arXiv subjects

G. M. Bruun

Publications and source records attributed to G. M. Bruun.

At least 19 recordsLinked to original sources

arXiv2026

Observation of low-lying impurity states in Bose-Einstein condensates

Impurities embedded in a Bose-Einstein Condensate (BEC) of 39K atoms are investigated with a pump-probe ejection spectroscopy sequence. The spectroscopic signal exhibits a strong feature corresponding to a Bose polaron in agreement with prior injection spectroscopy and theory. In addition, significant spectral weight at energies well below the energy of the polaron is observed, which is absent in injection spectroscopy. The energy and spectral weight of this signal are measured as a function of interaction strength and evolution time between the pump and probe pulses. We tentatively compare these results to two different theoretical models: a low-energy impurity state dressed by many bosonic excitations and a bipolaron state formed by two polarons due to attractive interactions mediated by the BEC. Such states can exist due to the large compressibility of the weakly interacting BEC. Both theories predict ejection spectra consistent with the low-energy signal, but only the bipolaron model is compatible with its spectral weight. These results indicate that lowenergy states below the usual polaron exist for strong interactions, calling for further experimental investigations

cond-mat.quant-gas↗

arXiv2025

Probing spatially resolved spin density correlations with trapped excitons

The rapidly growing class of atomically thin and tunable van der Waals materials is intensely investigated both in the context of fundamental science and for new technologies. There is in this connection a widespread need for new ways to probe the electronic properties of these layered materials, since their two-dimensional (2D) character make conventional probes less efficient. Here, we show how excitons trapped in a moiré lattice can be used as an optical probe for spatially resolved electron spin density correlations in such materials. The electrons in the material of interest virtually tunnel to the moiré lattice where they scatter on the excitons after which they tunnel back. This gives rise to an effective spin-dependent and spatially localised potential felt by the electrons, which in turn leads to energy shifts that can be measured spectroscopically in the exciton spectrum. Using second order perturbation theory combined with a solution to the exciton-electron scattering problem, we show that the electrons mediate an interaction between two excitons resulting in an energy shift proportional to their two-point spin density-density correlation function evaluated at the exciton positions. We then discuss two specific applications of our setup. First, we show that quantum phase transitions between different in-plane anti-ferromagnetic orders in a 2D lattice give rise to large and measurable shifts in the exciton spectrum in the critical regions. Second, we analyse how different pairing symmetries of superconducting phases can be probed. This demonstrates that our scheme opens up new ways to probe electron spin density correlations, which is a key property of many quantum phases predicted to exist in the new 2D materials.

cond-mat.mes-hall↗

arXiv2025

Dual Spectroscopy of Quantum Simulated Fermi-Hubbard Systems

Quantum gas microscopy with atoms in optical lattices provides remarkable insights into the real space properties of many-body systems, but does not directly reveal the nature of their fundamental excitation spectrum. Here, we demonstrate that radio-frequency spectroscopy can reveal the quasi-particle nature of doped quantum many-body systems, crucial for our understanding of, e.g., high-temperature superconductors. In particular, we showcase how the existence and energy of magnetic polaron quasi-particles in doped Fermi-Hubbard systems may be probed, revealed by hallmark peaks in the spectroscopic spectrum. In combination with fundamental dualities of the Fermi-Hubbard model, we describe how these findings may be tested using several experimental platforms.

cond-mat.quant-gas↗

arXiv2025

Probing a quantum spin liquid with equilibrium and nonequilibrium hole dynamics

The properties and experimental identification of quantum spin liquids (QSLs) remain an important topic with many fundamental questions. Here, we explore the dynamics of a single charge dopant (hole) in a $t$-$J_{1}$-$J_{2}$ model on a square lattice, which realizes a gapless $\mathbb{Z}_2$ QSL at half filling. Using a field theory approach based on the parton construction, which includes an infinite number of scatterings between the low-energy quasiparticle excitations of the QSL via a self-consistent Born approximation, we calculate both the equilibrium and nonequilibrium properties of the hole for weak and strong interactions. Quasiparticle branches as well as stringlike excitations of the holon are identified, and we furthermore explore the time-dependent spreading of a hole throughout the QSL after it has been injected at a given lattice site. The final ballistic expansion speed is shown to exhibit a nonmonotonic behavior as a quantum phase transition between an antiferromagnetic and the QSL phase is crossed, which is caused by a qualitative change in the fundamental kinematics of the interactions between the hole and the surrounding spins. Our results demonstrate how charge dopants can be used as a quantum probe for QSLs and are directly relevant to optical lattice experiments with single site resolution.

cond-mat.str-el↗

arXiv2023

Quantum beat spectroscopy of repulsive Bose polarons

The physics of impurities in a bosonic quantum environment is a paradigmatic and challenging many-body problem that remains to be understood in its full complexity. Here, this problem is investigated for impurities with strong repulsive interactions based on Ramsey interferometry in a quantum degenerate gas of 39K atoms. We observe an oscillatory signal that is consistent with a quantum beat between two co-existing coherent quasiparticle states: the attractive and repulsive polarons. The interferometric signal allows us to extract the polaron energies for a wide range of interaction strengths, complimenting earlier spectroscopic measurements. We furthermore identify several dynamical regimes towards the formation of the Bose polaron in good agreement with theory. Our results improve the understanding of quantum impurities interacting strongly with a bosonic environment, and demonstrate how quasiparticles as well as short-lived non-equilibrium many-body states can be probed using Ramsey interferometry.

cond-mat.quant-gas↗

arXiv2022

Nonequilibrium Hole Dynamics in Antiferromagnets: Damped Strings and Polarons

We develop a nonperturbative theory for hole dynamics in antiferromagnetic spin lattices, as described by the $t$-$J$ model. This is achieved by generalizing the selfconsistent Born approximation to nonequilibrium systems, making it possible to calculate the full time-dependent many-body wave function. Our approach reveals three distinct dynamical regimes, ultimately leading to the formation of magnetic polarons. Following the initial ballistic stage of the hole dynamics, coherent formation of string excitations gives rise to characteristic oscillations in the hole density. Their damping eventually leaves behind magnetic polarons that undergo ballistic motion with a greatly reduced velocity. The developed theory provides a rigorous framework for understanding nonequilibrium physics of defects in quantum magnets and quantitatively explains recent observations from cold-atom quantum simulations in the strong coupling regime.

cond-mat.quant-gas↗

arXiv2022

Mediated interactions between ions in quantum degenerate gases

We explore the interaction between two trapped ions mediated by a surrounding quantum degenerate Bose or Fermi gas. Using perturbation theory valid for weak atom-ion interaction, we show analytically that the interaction mediated by a Bose gas has a power-law behaviour for large distances whereas it has a Yukawa form for intermediate distances. For a Fermi gas, the mediated interaction is given by a power-law for large density and by a Ruderman-Kittel-Kasuya-Yosida form for low density. For strong atom-ion interactions, we use a diagrammatic theory to demonstrate that the mediated interaction can be a significant addition to the bare Coulomb interaction between the ions, when an atom-ion bound state is close to threshold. Finally, we show that the induced interaction leads to substantial and observable shifts in the ion phonon frequencies.

cond-mat.quant-gas↗

arXiv2021

Spatial structure of magnetic polarons in strongly interacting antiferromagnets

The properties of mobile impurities in quantum magnets are fundamental for our understanding of strongly correlated materials and may play a key role in the physics of high-temperature superconductivity. Hereby, the motion of hole-like defects through an antiferromagnet has been of particular importance. It creates magnetic frustrations that lead to the formation of a quasiparticle, whose complex structure continues to pose substantial challenges to theory and numerical simulations. In this article, we develop a non-perturbative theoretical approach to describe the microscopic properties of such magnetic polarons. Based on the self-consistent Born approximation, which is provenly accurate in the strong-coupling regime, we obtain a complete description of the polaron wave function by solving a set of Dyson-like equations that permit to compute relevant spin-hole correlation functions. We apply this new method to analyze the spatial structure of magnetic polarons in the strongly interacting regime and find qualitative differences from predictions of previously applied truncation schemes. Our calculations reveal a remarkably high spatial symmetry of the polaronic magnetization cloud and a surprising misalignment between its orientation and the polaron crystal momentum. The developed framework opens up an approach to the microscopic properties of doped quantum magnets and will enable detailed analyses of ongoing experiments based on cold-atom quantum simulations of the Fermi-Hubbard model.

cond-mat.str-el↗

arXiv2021

Topological transport of mobile impurities

We study the Hall response of topologically-trivial mobile impurities (Fermi polarons) interacting weakly with majority fermions forming a Chern-insulator background. This setting involves a rich interplay between the genuine many-body character of the polaron problem and the topological nature of the surrounding cloud. When the majority fermions are accelerated by an external field, a transverse impurity current can be induced. To quantify this polaronic Hall effect, we compute the drag transconductivity, employing controlled diagrammatic perturbation theory in the impurity-fermion interaction. We show that the impurity Hall drag is not simply proportional to the Chern number characterizing the topological transport of the insulator on its own - it also depends continuously on particle-hole breaking terms, to which the Chern number is insensitive. However, when the insulator is tuned across a topological phase transition, a sharp jump of the impurity Hall drag results, for which we derive an analytical expression. We describe how the Hall drag and jump can be extracted from a circular dichroic measurement of impurity excitation rates, particularly suited for ultracold gas experiments.

cond-mat.quant-gas↗

arXiv2020

Detecting chiral pairing and topological superfluidity using circular dichroism

Realising and probing topological superfluids is a key goal for fundamental science, with exciting technological promises. Here, we show that chiral $p_x+ip_y$ pairing in a two-dimensional topological superfluid can be detected through circular dichroism, namely, as a difference in the excitation rates induced by a clockwise and counter-clockwise circular drive. For weak pairing, this difference is to a very good approximation determined by the Chern number of the superfluid, whereas there is a non-topological contribution scaling as the superfluid gap squared that becomes signifiant for stronger pairing. This gives rise to a competition between the experimentally driven goal to maximise the critical temperature of the superfluid, and observing a signal given by the underlying topology. Using a combination of strong coupling Eliashberg and Berezinskii-Kosterlitz-Thouless theory, we analyse this tension for an atomic Bose-Fermi gas, which represents a promising platform for realising a chiral superfluid. We identify a wide range of system parameters where both the critical temperature is high and the topological contribution to the dichroic signal is dominant.

cond-mat.quant-gas↗

arXiv2020

Attractive and repulsive exciton-polariton interactions mediated by an electron gas

Realising strong photon-photon interactions in a solid-state setting is a major goal with far reaching potential for optoelectronic applications. Using Landau's quasiparticle framework combined with a microscopic many-body theory, we explore the interactions between exciton-polaritons and trions in a two-dimensional semiconductor injected with an electron gas inside a microcavity. We show that particle-hole excitations in the electron gas mediate an attractive interaction between the polaritons, whereas a trion-polariton interaction mediated by the exchange of an electron is either repulsive or attractive depending on the specific polariton branch. These mediated interactions are intrinsic to the quasiparticles and are also present in the absence of light. Importantly, they can be tuned to be more than an order of magnitude stronger than the direct polariton-polariton interaction in the absence of the electron gas, thereby providing a promising outlook for non-linear optical components. Finally, we compare our theoretical predictions with two recent experiments.

cond-mat.mes-hall↗

arXiv2020

Superfluid flow of polaron polaritons above Landau's critical velocity

We develop a theory for the interaction of light with superfluid optical media, describing the motion of quantum impurities that are created and dragged through the liquid by propagating photons. It is well known that a mobile impurity suffers dissipation due to phonon emission as soon as it moves faster than the speed of sound in the superfluid - Landau's critical velocity. Surprisingly we find that in the present hybrid light-matter setting, polaritonic impurities can be protected against environmental decoherence and be allowed to propagate well above the Landau velocity without jeopardizing the superfluid response of the medium.

cond-mat.quant-gas↗

arXiv2020

Mediated interactions and photon bound states in an exciton-polariton mixture

The quest to realise strongly interacting photons remains an outstanding challenge both for fundamental science and for applications. Here, we explore mediated photon-photon interactions in a highly imbalanced two-component mixture of exciton-polaritons in a semiconductor microcavity. Using a theory that takes into account non-perturbative correlations between the excitons as well as strong light-matter coupling, we demonstrate the high tunability of an effective interaction between quasiparticles formed by minority component polaritons interacting with a Bose-Einstein condensate (BEC) of a majority component polaritons. In particular, the interaction, which is mediated by the exchange of sound modes in the BEC can be made strong enough to support a bound state of two quasiparticles. Since these quasiparticles consist partly of photons, this in turn corresponds to a dimer state of photons propagating through the BEC. This gives rise to a new light transmission line where the bound state wave function is directly mapped onto correlations between outgoing photons. Our findings open up new routes for realising highly non-linear optical materials and novel hybrid light-matter quantum systems.

cond-mat.mes-hall↗

arXiv2020

Polariton dynamics in strongly interacting quantum many-body systems

We develop a theory for light propagating in an atomic Bose-Einstein condensate in the presence of strong interactions. The resulting many-body correlations are shown to have profound effects on the optical properties of this interacting medium. For weak atom-light coupling, there is a well-defined quasiparticle, the polaron-polariton, supporting light propagation with spectral features differing significantly from the noninteracting case. The damping of the polaron-polariton depends nonmonotonically on the light-matter coupling strength, initially increasing and then decreasing. This gives rise to an interesting crossover between two quasiparticles: a bare polariton and a polaron-polariton, separated by a complex and lossy mixture of light and matter.

cond-mat.quant-gas↗

arXiv2019

High Frequency Sound in a Unitary Fermi Gas

We present an experimental and theoretical study of the phonon mode in a unitary Fermi gas. Using two-photon Bragg spectroscopy, we measure excitation spectra at a momentum of approximately half the Fermi momentum, both above and below the superfluid critical temperature $T_\mathrm{c}$. Below $T_\mathrm{c}$, the dominant excitation is the Bogoliubov-Anderson (BA) phonon mode, driven by gradients in the phase of the superfluid order parameter. The temperature dependence of the BA phonon is consistent with a theoretical model based on the quasiparticle random phase approximation in which the dominant damping mechanism is via collisions with thermally excited quasiparticles. As the temperature is increased above $T_\mathrm{c}$, the phonon evolves into a strongly damped collisional mode, accompanied by an abrupt increase in spectral width. Our study reveals strong similarities between sound propagation in the unitary Fermi gas and liquid helium.

cond-mat.quant-gas↗

arXiv2019

Strong interactions and bi-excitons in a polariton mixture

We develop a many-body theory for the properties of exciton-polaritons interacting strongly with a Bose-Einstein condensate (BEC) of exciton-polaritons in another spin state. Interactions lead to the presence of a two-body bound state, the bi-exciton, giving rise to a Feshbach resonance in the polariton spectrum when its energy is equal to that of two free polaritons. Using the minimal set of terms to describe this resonance, our theory recovers the main findings of two experiments probing interaction effects for upper and lower polaritons in a BEC. This strongly supports that Feshbach physics has indeed been realized, and we furthermore extract the energy and decay of biexciton from the experimental data. The decay rate is predicted to be much larger than that coming from its dissociation into two free polaritons indicating that other decay channels are important.

cond-mat.quant-gas↗

arXiv2019

Analyzing a Bose polaron across resonant interactions

Recently, two independent experiments reported the observation of long-lived polarons in a Bose-Einstein condensate, providing an excellent setting to study the generic scenario of a mobile impurity interacting with a quantum reservoir. Here, we expand the experimental analysis by disentangling the effects of trap inhomogeneities and the many-body continuum in one of these experiments. This makes it possible to extract the energy of the polaron at a well-defined density as a function of the interaction strength. Comparisons with quantum Monte-Carlo as well as diagrammatic calculations show good agreement, and provide a more detailed picture of the polaron properties at stronger interactions than previously possible. Moreover, we develop a semi-classical theory for the motional dynamics and three-body loss of the polarons, which partly explains a previously unresolved discrepancy between theory and experimental observations for repulsive interactions. Finally, we utilize quantum Monte-Carlo calculations to demonstrate that the findings reported in the two experiments are consistent with each other.

cond-mat.quant-gas↗

arXiv2019

Dropping an impurity into a Chern insulator: a polaron view on topological matter

We investigate the properties of an impurity particle interacting with a Fermi gas in a Chern-insulating state. The interaction leads to the formation of an exotic polaron, which consists of a coherent superposition of the topologically-trivial impurity and the surrounding topological cloud. We characterize this intriguing topologically-composite object by calculating its transverse (Hall) conductivity, using diagrammatic as well as variational methods. The "polaronic Hall conductivity" is shown to be non-zero whenever the surrounding cloud is prepared in a non-trivial Chern insulating state, which we attribute to the transverse drag exerted by the dressing cloud on the impurity. In this way, the polaron partially inherits the topological properties of the Chern insulator through genuine interaction effects. This is also analysed at the microscopic level of wave functions, by identifying a "composite Berry curvature" for the polaron, which closely mimics the Berry curvature of the Chern insulator's band structure. Finally, we discuss how this interplay between topology and many-body correlations can be studied in cold-atom experiments, using available technologies.

cond-mat.quant-gas↗