arXiv subjects

G. Kim

Publications and source records attributed to G. Kim.

At least 19 recordsLinked to original sources

arXiv2026

From perovskite to infinite-layer nickelates: hole concentration from x-ray absorption

The difficulty of determining cation concentrations and oxygen stoichiometry in infinite-layer nickelate thin films has so far prevented clear experimental identification of the nickel electron configuration in the superconducting phase. We used soft x-ray absorption spectroscopy to study the successive changes in PrNiO$_x$ thin films at various intermediate stages of topotactic reduction with $x=2-3$. By comparing the Ni-$L$ edge spectra to single and double cluster ligand-field calculations, we find that none of our samples exhibit a pure $d^9$ configuration. Our quantitative analysis using the charge sum rule shows that even when films are maximally reduced, the averaged number of nickel $3d$ holes is 1.35. Superconducting samples have even higher values, calling into question the previously assumed limit of hole doping. Concomitant changes in the oxygen $K$-edge absorption spectra upon reduction indicate the presence of oxygen $2p$ holes, even in the most reduced films. Overall, our results suggest a complex interplay of hole doping mechanisms resulting from self-doping effects and oxygen non-stoichiometry.

cond-mat.supr-con↗

arXiv2025

Evolution of spin excitations in superconducting La$_{2-x}$Ca$_{x}$CuO$_{4-\delta}$ from the underdoped to the heavily overdoped regime

We investigate high-energy spin excitations in hole-doped La$_{2-x}$Ca$_{x}$CuO$_{4-\delta}$ films across a broad Ca doping range $x = 0.05-0.50$ using resonant inelastic x-ray scattering (RIXS). Polarization analysis and incident-photon energy detuning measurements confirm the persistence of collective paramagnon excitations up to $x = 0.50$. Consistent with previous studies on other cuprate families, we observe a pronounced crossover near $x = 0.15$, where paramagnon spectral weight is transferred to incoherent spin-flip excitations associated with the particle-hole continuum. The overall behavior of paramagnons in LCCO resembles that in other hole-doped cuprates and appears insensitive to the persistence of superconductivity at high doping levels in LCCO - up to at least $x = 0.50$, as demonstrated in prior work. These findings support the view that high-energy magnetic excitations probed by RIXS are not a major contributor to superconducting pairing, in line with theories of spin-fluctuation mediated superconductivity.

cond-mat.supr-con↗

arXiv2024

Performance of the prototype beam drift chamber for LAMPS at RAON with proton and Carbon-12 beams

Beam Drift Chamber (BDC) is designed to reconstruct the trajectories of incident rare isotope beams provided by RAON (Rare isotope Accelerator complex for ON-line experiments) into the experimental target of LAMPS (Large Acceptance Multi-Purpose Spectrometer). To conduct the performance test of the BDC, the prototype BDC (pBDC) is manufactured and evaluated with the high energy ion beams from HIMAC (Heavy Ion Medical Accelerator in Chiba) facility in Japan. Two kinds of ion beams, 100 MeV proton, and 200 MeV/u $^{12}$C, have been utilized for this evaluation, and the track reconstruction efficiency and position resolution have been measured as the function of applied high voltage. This paper introduces the construction details and presents the track reconstruction efficiency and position resolution of pBDC.

physics.ins-det↗

arXiv2024

Interplay between electronic and lattice superstructures in La$_{2-x}$Ca$_{x}$CuO$_{4}$

Complex oxides are well known to develop oxygen ordering patterns with well defined periodicities, but their interplay with electronic correlations remains largely unexplored. Here, we report resonant and non-resonant x-ray diffraction data indicating a four-unit-cell periodic superstructure related to oxygen vacancy ordering in La$_{2-x}$Ca$_{x}$CuO$_{4}$ films with doping levels from the underdoped ($x = 0.15$) to the extremely overdoped ($x = 0.50$) regime. Whereas the lattice superstructure is temperature independent up to 300 K, a strongly temperature dependent electronic charge density wave (CDW) is observed in the underdoped and slightly overdoped regimes ($x\leq0.20$). The periodicity, in-plane and out-of-plane correlation lengths of the CDW are locked in by the lattice superstructure. Our results highlight the necessity to consider lattice and electronic energetics on equal footing in the high-temperature oxygen-disordered phase to explain oxygen ordering phenomena in complex oxides.

cond-mat.str-el↗

arXiv2022

Twisted quantum interference in photoelectron holography with elliptically polarized fields

We perform a systematic analysis of how ultrafast photoelectron holography is influenced by an elliptically polarized field, with emphasis on quantum interference effects. We find that the interplay of the external field and the binding potential leads to twisted holographic patterns for low ellipticities and recover well-known angular offsets for high ellipticities. Using the Coulomb quantum-orbit strong-field approximation (CQSFA), we assess how the field ellipticity affects specific holographic patterns, such as the fan and the spider. The interplay of the external field and the binding potential leads to twisted holographic patterns in the fan, and to loss of contrast in the spider. This behavior can be traced back to interfering electron trajectories, and unequal changes in tunneling probability due to non-vanishing ellipticity. We also derive tunneling times analytically using the strong-field approximation (SFA), provide estimates for ellipticy ranges for which interference is expected to be prominent, and discuss how to construct continuous electron momentum distributions exploring the rotation symmetry around the origin.

quant-ph↗

arXiv2021

All-Optical and Microwave-Free Detection of Meissner Screening using Nitrogen-Vacancy Centers in Diamond

Microscopic studies on thin film superconductors play an important role for probing non-equilibrium phase transitions and revealing dynamics at the nanoscale. However, magnetic sensors with nanometer scale spatial and picosecond temporal resolution are essential for exploring these. Here, we present an all-optical, microwave-free method, that utilizes the negatively charged nitrogen-vacancy (NV) center in diamond as a non-invasive quantum sensor and enables the spatial detection of the Meissner state in a superconducting thin film. We place an NV implanted diamond membrane on a superconducting LSCO thin film. The strong B-field dependence of the NV photoluminescence (PL) allows us to investigate the Meissner screening in LSCO under an externally applied magnetic field in a non-resonant manner.

cond-mat.supr-con↗

arXiv2020

Dust polarized emission observations of NGC 6334; BISTRO reveals the details of the complex but organized magnetic field structure of the high-mass star-forming hub-filament network

[Abridged] Filaments and hubs have received special attention recently thanks to studies showing their role in star formation. While the column density and velocity structures of both filaments and hubs have been studied, their magnetic fields (B-field) are not yet characterized. We aim to understand the role of the B-field in the dynamical evolution of the NGC 6334 hub-filament network. We present new observations of the dust polarized emission at 850$\mu$m towards NGC 6334 obtained with the JCMT/POL-2. We study the distribution and dispersion of the polarized intensity ($PI$), the polarization fraction ($PF$), and the B-field angle ($\theta_{B}$). We derive the power spectrum of the intensity and $\theta_{B}$ along the ridge crest. Our analyses show a complex B-field structure when observed over the whole region ($\sim10$ pc), however, at smaller scales ($\sim1$ pc), $\theta_{B}$ varies coherently along the filaments. The observed power spectrum of $\theta_{B}$ can be well represented with a power law function with a slope $-1.33\pm0.23$, which is $\sim20\%$ shallower than that of $I$. This result is compatible with the properties of simulated filaments and may indicate the processes at play in the formation of filaments. $\theta_{B}$ rotates from being mostly perpendicular to the filament crests to mostly parallel as they merge with the hubs. This variation of $\theta_{B}$ may be tracing local velocity flows of matter in-falling onto the hubs. Our analysis suggests a variation of the energy balance along the crests of these filaments, from magnetically critical/supercritical at their far ends to magnetically subcritical near the hubs. We detect an increase of $PF$ towards the high-column density star cluster-forming hubs that may result from the increase of grain alignment efficiency due to stellar radiation from the newborn stars.

astro-ph.GA↗

arXiv2020

Distance, magnetic field and kinematics of a filamentary cloud LDN 1157

LDN 1157, is one of the several clouds situated in the cloud complex, LDN 1147/1158, represents a coma-shaped morphology with a well-collimated bipolar outflow emanating from a Class 0 protostar, LDN 1157-mm. The main goals of this work are (a) to map the inter-cloud magnetic field (ICMF) geometry of the region surrounding LDN 1157 to investigate its relationship with the cloud morphology, with the outflow direction and with the core magnetic field (CMF) geometry inferred from the mm- and sub-mm polarization results from the literature, and (b) to investigate the kinematic structure of the cloud. We carried out R-band polarization observations of the stars projected on the cloud to map the pc-scale magnetic field geometry and made spectroscopic observations of the entire cloud in 12CO, C18O and N2H+ (J=1-0) lines to investigate its kinematic structure. We obtained a distance of 340$\pm$3 pc to the LDN 1147/1158, complex based on the Gaia DR2 parallaxes and proper motion values of the three YSOs associated with the complex. A single filament of $\sim1.2$ pc in length and $\sim0.09$ pc in width is found to run all along the coma-shaped cloud. Based on the relationships between the ICMF, CMF, filament orientations, outflow direction, and the presence of an hour-glass morphology of the magnetic field, it is likely that the magnetic field had played an important role in the star formation process in LDN 1157. Combining the proper motions of the YSOs and the radial velocity of LDN 1147/1158 and another complex LDN 1172/1174 which is situated $\sim2$\dgr~east of it, we found that both the complexes are moving collectively toward the Galactic plane. The filamentary morphology of the east-west segment of LDN 1157 may have formed as a result of mass lost by ablation due to the interaction of the moving cloud with the ambient interstellar medium.

astro-ph.SR↗

arXiv2019

Proximity effect in [Nb(1.5nm)/Fe(x)]$_{10}$/Nb(50nm) superconducting/ferromagnet heterostructures

We have investigated the structural, magnetic and superconducting properties of [Nb(1.5nm)/Fe(x)]$_{10}$ superlattices deposited on a thick Nb(50nm) layer. Our investigation showed that the Nb(50nm) layer grows epitaxially at 800$^\circ$C on Al$_2$O$_3$(1$\bar{1}$02) substrate. Samples grown at this condition posses a high residual resistivity ratio of 15-20. By using neutron reflectometry we show that Fe/Nb superlattices with $x<$ 4 nm form a depth-modulated FeNb alloy with concentration of iron varying between 60% and 90%. This alloy has properties of a weak ferromagnet. Proximity of this weak ferromagnetic layer to a thick superconductor leads to an intermediate phase that is characterized by co-existing superconducting and normal-state domains. By increasing the thickness of the Fe layer to $x$ = 4 nm the intermediate phase disappears. We attribute the intermediate state to proximity induced non-homogeneous superconductivity in the periodic Fe/Nb structure.

cond-mat.supr-con↗

arXiv2019

Magnetic proximity effect in [Nb/Gd] superlattices seen by neutron scattering

We have used spin-polarized neutron reflectometry to investigate the magnetization profile of superlattices composed of ferromagnetic Gd and superconducting Nb layers. We have observed a partial suppression of ferromagnetic (F) order of Gd layers in [Gd($d_F$)/Nb(25nm)]$_{12}$ superlattices below the superconducting (S) transition of the Nb layers. The amplitude of the suppression decreases with increasing $d_F$. By analyzing the neutron spin asymmetry we conclude that the observed effect has an electromagnetic origin - the proximity-coupled S layers screen out the external magnetic field and thus suppress the F response of the Gd layers inside the structure. Our investigation demonstrates the considerable influence of electromagnetic effects on the magnetic properties of S/F systems.

cond-mat.supr-con↗

arXiv2010

A Robust Approach for the Growth of Epitaxial Spinel Ferrite Films

Heteroepitaxial spinel ferrites NiFe2O4 and CoFe2O4 films have been prepared by pulsed laser deposition (PLD) at various temperatures (175 - 690 {\deg}C) under ozone/oxygen pressure of 10 mTorr. Due to enhanced kinetic energy of ablated species at low pressure and enhanced oxidation power of ozone, epitaxy has been achieved at significantly lower temperatures than previously reported. Films grown at temperature below 550 {\deg}C show a novel growth mode, which we term "vertical step-flow" growth mode. Epitaxial spinel ferrite films with atomically flat surface over large areas and enhanced magnetic moment can be routinely obtained. Interestingly, the growth mode is independent of the nature of substrates (spinel MgAl2O4, perovskite SrTiO3, and rock salt MgO) and film thicknesses. The underlying growth mechanism is discussed.

cond-mat.mtrl-sci↗

arXiv2010

Study of the interactions of pions in the CALICE silicon-tungsten calorimeter prototype

A prototype silicon-tungsten electromagnetic calorimeter for an ILC detector was tested in 2007 at the CERN SPS test beam. Data were collected with electron and hadron beams in the energy range 8 to 80 GeV. The analysis described here focuses on the interactions of pions in the calorimeter. One of the main objectives of the CALICE program is to validate the Monte Carlo tools available for the design of a full-sized detector. The interactions of pions in the Si-W calorimeter are therefore confronted with the predictions of various physical models implemented in the GEANT4 simulation framework.

physics.ins-det↗

arXiv2010

Construction and Commissioning of the CALICE Analog Hadron Calorimeter Prototype

An analog hadron calorimeter (AHCAL) prototype of 5.3 nuclear interaction lengths thickness has been constructed by members of the CALICE Collaboration. The AHCAL prototype consists of a 38-layer sandwich structure of steel plates and highly-segmented scintillator tiles that are read out by wavelength-shifting fibers coupled to SiPMs. The signal is amplified and shaped with a custom-designed ASIC. A calibration/monitoring system based on LED light was developed to monitor the SiPM gain and to measure the full SiPM response curve in order to correct for non-linearity. Ultimately, the physics goals are the study of hadron shower shapes and testing the concept of particle flow. The technical goal consists of measuring the performance and reliability of 7608 SiPMs. The AHCAL was commissioned in test beams at DESY and CERN. The entire prototype was completed in 2007 and recorded hadron showers, electron showers and muons at different energies and incident angles in test beams at CERN and Fermilab.

physics.ins-det↗

arXiv2008

Design and Electronics Commissioning of the Physics Prototype of a Si-W Electromagnetic Calorimeter for the International Linear Collider

The CALICE collaboration is studying the design of high performance electromagnetic and hadronic calorimeters for future International Linear Collider detectors. For the electromagnetic calorimeter, the current baseline choice is a high granularity sampling calorimeter with tungsten as absorber and silicon detectors as sensitive material. A ``physics prototype'' has been constructed, consisting of thirty sensitive layers. Each layer has an active area of 18x18 cm2 and a pad size of 1x1 cm2. The absorber thickness totals 24 radiation lengths. It has been exposed in 2006 and 2007 to electron and hadron beams at the DESY and CERN beam test facilities, using a wide range of beam energies and incidence angles. In this paper, the prototype and the data acquisition chain are described and a summary of the data taken in the 2006 beam tests is presented. The methods used to subtract the pedestals and calibrate the detector are detailed. The signal-over-noise ratio has been measured at 7.63 +/- 0.01. Some electronics features have been observed; these lead to coherent noise and crosstalk between pads, and also crosstalk between sensitive and passive areas. The performance achieved in terms of uniformity and stability is presented.

physics.ins-det↗

arXiv2005

Formation, Manipulation, and Elasticity Measurement of a Nanometric Column of Water Molecules

Nanometer-sized columns of condensed water molecules are created by an atomic-resolution force microscope operated in ambient conditions. Unusual stepwise decrease of the force gradient associated with the thin water bridge in the tip-substrate gap is observed during its stretch, exhibiting regularity in step heights (~0.5 N/m) and plateau lengths (~1 nm). Such "quantized" elasticity is indicative of the atomic-scale stick-slip at the tip-water interface. A thermodynamic-instability-induced rupture of the water meniscus (5-nm long and 2.6-nm wide) is also found. This work opens a high-resolution study of the structure and the interface dynamics of a nanometric aqueous column.

physics.flu-dyn↗

arXiv2004

PES and XAS Study on Electronic Structures of Multiferroic RMnO$_3$ (R=Y, Er)

Electronic structures of multiferroic RMnO$_3$ (R=Y, Er) have been investigated by employing photoemission spectroscopy (PES) and x-ray absorption spectroscopy (XAS). We have found that Mn ions in RMnO$_3$ are in the trivalent high-spin state with the total spin of S=2. The occupied Mn ($d_{xz} - d_{yz}$) states lie deep below $\rm E_F$, while the occupied Mn ($d_{xy} - d_{x^2 -y^2}$) states overlap very much with the O $2p$ states. It is observed that the PES spectral intensity of Mn 3d states is negligible above the occupied O $2p$ bands, suggesting that YMnO$_3$ is likely to be a charge-transfer insulator. The Mn $d_{3z^2 -r^2}$ state is mostly unoccupied in the ferroelectric phase of YMnO$_3$.

cond-mat.mtrl-sci↗

arXiv2002

An ionization chamber for (n,z) reaction cross section measurements on gaseous targets

An ionization chamber with gaseous samples has been designed. It has been tested on the beam of the pulsed reactor IBR-30 of FLNP, JINR-Dubna. The experiment has been carried out with resonance neutrons. The exposed gas volume serves as a target for neutron beam. We have compared the chamber to samples on substrates, the background component due to Li and B microimpurities in this case is totally absent. It has been tested also the recovery capability of the chamber after the reactor power pulse using the protons from the 3He(n,p)3H reaction, alpha-particles from a U-source and a pulsed precision generator. Moreover the energy resolution of the chamber with its equipment has been carried out.

nucl-ex↗

arXiv1999

Dipole and Quadrupole Moments of Mirror Nuclei 8B and 8li

Magnetic dipole and electric quadrupole moments of the mirror nuclei 8Li and 8B are analysed in the framework of the multiparticle shell model by using two approaches : i) the one-particle spectroscopic factors and ii) the one-particle fractional parentage coefficients. These two approaches are compared both each to other and with a microscopic multicluster model. The one-particle nucleon states are calculated taking into account the continuum by the method of the expansion of the Sturm - Liouville functions. The experimental magnetic and quadrupole moments of 8Li and 8Bare reproduced well by using fractional parentage coefficients technique. The root mean-square radii and the radial density distributions are obtained for these nuclei.

nucl-th↗