arXiv subjects

G. L. van de Stolpe

Publications and source records attributed to G. L. van de Stolpe.

5 recordsLinked to original sources

arXiv2026

Laser-induced creation of coherent V2 centers in bulk-grown silicon carbide

Solid-state spin defects are promising qubits for quantum network nodes. A key challenge towards larger networks is creating defects with high yield into nanophotonic devices, while maintaining good optical and spin properties. Here, we demonstrate the creation of V2 centers in nanopillars fabricated from commercial bulk-grown 4H-silicon carbide using a pulsed above-bandgap (UV) laser. We observe an eleven-fold increase in the V2 center occurrence after UV laser illumination. These laser-induced V2 centers exhibit narrow optical linewidths and spectral diffusion rates comparable to naturally occurring V2 centers in nanopillars of the same material. Furthermore, we measure a spin coherence time of $T_{2}^{\mathrm{DD}} = 3.6 \pm 0.3~\text{ms}$ under dynamical decoupling, consistent with dephasing by the nuclear-spin bath. This demonstration of the in-situ, post-fabrication generation of coherent V2 centers in nanostructures in widely available bulk-grown 4H-SiC, shows the potential for above-bandgap laser illumination for scalable defect creation in integrated photonic devices.

quant-ph↗

arXiv2024

Improved Electron-Nuclear Quantum Gates for Spin Sensing and Control

The ability to sense and control nuclear spins near solid-state defects might enable a range of quantum technologies. Dynamically Decoupled Radio-Frequency (DDRF) control offers a high degree of design flexibility and long electron-spin coherence times. However, previous studies considered simplified models and little is known about optimal gate design and fundamental limits. Here, we develop a generalised DDRF framework that has important implications for spin sensing and control. Our analytical model, which we corroborate by experiments on a single NV center in diamond, reveals the mechanisms that govern the selectivity of gates and their effective Rabi frequencies, and enables flexible detuned gate designs. We apply these insights to numerically show a 60x sensitivity enhancement for detecting weakly coupled spins and study the optimisation of quantum gates in multi-qubit registers. These results advance the understanding for a broad class of gates and provide a toolbox for application-specific design, enabling improved quantum control and sensing.

quant-ph↗

arXiv2024

Check-probe spectroscopy of lifetime-limited emitters in bulk-grown silicon carbide

Solid-state single-photon emitters provide a versatile platform for exploring quantum technologies such as optically connected quantum networks. A key challenge is to ensure optical coherence and spectral stability of the emitters. Here, we introduce a high-bandwidth `check-probe' scheme to quantitatively measure (laser-induced) spectral diffusion and ionisation rates, as well as homogeneous linewidths. We demonstrate these methods on single V2 centers in commercially available bulk-grown 4H-silicon carbide. Despite observing significant spectral diffusion under laser illumination ($\gtrsim$ GHz/s), the optical transitions are narrow ($\sim$35 MHz), and remain stable in the dark ($\gtrsim$1 s). Through Landau-Zener-Stückelberg interferometry, we determine the optical coherence to be near-lifetime limited ($T_2 = 16.4(4)$ ns), hinting at the potential for using bulk-grown materials for developing quantum technologies. These results advance our understanding of spectral diffusion of quantum emitters in semiconductor materials, and may have applications for studying charge dynamics across other platforms.

quant-ph↗

arXiv2024

Mapping a 50-spin-qubit network through correlated sensing

Spins associated to optically accessible solid-state defects have emerged as a versatile platform for exploring quantum simulation, quantum sensing and quantum communication. Pioneering experiments have shown the sensing, imaging, and control of multiple nuclear spins surrounding a single electron-spin defect. However, the accessible size of these spin networks has been constrained by the spectral resolution of current methods. Here, we map a network of 50 coupled spins through high-resolution correlated sensing schemes, using a single nitrogen-vacancy center in diamond. We develop concatenated double-resonance sequences that identify spin-chains through the network. These chains reveal the characteristic spin frequencies and their interconnections with high spectral resolution, and can be fused together to map out the network. Our results provide new opportunities for quantum simulations by increasing the number of available spin qubits. Additionally, our methods might find applications in nano-scale imaging of complex spin systems external to the host crystal.

quant-ph↗

arXiv2023

Hyperpolarisation of nuclear spins: polarisation blockade

Efficient hyperpolarisation of nuclear spins via optically active defect centers, such as the nitrogen vacancy (NV) center in diamond, has great potential for enhancing NMR based quantum information processing and nanoscale magnetic resonance imaging. Recently, pulse-based protocols have been shown to efficiently transfer optically induced polarisation of the electron defect spin to surrounding nuclear spins -- at particular resonant pulse intervals. In this work, we investigate the performance of these protocols, both analytically and experimentally, with the electronic spin of a single NV defect. We find that whenever polarisation resonances of nuclear spins are near-degenerate with a `blocking' spin, which is single spin with stronger off-diagonal coupling to the electronic central spin, they are displaced out of the central resonant region -- without, in general, significant weakening of the resonance. We analyse the underlying physical mechanism and obtain a closed form expression for the displacement. We propose that spin blocking represents a common but overlooked effect in hyperpolarisation of nuclear spins and suggest solutions for improved protocol performance in the presence of (naturally occurring) blocking nuclear spins.

quant-ph↗