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G. F. Grinyer

Publications and source records attributed to G. F. Grinyer.

At least 19 recordsLinked to original sources

Direct measurement of Enhanced octupole collectivity in 148Dy

Excited states in $^{148}_{~66}$Dy were populated via $β^+/EC$ decay of $^{148m}$Ho using the GRIFFIN spectrometer at the TRIUMF ISAC-I facility. A combined measurement of the mean lifetime of the $3_1^-$ level using the Generalized Centroid Difference (GCD) method and branching fraction of the $3_1^-\rightarrow0_1^+$ $γ$-ray decay has been performed. From these results, an enhanced electric octupole $B(E3;3_1^-\rightarrow0_1^+)$ transition strength of 46(3)~W.u. has been determined in $^{148}_{~66}$Dy. This is the largest measured value across the closed neutron shell at $N=82$ and provides direct evidence of enhanced octupole collectivity beyond $Z=64$. The evolution of the $B(E3; 3^-_1 \rightarrow 0^+_1)$ strength along the $N=82$ isotonic chain is compared with quasiparticle random-phase approximation (QRPA) calculations using the SkI3 and SkM$^*$ Skyrme energy-density functionals, as well as with large-scale shell-model (SM) calculations. This result extends the boundaries of enhanced octupole collectivity far from the so-called `octupole magic numbers' $Z=56$ and $N=88$.

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First observation of the fine structure of the Pygmy Dipole Resonance in a nucleus away from stability via the $β^-$ decay of $^{92}$Rb to $^{92}$Sr

A comprehensive $γ$-ray spectroscopy study of excited states in $^{92}$Sr populated via $β^-$ decay of $^{92}$Rb ($J^π=0^-$, $Q_β=8095(6)$~keV) was performed with the GRIFFIN spectrometer at the Isotope Separator and Accelerator (ISAC) radioactive ion beam facility at TRIUMF. The high $γ$-ray efficiency of the GRIFFIN spectrometer combined with the intense rubidium beams produced allowed for 864 $γ$-ray transitions to be placed in the level scheme with 190 excited levels populated, most of them identified for the first time. The excitation energies of low-spin states in $^{92}$Sr are well reproduced by large-scale Shell Model calculations up to 5~MeV. The $β$-feeding intensities are in very good agreement with results from a recent study employing Modular Total Absorption Spectroscopy, indicating a significant suppression of the Pandemonium effect. The experimental picture reveals the energy level dependence of log~$ft$ values in unprecedented detail. These log~$ft$ values are well reproduced by Multiple-Commutator Model calculations that identify the features in the excited levels' wavefunctions that enable the population of high-lying levels with a low effective Q-value that belong to the Pygmy Dipole Resonance.

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Independent Validation of Octupole Collectivity in radium-224 through lifetime measurements of low-lying negative-parity states

The nucleus $^{224}$Ra is a key benchmark for octupole deformation and for theoretical descriptions of enhanced Schiff moments in reflection-asymmetric nuclei. While Coulomb-excitation measurements have established strong octupole collectivity in $^{224}$Ra, theoretical models predict that its intrinsic electric-dipole moment should be strongly quenched by a cancellation between macroscopic and microscopic contributions. Direct fast-timing measurements of the low-lying $J^π= 1^-_1$ and $3^-_1$ states populated following the $β$-decay of $^{224}$Fr at TRIUMF-ISAC were performed. Using the LaBr$_3$(Ce) detectors of the GRIFFIN array, mean lifetimes of $τ(1^-_1) = 444(6)$~ps and $τ(3^-_1) = 460(18)$~ps were obtained. The corresponding reduced transition probabilities agree with values inferred from Coulomb excitation, but are determined with substantially improved precision. These results provide an independent validation of the electromagnetic matrix elements associated with octupole collectivity in $^{224}$Ra and confirm a strongly-quenched intrinsic dipole moment of $D_0 \simeq 0.032~e\mathrm{fm}$. The present measurements therefore provide a stringent experimental benchmark for nuclear-structure models used in the interpretation of Schiff moments and future searches for non-zero electric dipole moments.

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Quenching of the proton $\pi0p_{3/2}$-$\pi0p_{1/2}$ spin-orbit splitting in $^{20}$O and the effect of the tensor force

We present the first direct measurement of the Z=6 shell gap in the neutron-rich 20O nucleus. The one-proton removal transfer reaction 2H(20O,3He)19N has been studied using the ACTAR TPC setup at GANIL. The use of ACTAR TPC enabled the measurement of low-cross section proton-removal reactions while preserving resolution. Eight p-hole states with l=1 were identified in 19N accounting for total strengths of 86% and 72% of the 0p3/2 and 0p1/2 single-particle orbitals, respectively. The energies and spectroscopic factors of the measured states allowed to determine the proton spin-orbit splitting 0p3/2 - 0p1/2 in 20O. The Z=6 shell gap has been established to be 5.30(14) MeV. These findings indicate a reduction of the Z=6 shell gap while adding neutrons to the sd-valence orbitals, consistent with the effects of the tensor force predicted by state-of-the-art shell model interaction SFO-tls while at variance with the emergence of a large Z=6 gap observed in other studies.

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Direct measurement of $^{59}$Cu($p$,$α$)$^{56}$Ni precludes a strong NiCu cycle in Type-I X-ray bursts

Model-observation comparisons of type-I X-ray bursts (XRBs) can reveal the properties of accreting neutron star systems, including the neutron star compactness. XRBs are powered by nuclear burning and a handful of reactions have been shown to impact the model results. Reactions in the NiCu cycles, featuring a competition between $^{59}$Cu($p$,$γ$)$^{60}$Zn and $^{59}$Cu($p$,$α$)$^{56}$Ni, have been shown to be among the most important reactions as they are a critical checkpoint in $rp$-process flow and significantly impact the light curves and burst ashes. We report a direct measurement of $^{59}$Cu($p$,$α$)$^{56}$Ni bringing stringent constraints on this reaction rate. New results rule out a strong NiCu cycle in XRBs, with a negligible degree of recycling, $\leq$5\% up to 1.5 GK. The new reaction rate, when varied within new uncertainty limits, shows no impact on one-zone XRB model light-curves tailored for clocked-burster $\tt{GS 1826-24}$, hence removing an important nuclear physics uncertainty in the model-observation comparison.

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Unbound neutron $\nu0d_{3/2}$ strength in $^{17}$C and the N=16 shell gap

Significant continuum strength has been observed to be populated in $^{17}$C produced in the d($^{16}$C,p) reaction at a beam energy of 17.2~MeV/nucleon. The strength appears at greater than $\sim$2~MeV above the single-neutron decay threshold and has been identified as arising from transfer into the neutron $0d_{3/2}$ orbital. Guided by shell model predictions the greater majority of the strength is associated with a 3/2$^+$ state at an excitation energy of 4.40$_{-0.14}^{+0.33}$ MeV and a much weaker 3/2$^+$ level at 5.60$_{-0.45}^{+1.35}$ MeV. The corresponding total widths were determined to be 3.45$_{-0.78}^{+1.82}$ and 1.6$_{-1.4}^{+4.6}$ MeV, respectively. From the backward angle proton differential cross sections and the branching ratios for neutron decay to the $^{16}$C(2$_{1}^{+}$) level, the corresponding spectroscopic factors to the ground state were deduced to be 0.47$\pm{10}$ and $<$0.09. Shell-model calculations employing the phenomenological SFO-tls interaction as well as Gamow Shell-Model calculations including continuum effects are in reasonable agreement with experiment, although the predicted strength lies at somewhat lower energy. The size of the N=16 shell gap ($\varepsilon_{ \nu0d_{3/2}}-\varepsilon _{ν1s_{1/2}}$) was estimated to be 5.08$_{-0.33}^{+0.43}$~MeV - some 1.3~MeV larger than found in the SFO-tls shell model calculation.

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Investigation of the Excited States of $^{114}\mathrm{Sn}$ Using the GRIFFIN Spectrometer at TRIUMF

The semi-magic $^{110-122}\mathrm{Sn}$ isotopes display signs of shape coexistence in their excited $0^+$ states, which, in contrast to the spherical $0^+$ ground states, are deformed. This paper investigates the nuclear structure of $^{114}\mathrm{Sn}$ using the competing $β^+$ decay and electron capture of a radioactive beam of $^{114}\mathrm{Sb}$ produced at the TRIUMF-ISAC facility using the GRIFFIN spectrometer. This study will allow for an in-depth understanding of the excited $0^+$ states in $^{114}\mathrm{Sn}$, by focusing on their decay patterns. In the present experiment, transitions at 856.2-keV and 1405.0-keV, which were observed in an earlier $β^+$ decay study but not placed in the $^{114}\mathrm{Sn}$ level scheme, have been assigned to the level scheme in connection to the $0^+_3$ level at 2156.0-keV. Properly assigning these transitions refines the level scheme and enhances our understanding of the nuclear structure in $^{114}\mathrm{Sn}$.

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Cross-shell states in $^{15}$C: a test for p-sd interactions

The low-lying structure of $^{15}$C has been investigated via the neutron-removal $^{16}$C$(d,t)$ reaction. Along with bound neutron sd-shell hole states, unbound p-shell hole states have been firmly confirmed. The excitation energies and the deduced spectroscopic factors of the cross-shell states are an important measure of the $[(p)^{-1}(sd)^{2}]$ neutron configurations in $^{15}$C. Our results show a very good agreement with shell-model calculations using the SFO-tls interaction for $^{15}$C. However, a modification of the $p$-$sd$ and $sd$-$sd$ monopole terms was applied in order to reproduce the $N=9$ isotone $^{17}$O. In addition, the excitation energies and spectroscopic factors have been compared to the first calculations of $^{15}$C with the $ab~ initio$ self-consistent Green's function method employing the NNLO$_{sat}$ interaction. The results show the sensitivity to the size of the $N=8$ shell gap and highlight the need of going beyond the current truncation scheme in the theory.

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First Evidence of Axial Shape Asymmetry and Configuration Coexistence in $^{74}$Zn: Suggestion for a Northern Extension of the $N=40$ Island of Inversion

The excited states of $N=44$ $^{74}$Zn were investigated via $γ$-ray spectroscopy following $^{74}$Cu $β$ decay. By exploiting $γ$-$γ$ angular correlation analysis, the $2_2^+$, $3_1^+$, $0_2^+$ and $2_3^+$ states in $^{74}$Zn were firmly established. The $γ$-ray branching and $E2/M1$ mixing ratios for transitions de-exciting the $2_2^+$, $3_1^+$ and $2_3^+$ states were measured, allowing for the extraction of relative $B(E2)$ values. In particular, the $2_3^+ \to 0_2^+$ and $2_3^+ \to 4_1^+$ transitions were observed for the first time. The results show excellent agreement with new microscopic large-scale shell-model calculations, and are discussed in terms of underlying shapes, as well as the role of neutron excitations across the $N=40$ gap. Enhanced axial shape asymmetry (triaxiality) is suggested to characterize $^{74}$Zn in its ground state. Furthermore, an excited $K=0$ band with a significantly larger softness in its shape is identified. A shore of the $N=40$ ``island of inversion'' appears to manifest above $Z=26$, previously thought as its northern limit in the chart of the nuclides.

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Neutrinoless Double Beta Decay

This White Paper, prepared for the Fundamental Symmetries, Neutrons, and Neutrinos Town Meeting related to the 2023 Nuclear Physics Long Range Plan, makes the case for double beta decay as a critical component of the future nuclear physics program. The major experimental collaborations and many theorists have endorsed this white paper.

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Improved measurement of the $0_2^+\rightarrow0_1^+$ E0 transition strength for $^{72}$Se using the SPICE spectrometer

The selenium isotopes lie at the heart of a tumultuous region of the nuclear chart where shape coexistence effects grapple with neutron-proton pairing correlations, triaxiality, and the impending proton dripline. In this work a study of $^{72}$Se by internal conversion electron and $γ$-ray spectroscopy was undertaken with the SPICE and TIGRESS arrays. New measurements of the branching ratio and lifetime of the $0_2^+$ state were performed yielding a determination of $ρ^2(E0;0_2^+{\rightarrow}0_1^+)=29(3)$ milliunits. two state mixing calculations were performed that highlighted the importance of interpretation of such $E0$ strength values in the context of shape-coexistence.

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High-precision half-life determination of $^{14}$O via direct $β$ counting

The half-life of the superallowed Fermi $β^+$ emitter $^{14}$O was determined to high precision via a direct $β$ counting experiment performed at the Isotope Separator and Accelerator (ISAC) facility at TRIUMF. The result, $T_{1/2}$($^{14}$O) = 70619.2(76) ms, is consistent with, but is more precise than, the world average obtained from 11 previous measurements. Combining the $^{14}$O half-life deduced in the present work with the previous most precise measurements of this quantity leads to a reduction in the overall uncertainty, by nearly a factor of 2. The new world average is $T_{1/2}$($^{14}$O) = 70619.6(63) ms with a reduced $χ^2$ value of 0.87 obtained from 8 degrees of freedom.

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Experimental investigation of ground-state properties of $^7$H with transfer reactions

The properties of nuclei with extreme neutron-to-proton ratios, far from those naturally occurring on Earth, are key to understand nuclear forces and how nucleons hold together to form nuclei. $^7$H, with six neutrons and a single proton, is the nuclear system with the most unbalanced neutron-to-proton ratio known so far. However, its sheer existence and properties are still a challenge for experimental efforts and theoretical models. Here we report experimental evidences on the formation of $^7$H as a resonance, detected with independent observables, and the first measurement of the structure of its ground state. The resonance is found at $\sim$0.7 MeV above the $^3$H+4n mass, with a narrow width of $\sim$0.2 MeV and a $1/2^+$ spin and parity. These data are consistent with a $^7$H as a $^3$H core surrounded by an extended four-neutron halo, with a unique four-neutron decay and a relatively long half-life thanks to neutron pairing; a prime example of new phenomena occurring in what would be the most pure-neutron nuclear matter we can access in the laboratory.

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LEGEND-1000 Preconceptual Design Report

We propose the construction of LEGEND-1000, the ton-scale Large Enriched Germanium Experiment for Neutrinoless $ββ$ Decay. This international experiment is designed to answer one of the highest priority questions in fundamental physics. It consists of 1000 kg of Ge detectors enriched to more than 90% in the $^{76}$Ge isotope operated in a liquid argon active shield at a deep underground laboratory. By combining the lowest background levels with the best energy resolution in the field, LEGEND-1000 will perform a quasi-background-free search and can make an unambiguous discovery of neutrinoless double-beta decay with just a handful of counts at the decay $Q$ value. The experiment is designed to probe this decay with a 99.7%-CL discovery sensitivity in the $^{76}$Ge half-life of $1.3\times10^{28}$ years, corresponding to an effective Majorana mass upper limit in the range of 9-21 meV, to cover the inverted-ordering neutrino mass scale with 10 yr of live time.

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First direct measurement of $^{59}$Cu(p,$α$)$^{56}$Ni: A step towards constraining the Ni-Cu cycle in the Cosmos

Reactions on the proton-rich nuclides drive the nucleosynthesis in Core-Collapse Supernovae (CCSNe) and in X-ray bursts (XRBs). CCSNe eject the nucleosynthesis products to the interstellar medium and hence are a potential inventory of p-nuclei, whereas in XRBs nucleosynthesis powers the light curves. In both astrophysical sites the Ni-Cu cycle, which features a competition between $^{59}$Cu(p,$α$)$^{56}$Ni and $^{59}$Cu(p,$γ$)$^{60}$Zn, could potentially halt the production of heavier elements. Here, we report the first direct measurement of $^{59}$Cu(p,$α$)$^{56}$Ni using a re-accelerated $^{59}$Cu beam and cryogenic solid hydrogen target. Our results show that the reaction proceeds predominantly to the ground state of $^{56}$Ni and the experimental rate has been found to be lower than Hauser-Feshbach-based statistical predictions. New results hint that the $νp$-process could operate at higher temperatures than previously inferred and therefore remains a viable site for synthesizing the heavier elements.

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High-Precision Branching Ratio Measurement and Spin Assignment Implications for $^{62}$Ga Superallowed $β$ Decay

A high-precision branching ratio measurement for the superallowed Fermi $β^{+}$ emitter $^{62}$Ga was performed with the Gamma-Ray Infrastructure for Fundamental Investigations of Nuclei (GRIFFIN) spectrometer at the Isotope Separator and Accelerator (ISAC) radioactive ion beam facility at TRIUMF. The high efficiency of the GRIFFIN spectrometer allowed 63 $γ$-ray transitions, with intensities down to $\approx$1 part per million (ppm) per $^{62}$Ga $β^{+}$ decay, to be placed in the level scheme of the daughter nucleus $^{62}$Zn, establishing the superallowed $β$ branching ratio for $^{62}$Ga decay to be 99.8577$^{+0.0023}_{-0.0029}\%$, a factor of 4 more precise than the previous world average. For several cascades, $γ-γ$ angular correlation measurements were performed to assign spins and/or determine the mixing ratios of transitions. In particular, the spin of the 2.342 MeV excited state in the daughter nucleus $^{62}$Zn was definitively assigned as $J = 0$. This assignment resolves a discrepancy between previous measurements and has important implications for the isospin symmetry breaking correction, $δ_{C1}$, in $^{62}$Ga superallowed Fermi $β$ decay.

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Low-lying single-particle structure of 17C and the N = 14 sub-shell closure

The first investigation of the single-particle structure of the bound states of 17C, via the d(16C, p) transfer reaction, has been undertaken. The measured angular distributions confirm the spin-parity assignments of 1/2+ and 5/2+ for the excited states located at 217 and 335 keV, respectively. The spectroscopic factors deduced for these states exhibit a marked single-particle character, in agreement with shell model and particle-core model calculations, and combined with their near degeneracy in energy provide clear evidence for the absence of the N = 14 sub-shell closure. The very small spectroscopic factor found for the 3/2+ ground state is consistent with theoretical predictions and indicates that the ν1d3/2 strength is carried by unbound states. With a dominant l = 0 valence neutron configuration and a very low separation energy, the 1/2+ excited state is a one-neutron halo candidate.

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Signature of a possible $α$-cluster state in $N=Z$ doubly-magic $^{56}$Ni

An inelastic $α$-scattering experiment on the unstable $N=Z$, doubly-magic $^{56}$Ni nucleus was performed in inverse kinematics at an incident energy of 50 A.MeV at GANIL. High multiplicity for $α$-particle emission was observed within the limited phase-space of the experimental setup. This observation cannot be explained by means of the statistical-decay model. The ideal classical gas model at $kT$ = 0.4 MeV reproduces fairly well the experimental momentum distribution and the observed multiplicity of $α$ particles corresponds to an excitation energy around 96 MeV. The method of distributed $mα$-decay ensembles is in agreement with the experimental results if we assume that the $α$-gas state in $^{56}$Ni exists at around $113^{+15}_{-17}$ MeV. These results suggest that there may exist an exotic state consisting of many $α$ particles at the excitation energy of $113^{+15}_{-17}$ MeV.

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