arXiv subjects

G. Gatti

Publications and source records attributed to G. Gatti.

At least 19 recordsLinked to original sources

arXiv2026

Electron-phonon coupling across the TMD/hBN van der Waals interface

Many-body interactions can couple electronic states in one layer with collective excitations in the adjacent layer, providing a route to tailor properties of heterostructures. However, detecting and quantifying interlayer many-body interactions proved a major challenge. Here, we demonstrate that quasiparticles in monolayer transition metal dichalcogenides (TMDs) are dressed by a remote cloud of phonons in the adjacent hexagonal boron nitride slab. Using angle resolved photoemission, we identify replica bands in the TMDs which are a clear fingerprint of long-range electron-phonon interaction. We develop a modified Fröhlich model that shows semi-quantitative agreement with the experimental spectral functions. Our analysis shows that remote electron-phonon coupling is a generic property of interfaces with hBN. This has implications for electron mobilities in 2D materials, for superconductivity and possibly for moiré correlated phases.

cond-mat.mtrl-sci↗

arXiv2025

Fermi surface and pseudogap in highly doped Sr$_{2}$IrO$_{4}$

The fate of the Fermi surface in bulk electron-doped Sr$_{2}$IrO$_{4}$ remains elusive, as does the origin and extension of its pseudogap phase. Here, we use high-resolution angle-resolved photoelectron spectroscopy (ARPES) to investigate the electronic structure of Sr$_{2-x}$La$_{x}$IrO$_{4}$ up to $x=0.2$, a factor of two higher than in previous work. We find that the antinodal pseudogap persists up to the highest doping level, and thus beyond the sharp increase in Hall carrier density to $\simeq 1+x$ recently observed above $x^{*}\simeq 0.16$ [Y.-T. Hsu et al., Nature Physics 20, 1593 (2024)]. This suggests that doped iridates host a unique phase of matter in which a large Hall density coexists with an anisotropic pseudogap, breaking up the Fermi surface into disconnected arcs. The temperature boundary of the pseudogap is $T^{*}\simeq 200$ K for $x=0.2$, comparable to cuprates and to the energy scale of short range antiferromagnetic correlations in cuprates and iridates.

cond-mat.str-el↗

arXiv2024

Technical Status Report on Plasma Components and Systems in the context of EuPRAXIA

The EuPRAXIA project aims to construct two state-of-the-art accelerator facilities based on plasma accelerator technology. Plasma-based accelerators offer the possibility of a significant reduction in facility size and cost savings over current radio frequency (RF) accelerators. The two facilities - one laser-driven one a beam-driven - are envisioned to provide electron beams with an energy in the range of 1-5 GeV and beam quality comparable to existing RF machines. This will enable a versatile portfolio of applications from compact free-electron laser (FEL) drivers to sources for medical and industrial imaging. At the heart of both facilities is the use of plasma-based accelerator components and systems which encompass not only the accelerating medium itself, but also a range of auxiliary systems such as plasma-based electron beam optics and plasma-based mirrors for high-intensity lasers. From a technical standpoint, a high-degree of control over these plasma devices will be essential for EuPRAXIA to achieve its target performance goals. The ability to diagnose and characterize these plasma devices and to simulate their operation will be further essential success factors. Additionally, compatibility with extended operation at high-repetition rates and integration into the accelerator beamline will also prove crucial. In this work, we aim to review the current status of plasma components and related systems for both laser-driven and beam-driven plasma accelerators and to assess challenges to be addressed regarding implementation at future EuPRAXIA facilities.

physics.plasm-ph↗

arXiv2024

Nature of metallic and insulating domains in the CDW system 1T-TaSe2

We study the electronic structure of bulk 1T-TaSe$_2$ in the charge density wave phase at low temperature. Our spatially and angle resolved photoemission (ARPES) data show insulating areas coexisting with metallic regions characterized by a chiral Fermi surface and moderately correlated quasiparticle bands. Additionally, high-resolution laser ARPES reveals variations in the metallic regions, with series of low-energy states, whose energy, number and dispersion can be explained by the formation of quantum well states of different thicknesses. Dynamical mean field theory calculations show that the observed rich behaviour can be rationalized by assuming occasional stacking faults of the charge density wave. Our results indicate that the diverse electronic phenomena reported previously in 1T-TaSe$_2$ are dictated by the stacking arrangement and the resulting quantum size effects while correlation effects play a secondary role.

cond-mat.str-el↗

arXiv2024

Light-induced renormalization of the band structure of chiral tellurium

Chirality in tellurium derives from a Peierls distortion driven by strong electron-phonon coupling, making this material a unique candidate for observing a light-induced topological phase transition. By using time- and angle-resolved photoelectron spectroscopy (trARPES), we reveal that upon near-infrared photoexcitation the Peierls gap is modulated by displacively excited coherent phonons with $\mathrm{A_{1g}}$ symmetry as well as chiral-symmetry-breaking $\mathrm{E'_{LO}}$ modes. By comparison with state-of-the-art TDDFT+U calculations, we reveal the microscopic origin of the in-phase oscillations of band edges, due to phonon-induced modulation of the effective Hubbard $U$ term.

cond-mat.mtrl-sci↗

arXiv2024

Spatial characterization of debris ejection from the interaction of a tightly focused PW-laser pulse with metal targets

We present a novel scheme for rapid quantitative analysis of debris generated during experiments with solid targets following relativistic laser-plasma interaction at high-power laser facilities. Experimental data indicates that predictions by available modelling for non-mass-limited targets are reasonable, with debris on the order of hundreds ug-per-shot. We detect for the first time that several % of the debris is ejected directional following the target normal (rear- and interaction side); and confirm previous work that found the debris ejection in direction of the interaction side to be larger than on the side of the target rear.

physics.plasm-ph↗

arXiv2023

Orbital-selective metal skin induced by alkali-metal-dosing Mott-insulating Ca$_2$RuO$_4$

Doped Mott insulators are the starting point for interesting physics such as high temperature superconductivity and quantum spin liquids. For multi-band Mott insulators, orbital selective ground states have been envisioned. However, orbital selective metals and Mott insulators have been difficult to realize experimentally. Here we demonstrate by photoemission spectroscopy how Ca$_2$RuO$_4$, upon alkali-metal surface doping, develops a single-band metal skin. Our dynamical mean field theory calculations reveal that homogeneous electron doping of Ca$_2$RuO$_4$ results in a multi-band metal. All together, our results provide compelling evidence for an orbital-selective Mott insulator breakdown, which is unachievable via simple electron doping. Supported by a cluster model and cluster perturbation theory calculations, we demonstrate a novel type of skin metal-insulator transition induced by surface dopants that orbital-selectively hybridize with the bulk Mott state and in turn produce coherent in-gap states.

cond-mat.str-el↗

arXiv2023

The fate of quasiparticles at high-temperature

We study the temperature evolution of quasiparticles in the correlated metal Sr$_2$RuO$_4$. Our angle resolved photoemission data show that quasiparticles persist up to temperatures above 200~K, far beyond the Fermi liquid regime. Extracting the quasiparticle self-energy we demonstrate that the quasiparticle residue $Z$ increases with increasing temperature. Quasiparticles eventually disappear on approaching the bad metal state of Sr$_2$RuO$_4$ not by losing weight but via excessive broadening from super-Planckian scattering. We further show that the Fermi surface of Sr$_2$RuO$_4$ - defined as the loci where the spectral function peaks - deflates with increasing temperature. These findings are in semi-quantitative agreement with dynamical mean field theory calculations.

cond-mat.str-el↗

arXiv2022

Mode Control of Electro-Magnetic Pulses in the VHF Band

We present experimental results for the controlled mitigation of electromagnetic pulses (EMP) produced in interactions of the 1PW high-power 30fs Ti:Sa laser VEGA-3 with matter. This study aims at the band of very high frequencies (VHF), notably hundreds of MHz, comprising the fundamental cavity modes of the rectangular VEGA-3 vacuum chamber. We demonstrate mode suppression by tailoring of the laser-produced space charge distribution.

physics.plasm-ph↗

arXiv2022

Electronic structure of the highly conductive perovskite oxide SrMoO$_3$

We use angle-resolved photoemission to map the Fermi surface and quasiparticle dispersion of bulk-like thin films of SrMoO$_3$ grown by pulsed laser deposition. The electronic self-energy deduced from our data reveals weak to moderate correlations in SrMoO$_3$, consistent with our observation of well-defined electronic states over the entire occupied band width. We further introduce spectral function calculations that combine dynamical mean-field theory with an unfolding procedure of density functional calculations and demonstrate good agreement of this approach with our experiments.

cond-mat.str-el↗

arXiv2020

Ion acceleration by an ultrashort laser pulse interacting with a near-critical-density gas jet

We demonstrate laser-driven Helium ion acceleration with cut-off energies above 25 MeV and peaked ion number above $10^8$ /MeV for 22(2) MeV projectiles from near-critical density gas jet targets. We employed shock gas jet nozzles at the high-repetition-rate (HRR) VEGA-2 laser system with 3 J in pulses of 30 fs focused down to intensities in the range between $9\times10^{19}$ W/cm$^2$ and $1.2\times10^{20}$ W/cm$^2$. We demonstrate acceleration spectra with minor shot-to-shot changes for small variations in the target gas density profile. Difference in gas profiles arise due to nozzles being exposed to a experimental environment, partially ablating and melting.

physics.plasm-ph↗

arXiv2020

A quasi-monoenergetic short time duration compact proton source for probing high energy density states of matter

We report on the development of a highly directional, narrow energy band, short time duration proton beam operating at high repetition rate, suitable for measurements of stopping power in high energy density plasmas as well as other applications. The protons are generated with an ultrashort-pulse laser interacting with a solid target and converted to a pencil-like narrow-band beam using a compact magnet-based energy selector. We experimentally demonstrate the production of a proton beam with an energy of 500 keV and energy spread well below 10%, and a pulse duration of 260 ps. The energy loss of this beam is measured in a 2 $μ$m thick solid Mylar target and found to be in within 1% of theoretical predictions. The short time duration of the proton pulse makes it particularly well suited for applications involving the probing of highly transient plasma states produced in laser-matter interaction experiments, in particular measurements of proton stopping power.

physics.plasm-ph↗

arXiv2020

Integrated quantitative PIXE analysis and EDX spectroscopy using a laser-driven particle source

Among the existing elemental characterization techniques, Particle Induced X-ray Emission (PIXE) and Energy Dispersive X-ray (EDX) spectroscopy are two of the most widely used in different scientific and technological fields. Here we present the first quantitative laser-driven PIXE and laser-driven EDX experimental investigation performed at the Centro de Láseres Pulsados in Salamanca. Thanks to their potential for compactness and portability, laser-driven particle sources are very appealing for materials science applications, especially for materials analysis techniques. We demonstrate the possibility to exploit the X-ray signal produced by the co-irradiation with both electrons and protons to identify the elements in the sample. We show that, using the proton beam only, we can successfully obtain quantitative information about the sample structure through laser-driven PIXE analysis. These results pave the way towards the development of a compact and multi-functional apparatus for the elemental analysis of materials based on a laser-driven particle source.

physics.plasm-ph↗

arXiv2019

Light-induced renormalization of the Dirac quasiparticles in the nodal-line semimetal ZrSiSe

In nodal-line semimetals linearly dispersing states form Dirac loops in the reciprocal space, with high degree of electron-hole symmetry and almost-vanishing density of states near the Fermi level. The result is reduced electronic screening and enhanced correlations between Dirac quasiparticles. Here we investigate the electronic structure of ZrSiSe, by combining time- and angle-resolved photoelectron spectroscopy with ab initio density functional theory (DFT) complemented by an extended Hubbard model (DFT +U +V). We show that electronic correlations are reduced on an ultrashort timescale by optical excitation of high-energy electrons-hole pairs, which transiently screen the Coulomb interaction. Our findings demonstrate an all-optical method for engineering the band structure of a quantum material.

cond-mat.str-el↗

arXiv2019

Towards an in situ, full-power gauge of the focal-volume intensity of petawatt-class lasers

About 50 years ago, Sarachick and Schappert [Phys. Rev. D. 1, 2738 (1970)] showed that relativistic Thomson scattering leads to wavelength shifts that are proportional to the laser intensity. About 28 years later Chen et al. [Nature 396, 653 (1998)] used these shifts to estimate their laser intensity near 10^18 W/cm^2. More recently there have been several theoretical studies aimed at exploiting nonlinear Thomson scattering as a tool for direct measurement of intensities well into the relativistic regime. We present the first quantitative study of this approach for intensities between 10^18 and 10^19 W/cm^2. We show that the spectral shifts are in reasonable agreement with estimates of the peak intensity extracted from images of the focal area obtained at reduced power. Finally, we discuss the viability of the approach, its range of usefulness and how it might be extended to gauge intensities well in excess of 10^19 W/cm^2.

physics.plasm-ph↗

arXiv2019

Evidence of large polarons in photoemission band mapping of the perovskite semiconductor CsPbBr$_3$

Lead-halide perovskite (LHP) semiconductors are emergent optoelectronic materials with outstanding transport properties which are not yet fully understood. We find signatures of large polaron formation in the electronic structure of the inorganic LHP CsPbBr$_3$ by means of angle-resolved photoelectron spectroscopy. The experimental valence band dispersion shows a hole effective mass $0.26\pm0.02\,\,m_e$, 50% heavier than the bare mass $m_0 =0.17 m_e$ predicted by density functional theory. Calculations of electron-phonon coupling indicate that phonon dressing of the carriers mainly occurs via distortions of the Pb-Br bond with a Fröhlich coupling parameter $α=1.82$. A good agreement with our experimental data is obtained within the Feynmann polaron model, validating a viable theorical method to predict the carrier effective mass of LHPs ab-initio.

cond-mat.mtrl-sci↗

arXiv2019

A 2D scintillator based proton detector for HRR experiments

We present a scintillator based detector able to measure both spatial and energy information at High repetition rate (HRR) with a relatively simple design. It has been built at the Center of Pulsed Laser (CLPU) in Salamanca and tested in the proton accelerator at the Centro de Micro-Analisis de Materiales (CMAM) in Madrid. The detector has been demonstrated to work in HRR mode by reproducing the performance of the radiochromic film detector. It represents a new class of on-line detectors for Laser-plasma physics experiments in the new emerging High Power and HRR laser systems.

physics.ins-det↗

arXiv2018

Generation of high energy laser-driven electron and proton sources with the 200 TW system VEGA 2 at the Centro de Laseres Pulsados

The Centro de Laseres Pulsados in Salamanca Spain has recently started operation phase and the first User access period on the 6 J 30 fs 200 TW system (VEGA 2) already started at the beginning of 2018. In this paper we report on two commissioning experiments recently performed on the VEGA 2 system in preparation for the user campaign. VEGA 2 system has been tested in different configurations depending on the focusing optics and targets used. One configuration (long focal length f=130 cm) is for under-dense laser-matter interaction where VEGA 2 is focused onto a low density gas-jet generating electron beams (via laser wake field acceleration mechanism) with maximum energy up to 500 MeV and an X-ray betatron source with a 10 keV critical energy. A second configuration (short focal length f=40 cm) is for over-dense laser-matter interaction where VEGA 2 is focused onto an 5 microns thick Al target generating a proton beam with a maximum energy of 10 MeV and average energy of 7-8 MeV and temperature of 2.5 MeV. In this paper we present preliminary experimental results.

physics.plasm-ph↗