arXiv subjects

G. M. Tveten

Publications and source records attributed to G. M. Tveten.

At least 37 records · Page 2Linked to original sources

arXiv2019

Restricted spin-range correction in the Oslo Method: The example of nuclear level density and $γ$-ray strength function from $^{239}\mathrm{Pu}(\mathrm{d,p}γ)^{240}\mathrm{Pu}$

The Oslo Method has been applied to particle-$γ$ coincidences following the $^{239}\mathrm{Pu}$(d,p) reaction to obtain the nuclear level density (NLD) and $γ$-ray strength function ($γ$SF) of $^{240}\mathrm{Pu}$. The experiment was conducted with a 12 MeV deuteron beam at the Oslo Cyclotron Laboratory. The low spin transfer of this reaction leads to a spin-parity mismatch between populated and intrinsic levels. This is a challenge for the Oslo Method as it can have a significant impact on the extracted NLD and $γ$SF. We have developed an iterative approach to ensure consistent results even for cases with a large spin-parity mismatch, in which we couple Green's Function Transfer calculations of the spin-parity dependent population cross-section to the nuclear decay code RAINIER. The resulting $γ$SF shows a pronounced enhancement between 2-4 MeV that is consistent with the location of the low-energy orbital $M1$ scissors mode.

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arXiv2019

First experimental constraint on the $^{191}$Os$(n,γ)$ reaction rate relevant to $s$-process nucleosynthesis

The nuclear level density and $γ$-decay strength of $^{192}$Os have been extracted using particle-$γ$ coincidence data from the $^{192}$Os($α,α^\primeγ$)$^{192}$Os reaction by means of the Oslo method. The level density is found to be a rather smooth function of excitation energy, approximately following the constant temperature model. The $γ$-decay strength is compared to photoneutron cross-section data above the neutron separation energy, and to $E1$ and $M1$ strengths for nuclei in this mass region derived from primary transitions following neutron capture. Our results are in good agreement with these previous data and draw a consistent picture of the $γ$-strength function in the range $E_γ\approx 1.5-6 $ MeV. Using the measured nuclear level density and $γ$-decay strength as input to the nuclear-reaction code TALYS, we provide the first experimentally constrained Maxwellian-averaged cross section (MACS) for the $^{191}$Os($n,γ$)$^{192}$Os reaction relevant to $s$-process nucleosynthesis. The systematic uncertainties introduced by the normalization procedure of the level density and $γ$-strength function were investigated and propagated to the calculated Maxwellian-averaged cross section. The obtained result of the Maxwellian-averaged cross section at $k_BT=30$ keV, $\langle σ\rangle_{n,γ}=1134\pm 375$ mb, is in very good agreement with the theoretical estimate provided by the KADoNiS project, giving experimental support to the adopted KADoNiS value. Good agreement is also found with MACS values obtained from other libraries, such as TENDL-2017, ENDF/B-VII.0, and JEFF.

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arXiv2019

Nuclear level densities and gamma-ray strength functions of $^{180,181,182}$Ta

Particle-$γ$ coincidence experiments were performed at the Oslo Cyclotron Laboratory with the $^{181}$Ta(d,X) and $^{181}$Ta($^{3}$He,X) reactions, to measure the nuclear level densities (NLDs) and $γ$-ray strength functions ($γ$SFs) of $^{180, 181, 182}$Ta using the Oslo method. The Back-shifted Fermi-Gas, Constant Temperature plus Fermi Gas, and Hartree-Fock-Bogoliubov plus Combinatorial models where used for the absolute normalisations of the experimental NLDs at the neutron separation energies. The NLDs and $γ$SFs are used to calculate the corresponding $^{181}$Ta(n,$γ$) cross sections and these are compared to results from other techniques. The energy region of the scissors resonance strength is investigated and from the data and comparison to prior work it is concluded that the scissors strength splits into two distinct parts. This splitting may allow for the determination of triaxiality and a $γ$ deformation of $14.9^{\circ} \pm 1.8^{\circ}$ was determined for $^{181}$Ta.

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arXiv2019

Impact of restricted spin-ranges in the Oslo Method: The example of (d,p)$^{240}\mathrm{Pu}$

In this paper we present the first systematic analysis of the impact of the populated vs. intrinsic spin distribution on the nuclear level density and $γ$-ray strength function retrieved through the Oslo Method. We illustrate the effect of the spin distribution on the recently performed $^{239}\mathrm{Pu}$(d,p$γ$)$^{240}\mathrm{Pu}$ experiment using a 12 MeV deuteron beam performed at the Oslo Cyclotron Lab. In the analysis we couple state-of-the-art calculations for the populated spin-distributions with the Monte-Carlo nuclear decay code RAINIER to compare Oslo Method results to the known input. We find that good knowledge of the populated spin distribution is crucial and show that the populated distribution has a significant impact on the extracted nuclear level density and $γ$-ray strength function for the $^{239}\mathrm{Pu}$(d,p$γ$)$^{240}\mathrm{Pu}$ case.

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arXiv2018

The $γ$-ray strength function for Thallium isotopes relevant to the $^{205}$Pb - $^{205}$Tl chronometry

Photoneutron cross sections were measured for $^{203}$Tl and $^{205}$Tl at energies between the one- and two-neutron thresholds using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. Our new measurement results in cross sections significantly different from the previously reported bremsstrahlung experiment, leading to rather different GDR parameters, in particular to lower GDR peak energies and higher peak cross sections. The photoneutron data are used to constrain the $γ$-ray strength function on the basis of the Hartree-Fock-Bogolyubov plus quasi-particle random phase approximation using the Gogny D1M interaction. Supplementing the experimentally constrained $γ$-ray strength function with the zero-limit E1 and M1 contributions for the de-excitation mode, we estimate the Maxwellian-averaged cross section for the s-process branching-point nucleus $^{204}$Tl in the context of the $^{205}$Pb - $^{205}$Tl chronometry.

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arXiv2018

Photoneutron cross sections for Ni isotopes: Toward understanding $(n,γ)$ cross sections relevant to the weak s-process nucleosynthesis

Photoneutron cross sections were measured for $^{58}$Ni, $^{60}$Ni, $^{61}$Ni, and $^{64}$Ni at energies between the one-neutron and two-neutron thresholds using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. The new photoneutron data are used to extract the $γ$-ray strength function above the neutron threshold complementing the information obtained by the Oslo method below the threshold. We discuss radiative neutron capture cross sections and the Maxwellian-averaged cross sections for Ni isotopes including $^{63}$Ni, a branching point nucleus along the weak s-process path. The cross sections are calculated with the experimentally constrained $γ$-ray strength functions from the Hartree-Fock-Bogolyubov plus quasi-particle-random phase approximation based on the Gogny D1M interaction for both $E1$ and $M1$ components and supplemented with the $M1$ upbend.

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arXiv2018

Experimental $γ$-decay strength in $^{59, 60}$Ni compared with microscopic calculations

Nuclear level densities and $γ$-ray strength functions have been extracted for $^{59, 60}\rm{Ni}$, using the Oslo method on data sets from the $^{60}$Ni($^{3}$He,$^{3}$He$^{\prime}γ$)$^{60}$Ni and $^{60}$Ni($^{3}$He,$αγ$)$^{59}$Ni reactions. Above the neutron separation energy, S$_n$, we have measured the $γ$-ray strength functions for $^{61}$Ni and $^{60}$Ni in photoneutron experiments. The low-energy part of the $^{59,60}$Ni $γ$-ray strength functions show an increase for decreasing $γ$ energies. The experimental $γ$-ray strength functions are compared with $M1$ $γ$-ray strength functions calculated within the shell model. The $E1$ $γ$-ray strength function of $^{60}$Ni has been calculated using the QTBA framework. The QTBA calculations describe the data above $E_γ\approx$ 7 MeV, while the shell-model calculations agree qualitatively with the low energy part of the $γ$-ray strength function. Hence, we give a plausible explanation of the observed shape of the $γ$-decay strength.

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arXiv2018

The gamma-ray strength function of $^{89}$Y and $^{90}$Y

In this work, we present new data on the $^{89}$Y($γ$,n) cross section studied with a quasi-monochromatic photon beam produced at the NewSUBARU synchrotron radiation facility in Japan contributing torwards resolving a long standing discrepancy between existing measurements of this cross section. Results for $γ$-ray strength function below threshold obtained by applying the Oslo method to $^{89}$Y($p,p'γ$)$^{89}$Y coincidences combined with the $^{89}$Y($γ$,n) data this providing experimental data for the $γ$-ray strength function of $^{89}$Y for $γ$ energies in the range of $\approx 1.6$ Mev to $\approx$ 20 MeV. A low-energy enhancement is seen for $γ$-rays below $\approx 2.5$ MeV. Shell-model calculations indicate that this feature is caused by strong, low-energy $M1$ transitions at high excitation energies. The nuclear level density and $γ$-ray strength function have been extracted from $^{89}$Y($d,p γ$)$^{90}$Y coincidences using the Oslo method. Using the ($γ,n$) and ($d,pγ$) data as experimental constraints, we have calculated the $^{89}$Y($n,γ$)$^{90}$Y cross section with the TALYS reaction code. Our results have been compared with directly measured (n,$γ$) cross sections and evaluations. The $N=50$ isotope $^{89}$Y is an important bottleneck in the s-process and the magnitude of the $^{89}$Y(n,$γ)$ cross section is key to understanding how s-process stars produce heavy isotopes.

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arXiv2018

Verification of detailed balance for $γ$ absorption and emission in Dy isotopes

The photo-neutron cross sections of $^{162,163}\rm{Dy}$ have been measured for the first time in an energy region from the neutron threshold ($S_n$) up to $\approx$ $13$~MeV. The ($γ$,n) reaction was induced with quasi-monochromatic laser Compton-scattered $γ$ rays, produced at the NewSUBARU laboratory. The corresponding $γ$-ray strength functions ($γ$SF) have been calculated from the photo-neutron cross sections. The data are compared to reanalyzed $γ$SFs of $^{160-164}\rm{Dy}$, which are measured below $S_n$. The excellent agreement with the photo-neutron data at $S_n$ confirms the principle of detailed balance. Thus, a complete $γ$SF is established covering in total the energy region of 1 MeV $\leq$ E$_γ$ $\leq$ 13 MeV. These mid-shell well-deformed dysprosium isotopes all show scissors resonances with very similar structures. We find that our data predict the same integrated scissors strength as ($γ,γ^\prime$) data when integrated over the same energy range, which shows that the scissors mode very likely is consistent with the generalized Brink hypothesis. Finally, using the $γ$SFs as input in the reaction code TALYS, we have deduced radiative neutron-capture cross sections and compared them to direct measurements. We find a very good agreement within the uncertainties, which gives further support to the experimentally determined $γ$SFs.

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arXiv2018

Gamma-widths, lifetimes and fluctuations in the nuclear quasi-continuum

Statistical $γ$-decay from highly excited states is determined by the nuclear level density (NLD) and the $γ$-ray strength function ($γ$SF). These average quantities have been measured for several nuclei using the Oslo method. For the first time, we exploit the NLD and $γ$SF to evaluate the $γ$-width in the energy region below the neutron binding energy, often called the quasi-continuum region. The lifetimes of states in the quasi-continuum are important benchmarks for a theoretical description of nuclear structure and dynamics at high temperature. The lifetimes may also have impact on reaction rates for the rapid neutron-capture process, now demonstrated to take place in neutron star mergers.

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arXiv2017

Energy dependence of the prompt $γ$-ray emission from the $(d,p)$-induced fission of $^{234}\mathrm{U}^{}$ and $^{240}\mathrm{Pu}^{}$

Prompt fission $γ$-rays are responsible for approximately 5\% of the total energy released in fission, and therefore important to understand when modelling nuclear reactors. In this work we present prompt $γ$-ray emission characteristics in fission, for the first time as a function of the nuclear excitation energy of the fissioning system. Emitted $γ$-ray spectra were measured, and $γ$-ray multiplicities and average and total $γ$ energies per fission were determined for the $^{233}$U(d,pf) reaction for excitation energies between 4.8 and 10 MeV, and for the $^{239}$Pu(d,pf) reaction between 4.5 and 9 MeV. The spectral characteristics show no significant change as a function of excitation energy above the fission barrier, despite the fact that an extra $\sim$5 MeV of energy is potentially available in the excited fragments for $γ$-decay. The measured results are compared to model calculations made for prompt $γ$-ray emission with the fission model code GEF. Further comparison with previously obtained results from thermal neutron induced fission is made to characterize possible differences arising from using the surrogate (d,p) reaction.

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arXiv2017

Low-energy enhancement and fluctuations of $γ$-ray strength functions in $^{56,57}$Fe: test of the Brink-Axel hypothesis

Nuclear level densities and $γ$-ray strength functions of $^{56,57}$Fe have been extracted from proton-$γ$ coincidences. A low-energy enhancement in the $γ$-ray strength functions up to a factor of 30 over common theoretical E1 models is confirmed. Angular distributions of the low-energy enhancement in $^{57}$Fe indicate its dipole nature, in agreement with findings for $^{56}$Fe. The high statistics and the excellent energy resolution of the large-volume LaBr$_{3}$(Ce) detectors allowed for a thorough analysis of $γ$ strength as function of excitation energy. Taking into account the presence of strong Porter-Thomas fluctuations, there is no indication of any significant excitation-energy dependence in the $γ$-ray strength function, in support of the generalized Brink-Axel hypothesis.

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arXiv2017

Is the generalized Brink-Axel hypothesis valid?

Experimental results of the $^{237}$Np($d, p γ)^{238}$Np reaction are presented, which verifies the generalized Brink-Axel (gBA) hypothesis for $γ$ transitions between states in the quasi-continuum. The gBA hypothesis holds not only for specific collective resonances, but for the full dipole strength below the neutron separation energy. We discuss the validity of the gBA hypothesis also for lighter systems like $^{92}$Zr where the concept of a unique $γ$-ray strength function ($γ$SF) is problematic due to large Porter-Thomas fluctuations. Methods for studying the $γ$SF and the fluctuations as function of excitation energy are presented.

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arXiv2016

Study of the 238U(d,p) surrogate reaction via the simultaneous measurement of gamma-decay and fission probabilities

We investigated the 238U(d,p) reaction as a surrogate for the n + 238U reaction. For this purpose we measured for the first time the gamma-decay and fission probabilities of 239U* simultaneously and compared them to the corresponding neutron-induced data. We present the details of the procedure to infer the decay probabilities, as well as a thorough uncertainty analysis, including parameter correlations. Calculations based on the continuum-discretized coupled-channels and distorted-wave Born approximations were used to correct our data from detected protons originating from elastic and inelastic deuteron breakup. In the region where the fission and gamma-decay probabilities compete, the corrected fission probability is in agreement with neutron-induced data, whereas the gamma-decay probability is much higher than the neutron-induced data. The performed statistical-model calculations are not able to explain these results.

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arXiv2016

Completing the nuclear reaction puzzle of the nucleosynthesis of 92Mo

One of the greatest questions for modern physics to address is how elements heavier than iron are created in extreme, astrophysical environments. A particularly challenging part of that question is the creation of the so-called p-nuclei, which are believed to be mainly produced in some types of supernovae. The lack of needed nuclear data presents an obstacle in nailing down the precise site and astrophysical conditions. In this work, we present for the first time measurements on the nuclear level density and average strength function of $^{92}$Mo. State-of-the-art p-process calculations systematically underestimate the observed solar abundance of this isotope. Our data provide stringent constraints on the $^{91}$Nb$(p,γ)^{92}$Mo reaction rate, which is the last unmeasured reaction in the nucleosynthesis puzzle of $^{92}$Mo. Based on our results, we conclude that the $^{92}$Mo abundance anomaly is not due to the nuclear physics input to astrophysical model calculations.

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arXiv2016

Experimentally constrained ($p,γ$)$^{89}$Y and ($n,γ$)$^{89}$Y reaction rates relevant to the $p$-process nucleosynthesis

The nuclear level density and the $γ$-ray strength function have been extracted for $^{89}$Y, using the Oslo Method on $^{89}$Y($p,p' γ$)$^{89}$Y coincidence data. The $γ$-ray strength function displays a low-energy enhancement consistent with previous observations in this mass region ($^{93-98}$Mo). Shell-model calculations give support that the observed enhancement is due to strong, low-energy $M1$ transitions at high excitation energies. The data were further used as input for calculations of the $^{88}$Sr($p,γ$)$^{89}$Y and $^{88}$Y($n,γ$)$^{89}$Y cross sections with the TALYS reaction code. Comparison with cross-section data, where available, as well as with values from the BRUSLIB library, shows a satisfying agreement.

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arXiv2016

The structure of low-lying states in ${}^{140}$Sm studied by Coulomb excitation

The electromagnetic structure of $^{140}$Sm was studied in a low-energy Coulomb excitation experiment with a radioactive ion beam from the REX-ISOLDE facility at CERN. The $2^+$ and $4^+$ states of the ground-state band and a second $2^+$ state were populated by multi-step excitation. The analysis of the differential Coulomb excitation cross sections yielded reduced transition probabilities between all observed states and the spectroscopic quadrupole moment for the $2_1^+$ state. The experimental results are compared to large-scale shell model calculations and beyond-mean-field calculations based on the Gogny D1S interaction with a five-dimensional collective Hamiltonian formalism. Simpler geometric and algebraic models are also employed to interpret the experimental data. The results indicate that $^{140}$Sm shows considerable $γ$ softness, but in contrast to earlier speculation no signs of shape coexistence at low excitation energy. This work sheds more light on the onset of deformation and collectivity in this mass region.

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arXiv2016

Statistical properties of $^{243}$Pu, and $^{242}$Pu(n,$γ$) cross section calculation

The level density and gamma-ray strength function (gammaSF) of 243Pu have been measured in the quasi-continuum using the Oslo method. Excited states in 243Pu were populated using the 242Pu(d,p) reaction. The level density closely follows the constant-temperature level density formula for excitation energies above the pairing gap. The gammaSF displays a double-humped resonance at low energy as also seen in previous investigations of actinide isotopes. The structure is interpreted as the scissors resonance and has a centroid of omega_{SR}=2.42(5)MeV and a total strength of B_{SR}=10.1(15)mu_N^2, which is in excellent agreement with sum-rule estimates. The measured level density and gammaSF were used to calculate the 242Pu(n,gamma) cross section in a neutron energy range for which there were previously no measured data.

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