arXiv subjects

G. Hétet

Publications and source records attributed to G. Hétet.

At least 19 recordsLinked to original sources

arXiv2026

Measurement of a quantum system using spin-mechanical conversion

Levitated macroscopic particles exhibiting quantum mechanical effects are garnering increased attention as a means for precision sensing and testing quantum mechanics. Defects in diamond, such as the nitrogen-vacancy (NV) centre possess optically-addressable spins with long coherence times at room temperature and offer an intriguing system to examine quantum spin dynamics coupled to a macroscopic classical particle. In this work, we convert the outcome of a quantum measurement on an ensemble of spins into a macroscopic rotation of the host particle via spin-mechanical coupling. Following a sequence of green laser and microwave control pulses, spin-mechanical coupling between the final qubit spin state and the host particle -- an electrically-levitated diamond -- exerts a torque on the particle that deflects a weak near-infra-red laser beam. We measure spin readout contrast in excess of 70\%, and demonstrate pulsed mechanical detection of coherent Rabi oscillations, spin-echo interferometry and $T_1$-induced relaxation. We directly measure with temporal resolution the particle reorientation from a 60\,attonewton-metre spin torque induced by flipping the spins. Our results open up interesting new opportunities for levitated spin-mechanical systems using pulsed control, from improved sensing to the prospect of realising macroscopic quantum superposition states.

quant-ph↗

arXiv2024

Nuclear Magnetic Resonance with a Levitating Micro-Particle

Nuclear Magnetic Resonance (NMR) spans diverse fields from biology to quantum science. Employing NMR on a floating object could unveil novel possibilities beyond conventional operational paradigms. Here, we observe Nuclear Magnetic Resonance (NMR) within a levitating micro-diamond using the nuclear spins of nitrogen-14 atoms. By tightly confining the angular degrees of freedom of the diamond in a Paul trap, we achieve efficient hyperfine interaction between optically polarized electronic spins of nitrogen-vacancy centers and the $^{14}$N nuclear spin, enabling nuclear spin polarization and quantum state read-out revealing coherence times up to hundreds of microseconds. This represents the longest recorded spin coherence time in a levitated system, surpassing previous records by three orders of magnitude. Our results offer promise for various applications, including cooling macroscopic particles to their motional ground state and exploring geometric phases for gyroscopy.

quant-ph↗

arXiv2022

Spin-Relaxation of Dipolar-Coupled Nitrogen-Vacancy Centers : The role of Double-flip Processes

We study relaxation processes of the spins of dipolar-coupled negatively charged nitrogen vacancy (NV$^-$) centers under transverse electric and magnetic fields. Specifically, we uncover regimes where flip-flop, double-flip processes as well as mixing induced by local electric fields play a significant role in NV-NV cross-relaxation. Our results are relevant for understanding decoherence in many-body spin systems as well as for high sensitivity magneto- and electro-metry with long-lived interacting solid-state spins. As a proof of principle, we present an orientation and microwave-free magnetometer based on cross-relaxation.

quant-ph↗

arXiv2021

Angle Locking of a Levitating Diamond using Spin-Diamagnetism

The negatively charged nitrogen-vacancy (NV) center in nano- or micro- diamonds has emerged as a promising magnetic field sensor, as a candidate for hyper-polarizing paramagnetic species, as well as a tool for spin-mechanics at the nanoscale. However, NV-doped diamonds are presently not straightforwardly employable for these applications in a liquid or when levitating under atmospheric pressures due to the random angular Brownian motion which tends to rotate the NV quantization axis over the course of the measurments. Here, we report on angle locking of the crystalline axis of a trapped micro-diamond along an external magnetic field. Specifically, we use spin population inversion after a ground state level crossing of the NV center to turn the diamond into a diamagnet. The diamond crystalline axis naturally aligns to the magnetic field with high precision and in the absence of micro-wave, offering bright prospects for applications in biology and spin-mechanical platforms.

quant-ph↗

arXiv2021

Magnetic-Torque Enhanced by Tunable Dipolar interactions

We use tunable dipolar-interactions between the spins of nitrogen-vacancy (NV) centers in diamond to rotate a diamond crystal. Specifically, we employ cross-relaxation between the electronic spin of pairs of NV centers in a trapped diamond to enhance the anisotropic NV paramagnetism and thus to increase the associated spin torque. Our observations open a path towards the use of mechanical oscillators to detect paramagnetic defects that lack optical transitions, to investigation of angular momentum conservation in spin relaxation processes and to novel means of cooling the motion of mechanical oscillators.

cond-mat.mes-hall↗

arXiv2020

Optical Detection of Paramagnetic Defects in a CVD-grown Diamond

The electronic spins of the nitrogen-vacancy centers (NV centers) in Chemical-Vapor-Deposition (CVD) grown diamonds form ideal probes of magnetic fields and temperature, as well as promising qu-bits for quantum information processing. Studying and controlling the magnetic environment of NV centers in such high purity crystals is thus essential for these applications. We demonstrate optical detection of paramagnetic species, such as hydrogen-related complexes, in a CVD-grown diamond. The resonant transfer of the NV centers' polarized electronic spins to the electronic spins of these species generates conspicuous features in the NV photoluminescence by employing magnetic field scans along the [100] crystal direction. Our results offer prospects for more detailed studies of CVD-grown processes as well as for coherent control of the spin of novel classes of hyper-polarized paramagnetic species.

quant-ph↗

arXiv2020

Coherent Microwave Control of a Nuclear Spin Ensemble at Room Temperature

We use nominally forbidden electron-nuclear spin transitions in nitrogen-vacancy (NV) centers in diamond to demonstrate coherent manipulation of a nuclear spin ensemble using microwave fields at room temperature. We show that employing an off-axis magnetic field with a modest amplitude($\approx$ 0.01 T) at an angle with respect to the NV natural quantization axes is enough to tilt the direction of the electronic spins, and enable efficient spin exchange with the nitrogen nuclei of the NV center. We could then demonstrate fast Rabi oscillations on electron-nuclear spin exchanging transitions, coherent population trapping and polarization of nuclear spin ensembles in the microwave regime. Coupling many electronic spins of NV centers to their intrinsic nuclei offers full scalability with respect to the number of controllable spins and provides prospects for transduction. In particular, the technique could be applied to long-lived storage of microwave photons and to the coupling of nuclear spins to mechanical oscillators in the resolved sideband regime.

quant-ph↗

arXiv2020

Spin-mechanics with levitating ferromagnetic particles

We propose and demonstrate first steps towards schemes where the librational mode of levitating ferromagnets is strongly coupled to the electronic spin of Nitrogen-Vacancy (NV) centers in diamond. Experimentally, we levitate ferromagnets in a Paul trap and employ magnetic fields to attain oscillation frequencies in the hundreds of kHz range with Q factors close to $10^4$. These librational frequencies largely exceed the decoherence rate of NV centers in typical CVD grown diamonds offering prospects for sideband resolved operation. We also prepare and levitate composite diamond-ferromagnet particles and demonstrate both coherent spin control of the NV centers and read-out of the particle libration using the NV spin. Our results will find applications in ultra-sensitive gyroscopy and bring levitating objects a step closer to spin-mechanical experiments at the quantum level.

quant-ph↗

arXiv2019

Spin-Cooling of the Motion of a Trapped Diamond

Observing and controlling macroscopic quantum systems has long been a driving force in research on quantum physics. In this endeavor, strong coupling between individual quantum systems and mechanical oscillators is being actively pursued. While both read-out of mechanical motion using coherent control of spin systems and single spin read-out using pristine oscillators have been demonstrated, temperature control of the motion of a macroscopic object using long-lived electronic spins has not been reported. Here, we observe both a spin-dependent torque and spin-cooling of the motion of a trapped microdiamond. Using a combination of microwave and laser excitation enables the spin of nitrogen-vacancy centers to act on the diamond orientation and to cool the diamond libration via a dynamical back-action. Further, driving the system in the non-linear regime, we demonstrate bistability and self-sustained coherent oscillations stimulated by the spin-mechanical coupling, which offers prospects for spin-driven generation of non-classical states of motion. Such a levitating diamond operated as a compass with controlled dissipation has implications in high-precision torque sensing, emulation of the spin-boson problem and probing of quantum phase transitions. In the single spin limit and employing ultra-pure nano-diamonds, it will allow quantum non-demolition read-out of the spin of nitrogen-vacancy centers under ambient conditions, deterministic entanglement between distant individual spins and matter-wave interferometry.

quant-ph↗

arXiv2019

Sub-GHz linewidths ensembles of SiV centers in a diamond nano-pyramid revealed by charge state conversion

Producing nano-structures with embedded bright ensembles of lifetime-limited emitters is a challenge with potential high impact in a broad range of physical sciences. In this work, we demonstrate controlled charge transfer to and from dark states exhibiting very long lifetimes in high density ensembles of SiV centers hosted in a CVD-grown diamond nano-pyramid. Further, using a combination of resonant photoluminescence excitation and a frequency-selective persistent hole burning technique that exploits such charge state transfer, we could demonstrate close to lifetime-limited linewidths from the SiV centers. Such a nanostructure with thousands of bright narrow linewidth emitters in a volume much below $λ^3$ will be useful for coherent light-matter coupling, for biological sensing, and nanoscale thermometry.

quant-ph↗

arXiv2018

Ramsey interferences and spin echoes from electron spins inside a levitating macroscopic particle

We report observations of Ramsey interferences and spin echoes from electron spins inside a levitating macroscopic particle. The experiment is realized using nitrogen-vacancy (NV) centers hosted in a micron-sized diamond stored in a Paul trap both under atmospheric conditions and under vacuum. Spin echoes are used to show that the Paul trap preserves the coherence time of the embedded electron spins for more than microseconds. Conversely, the NV spin is employed to demonstrate high angular stability of the diamond even under vacuum. These results are significant steps towards strong coupling of NV spins to the rotational mode of levitating diamonds.

quant-ph↗

arXiv2018

Diamond nano-pyramids with narrow linewidth SiV centers for quantum technologies

Color centers in diamond are versatile solid state atomic-like systems suitable for quantum technological applications. In particular, the negatively charged silicon vacancy center (SiV) can exhibit a narrow photoluminescence (PL) line and lifetime-limited linewidth in bulk diamonds at cryogenic temperature. We present a low-temperature study of chemical vapour deposition (CVD)-grown diamond nano-pyramids containing SiV centers. The PL spectra feature a bulk-like zero-phonon line with ensembles of SiV centers, with a linewidth below 10 GHz which demonstrates very low crystal strain for such a nano-object.

quant-ph↗

arXiv2017

Coherent Population Trapping with a controlled dissipation: applications in optical metrology

We analyze the properties of a pulsed Coherent Population Trapping protocol that uses a controlled decay from the excited state in a $Λ$-level scheme. We study this problem analytically and numerically and find regimes where narrow transmission, absorption, or fluorescence spectral lines occur. We then look for optimal frequency measurements using these spectral features by computing the Allan deviation in the presence of ground state decoherence and show that the protocol is on a par with Ramsey-CPT. We discuss possible implementations with ensembles of alkali atoms and single ions and demonstrate that typical pulsed-CPT experiments that are realized on femto-second time-scales can be implemented on micro-seconds time-scales using this scheme.

quant-ph↗

arXiv2017

Strong Coupling between a Single NV Spin and the Rotational Mode of Diamonds Levitating in an Ion Trap

A scheme for strong coupling between a single atomic spin and the rotational mode of levitating nanoparticles is proposed. The idea is based on spin read-out of NV centers embedded in aspherical nanodiamonds levitating in an ion trap. We show that the asymmetry of the diamond induces a rotational confinement in the ion trap. Using a weak homogeneous magnetic field and a strong microwave driving we then demonstrate that the spin of the NV center can be strongly coupled to the rotational motion of the diamond.

quant-ph↗

arXiv2017

Diamonds levitating in a Paul trap under vacuum: measurements of laser-induced heating via NV center thermometry

We present measurements of the Electronic Spin Resonance (ESR) of Nitrogen Vacancy (NV) centers in diamonds that are levitating in a ring Paul trap under vacuum. We observe ESR spectra of NV centers embedded in micron-sized diamonds at vacuum pressures down to $2\times 10^{-1}$ mbar, limited by the green laser heating of the diamond. We also observe the NV photoluminescence at vacuum pressures down to $10^{-2}$ mbar and discuss the steps required to control the NV spin under ultra-high vacuum.

quant-ph↗

arXiv2015

Coherent population trapping of a single nuclear spin under ambient conditions

Coherent control of quantum systems has far-reaching implications in quantum engineering. In this context, coherent population trapping (CPT) involving dark resonances has played a prominent role, leading to a wealth of major applications including laser cooling of atoms and molecules, optical magnetometry, light storage and highly precise atomic clocks. Extending CPT methods to individual solid-state quantum systems has been only achieved in cryogenic environments for electron spin impurities and superconducting circuits. Here, we demonstrate efficient CPT of a single nuclear spin in a room temperature solid. To this end, we make use of a three-level system with a $Λ$-configuration in the microwave domain, which consists of nuclear spin states addressed through their hyperfine coupling to the electron spin of a single nitrogen-vacancy defect in diamond. Dark state pumping requires a relaxation mechanism which, in atomic systems, is simply provided by spontaneous emission. In this work, the relaxation process is externally controlled through incoherent optical pumping and separated in time from consecutive coherent microwave excitations of the nuclear spin $Λ$-system. Such a pumping scheme with controlled relaxation allows us (i) to monitor the sequential accumulation of population into the dark state and (ii) to reach a new regime of CPT dynamics for which periodic arrays of dark resonances can be observed, owing to multiple constructive interferences. This work offers new prospects for quantum state preparation, information storage in hybrid quantum systems and metrology.

quant-ph↗

arXiv2013

Quantum Memory with a controlled homogeneous splitting

We propose a quantum memory protocol where a input light field can be stored onto and released from a single ground state atomic ensemble by controlling dynamically the strength of an external static and homogeneous field. The technique relies on the adiabatic following of a polaritonic excitation onto a state for which the forward collective radiative emission is forbidden. The resemblance with the archetypal Electromagnetically-Induced-Transparency (EIT) is only formal because no ground state coherence based slow-light propagation is considered here. As compared to the other grand category of protocols derived from the photon-echo technique, our approach only involves a homogeneous static field. We discuss two physical situations where the effect can be observed, and show that in the limit where the excited state lifetime is longer than the storage time, the protocols are perfectly efficient and noise-free. We compare the technique to other quantum memories, and propose atomic systems where the experiment can be realized.

quant-ph↗

arXiv2013

Atom-atom entanglement by single-photon detection

A scheme for entangling distant atoms is realized, as proposed in the seminal paper by Cabrillo et al. [Phys. Rev. A 59, 1025 (1999)]. The protocol is based on quantum interference and detection of a single photon scattered from two effectively one meter distant laser-cooled and trapped atomic ions. The detection of a single photon heralds entanglement of two internal states of the trapped ions with high rate and with a fidelity limited mostly by atomic motion. Control of the entangled state phase is demonstrated by changing the path length of the single-photon interferometer.

quant-ph↗