticipated relationship $Δ(r)\propto n(r)$ is confirmed throughout, and exhibits an electron-dopant interaction energy $J^*$=145$meV\cdot nm^2$. These observations reveal how magnetic dopant atoms actually generate the TI mass gap locally and that, to achieve the novel physics expected of time-reversal-symmetry breaking TI materials, control of the resulting Dirac-mass gap disorder will be essential.

cond-mat.mtrl-sci↗

Observation of an electron band above the Fermi level in FeTe$_{0.55}$Se$_{0.45}$ from \emph{in-situ} surface doping

We used \emph{in-situ} potassium (K) evaporation to dope the surface of the iron-based superconductor FeTe$_{0.55}$Se$_{0.45}$. The systematic study of the bands near the Fermi level confirms that electrons are doped into the system, allowing us to tune the Fermi level of this material and to access otherwise unoccupied electronic states. In particular, we observe an electron band located above the Fermi level before doping that shares similarities with a small three-dimensional pocket observed in the cousin, heavily-electron-doped KFe$_{2-x}$Se$_2$ compound.

cond-mat.supr-con↗

Spectral weight transfer in strongly correlated Fe$_{1.03}$Te

The temperature dependence of the in-plane optical conductivity has been determined for Fe$_{1.03}$Te above and below the magnetic and structural transition at $T_N\simeq 68$ K. The electron and hole pockets are treated as two separate electronic subsystems; a strong, broad Drude response that is largely temperature independent, and a much weaker, narrow Drude response with a strong temperature dependence. Spectral weight is transferred from high to low frequency below $T_N$, resulting in the dramatic increase of both the low-frequency conductivity and the related plasma frequency. The change in the plasma frequency is due to an increase in the carrier concentration resulting from the closing of the pseudogap on the electron pocket, as well as the likely decrease of the effective mass in the antiferromagnetic state.

cond-mat.str-el↗

Nearly Perfect Fluidity in a High Temperature Superconductor

Perfect fluids are characterized as having the smallest ratio of shear viscosity to entropy density, η/s, consistent with quantum uncertainty and causality. So far, nearly perfect fluids have only been observed in the Quark-Gluon Plasma (QGP) and in unitary atomic Fermi gases (UFG), exotic systems that are amongst the hottest and coldest objects in the known universe, respectively. We use Angle Resolve Photoemission Spectroscopy (ARPES) to measure the temperature dependence of an electronic analogue of η/s in an optimally doped cuprate high temperature superconductor, finding it too is a nearly perfect fluid around, and above, its superconducting transition temperature Tc.

cond-mat.str-el↗

Optically induced superconductivity in striped La2-xBaxCuO4 by polarization-selective excitation in the near infrared

We show that superconducting interlayer coupling, which coexists with and is depressed by stripe order in La1.885Ba0.115CuO4, can be enhanced by excitation with near-infrared laser pulses. For temperatures lower than Tc = 13 K, we observe a blue-shift of the equilibrium Josephson plasma resonance, detected by terahertz-frequency reflectivity measurements. Key to this measurement is the ability to probe the optical properties at frequencies as low as 150 GHz, detecting the weak interlayer coupling strengths. For T > Tc a similar plasma resonance, absent at equilibrium, is induced up to the spin-ordering temperature TSO = 40 K. These effects are reminiscent but qualitatively different from the light-induced superconductivity observed by resonant phonon excitation in La1.675Eu0.2Sr0.125CuO6.5. Importantly, enhancement of the below-Tc interlayer coupling and its appearance above Tc are preferentially achieved when the near-infrared pump light is polarized perpendicular to the superconducting planes, likely due to more effective melting of stripe order and the less effective excitation of quasiparticles from the Cooper pair condensate when compared to in-plane excitation.

cond-mat.supr-con↗

Inhomogeneous slowing down of spin fluctuations induced by charge stripe order in 1/8-doped lanthanum cuprates

We report $^{139}$La nuclear magnetic resonance (NMR) measurements on La$_{2-x}$Sr$_x$CuO$_4$ ($0.07\leq x \leq 0.15$) and La$_{2-x}$Ba$_x$CuO$_4$ ($x=1/8$) single crystals, focusing on the spin freezing observed in 1/8-doped lanthanum cuprates. Charge stripe order seems to induce the inhomogeneous slowing down of spin fluctuations toward spin order and compete with superconductivity.

cond-mat.supr-con↗

Bulk Signatures of Pressure-Induced Band Inversion and Topological Phase Transitions in Pb$_{1-x}$Sn$_x$Se

The characteristics of topological insulators are manifested in both their surface and bulk properties, but the latter remain to be explored. Here we report bulk signatures of pressure-induced band inversion and topological phase transitions in Pb$_{1-x}$Sn$_x$Se ($x=$0.00, 0.15, and 0.23). The results of infrared measurements as a function of pressure indicate the closing and the reopening of the band gap as well as a maximum in the free carrier spectral weight. The enhanced density of states near the band gap in the topological phase give rise to a steep interband absorption edge. The change of density of states also yields a maximum in the pressure dependence of the Fermi level. Thus our conclusive results provide a consistent picture of pressure-induced topological phase transitions and highlight the bulk origin of the novel properties in topological insulators.

cond-mat.mtrl-sci↗

Superconductivity induced by In substitution into the topological crystalline insulator Pb(0.5)Sn(0.5)Te

Indium substitution turns the topological crystalline insulator (TCI) Pb$_{0.5}$Sn$_{0.5}$Te into a possible topological superconductor. To investigate the effect of the indium concentration on the crystal structure and superconducting properties of (Pb$_{0.5}$Sn$_{0.5}$)$_{1-x}$In$_{x}$Te, we have grown high-quality single crystals using a modified floating-zone method, and have performed systematic studies for indium content in the range $0\leq x\leq 0.35$. We find that the single crystals retain the rock salt structure up to the solubility limit of indium ($x\sim0.30$). Experimental dependences of the superconducting transition temperature ($T_c$) and the upper critical magnetic field ($H_{c2}$) on the indium content $x$ have been measured. The maximum $T_c$ is determined to be 4.7 K at $x=0.30$, with $μ_0H_{c2}(T=0)\approx 5$ T.

cond-mat.supr-con↗

Evolution from incoherent to coherent electronic states and its implications to superconductivity in FeTe1-xSex

We have performed systematic angle-resolved photoemission spectroscopy (ARPES) of iron-chalcogenide superconductor FeTe1-xSex to elucidate the electronic states relevant to the superconductivity. While the Fermi-surface shape is nearly independent of x, we found that the ARPES spectral line shape shows prominent x dependence. A broad ARPES spectrum characterized by a small quasiparticle weight at x = 0, indicative of incoherent electronic states, becomes progressively sharper with increasing x, and a well-defined quasiparticle peak appears around x = 0.45 where bulk superconductivity is realized. The present result suggests the evolution from incoherent to coherent electronic states and its close relationship to the emergence of superconductivity.

cond-mat.supr-con↗

Absence of a Proximity Effect in a Topological Insulator on a Cuprate Superconductor: Bi2Se3/Bi2Sr2CaCu2O8

Proximity-induced superconductivity in a 3D topological insulator represents a new avenue for observing zero-energy Majorana fermions inside vortex cores. Relatively small gaps and low transition temperatures of conventional s-wave superconductors put the hard constraints on these experiments. Significantly larger gaps and higher transition temperatures in cuprate superconductors might be an attractive alternative to considerably relax these constraints, but it is not clear whether the proximity effect would be effective in heterostructures involving cuprates and topological insulators. Here, we present angle-resolved photoemission studies of thin Bi2Se3 films grown in-situ on optimally doped Bi2Sr2CaCu2O8 substrates that show the absence of proximity-induced gaps on the surfaces of Bi2Se3 films as thin as a 1.5 quintuple layer. These results suggest that the superconducting proximity effect between a cuprate superconductor and a topological insulator is strongly suppressed, likely due to a very short coherence length along the c-axis, incompatible crystal and pairing symmetries at the interface, small size of the topological surface state Fermi surface and adverse effects of a strong spin-orbit coupling in the topological material.

cond-mat.supr-con↗

Power Law Like Correlation between Condensation Energy and Superconducting Transition Temperatures in Iron Pnictide/Chalcogenide Superconductors: Beyond the BCS Understanding

Superconducting condensation energy $U_0^{int}$ has been determined by integrating the electronic entropy in various iron pnictide/chalcogenide superconducting systems. It is found that $U_0^{int}\propto T_c^n$ with $n$ = 3 to 4, which is in sharp contrast to the simple BCS prediction $U_0^{BCS}=1/2N_FΔ_s^2$ with $N_F$ the quasiparticle density of states at the Fermi energy, $Δ_s$ the superconducting gap. A similar correlation holds if we compute the condensation energy through $U_0^{cal}=3γ_n^{eff}Δ_s^2/4π^2k_B^2$ with $γ_n^{eff}$ the effective normal state electronic specific heat coefficient. This indicates a general relationship $γ_n^{eff} \propto T_c^m$ with $m$ = 1 to 2, which is not predicted by the BCS scheme. A picture based on quantum criticality is proposed to explain this phenomenon.

cond-mat.supr-con↗

Evidence of Chiral Order in the Charge-Ordered Phase of Superconducting La1.875Ba0.125Cuo4 Single Crystals Using Polar Kerr-Effect Measurements

High resolution polar Kerr effect (PKE) measurements were performed on La1.875Ba0.125Cuo4 single crystals revealing that a finite Kerr signal is measured below an onset temperature-T_K that coincides with charge ordering transition temperature T_{CO}. We further show that the sign of the Kerr signal cannot be trained with magnetic field, is found to be the same of opposite sides of the same crystal, and is odd with respect to strain in the diagonal direction of the unit cell. These observations are consistent with a chiral "gyrotropic" order above T_c for La1.875Ba0.125Cuo4; similarities to other cuprates suggest that it is a universal property in the pseudogap regime.

cond-mat.str-el↗

Direct observation of dynamic charge stripes in La2-xSrxNiO4

The insulator-to-metal transition continues to be a challenging subject, especially when electronic correlations are strong. In layered compounds, such as La2-xSrxNiO4 and La2-xBaxCuO4, the doped charge carriers can segregate into periodically-spaced charge stripes separating narrow domains of antiferromagnetic order. Although there have been theoretical proposals of dynamically fluctuating stripes, direct spectroscopic evidence of charge-stripe fluctuations has been lacking. Here we report the detection of critical lattice fluctuations, driven by charge-stripe correlations, in La2-xSrxNiO4 using inelastic neutron scattering. This scattering is detected at large momentum transfers where the magnetic form factor suppresses the spin fluctuation signal. The lattice fluctuations associated with the dynamic charge stripes are narrow in q and broad in energy. They are strongest near the charge stripe melting temperature. Our results open the way towards the quantitative theory of dynamic stripes and for directly detecting dynamical charge stripes in other strongly-correlated systems, including high-temperature superconductors such as La2-xSrxCuO4.

cond-mat.str-el↗