arXiv subjects

G. Montambaux

Publications and source records attributed to G. Montambaux.

At least 19 recordsLinked to original sources

arXiv2023

Paramagnetic singularities of the orbital magnetism in graphene with a moiré potential

The recent detection of the singular diamagnetism of Dirac electrons in a single graphene layer paved a new way of probing 2D quantum materials through the measurement of equilibrium orbital currents which cannot be accessed in usual transport experiments. Among the theoretical predictions is an intriguing orbital paramagnetism at saddle points of the dispersion relation. Here we present magnetisation measurements in graphene monolayers aligned on hexagonal boron nitride (hBN)crystals. Beside the sharp diamagnetic McClure response at the Dirac point, we detect extra diamagnetic singularities at the satellite Dirac points (sDP) of the moiré lattice. Surrounding these diamagnetic satellite peaks, we also observe paramagnetic peaks located at the chemical potential of the saddle points of the Graphene moiré band structure and relate them to the presence of van Hove logarithmic singularities in the density of states. These findings reveal the long ago predicted anomalous paramagnetic orbital response in 2D systems when the Fermi energy is tuned to the vicinity of saddle points.

cond-mat.mes-hall↗

arXiv2021

Detection of graphene's divergent orbital diamagnetism at the Dirac point

The electronic properties of graphene have been intensively investigated over the last decade, and signatures of the remarkable features of its linear Dirac spectrum have been displayed using transport and spectroscopy experiments. In contrast, the orbital magnetism of graphene, which is one of the most fundamental signature of the characteristic Berry phase of graphene's electronic wave functions, has not yet been measured in a single flake. In particular, the striking prediction of a divergent diamagnetic response at zero doping calls for an experimental test. Using a highly sensitive Giant Magnetoresistance sensor (GMR) we have measured the gate voltage-dependent magnetization of a single graphene monolayer encapsulated between boron nitride crystals. The signal exhibits a diamagnetic peak at the Dirac point whose magnetic field and temperature dependences agree with theoretical predictions starting from the work of Mc Clure \cite{McClure1956}. Our measurements open a new field of investigation of orbital currents in graphene and 2D topological materials, offering a new means to monitor Berry phase singularities and explore correlated states generated by combined effects of Coulomb interactions, strain or moiré potentials.

cond-mat.mes-hall↗

arXiv2020

Semi-Dirac Transport and Anisotropic Localization in Polariton Honeycomb Lattices

Compression dramatically changes the transport and localization properties of graphene. This is intimately related to the change of symmetry of the Dirac cone when the particle hopping is different along different directions of the lattice. In particular, for a critical compression, a semi-Dirac cone is formed with massless and massive dispersions along perpendicular directions. Here we show direct evidence of the highly anisotropic transport of polaritons in a honeycomb lattice of coupled micropillars implementing a semi-Dirac cone. If we optically induce a vacancy-like defect in the lattice, we observe an anisotropically localized polariton distribution in a single sublattice, a consequence of the semi-Dirac dispersion. Our work opens up new horizons for the study of transport and localization in lattices with chiral symmetry and exotic Dirac dispersions.

cond-mat.mes-hall↗

arXiv2018

Tilted and type-III Dirac cones emerging from flat bands in photonic orbital graphene

The extraordinary electronic properties of Dirac materials, the two-dimensional partners of Weyl semimetals, arise from the linear crossings in their band structure. When the dispersion around the Dirac points is tilted, the emergence of intricate transport phenomena has been predicted, such as modified Klein tunnelling, intrinsic anomalous Hall effects and ferrimagnetism. However, Dirac materials are rare, particularly with tilted Dirac cones. Recently, artificial materials whose building blocks present orbital degrees of freedom have appeared as promising candidates for the engineering of exotic Dirac dispersions. Here we take advantage of the orbital structure of photonic resonators arranged in a honeycomb lattice to implement photonic lattices with semi-Dirac, tilted and, most interestingly, type-III Dirac cones that combine flat and linear dispersions. The tilted cones emerge from the touching of a flat and a parabolic band with a non-trivial topological charge. These results open the way to the synthesis of orbital Dirac matter with unconventional transport properties and, in combination with polariton nonlinearities, to the study of topological and Dirac superfluids in photonic lattices.

cond-mat.mes-hall↗

arXiv2018

Landau levels, response functions and magnetic oscillations from a generalized Onsager relation

A generalized semiclassical quantization condition for cyclotron orbits was recently proposed by Gao and Niu \cite{Gao}, that goes beyond the Onsager relation \cite{Onsager}. In addition to the integrated density of states, it formally involves magnetic response functions of all orders in the magnetic field. In particular, up to second order, it requires the knowledge of the spontaneous magnetization and the magnetic susceptibility, as was early anticipated by Roth \cite{Roth}. We study three applications of this relation focusing on two-dimensional electrons. First, we obtain magnetic response functions from Landau levels. Second we obtain Landau levels from response functions. Third we study magnetic oscillations in metals and propose a proper way to analyze Landau plots (i.e. the oscillation index $n$ as a function of the inverse magnetic field $1/B$) in order to extract quantities such as a zero-field phase-shift. Whereas the frequency of $1/B$-oscillations depends on the zero-field energy spectrum, the zero-field phase-shift depends on the geometry of the cell-periodic Bloch states via two contributions: the Berry phase and the average orbital magnetic moment on the Fermi surface. We also quantify deviations from linearity in Landau plots (i.e. aperiodic magnetic oscillations), as recently measured in surface states of three-dimensional topological insulators and emphasized by Wright and McKenzie \cite{Wright}.

cond-mat.mes-hall↗

arXiv2015

Diffusion of Dirac fermions across a topological merging transition in two dimensions

A continuous deformation of a Hamiltonian possessing at low energy two Dirac points of opposite chiralities can lead to a gap opening by merging of the two Dirac points. In two dimensions, the critical Hamiltonian possesses a semi-Dirac spectrum: linear in one direction but quadratic in the other. We study the transport properties across such a transition, from a Dirac semi-metal through a semi-Dirac phase towards a gapped phase. Using both a Boltzmann approach and a diagrammatic Kubo approach, we describe the conductivity tensor within the diffusive regime. In particular, we show that both the anisotropy of the Fermi surface and the Dirac nature of the eigenstates combine to give rise to anisotropic transport times, manifesting themselves through an unusual matrix self-energy.

cond-mat.mes-hall↗

arXiv2015

Rapid magnetic oscillations and magnetic breakdown in quasi-1D conductors

We review the physics of magnetic quantum oscillations in quasi-one dimensional conductors with an open Fermi surface, in the presence of modulated order. We emphasize the difference between situations where a modulation couples states on the same side of the Fermi surface and a modulation couples states on opposite sides of the Fermi surface. We also consider cases where several modulations coexist, which may lead to a complex reorganization of the Fermi surface. The interplay between nesting effects and magnetic breakdown is discussed. The experimental situation is reviewed.

cond-mat.mtrl-sci↗

arXiv2015

Tunable orbital susceptibility in $α$-${\cal T}_3$ tight-binding models

We study the importance of interband effects on the orbital susceptibility of three bands $α$-${\cal T}_3$ tight-binding models. The particularity of these models is that the coupling between the three energy bands (which is encoded in the wavefunctions properties) can be tuned (by a parameter $α$) without any modification of the energy spectrum. Using the gauge-invariant perturbative formalism that we have recently developped, we obtain a generic formula of the orbital susceptibility of $α$-${\cal T}_3$ tight-binding models. Considering then three characteristic examples that exhibit either Dirac, semi-Dirac or quadratic band touching, we show that by varying the parameter $α$ and thus the wavefunctions interband couplings, it is possible to drive a transition from a diamagnetic to a paramagnetic peak of the orbital susceptibility at the band touching. In the presence of a gap separating the dispersive bands, we show that the susceptibility inside the gap exhibits a similar dia to paramagnetic transition.

cond-mat.quant-gas↗

arXiv2014

Orbital magnetism of coupled bands models

We develop a gauge-independent perturbation theory for the grand potential of itinerant electrons in two-dimensional tight-binding models in the presence of a perpendicular magnetic field. At first order in the field, we recover the result of the so-called {\it modern theory of orbital magnetization} and, at second order, deduce a new general formula for the orbital susceptibility. In the special case of two coupled bands, we relate the susceptibility to geometrical quantities such as the Berry curvature. Our results are applied to several two-band -- either gapless or gapped -- systems. We point out some surprising features in the orbital susceptibility -- such as in-gap diamagnetism or parabolic band edge paramagnetism -- coming from interband coupling. From that we draw general conclusions on the orbital magnetism of itinerant electrons in multi-band tight-binding models.

cond-mat.mes-hall↗

arXiv2014

Measure of Diracness in two-dimensional semiconductors

We analyze the low-energy properties of two-dimensional direct-gap semiconductors, such as for example the transition-metal dichalcogenides MoS$_2$, WS$_2$, and their diselenide analogues MoSe$_2$, WSe$_2$, etc., which are currently intensively investigated. In general, their electrons have a mixed character -- they can be massive Dirac fermions as well as simple Schrödinger particles. We propose a measure (Diracness) for the degree of mixing between the two characters and discuss how this quantity can in principle be extracted experimentally, within magneto-transport measurements, and numerically via ab initio calculations.

cond-mat.mes-hall↗

arXiv2013

Magnetic spectrum of trigonally warped bilayer graphene - semiclassical analysis, zero modes, and topological winding numbers

We investigate the fine structure in the energy spectrum of bilayer graphene in the presence of various stacking defaults, such as a translational or rotational mismatch. This fine structure consists of four Dirac points that move away from their original positions as a consequence of the mismatch and eventually merge in various manners. The different types of merging are described in terms of topological invariants (winding numbers) that determine the Landau-level spectrum in the presence of a magnetic field as well as the degeneracy of the levels. The Landau-level spectrum is, within a wide parameter range, well described by a semiclassical treatment that makes use of topological winding numbers. However, the latter need to be redefined at zero energy in the high-magnetic-field limit as well as in the vicinity of saddle points in the zero-field dispersion relation.

cond-mat.mes-hall↗

arXiv2013

From dia- to paramagnetic orbital susceptibility of Dirac cones

We study the orbital susceptibility of coupled energy bands with a pair of Dirac points, as in graphene. We show that different systems having the same zero-field energy spectrum exhibit strong differences in their orbital magnetic response at zero energy, ranging from diamagnetism (graphene) to paramagnetism (dice lattice). A lattice model is introduced which interpolates continuously between these two limits. This striking behavior is related to a Berry phase varying continuously from pi to 0. These predictions could be tested with cold atoms in an optical lattice

cond-mat.mes-hall↗

arXiv2012

Manipulation of Dirac points in graphene-like crystals

We review different scenarios for the motion and merging of Dirac points in two dimensional crystals. These different types of merging can be classified according to a winding number (a topological Berry phase) attached to each Dirac point. For each scenario, we calculate the Landau level spectrum and show that it can be quantitatively described by a semiclassical quantization rule for the constant energy areas. This quantization depends on how many Dirac points are enclosed by these areas. We also emphasize that different scenarios are characterized by different numbers of topologically protected zero energy Landau levels

cond-mat.mes-hall↗

arXiv2012

Geometry-related magnetic interference patterns in long SNS Josephson junctions

We have measured the critical current dependence on the magnetic flux of two long SNS junctions differing by the normal wire geometry. The samples are made by a Au wire connected to W contacts, via Focused Ion Beam assisted deposition. We could tune the magnetic pattern from the monotonic gaussian-like decay of a quasi 1D normal wire to the Fraunhofer-like pattern of a square normal wire. We explain the monotonic limit with a semiclassical 1D model, and we fit both field dependences with numerical simulations of the 2D Usadel equation. Furthermore, we observe both integer and fractional Shapiro steps. The magnetic flux dependence of the integer steps reproduces as expected that of the critical current Ic, while fractional steps decay slower with the flux than Ic.

cond-mat.mes-hall↗

arXiv2011

The Zak phase and the existence of edge states in graphene

We develop a method to predict the existence of edge states in graphene ribbons for a large class of boundaries. This approach is based on the bulk-edge correspondence between the quantized value of the Zak phase Z(k), which is a Berry phase across an appropriately chosen one-dimensional Brillouin zone, and the existence of a localized state of momentum k at the boundary of the ribbon. This bulk-edge correspondence is rigorously demonstrated for a one dimensional toy model as well as for graphene ribbons with zigzag edges. The range of k for which edge states exist in a graphene ribbon is then calculated for arbitrary orientations of the edges. Finally, we show that the introduction of an anisotropy leads to a topological transition in terms of the Zak phase, which modifies the localization properties at the edges. Our approach gives a new geometrical understanding of edge states, it confirms and generalizes the results of several previous works.

cond-mat.mes-hall↗

arXiv2011

Emergence of Dirac Electron Pair in Charge Ordered State of Organic Conductor $α$-(BEDT-TTF)$_2$I$_3$

We re-examine the band structure of the stripe charge ordered state of $α$-(BEDT-TTF)$_2$I$_3$ under pressure by using an extended Hubbard model within the Hartree mean-field theory. By increasing pressure, we find a topological transition from a conventional insulator with a single-minimum in the dispersion relation at the M-point in the Brillouin zone, towards a new phase which exhibits a double-minimum. This transition is characterized by the appearance of a pair of Dirac electrons with a finite mass. Using the Luttinger-Kohn representation at the M-point, it is shown that such a variation of the band structure can be described by an effective $2 \times 2$ low energy Hamiltonian with a single driving parameter. The topological nature of this transition is confirmed by the calculation of the Berry curvature which vanishes in the conventional phase and has a double peak structure with opposite signs in the new phase. We compare the structure of this transition with a simpler situation which occurs in two-component systems, like boron-nitride.

cond-mat.mes-hall↗

arXiv2011

Topologically Protected Zero Modes in Twisted Bilayer Graphene

We show that the twisted graphene bilayer can reveal unusual topological properties at low energies, as a consequence of a Dirac-point splitting. These features rely on a symmetry analysis of the electron hopping between the two layers of graphene and we derive a simplified effective low-energy Hamiltonian which captures the essential topological properties of twisted bilayer graphene. The corresponding Landau levels peculiarly reveal a degenerate zero-energy mode which cannot be lifted by strong magnetic fields.

cond-mat.mes-hall↗

arXiv2010

Topological Berry phase and semiclassical quantization of cyclotron orbits for two dimensional electrons in coupled band models

The semiclassical quantization of cyclotron orbits for two-dimensional Bloch electrons in a coupled two band model with a particle-hole symmetric spectrum is considered. As concrete examples, we study graphene (both mono and bilayer) and boron nitride. The main focus is on wave effects -- such as Berry phase and Maslov index -- occurring at order $\hbar$ in the semiclassical quantization and producing non-trivial shifts in the resulting Landau levels. Specifically, we show that the index shift appearing in the Landau levels is related to a topological part of the Berry phase -- which is basically a winding number of the direction of the pseudo-spin 1/2 associated to the coupled bands -- acquired by an electron during a cyclotron orbit and not to the complete Berry phase, as commonly stated. As a consequence, the Landau levels of a coupled band insulator are shifted as compared to a usual band insulator. We also study in detail the Berry curvature in the whole Brillouin zone on a specific example (boron nitride) and show that its computation requires care in defining the "k-dependent Hamiltonian" H(k), where k is the Bloch wavevector.

cond-mat.mes-hall↗