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G. J. Lane

Publications and source records attributed to G. J. Lane.

At least 37 records · Page 2Linked to original sources

First direct observation of isomeric decay in neutron-rich odd-odd $^{186}$Ta

De-excitation $γ$ rays associated with an isomeric state of $^{186}$Ta were investigated. The isomers were produced in multinucleon transfer reactions between a $^{136}$Xe beam and a natural W target, and were collected and separated by the KEK Isotope Separation System. Two $γ$ transitions with energies of 161.1(2) and 186.8(1) keV associated with an isomeric decay were observed for the first time. The half-life of the isomeric state of the neutral atom $^{186 \rm m}$Ta was deduced as 17(2) s. Based on the comparison with the previous measurements of the isomeric state using the ESR storage ring at GSI Darmstadt and the coupling of angular momenta of individual particle orbitals in odd-odd nuclei, a decay scheme of $^{186 \rm m}$Ta was proposed.

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Quenching factor measurements of sodium nuclear recoils in NaI:Tl determined by spectrum fitting

We have performed measurements of sodium nuclear recoils in NaI:Tl crystals, following scattering by neutrons produced in a $^{7}$Li(p,n)$^{7}$Be reaction. Understanding the light output from such recoils, which is reduced relative to electrons of equivalent energy by the quenching factor, is critical to interpret dark matter experiments that search for nuclear scattering interactions. We have developed a spectrum-fitting methodology to extract the quenching factor from our measurements, and report quenching factors for nuclear recoil energies between 36 and 401 keV. Our results agree with other recent quenching factor measurements that use quasi-monoenergetic neutron sources. The new method will be applied in the future to the NaI:Tl crystals used in the SABRE experiment.

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Characterization of SABRE crystal NaI-33 with direct underground counting

Ultra-pure NaI(Tl) crystals are the key element for a model-independent verification of the long standing DAMA result and a powerful means to search for the annual modulation signature of dark matter interactions. The SABRE collaboration has been developing cutting-edge techniques for the reduction of intrinsic backgrounds over several years. In this paper we report the first characterization of a 3.4 kg crystal, named NaI-33, performed in an underground passive shielding setup at LNGS. NaI-33 has a record low $^{39}$K contamination of 4.3$\pm$0.2 ppb as determined by mass spectrometry. We measured a light yield of 11.1$\pm$0.2 photoelectrons/keV and an energy resolution of 13.2% (FWHM/E) at 59.5 keV. We evaluated the activities of $^{226}$Ra and $^{228}$Th inside the crystal to be $5.9\pm0.6 μ$Bq/kg and $1.6\pm0.3 μ$Bq/kg, respectively, which would indicate a contamination from $^{238}$U and $^{232}$Th at part-per-trillion level. We measured an activity of 0.51$\pm$0.02 mBq/kg due to $^{210}$Pb out of equilibrium and a $α$ quenching factor of 0.63$\pm$0.01 at 5304 keV. We illustrate the analyses techniques developed to reject electronic noise in the lower part of the energy spectrum. A cut-based strategy and a multivariate approach indicated a rate, attributed to the intrinsic radioactivity of the crystal, of $\sim$1 count/day/kg/keV in the [5-20] keV region.

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Ground-state and decay properties of neutron-rich 106Nb

The ground-state properties of neutron-rich 106Nb and its beta decay into 106Mo have been studied using the CARIBU radioactive-ion-beam facility at Argonne National Laboratory. Niobium-106 ions were extracted from a 252Cf fission source and mass separated before being delivered as low-energy beams to the Canadian Penning Trap, as well as the X-Array and SATURN beta-decay-spectroscopy station. The measured 106Nb ground-state mass excess of -66202.0(13) keV is consistent with a recent measurement but has three times better precision; this work also rules out the existence of a second long-lived, beta-decaying state in 106Nb above 5 keV in excitation energy. The decay half-life of 106Nb was measured to be 1.097(21) s, which is 8% longer than the adopted value. The level scheme of the decay progeny, 106Mo, has been expanded up to approximately 4 MeV. The distribution of decay strength and considerable population of excited states in 106Mo of J >= 3 emphasises the need to revise the adopted Jpi = 1- ground-state spin-parity assignment of 106Nb; it is more likely to be J => 3.

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Properties of 187Ta revealed through isomeric decay

Mass-separated 187Ta in a high-spin isomeric state has been produced for the first time by multi-nucleon transfer reactions, employing an argon gas stopping cell and laser ionisation. Internal gamma rays revealed a 7.3 s isomer at 1778 keV, which decays through a rotational band with perturbations associated with the approach to a prolate-oblate shape transition. Model calculations show less influence from triaxiality compared to heavier elements in the same mass region. The isomer decay reduced E2 hindrance factor of 27 supports the interpretation that axial symmetry is approximately conserved.

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Improved precision on the experimental E0 decay branching ratio of the Hoyle state

Stellar carbon synthesis occurs exclusively via the $3α$ process, in which three $α$ particles fuse to form $^{12}$C in the excited Hoyle state, followed by electromagnetic decay to the ground state. The Hoyle state is above the $α$ threshold, and the rate of stellar carbon production depends on the radiative width of this state. The radiative width cannot be measured directly, and must instead be deduced by combining three separately measured quantities. One of these quantities is the $E0$ decay branching ratio of the Hoyle state, and the current $10$\% uncertainty on the radiative width stems mainly from the uncertainty on this ratio. The $E0$ branching ratio was deduced from a series of pair conversion measurements of the $E0$ and $E2$ transitions depopulating the $0^+_2$ Hoyle state and $2^+_1$ state in $^{12}$C, respectively. The excited states were populated by the $^{12}$C$(p,p^\prime)$ reaction at 10.5 MeV beam energy, and the pairs were detected with the electron-positron pair spectrometer, Super-e, at the Australian National University. The deduced branching ratio required knowledge of the proton population of the two states, as well as the alignment of the $2^+_1$ state in the reaction. For this purpose, proton scattering and $γ$-ray angular distribution experiments were also performed. An $E0$ branching ratio of $Γ^{E0}_π/Γ=8.2(5)\times10^{-6}$ was deduced in the current work, and an adopted value of $Γ^{E0}_π/Γ=7.6(4)\times10^{-6}$ is recommended based on a weighted average of previous literature values and the new result. The new recommended value for the $E0$ branching ratio is about 14% larger than the previous adopted value of $Γ^{E0}_π/Γ=6.7(6)\times10^{-6}$, while the uncertainty has been reduced from 9% to 5%.

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Emerging nuclear collectivity in $^{124-130}$Te

The emergence of nuclear collectivity near doubly-magic $^{132}$Sn was explored along the stable, even-even $^{124-130}$Te isotopes. Preliminary measurements of the $B(E2;4^{+}_{1}\rightarrow2^{+}_{1})$ transition strengths are reported from Coulomb excitation experiments primarily aimed at measuring the $g$ factors of the $4^{+}_{1}$ states. Isotopically enriched Te targets were excited by 198-205 MeV $^{58}$Ni beams. A comparison of transition strengths obtained is made to large-scale shell-model calculations with successes and limitations discussed.

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$E0$ transition strength in stable Ni isotopes

Excited states in $^{58,60,62}$Ni were populated via inelastic proton scattering at the Australian National University as well as via inelastic neutron scattering at the University of Kentucky Accelerator Laboratory. The Super-e electron spectrometer and the CAESAR Compton-suppressed HPGe array were used in complementary experiments to measure conversion coefficients and $δ(E2/M1)$ mixing ratios, respectively, for a number of $2^+ \rightarrow 2^+$ transitions. The data obtained were combined with lifetimes and branching ratios to determine $E0$, $M1$, and $E2$ transition strengths between $2^+$ states. The $E0$ transition strengths between $0^+$ states were measured using internal conversion electron spectroscopy and compare well to previous results from internal pair formation spectroscopy. The $E0$ transition strengths between the lowest-lying $2^+$ states were found to be consistently large for the isotopes studied.

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First-excited state $g$ factors in the stable, even Ge and Se isotopes

Transient-field $g$-factor measurements in inverse kinematics were performed for the first-excited states of the stable, even isotopes of Ge and Se. The $g$ factors of $^{74}$Ge and $^{74}$Se were measured simultaneously using a cocktail beam, which eliminates most possible sources of systematic error in a relative $g$-factor measurement. The results are $g(^{74}{\rm Se})/g(^{74}{\rm Ge})=1.34(7)$, $g(^{70}{\rm Ge})/g(^{74}{\rm Ge}) = 1.16(15)$, $g(^{72}{\rm Ge})/g(^{74}{\rm Ge})=0.92(13)$, $g(^{76}{\rm Ge})/g(^{74}{\rm Ge})=0.88(5)$, $g(^{76}{\rm Se})/g(^{74}{\rm Se})=0.96(7)$, $g(^{78}{\rm Se})/g(^{74}{\rm Se})=0.82(5)$, $g(^{80}{\rm Se})/g(^{74}{\rm Se})=0.99(7)$ and $g(^{82}{\rm Se})/g(^{74}{\rm Se})=1.19(6)$. The measured $g$-factor ratios are in agreement with ratios from previous measurements, despite considerable variation in previous reported absolute values. The absolute values of the $g$ factors remain uncertain, however the Rutgers parametrization was used to set the transient-field strength and then compare the experimental $g$ factors with shell-model calculations based on the JUN45 and jj44b interactions. Modest agreement was found between experiment and theory for both interactions. The shell model calculations indicate that the $g(2^+_1)$ values and trends are determined largely by the balance of the spin carried by orbital motion of the protons.

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The SABRE project and the SABRE PoP

SABRE aims to directly measure the annual modulation of the dark matter interaction rate with NaI(Tl) crystals. A modulation compatible with the standard hypothesis in which our Galaxy is embedded in a dark matter halo has been measured by the DAMA experiment in the same target material. Other direct detection experiments, using different target materials, seem to exclude the interpretation of such modulation in the simplest scenario of WIMP-nucleon elastic scattering. The SABRE experiment aims to carry out an independent search with sufficient sensitivity to confirm or refute the DAMA claim. The SABRE concept and goal is to obtain a background rate of the order of 0.1 cpd/kg/keVee in the energy region of interest. This challenging goal is achievable by operating high-purity crystals inside a liquid scintillator veto for active background rejection. In addition, twin detectors will be located in the northern and southern hemispheres to identify possible contributions to the modulation from seasonal or site-related effects. The SABRE project includes an initial Proof-of-Principle phase at LNGS (Italy), to assess the radio-purity of the crystals and the efficiency of the liquid scintillator veto. This paper describes the general concept of SABRE and the expected sensitivity to WIMP annual modulation.

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Monte Carlo simulation of the SABRE PoP background

SABRE (Sodium-iodide with Active Background REjection) is a direct dark matter search experiment based on an array of radio-pure NaI(Tl) crystals surrounded by a liquid scintillator veto. Twin SABRE experiments in the Northern and Southern Hemispheres will differentiate a dark matter signal from seasonal and local effects. The experiment is currently in a Proof-of-Principle (PoP) phase, whose goal is to demonstrate that the background rate is low enough to carry out an independent search for a dark matter signal, with sufficient sensitivity to confirm or refute the DAMA result during the following full-scale experimental phase. The impact of background radiation from the detector materials and the experimental site needs to be carefully investigated, including both intrinsic and cosmogenically activated radioactivity. Based on the best knowledge of the most relevant sources of background, we have performed a detailed Monte Carlo study evaluating the expected background in the dark matter search spectral region. The simulation model described in this paper guides the design of the full-scale experiment and will be fundamental for the interpretation of the measured background and hence for the extraction of a possible dark matter signal.

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Probing the $N = 14$ subshell closure: $g$ factor of the $^{26}$Mg(2$^+_1$) state

The first-excited state $g$~factor of $^{26}$Mg has been measured relative to the $g$ factor of the $^{24}$Mg($2^+_1$) state using the high-velocity transient-field technique, giving $g=+0.86\pm0.10$. This new measurement is in strong disagreement with the currently adopted value, but in agreement with the $sd$-shell model using the USDB interaction. The newly measured $g$ factor, along with $E(2^+_1)$ and $B(E2)$ systematics, signal the closure of the $νd_{5/2}$ subshell at $N=14$. The possibility that precise $g$-factor measurements may indicate the onset of neutron $pf$ admixtures in first-excited state even-even magnesium isotopes below $^{32}$Mg is discussed and the importance of precise excited-state $g$-factor measurements on $sd$~shell nuclei with $N\neq Z$ to test shell-model wavefunctions is noted.

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Identification of significant $E0$ strength in the $2^+_2 \rightarrow 2^+_1$ transitions of $^{58, 60, 62}$Ni

The $E0$ transition strength in the $2^+_2 \rightarrow 2^+_1$ transitions of $^{58,60,62}$Ni have been determined for the first time following a series of measurements at the Australian National University (ANU) and the University of Kentucky (UK). The CAESAR Compton-suppressed HPGe array and the Super-e solenoid at ANU were used to measure the $δ(E2/M1)$ mixing ratio and internal conversion coefficient of each transition following inelastic proton scattering. Level half-lives, $δ(E2/M1)$ mixing ratios and $γ$-ray branching ratios were measured at UK following inelastic neutron scattering. The new spectroscopic information was used to determine the $E0$ strengths. These are the first $2^+ \rightarrow 2^+$ $E0$ transition strengths measured in nuclei with spherical ground states and the $E0$ component is found to be unexpectedly large; in fact, these are amongst the largest $E0$ transition strengths in medium and heavy nuclei reported to date.

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High-spin spectroscopy and shell-model interpretation of the N < 126 radium isotopes $^{212}$Ra and $^{213}$Ra

The level structures of $^{212}$Ra and $^{213}$Ra have been established via time-correlated $γ$-ray spectroscopy following the $^{204}$Pb($^{12}$C,4$n$)$^{212}$Ra and $^{204}$Pb($^{13}$C,4$n$)$^{213}$Ra reactions. In $^{212}$Ra, levels up to $\sim 6.2$ MeV were identified and firm spin-parity assignments were achieved to a $J^π = 19^+$ isomer with a mean life of 31(3) ns. For $^{213}$Ra the corresponding values were $\sim 4.5$ MeV in excitation energy and $J^π = 33/2^+$. Two isomeric states with $J^π= 23/2^+$, $τ= 27(3)$ ns and $J^π= 33/2^+$, $τ= 50(3)$ ns were discovered in $^{213}$Ra. The experimental data were compared with semiempirical shell-model calculations, which allowed dominant configurations to be assigned to most of the observed levels.

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Perturbed angular distributions with LaBr$_3$ detectors: the $g$ factor of the first ${10^+}$ state in $^{110}$Cd revisited

The Time Differential Perturbed Angular Distribution technique with LaBr$_3$ detectors has been applied to the $I^π= \frac{11}{2}^-$ isomeric state ($E_x = 846$ keV, $τ=107$~ns) in $^{107}$Cd, which was populated and recoil-implanted into a gadolinium host following the $^{98}$Mo($^{12}$C, $3n$)$^{107}$Cd reaction. The static hyperfine field strength of Cd recoil implanted into gadolinium was thus measured, together with the fraction of nuclei implanted into field-free sites, under similar conditions as pertained for a previous implantation perturbed angular distribution $g$-factor measurement on the $I^π= 10^+$ state in $^{110}$Cd. The $^{110}$Cd $g(10^+)$ value was thereby re-evaluated, bringing it into agreement with the value expected for a seniority-two $νh_{\frac{11}{2}}$ configuration.

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Fast Rotation of the N=Z Nucleus 36Ar

A highly-deformed rotational band has been identified in the N=Z nucleus 36Ar. At high spin the band is observed to its presumed termination at I=16+, while at low spin it has been firmly linked to previously known states in 36Ar. Spins, parities, and absolute excitation energies have thus been determined throughout the band. Lifetime measurements establish a large low-spin quadrupole deformation (beta_2=0.46+-0.03) and indicate a decreasing collectivity as the band termination is approached. With effectively complete spectroscopic information and a valence space large enough for significant collectivity to develop, yet small enough to be meaningfully approached from the shell model perspective, this rotational band in 36Ar provides many exciting opportunities to test and compare complementary models of collective motion in nuclei.

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Incipient magnetic rotation? A magnetic dipole band in 104Cd

High spin states of the nucleus 104Cd have been studied using the Gammapshere array. The level scheme for 104Cd has been revised and evidence for a structure consisting of magnetic dipole transitions is presented. Shell model calculations, published previously, are invoked to support an interpretation of this structure as an incpient case of magnetic rotation where the transversal magnetic dipole moment is not strong enough to break the signature symmetry.

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Collective T=0 pairing in N=Z nuclei? Pairing vibrations around 56Ni revisited

We present a new analysis of the pairing vibrations around 56Ni, with emphasis on odd-odd nuclei. This analysis of the experimental excitation energies is based on the subtraction of average properties that include the full symmetry energy together with volume, surface and Coulomb terms. The results clearly indicate a collective behavior of the isovector pairing vibrations and do not support any appreciable collectivity in the isoscalar channel.

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