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G. Karapetrov

Publications and source records attributed to G. Karapetrov.

At least 37 records · Page 2Linked to original sources
arXiv2016

Superconductivity and hybrid soft modes in TiSe$_2$

The competition between superconductivity and other ground states of solids is one of the challenging topics in condensed matter physics. Apart from high-temperature superconductors [1,2] this interplay also plays a central role in the layered transition-metal dichalcogenides, where superconductivity is stabilized by suppressing charge-density-wave order to zero temperature by intercalation [3] or applied pressure [4-7]. 1T-TiSe$_2$ forms a prime example, featuring superconducting domes on intercalation as well as under applied pressure. Here, we present high energy-resolution inelastic x-ray scattering measurements of the CDW soft phonon mode in intercalated Cu$_x$TiSe$_2$ and pressurized 1T-TiSe$_2$ along with detailed ab-initio calculations for the lattice dynamical properties and phonon-mediated superconductivity. We find that the intercalation-induced superconductivity can be explained by a solely phonon-mediated pairing mechanism, while this is not possible for the superconducting phase under pressure. We argue that a hybridization of phonon and exciton modes in the pairing mechanism is necessary to explain the full observed temperature-pressure-intercalation phase diagram. These results indicate that 1T-TiSe$_2$ under pressure is close to the elusive state of the excitonic insulator.

cond-mat.supr-con↗
arXiv2015

Emergence of coherence in the charge-density wave state of 2H-NbSe$_2$

A charge-density wave (CDW) state has a broken symmetry described by a complex order parameter with an amplitude and a phase. The conventional view, based on clean, weak-coupling systems, is that a finite amplitude and long-range phase coherence set in simultaneously at the CDW transition temperature T$_{cdw}$. Here we investigate, using photoemission, X-ray scattering and scanning tunneling microscopy, the canonical CDW compound 2H-NbSe$_2$ intercalated with Mn and Co, and show that the conventional view is untenable. We find that, either at high temperature or at large intercalation, CDW order becomes short-ranged with a well-defined amplitude that impacts the electronic dispersion, giving rise to an energy gap. The phase transition at T$_{cdw}$ marks the onset of long-range order with global phase coherence, leading to sharp electronic excitations. Our observations emphasize the importance of phase fluctuations in strongly coupled CDW systems and provide insights into the significance of phase incoherence in `pseudogap' states.

cond-mat.str-el↗
arXiv2015

Superconducting properties of sulfur-doped iron selenide

The recent discovery of high-temperature superconductivity in single-layer iron selenide has generated significant experimental interest for optimizing the superconducting properties of iron-based superconductors through the lattice modification. For simulating the similar effect by changing the chemical composition due to S doping, we investigate the superconducting properties of high-quality single crystals of FeSe$_{1-x}$S$_{x}$ ($x$=0, 0.04, 0.09, and 0.11) using magnetization, resistivity, the London penetration depth, and low temperature specific heat measurements. We show that the introduction of S to FeSe enhances the superconducting transition temperature $T_{c}$, anisotropy, upper critical field $H_{c2}$, and critical current density $J_{c}$. The upper critical field $H_{c2}(T)$ and its anisotropy are strongly temperature dependent, indicating a multiband superconductivity in this system. Through the measurements and analysis of the London penetration depth $λ_{ab}(T)$ and specific heat, we show clear evidence for strong coupling two-gap $s$-wave superconductivity. The temperature-dependence of $λ_{ab}(T)$ calculated from the lower critical field and electronic specific heat can be well described by using a two-band model with $s$-wave-like gaps. We find that a $d$-wave and single-gap BCS theory under the weak-coupling approach can not describe our experiments. The change of specific heat induced by the magnetic field can be understood only in terms of multiband superconductivity.

cond-mat.supr-con↗
arXiv2014

Neutron Reflectometry Studies on Magnetic Stripe Domains in Permalloy/Superconductor bilayers

We explored changes in magnetic domain structures in a magnetic layer due to the onset of the superconductivity of an adjacent superconductive layer using neutron reflectometry. Magnetic domain structures in 1~$μ$m thick permalloy (Py) films were studied as functions of magnetic field, temperature and under the influence of the onset of superconductivity in a neighboring layer. Bragg peaks in the off-specular scattering were observed at low fields following saturation with an in-plane field, which are attributed to the quasi-parallel magnetic stripes along the field direction. During the magnetization reversal from saturation, the stripe pattern shows increases in the period, the transverse coherence length (\textit{i.e.}, perpendicular to the stripes) and the amplitude of the out-of-plane magnetization component. The coherence length of the magnetic stripes is anisotropic in the remnant state with the longitudinal coherence length (\textit{i.e.}, along the stripes) being larger than the transverse one. The stripe period shows a weak temperature dependence between 300~K and 3~K, but no abrupt change in the period is observed when the temperature crosses the superconducting critical temperature.

cond-mat.mes-hall↗
arXiv2013

Magnetization Properties and Vortex Phase Diagram in CuxTiSe2 Single Crystals

We have investigated the magnetization properties and flux dynamics of superconducting Cu$_x$TiSe$_2$ single crystals within wide range of copper concentrations. We find that the superconducting anisotropy is low and independent on copper concentration ($γ\sim1.7$), except in the case of strongly underdoped samples ($x\leq0.06$) that show a gradual increase in anisotropy to $γ\sim1.9$. The vortex phase diagram in this material is characterized by broad region of vortex liquid phase that is unusual for such low-$T_c$ superconductor with low anisotropy. Below the irreversibility line the vortex solid state supports relatively low critical current densities as compared to the depairing current limit ($J_c/J_0\sim10^{-7}$). All this points out that local fluctuations in copper concentration have little effect on bulk pinning properties in this system.

cond-mat.supr-con↗
arXiv2013

Heat Capacity of Single Crystal CuxTiSe2 Superconductors

We present heat capacity measurements on a series of superconducting Cu$_x$TiSe$_2$ single crystals with different Cu content down to 600 mK and up to 1 T performed by ac microcalorimetry. The samples cover a large portion of the phase diagram from an underdoped to a slightly overdoped region with an increasing superconducting critical temperature and the charge density wave (CDW) order gradually suppressed. The electronic heat capacity as a function of normalized temperature $T/T_c$ shows no difference regardless of the concentration of copper, i.e., regardless of how much the CDW order is developed in the samples. The data analysis reveals consistently a single s-wave gap with an intermediate coupling strength $2Δ/k_BT_c$ = 3.7 for all samples.

cond-mat.supr-con↗
arXiv2012

Evidence of Vortex Jamming in Abrikosov Vortex Flux Flow Regime

We report on dynamics of non-local Abrikosov vortex flow in mesoscopic superconducting Nb channels. Magnetic field dependence of the non-local voltage induced by the flux flow shows that vortices form ordered vortex chains. Voltage asymmetry (rectification) with respect to the direction of vortex flow is evidence that vortex jamming strongly moderates vortex dynamics in mesoscopic geometries. The findings can be applied to superconducting devices exploiting vortex dynamics and vortex manipulation, including superconducting wires with engineered pinning centers.

cond-mat.supr-con↗
arXiv2011

Electron-Phonon Coupling and the Soft Phonon Mode in TiSe$_2$

We report high-resolution inelastic x-ray measurements of the soft phonon mode in the charge-density-wave compound TiSe$_2$. We observe a complete softening of a transverse optic phonon at the L point, i.e. q = (0.5, 0, 0.5), at T ~ T_{CDW}. Renormalized phonon energies are observed over a large wavevector range $(0.3, 0, 0.5) \le \mathbf{q} \le (0.5, 0, 0.5)$. Detailed ab-initio calculations for the electronic and lattice dynamical properties of TiSe2 are in quantitative agreement with experimental frequencies for the phonon branch involving the soft mode. The observed broad range of renormalized phonon frequencies is directly related to a broad peak in the electronic susceptibility stabilizing the charge-density-wave ordered state. Our analysis demonstrates that a conventional electron-phonon coupling mechanism can explain a structural instability and the charge-density-wave order in TiSe_2 although other mechanisms might further boost the transition temperature.

cond-mat.str-el↗
arXiv2010

Muon spin rotation study of the magnetic penetration depth in the intercalated graphite superconductor CaC6

We report temperature- and magnetic field-dependent bulk muon spin rotation measurements in a c-axis oriented superconductor CaC6 in the mixed state. Using both a simple second moment analysis and the more precise analytical Ginzburg-Landau model, we obtained a field independent in-plane magnetic penetration depth λab (0) = 72(3) nm. The temperature dependencies of the normalized muon spin relaxation rate and of the normalized superfluid density result to be identical, and both are well represented by the clean limit BCS model with 2Δ/kB Tc = 3.6(1), suggesting that CaC6 is a fully gapped BCS superconductor in the clean limit regime.

cond-mat.supr-con↗
arXiv2009

Transverse instabilities of multiple vortex chains in superconductor-ferromagnet bilayers

Using scanning tunneling microscopy and Ginzburg-Landau simulations we explore vortex configurations in magnetically coupled NbSe$_2$-Permalloy superconductor-ferromagnet bilayer. The Permalloy film with stripe domain structure induces periodic local magnetic induction in the superconductor creating a series of pinning-antipinning channels for externally added magnetic flux quanta. Such laterally confined Abrikosov vortices form quasi-1D arrays (chains). The transitions between multichain states occur through propagation of kinks at the intermediate fields. At high fields we show that the system becomes non-linear due to a change in both the number of vortices and the confining potential. The longitudinal instabilities of the resulting vortex structures lead to vortices `levitating' in the anti-pinning channels.

cond-mat.supr-con↗
arXiv2008

Guiding superconducting vortices by magnetic domain walls

We demonstrate a unique prospect for inducing anisotropic vortex pinning and manipulating the directional motion of vortices using the stripe domain patterns of a uniaxial magnetic film in a the superconducting/ferromagnetic hybrid. Our observations can be described by a model, which considers interactions between magnetic charges of vortices and surface magnetic charges of domains resulting in the enhanced pinning of vortices on domain walls.

cond-mat.supr-con↗
arXiv2004

Oscillatory Thickness Dependence of the Coercive Field in Magnetic 3D Anti-Dot Arrays

We present studies on magnetic nano-structures with 3D architectures, fabricated using electrodeposition in the pores of well-ordered templates prepared by self-assembly of polystyrene latex spheres. The coercive field is found to demonstrate an oscillatory dependence on film thickness reflecting the patterning transverse to the film plane. Our results demonstrate that 3D patterned magnetic materials are prototypes of a new class of geometrical multilayer structures in which the layering is due to local shape effects rather then compositional differences.

cond-mat.mes-hall↗
arXiv2002

Anisotropy of the Upper Critical Field and Critical Current in Single Crystal MgB$_2$

We report on specific heat, high magnetic field transport and $ac-$susceptibility measurements on magnesium diboride single crystals. The upper critical field $H_{c2}$ for magnetic fields perpendicular and parallel to the Mg and B planes is presented for the first time in the entire temperature range. A very different temperature dependence has been observed in the two directions which yields to a temperature dependent anisotropy with $Γ\sim$ 5 at low temperatures and about 2 near $T_c$. A peak effect is observed in susceptibility measurements for $H \sim $2 T parallel to the $c-$axis and the critical current density presnts a sharp maximum for $H$ parallel to the ab-plane.

cond-mat.supr-con↗
arXiv2002

Superconducting Transition and Phase Diagram of Single Crystal MgB2

The superconducting phase diagram of MgB2 was determined from magnetization, magneto-transport and the first single-crystal specific heat measurements. A zero-temperature in-plane coherence length of 8 nm is determined. The superconducting anisotropy increases from a value around 2 near Tc to above 4.5 at 22 K. For H||c a pronounced peak effect in the critical current occurs at the upper critical field. Evidence for a surface superconducting state is presented for H||c which might account for the wide spread in reported values of the anisotropy.

cond-mat.supr-con↗
arXiv2002

Two-Band Superconductivity in MgB2

The study of the anisotropic superconductor MgB2 using a combination of scanning tunneling microscopy and spectroscopy reveals two distinct energy gaps at Delta1=2.3 meV and Delta2=7.1 meV. Different spectral weights of the partial superconducting density of states (PDOS) are a reflection of different tunneling directions in this multi-band system. Our experimental observations are consistent with the existence of two-band superconductivity in the presence of interband superconducting pair interaction and quasiparticle scattering. Temperature evolution of the tunneling spectra follows the BCS scenario with both gaps vanishing at the bulk Tc. Indeed, the study of tunneling junctions exhibiting only the small gap (c-axis tunneling) clearly and reproducibly show that this gap persists up to the bulk Tc. The data confirm the importance of Fermi-surface sheet dependent superconductivity in MgB2 proposed in the multigap model by Liu et al.

cond-mat.supr-con↗
arXiv2002

Effect of High Energy Heavy Ion Irradiation on c-axis Oriented MgB2 Films

We report on the transport, magnetization, and scanning tunneling spectroscopy measurements on c-axis oriented thin films of MgB2 irradiated with high energy heavy ions of uranium and gold. We find a slight shift in the irreversibility and upper critical field lines to higher temperatures after irradiation. In addition, we observe an increase in the critical current at high temperatures near Tc2 and only a small change at low temperatures. Furthermore, we find no evidence for the existence of anisotropic pinning induced by heavy ion irradiation in this material. Tunneling spectra in an irradiated sample show a double gap structure with a flat background and very low zero-bias conductance, behaving in much the same way as the pristine unirradiated sample.

cond-mat.supr-con↗
arXiv2001

Scanning Tunneling Spectroscopy in MgB2

We present scanning tunneling microscopy measurements of the surface of superconducting MgB2 with a critical temperature of 39K. In zero magnetic field the conductance spectra can be analyzed in terms of the standard BCS theory with a smearing parameter Gamma. The value of the superconducting gap is 5.2 meV at 4.2 K, with no experimentally significant variation across the surface of the sample. The temperature dependence of the gap follows the BCS form, fully consistent with phonon-mediated superconductivity in this novel superconductor. The application of a magnetic field induces strong pair-breaking as seen in the conductance spectra in fields up to 6 T.

cond-mat.supr-con↗