arXiv subjects

G. H. Ma

Publications and source records attributed to G. H. Ma.

4 recordsLinked to original sources

arXiv2005

Ultrafast and Large Third-order Nonlinear Optical Properties of CdS Nanocrystals in Polymeric Film

We report the ultrafast and large third-order nonlinear optical properties of CdS nanocrystals (NCs) embedded in a polymeric film. The CdS NCs of 2-nm radius are synthesized by an ion exchange method and highly concentrated in the two layers near the surfaces of the polymeric film. The two-photon absorption coefficient and the optical Kerr coefficient are measured with laser pulses of 250-fs duration at 800-nm wavelength. The one-photon and two-photon figures of merit are determined to be 3.1 and 1.3, respectively, at irradiance of 2 GW/cm2. The observed nonlinearities have a recovery time of ~ 1 ps. The two-photon-generated free carrier effects have also been observed and discussed. These results demonstrate that CdS NCs embedded in polymeric film are a promising candidate for optical switching applications.

cond-mat.mtrl-sci↗

arXiv2005

Excitonic nonlinear absorption in CdS nanocrystals studied using Z-scan technique

Irradiance dependence of excitonic nonlinear absorption in Cadmium Sulfide (CdS) nanocrystals has been studied by using Z-scan method with nanosecond laser pulses. The wavelength dependence of nonlinear absorption has also been measured near the excitonic transition of 1S(e)-1S3/2(h). We observe the saturable absorption, which can be described by a third-order and a fifth-order nonlinear process for both 3.0-nm-sized and 2.3-nm-sized CdS nanocrystals. The experimental results show that the excitonic nonlinear absorption of CdS nanocrystals is greatly enhanced with decreasing particle size. A two-level model is utilized to explain both irradiance and wavelength dependence of the excitonic nonlinearity.

cond-mat.mtrl-sci↗

arXiv2005

Terahertz generation in Czochralski grown periodically poled Mg:Y:LiNbO3 via optical rectification

Using a canonical pump-probe experimental technique, we studied the terahertz (THz) waves generation and detection via optical rectification and mixing in Czochralski-grown periodically poled Mg:Y:LiNbO3 (PPLN) crystals. THz waves with frequencies at 1.37 THz and 0.68 THz as well as 1.8 THz were obtained for PPLN with nonlinear grating periods of 0.03 and 0.06 mm, respectively. A general theoretical model was developed by considering the dispersion and damping of low frequency phonon-polariton mode. Our results show that THz waves are generated in forward and backward directions via pumping pulse rectification. The generated THz waves depend on the spectral shape of the laser pulses, quasi-phase mismatches and dispersion characteristics of a crystal.

physics.optics↗

arXiv2003

Ultrafast absorptive and refractive nonlinearities in multi-walled carbon nanotube film

By using femtosecond laser pulses at a wavelength range from 720 to 780 nm, we have observed absorptive and refractive nonlinearities in a film of multi-walled carbon nanotubes grown mainly along the direction perpendicular to the surface of quartz substrate. The Z-scans show that both absorptive and refractive nonlinearities are of negative and cubic nature in the laser irradiance range from a few to 300 GW/cm^2. The magnitude of the third-order nonlinear susceptibility,chi-(3), is of an order of 10^-11 esu. The degenerate pump-probe measurement reveals a relaxation time of 2 ps.

cond-mat.mtrl-sci↗